Comparison between WGS membrane reactors operating with and without sweep gas: Limiting conditions for co-current flow

Autores
Adrover, María Esperanza; Borio, Daniel Oscar; Pedernera, Marisa Noemi
Año de publicación
2017
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
In this work, a comparative study is carried out to analyze the behavior of a water gas shift membrane reactor operating with and without sweep gas. The present study includes thermal effects that play a key role in reaction and permeation rates involved in the membrane reactor. Based on a 1-D mathematical model, the effect of the most important operating variables on the membrane reactor performance is comparatively studied. Additionally, novel algebraic expressions are developed when operating without sweep gas, that only depend on inlet variables to calculate the limiting membrane reactor conversions and recovery values. An algebraic equation is developed to estimate limiting recovery when operating with sweep gas. The dependence of limiting membrane reactor conversion and recovery values operating with and without sweep gas on operating parameters is included. From the comparative analysis, some guidelines for an improved operation of the membrane reactor are proposed.
Fil: Adrover, María Esperanza. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Planta Piloto de Ingeniería Química. Universidad Nacional del Sur. Planta Piloto de Ingeniería Química; Argentina
Fil: Borio, Daniel Oscar. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Planta Piloto de Ingeniería Química. Universidad Nacional del Sur. Planta Piloto de Ingeniería Química; Argentina
Fil: Pedernera, Marisa Noemi. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Planta Piloto de Ingeniería Química. Universidad Nacional del Sur. Planta Piloto de Ingeniería Química; Argentina
Materia
Limiting Conversion
Membrane Reactor
Reactor Analysis
Sweep Gas
Wgs
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/39988
Acceder
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oai_identifier_str oai:ri.conicet.gov.ar:11336/39988
network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Comparison between WGS membrane reactors operating with and without sweep gas: Limiting conditions for co-current flowAdrover, María EsperanzaBorio, Daniel OscarPedernera, Marisa NoemiLimiting ConversionMembrane ReactorReactor AnalysisSweep GasWgshttps://purl.org/becyt/ford/2.4https://purl.org/becyt/ford/2In this work, a comparative study is carried out to analyze the behavior of a water gas shift membrane reactor operating with and without sweep gas. The present study includes thermal effects that play a key role in reaction and permeation rates involved in the membrane reactor. Based on a 1-D mathematical model, the effect of the most important operating variables on the membrane reactor performance is comparatively studied. Additionally, novel algebraic expressions are developed when operating without sweep gas, that only depend on inlet variables to calculate the limiting membrane reactor conversions and recovery values. An algebraic equation is developed to estimate limiting recovery when operating with sweep gas. The dependence of limiting membrane reactor conversion and recovery values operating with and without sweep gas on operating parameters is included. From the comparative analysis, some guidelines for an improved operation of the membrane reactor are proposed.Fil: Adrover, María Esperanza. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Planta Piloto de Ingeniería Química. Universidad Nacional del Sur. Planta Piloto de Ingeniería Química; ArgentinaFil: Borio, Daniel Oscar. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Planta Piloto de Ingeniería Química. Universidad Nacional del Sur. Planta Piloto de Ingeniería Química; ArgentinaFil: Pedernera, Marisa Noemi. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Planta Piloto de Ingeniería Química. Universidad Nacional del Sur. Planta Piloto de Ingeniería Química; ArgentinaPergamon-Elsevier Science Ltd2017-02info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/39988Adrover, María Esperanza; Borio, Daniel Oscar; Pedernera, Marisa Noemi; Comparison between WGS membrane reactors operating with and without sweep gas: Limiting conditions for co-current flow; Pergamon-Elsevier Science Ltd; International Journal of Hydrogen Energy; 42; 8; 2-2017; 5139-51490360-3199CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/doi/10.1016/j.ijhydene.2016.11.075info:eu-repo/semantics/altIdentifier/url/https://www.sciencedirect.com/science/article/pii/S036031991633364Xinfo:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-10-22T11:05:34Zoai:ri.conicet.gov.ar:11336/39988instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-10-22 11:05:34.741CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Comparison between WGS membrane reactors operating with and without sweep gas: Limiting conditions for co-current flow
title Comparison between WGS membrane reactors operating with and without sweep gas: Limiting conditions for co-current flow
spellingShingle Comparison between WGS membrane reactors operating with and without sweep gas: Limiting conditions for co-current flow
