Human health risk associated to particulate matter and polycyclic aromatic hydrocarbon levels and their relation with preponderant sources in Gran La Plata, Argentina

Autores
Giuliani, Daniela Silvana; Colman Lerner, Jorge Esteban; Porta, Atilio Andrés
Año de publicación
2021
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
Levels of suspended particulate matter (PM) of both fractions PM₁₀ and PM2.5 in ambient air were monitored in three areas of Gran La Plata: industrial, urban, and residential (2017-2019). Associated polycyclic aromatic hydrocarbons (PAHs) and nitropolycyclic aromatic hydrocarbons (NPAHs) to PM were also determined and possible emission sources were identified. Assessment of health risk to PM exposure and associated compounds was realized. Results showed a decrease in levels of PM₁₀ in each area along the period studied, especially in the industrial area. Decreases in PM2.5 levels were also observed in urban and residential areas over the years, although the trend is not as marked as with PM₁₀ levels. Then, PM2.5 levels in the industrial area have remained practically constant. The 89% of both PM₁₀ and PM2.5 annual mean exceeds the WHO reference values. The presence of most of the 16 US EPA priority PAHs studied was found with a detection frequency greater than 60% and it was possible to identify the importance of the contributions of vehicular emissions as predominant sources of PAH emission. From the calculations of the risk of contracting cancer throughout life (LCR), in the case of adults, the US EPA limits were not complied in the industrial and urban areas and in both fractions of PM. From the evaluation of the burden of disease (EBD), the calculated relative risks of mortality were very similar for the studied districts, being the relative risk in La Plata slightly lower, about 3-5%, than those in Berisso and Ensenada.
Facultad de Ciencias Exactas
Centro de Investigaciones del Medioambiente
Centro de Investigación y Desarrollo en Ciencias Aplicadas
Materia
Ciencias Exactas
PM
PAHs
Vehicular emissions
Lifetime cancer risk
Environmental burden of disease
Gran La Plata Argentina
Nivel de accesibilidad
acceso abierto
Condiciones de uso
http://creativecommons.org/licenses/by-nc-sa/4.0/
Repositorio
SEDICI (UNLP)
Institución
Universidad Nacional de La Plata
OAI Identificador
oai:sedici.unlp.edu.ar:10915/130464

id SEDICI_6ee97b576f1f83fe6fa5009a3bdd50f4
oai_identifier_str oai:sedici.unlp.edu.ar:10915/130464
network_acronym_str SEDICI
repository_id_str 1329
network_name_str SEDICI (UNLP)
spelling Human health risk associated to particulate matter and polycyclic aromatic hydrocarbon levels and their relation with preponderant sources in Gran La Plata, ArgentinaGiuliani, Daniela SilvanaColman Lerner, Jorge EstebanPorta, Atilio AndrésCiencias ExactasPMPAHsVehicular emissionsLifetime cancer riskEnvironmental burden of diseaseGran La Plata ArgentinaLevels of suspended particulate matter (PM) of both fractions PM₁₀ and PM<sub>2.5</sub> in ambient air were monitored in three areas of Gran La Plata: industrial, urban, and residential (2017-2019). Associated polycyclic aromatic hydrocarbons (PAHs) and nitropolycyclic aromatic hydrocarbons (NPAHs) to PM were also determined and possible emission sources were identified. Assessment of health risk to PM exposure and associated compounds was realized. Results showed a decrease in levels of PM₁₀ in each area along the period studied, especially in the industrial area. Decreases in PM<sub>2.5</sub> levels were also observed in urban and residential areas over the years, although the trend is not as marked as with PM₁₀ levels. Then, PM<sub>2.5</sub> levels in the industrial area have remained practically constant. The 89% of both PM₁₀ and PM<sub>2.5</sub> annual mean exceeds the WHO reference values. The presence of most of the 16 US EPA priority PAHs studied was found with a detection frequency greater than 60% and it was possible to identify the importance of the contributions of vehicular emissions as predominant sources of PAH emission. From the calculations of the risk of contracting cancer throughout life (LCR), in the case of adults, the US EPA limits were not complied in the industrial and urban areas and in both fractions of PM. From the evaluation of the burden of disease (EBD), the calculated relative risks of mortality were very similar for the studied districts, being the relative risk in La Plata slightly lower, about 3-5%, than those in Berisso and Ensenada.Facultad de Ciencias ExactasCentro de Investigaciones del MedioambienteCentro de Investigación y Desarrollo en Ciencias