Plasticized Mechanical Recycled PLA Films Reinforced with Microbial Cellulose Particles Obtained from Kombucha Fermented in Yerba Mate Waste

Autores
Agüero, Ángel; Corral Perianes, Esther; Abarca de las Muelas, Sara Soledad; Lascano, Diego; de la Fuente García Soto, María del Mar; Peltzer, Mercedes Ana; Balart, Rafael; Arrieta, Marina Patricia
Año de publicación
2023
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
In this study, yerba mate waste (YMW) was used to produce a kombucha beverage, and the obtained microbial cellulose produced as a byproduct (KMW) was used to reinforce a mechanically recycled poly(lactic acid) (r-PLA) matrix. Microbial cellulosic particles were also produced in pristine yerba mate for comparison (KMN). To simulate the revalorization of the industrial PLA products rejected during the production line, PLA was subjected to three extrusion cycles, and the resultant pellets (r3-PLA) were then plasticized with 15 wt.% of acetyl tributyl citrate ester (ATBC) to obtain optically transparent and flexible films by the solvent casting method. The plasticized r3-PLA-ATBC matrix was then loaded with KMW and KMN in 1 and 3 wt.%. The use of plasticizer allowed a good dispersion of microbial cellulose particles into the r3-PLA matrix, allowing us to obtain flexible and transparent films which showed good structural and mechanical performance. Additionally, the obtained films showed antioxidant properties, as was proven by release analyses conducted in direct contact with a fatty food simulant. The results suggest the potential interest of these recycled and biobased materials, which are obtained from the revalorization of food waste, for their industrial application in food packaging and agricultural films.
Fil: Agüero, Ángel. Universidad Politécnica de Valencia. Instituto de Tecnología de Materiales; España. Universidad Politécnica de Madrid; España
Fil: Corral Perianes, Esther. Universidad Politécnica de Madrid; España
Fil: Abarca de las Muelas, Sara Soledad. Universidad Politécnica de Madrid; España
Fil: Lascano, Diego. Universidad Politécnica de Valencia. Instituto de Tecnología de Materiales; España
Fil: de la Fuente García Soto, María del Mar. Universidad Politécnica de Madrid; España
Fil: Peltzer, Mercedes Ana. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Universidad Nacional de Quilmes. Departamento de Ciencia y Tecnología. Área Ingeniería en Alimentos; Argentina
Fil: Balart, Rafael. Universidad Politécnica de Valencia. Instituto de Tecnología de Materiales; España
Fil: Arrieta, Marina Patricia. Universidad Politécnica de Madrid; España
Materia
CELLULOSE
FOOD PACKAGING
KOMBUCHA
PLA
YERBA MATE
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/218953
Acceder
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oai_identifier_str oai:ri.conicet.gov.ar:11336/218953
network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Plasticized Mechanical Recycled PLA Films Reinforced with Microbial Cellulose Particles Obtained from Kombucha Fermented in Yerba Mate WasteAgüero, ÁngelCorral Perianes, EstherAbarca de las Muelas, Sara SoledadLascano, Diegode la Fuente García Soto, María del MarPeltzer, Mercedes AnaBalart, RafaelArrieta, Marina PatriciaCELLULOSEFOOD PACKAGINGKOMBUCHAPLAYERBA MATEhttps://purl.org/becyt/ford/2.11https://purl.org/becyt/ford/2In this study, yerba mate waste (YMW) was used to produce a kombucha beverage, and the obtained microbial cellulose produced as a byproduct (KMW) was used to reinforce a mechanically recycled poly(lactic acid) (r-PLA) matrix. Microbial cellulosic particles were also produced in pristine yerba mate for comparison (KMN). To simulate the revalorization of the industrial PLA products rejected during the production line, PLA was subjected to three extrusion cycles, and the resultant pellets (r3-PLA) were then plasticized with 15 wt.% of acetyl tributyl citrate ester (ATBC) to obtain optically transparent and flexible films by the solvent casting method. The plasticized r3-PLA-ATBC matrix was then loaded with KMW and KMN in 1 and 3 wt.%. The use of plasticizer allowed a good dispersion of microbial cellulose particles into the r3-PLA matrix, allowing us to obtain flexible and transparent films which showed good structural and mechanical performance. Additionally, the obtained films showed antioxidant properties, as was proven by release analyses conducted in direct contact with a fatty food simulant. The results suggest the potential interest of these recycled and biobased materials, which are obtained from the revalorization of food waste, for their industrial application in food packaging and agricultural films.Fil: Agüero, Ángel. Universidad Politécnica de Valencia. Instituto de Tecnología de Materiales; España. Universidad Politécnica de Madrid; EspañaFil: Corral Perianes, Esther. Universidad Politécnica de Madrid; EspañaFil: Abarca de las Muelas, Sara Soledad. Universidad Politécnica de Madrid; EspañaFil: Lascano, Diego. Universidad Politécnica de Valencia. Instituto de Tecnología de Materiales; EspañaFil: de la Fuente García Soto, María del Mar. Universidad Politécnica de Madrid; EspañaFil: Peltzer, Mercedes Ana. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Universidad Nacional de Quilmes. Departamento de Ciencia y Tecnología. Área Ingeniería en Alimentos; ArgentinaFil: Balart, Rafael. Universidad Politécnica de Valencia. Instituto de Tecnología de Materiales; EspañaFil: Arrieta, Marina Patricia. Universidad Politécnica de Madrid; EspañaMultidisciplinary Digital Publishing Institute2023-01info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/218953Agüero, Ángel; Corral Perianes, Esther; Abarca de las Muelas, Sara Soledad; Lascano, Diego; de la Fuente García Soto, María del Mar; et al.; Plasticized Mechanical Recycled PLA Films Reinforced with Microbial Cellulose Particles Obtained from Kombucha Fermented in Yerba Mate Waste; Multidisciplinary Digital Publishing Institute; Polymers; 15; 2; 1-2023; 1-192073-4360CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://www.mdpi.com/2073-4360/15/2/285info:eu-repo/semantics/altIdentifier/doi/10.3390/polym15020285info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T09:36:12Zoai:ri.conicet.gov.ar:11336/218953instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 09:36:12.319CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Plasticized Mechanical Recycled PLA Films Reinforced with Microbial Cellulose Particles Obtained from Kombucha Fermented in Yerba Mate Waste
title Plasticized Mechanical Recycled PLA Films Reinforced with Microbial Cellulose Particles Obtained from Kombucha Fermented in Yerba Mate Waste
spellingShingle Plasticized Mechanical Recycled PLA Films Reinforced with Microbial Cellulose Particles Obtained from Kombucha Fermented in Yerba Mate Waste
Agüero, Ángel
CELLULOSE
FOOD PACKAGING
KOMBUCHA
PLA
YERBA MATE
title_short Plasticized Mechanical Recycled PLA Films Reinforced with Microbial Cellulose Particles Obtained from Kombucha Fermented in Yerba Mate Waste
title_full Plasticized Mechanical Recycled PLA Films Reinforced with Microbial Cellulose Particles Obtained from Kombucha Fermented in Yerba Mate Waste
title_fullStr Plasticized Mechanical Recycled PLA Films Reinforced with Microbial Cellulose Particles Obtained from Kombucha Fermented in Yerba Mate Waste
title_full_unstemmed Plasticized Mechanical Recycled PLA Films Reinforced with Microbial Cellulose Particles Obtained from Kombucha Fermented in Yerba Mate Waste
title_sort Plasticized Mechanical Recycled PLA Films Reinforced with Microbial Cellulose Particles Obtained from Kombucha Fermented in Yerba Mate Waste
dc.creator.none.fl_str_mv Agüero, Ángel
Corral Perianes, Esther
Abarca de las Muelas, Sara Soledad
Lascano, Diego
de la Fuente García Soto, María del Mar
Peltzer, Mercedes Ana
Balart, Rafael
Arrieta, Marina Patricia
author Agüero, Ángel
author_facet Agüero, Ángel
Corral Perianes, Esther
Abarca de las Muelas, Sara Soledad
Lascano, Diego
de la Fuente García Soto, María del Mar
Peltzer, Mercedes Ana
Balart, Rafael
Arrieta, Marina Patricia
author_role author
author2 Corral Perianes, Esther
Abarca de las Muelas, Sara Soledad
Lascano, Diego
de la Fuente García Soto, María del Mar
Peltzer, Mercedes Ana
Balart, Rafael
Arrieta, Marina Patricia
author2_role author
author
author
author
author
author
author
dc.subject.none.fl_str_mv CELLULOSE
FOOD PACKAGING
KOMBUCHA
PLA
YERBA MATE
topic CELLULOSE
FOOD PACKAGING
KOMBUCHA
PLA
YERBA MATE
purl_subject.fl_str_mv https://purl.org/becyt/ford/2.11
https://purl.org/becyt/ford/2
dc.description.none.fl_txt_mv In this study, yerba mate waste (YMW) was used to produce a kombucha beverage, and the obtained microbial cellulose produced as a byproduct (KMW) was used to reinforce a mechanically recycled poly(lactic acid) (r-PLA) matrix. Microbial cellulosic particles were also produced in pristine yerba mate for comparison (KMN). To simulate the revalorization of the industrial PLA products rejected during the production line, PLA was subjected to three extrusion cycles, and the resultant pellets (r3-PLA) were then plasticized with 15 wt.% of acetyl tributyl citrate ester (ATBC) to obtain optically transparent and flexible films by the solvent casting method. The plasticized r3-PLA-ATBC matrix was then loaded with KMW and KMN in 1 and 3 wt.%. The use of plasticizer allowed a good dispersion of microbial cellulose particles into the r3-PLA matrix, allowing us to obtain flexible and transparent films which showed good structural and mechanical performance. Additionally, the obtained films showed antioxidant properties, as was proven by release analyses conducted in direct contact with a fatty food simulant. The results suggest the potential interest of these recycled and biobased materials, which are obtained from the revalorization of food waste, for their industrial application in food packaging and agricultural films.