Adrover, María Esperanza
Limiting Conversion
Membrane Reactor
Reactor Analysis
Sweep Gas
Wgs
title_short Comparison between WGS membrane reactors operating with and without sweep gas: Limiting conditions for co-current flow
title_full Comparison between WGS membrane reactors operating with and without sweep gas: Limiting conditions for co-current flow
title_fullStr Comparison between WGS membrane reactors operating with and without sweep gas: Limiting conditions for co-current flow
title_full_unstemmed Comparison between WGS membrane reactors operating with and without sweep gas: Limiting conditions for co-current flow
title_sort Comparison between WGS membrane reactors operating with and without sweep gas: Limiting conditions for co-current flow
dc.creator.none.fl_str_mv Adrover, María Esperanza
Borio, Daniel Oscar
Pedernera, Marisa Noemi
author Adrover, María Esperanza
author_facet Adrover, María Esperanza
Borio, Daniel Oscar
Pedernera, Marisa Noemi
author_role author
author2 Borio, Daniel Oscar
Pedernera, Marisa Noemi
author2_role author
author
dc.subject.none.fl_str_mv Limiting Conversion
Membrane Reactor
Reactor Analysis
Sweep Gas
Wgs
topic Limiting Conversion
Membrane Reactor
Reactor Analysis
Sweep Gas
Wgs
purl_subject.fl_str_mv https://purl.org/becyt/ford/2.4
https://purl.org/becyt/ford/2
dc.description.none.fl_txt_mv In this work, a comparative study is carried out to analyze the behavior of a water gas shift membrane reactor operating with and without sweep gas. The present study includes thermal effects that play a key role in reaction and permeation rates involved in the membrane reactor. Based on a 1-D mathematical model, the effect of the most important operating variables on the membrane reactor performance is comparatively studied. Additionally, novel algebraic expressions are developed when operating without sweep gas, that only depend on inlet variables to calculate the limiting membrane reactor conversions and recovery values. An algebraic equation is developed to estimate limiting recovery when operating with sweep gas. The dependence of limiting membrane reactor conversion and recovery values operating with and without sweep gas on operating parameters is included. From the comparative analysis, some guidelines for an improved operation of the membrane reactor are proposed.
Fil: Adrover, María Esperanza. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Planta Piloto de Ingeniería Química. Universidad Nacional del Sur. Planta Piloto de Ingeniería Química; Argentina
Fil: Borio, Daniel Oscar. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Planta Piloto de Ingeniería Química. Universidad Nacional del Sur. Planta Piloto de Ingeniería Química; Argentina
Fil: Pedernera, Marisa Noemi. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Planta Piloto de Ingeniería Química. Universidad Nacional del Sur. Planta Piloto de Ingeniería Química; Argentina
description In this work, a comparative study is carried out to analyze the behavior of a water gas shift membrane reactor operating with and without sweep gas. The present study includes thermal effects that play a key role in reaction and permeation rates involved in the membrane reactor. Based on a 1-D mathematical model, the effect of the most important operating variables on the membrane reactor performance is comparatively studied. Additionally, novel algebraic expressions are developed when operating without sweep gas, that only depend on inlet variables to calculate the limiting membrane reactor conversions and recovery values. An algebraic equation is developed to estimate limiting recovery when operating with sweep gas. The dependence of limiting membrane reactor conversion and recovery values operating with and without sweep gas on operating parameters is included. From the comparative analysis, some guidelines for an improved operation of the membrane reactor are proposed.
publishDate 2017
dc.date.none.fl_str_mv 2017-02
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/39988
Adrover, María Esperanza; Borio, Daniel Oscar; Pedernera, Marisa Noemi; Comparison between WGS membrane reactors operating with and without sweep gas: Limiting conditions for co-current flow; Pergamon-Elsevier Science Ltd; International Journal of Hydrogen Energy; 42; 8; 2-2017; 5139-5149
0360-3199
CONICET Digital
CONICET
url http://hdl.handle.net/11336/39988
identifier_str_mv Adrover, María Esperanza; Borio, Daniel Oscar; Pedernera, Marisa Noemi; Comparison between WGS membrane reactors operating with and without sweep gas: Limiting conditions for co-current flow; Pergamon-Elsevier Science Ltd; International Journal of Hydrogen Energy; 42; 8; 2-2017; 5139-5149
0360-3199
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/doi/10.1016/j.ijhydene.2016.11.075
info:eu-repo/semantics/altIdentifier/url/https://www.sciencedirect.com/science/article/pii/S036031991633364X
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv Pergamon-Elsevier Science Ltd
publisher.none.fl_str_mv Pergamon-Elsevier Science Ltd
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 12.982451

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