Aplicadas2021-07info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionArticulohttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdf35226-35241http://sedici.unlp.edu.ar/handle/10915/130464enginfo:eu-repo/semantics/altIdentifier/issn/1614-7499info:eu-repo/semantics/altIdentifier/issn/0944-1344info:eu-repo/semantics/altIdentifier/doi/10.1007/s11356-021-13138-8info:eu-repo/semantics/altIdentifier/pmid/33666842info:eu-repo/semantics/openAccesshttp://creativecommons.org/licenses/by-nc-sa/4.0/Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International (CC BY-NC-SA 4.0)reponame:SEDICI (UNLP)instname:Universidad Nacional de La Platainstacron:UNLP2025-09-29T11:32:26Zoai:sedici.unlp.edu.ar:10915/130464Institucionalhttp://sedici.unlp.edu.ar/Universidad públicaNo correspondehttp://sedici.unlp.edu.ar/oai/snrdalira@sedici.unlp.edu.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:13292025-09-29 11:32:27.227SEDICI (UNLP) - Universidad Nacional de La Platafalse
dc.title.none.fl_str_mv Human health risk associated to particulate matter and polycyclic aromatic hydrocarbon levels and their relation with preponderant sources in Gran La Plata, Argentina
title Human health risk associated to particulate matter and polycyclic aromatic hydrocarbon levels and their relation with preponderant sources in Gran La Plata, Argentina
spellingShingle Human health risk associated to particulate matter and polycyclic aromatic hydrocarbon levels and their relation with preponderant sources in Gran La Plata, Argentina
Giuliani, Daniela Silvana
Ciencias Exactas
PM
PAHs
Vehicular emissions
Lifetime cancer risk
Environmental burden of disease
Gran La Plata Argentina
title_short Human health risk associated to particulate matter and polycyclic aromatic hydrocarbon levels and their relation with preponderant sources in Gran La Plata, Argentina
title_full Human health risk associated to particulate matter and polycyclic aromatic hydrocarbon levels and their relation with preponderant sources in Gran La Plata, Argentina
title_fullStr Human health risk associated to particulate matter and polycyclic aromatic hydrocarbon levels and their relation with preponderant sources in Gran La Plata, Argentina
title_full_unstemmed Human health risk associated to particulate matter and polycyclic aromatic hydrocarbon levels and their relation with preponderant sources in Gran La Plata, Argentina
title_sort Human health risk associated to particulate matter and polycyclic aromatic hydrocarbon levels and their relation with preponderant sources in Gran La Plata, Argentina
dc.creator.none.fl_str_mv Giuliani, Daniela Silvana
Colman Lerner, Jorge Esteban
Porta, Atilio Andrés
author Giuliani, Daniela Silvana
author_facet Giuliani, Daniela Silvana
Colman Lerner, Jorge Esteban
Porta, Atilio Andrés
author_role author
author2 Colman Lerner, Jorge Esteban
Porta, Atilio Andrés
author2_role author
author
dc.subject.none.fl_str_mv Ciencias Exactas
PM
PAHs
Vehicular emissions
Lifetime cancer risk
Environmental burden of disease
Gran La Plata Argentina
topic Ciencias Exactas
PM
PAHs
Vehicular emissions
Lifetime cancer risk
Environmental burden of disease
Gran La Plata Argentina
dc.description.none.fl_txt_mv Levels of suspended particulate matter (PM) of both fractions PM₁₀ and PM<sub>2.5</sub> in ambient air were monitored in three areas of Gran La Plata: industrial, urban, and residential (2017-2019). Associated polycyclic aromatic hydrocarbons (PAHs) and nitropolycyclic aromatic hydrocarbons (NPAHs) to PM were also determined and possible emission sources were identified. Assessment of health risk to PM exposure and associated compounds was realized. Results showed a decrease in levels of PM₁₀ in each area along the period studied, especially in the industrial area. Decreases in PM<sub>2.5</sub> levels were also observed in urban and residential areas over the years, although the trend is not as marked as with PM₁₀ levels. Then, PM<sub>2.5</sub> levels in the industrial area have remained practically constant. The 89% of both PM₁₀ and PM<sub>2.5</sub> annual mean exceeds the WHO reference values. The presence of most of the 16 US EPA priority PAHs studied was found with a detection frequency greater than 60% and it was possible to identify the importance of the contributions of vehicular emissions as predominant sources of PAH emission. From the calculations of the risk of contracting cancer throughout life (LCR), in the case of adults, the US EPA limits were not complied in the industrial and urban areas and in both fractions of PM. From the evaluation of the burden of disease (EBD), the calculated relative risks of mortality were very similar for the studied districts, being the relative risk in La Plata slightly lower, about 3-5%, than those in Berisso and Ensenada.