Fil: Agüero, Ángel. Universidad Politécnica de Valencia. Instituto de Tecnología de Materiales; España. Universidad Politécnica de Madrid; España
Fil: Corral Perianes, Esther. Universidad Politécnica de Madrid; España
Fil: Abarca de las Muelas, Sara Soledad. Universidad Politécnica de Madrid; España
Fil: Lascano, Diego. Universidad Politécnica de Valencia. Instituto de Tecnología de Materiales; España
Fil: de la Fuente García Soto, María del Mar. Universidad Politécnica de Madrid; España
Fil: Peltzer, Mercedes Ana. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Universidad Nacional de Quilmes. Departamento de Ciencia y Tecnología. Área Ingeniería en Alimentos; Argentina
Fil: Balart, Rafael. Universidad Politécnica de Valencia. Instituto de Tecnología de Materiales; España
Fil: Arrieta, Marina Patricia. Universidad Politécnica de Madrid; España
description In this study, yerba mate waste (YMW) was used to produce a kombucha beverage, and the obtained microbial cellulose produced as a byproduct (KMW) was used to reinforce a mechanically recycled poly(lactic acid) (r-PLA) matrix. Microbial cellulosic particles were also produced in pristine yerba mate for comparison (KMN). To simulate the revalorization of the industrial PLA products rejected during the production line, PLA was subjected to three extrusion cycles, and the resultant pellets (r3-PLA) were then plasticized with 15 wt.% of acetyl tributyl citrate ester (ATBC) to obtain optically transparent and flexible films by the solvent casting method. The plasticized r3-PLA-ATBC matrix was then loaded with KMW and KMN in 1 and 3 wt.%. The use of plasticizer allowed a good dispersion of microbial cellulose particles into the r3-PLA matrix, allowing us to obtain flexible and transparent films which showed good structural and mechanical performance. Additionally, the obtained films showed antioxidant properties, as was proven by release analyses conducted in direct contact with a fatty food simulant. The results suggest the potential interest of these recycled and biobased materials, which are obtained from the revalorization of food waste, for their industrial application in food packaging and agricultural films.
publishDate 2023
dc.date.none.fl_str_mv 2023-01
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/218953
Agüero, Ángel; Corral Perianes, Esther; Abarca de las Muelas, Sara Soledad; Lascano, Diego; de la Fuente García Soto, María del Mar; et al.; Plasticized Mechanical Recycled PLA Films Reinforced with Microbial Cellulose Particles Obtained from Kombucha Fermented in Yerba Mate Waste; Multidisciplinary Digital Publishing Institute; Polymers; 15; 2; 1-2023; 1-19
2073-4360
CONICET Digital
CONICET
url http://hdl.handle.net/11336/218953
identifier_str_mv Agüero, Ángel; Corral Perianes, Esther; Abarca de las Muelas, Sara Soledad; Lascano, Diego; de la Fuente García Soto, María del Mar; et al.; Plasticized Mechanical Recycled PLA Films Reinforced with Microbial Cellulose Particles Obtained from Kombucha Fermented in Yerba Mate Waste; Multidisciplinary Digital Publishing Institute; Polymers; 15; 2; 1-2023; 1-19
2073-4360
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://www.mdpi.com/2073-4360/15/2/285
info:eu-repo/semantics/altIdentifier/doi/10.3390/polym15020285
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv Multidisciplinary Digital Publishing Institute
publisher.none.fl_str_mv Multidisciplinary Digital Publishing Institute
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 13.070432

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