Facultad de Ciencias Exactas
Centro de Investigaciones del Medioambiente
Centro de Investigación y Desarrollo en Ciencias Aplicadas
description Levels of suspended particulate matter (PM) of both fractions PM₁₀ and PM<sub>2.5</sub> in ambient air were monitored in three areas of Gran La Plata: industrial, urban, and residential (2017-2019). Associated polycyclic aromatic hydrocarbons (PAHs) and nitropolycyclic aromatic hydrocarbons (NPAHs) to PM were also determined and possible emission sources were identified. Assessment of health risk to PM exposure and associated compounds was realized. Results showed a decrease in levels of PM₁₀ in each area along the period studied, especially in the industrial area. Decreases in PM<sub>2.5</sub> levels were also observed in urban and residential areas over the years, although the trend is not as marked as with PM₁₀ levels. Then, PM<sub>2.5</sub> levels in the industrial area have remained practically constant. The 89% of both PM₁₀ and PM<sub>2.5</sub> annual mean exceeds the WHO reference values. The presence of most of the 16 US EPA priority PAHs studied was found with a detection frequency greater than 60% and it was possible to identify the importance of the contributions of vehicular emissions as predominant sources of PAH emission. From the calculations of the risk of contracting cancer throughout life (LCR), in the case of adults, the US EPA limits were not complied in the industrial and urban areas and in both fractions of PM. From the evaluation of the burden of disease (EBD), the calculated relative risks of mortality were very similar for the studied districts, being the relative risk in La Plata slightly lower, about 3-5%, than those in Berisso and Ensenada.
publishDate 2021
dc.date.none.fl_str_mv 2021-07
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
Articulo
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://sedici.unlp.edu.ar/handle/10915/130464
url http://sedici.unlp.edu.ar/handle/10915/130464
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/issn/1614-7499
info:eu-repo/semantics/altIdentifier/issn/0944-1344
info:eu-repo/semantics/altIdentifier/doi/10.1007/s11356-021-13138-8
info:eu-repo/semantics/altIdentifier/pmid/33666842
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
http://creativecommons.org/licenses/by-nc-sa/4.0/
Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International (CC BY-NC-SA 4.0)
eu_rights_str_mv openAccess
rights_invalid_str_mv http://creativecommons.org/licenses/by-nc-sa/4.0/
Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International (CC BY-NC-SA 4.0)
dc.format.none.fl_str_mv application/pdf
35226-35241
dc.source.none.fl_str_mv reponame:SEDICI (UNLP)
instname:Universidad Nacional de La Plata
instacron:UNLP
reponame_str SEDICI (UNLP)
collection SEDICI (UNLP)
instname_str Universidad Nacional de La Plata
instacron_str UNLP
institution UNLP
repository.name.fl_str_mv SEDICI (UNLP) - Universidad Nacional de La Plata
repository.mail.fl_str_mv alira@sedici.unlp.edu.ar
_version_ 1844616203973165056
score 13.070432