Dynamic response of an irreversible reaction system to a pulsed perturbation

Autores
Albano, Ezequiel Vicente
Año de publicación
1999
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
The dynamic response of the ZGB surface reaction lattice gas model, for the catalyzed reaction, is studied by means of Monte-Carlo simulations in the neighborhood of its second order irreversible phase transition (IPT). It is found that shortly after driving a stationary configuration into the absorbing state, the relaxation of the system can be well described by a stretched exponential behavior. The dependence of the relaxation characteristic time and the induced changes on the coverage of the reactants, on both, the intensity and the period of the pulsed perturbation, are systematically investigated. The obtained insights can straightforwardly be extended to a wide variety of irreversible systems exhibiting second order IPT's, such as directed percolation, forest fire models, the contact process, branching annihilating walkers, catalyzed reactions, etc.
Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas
Materia
Física
Química
ZGB
IPT
Nivel de accesibilidad
acceso abierto
Condiciones de uso
http://creativecommons.org/licenses/by/4.0/
Repositorio
SEDICI (UNLP)
Institución
Universidad Nacional de La Plata
OAI Identificador
oai:sedici.unlp.edu.ar:10915/134087
Acceder
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oai_identifier_str oai:sedici.unlp.edu.ar:10915/134087
network_acronym_str SEDICI
repository_id_str 1329
network_name_str SEDICI (UNLP)
spelling Dynamic response of an irreversible reaction system to a pulsed perturbationAlbano, Ezequiel VicenteFísicaQuímicaZGBIPTThe dynamic response of the ZGB surface reaction lattice gas model, for the catalyzed reaction, is studied by means of Monte-Carlo simulations in the neighborhood of its second order irreversible phase transition (IPT). It is found that shortly after driving a stationary configuration into the absorbing state, the relaxation of the system can be well described by a stretched exponential behavior. The dependence of the relaxation characteristic time and the induced changes on the coverage of the reactants, on both, the intensity and the period of the pulsed perturbation, are systematically investigated. The obtained insights can straightforwardly be extended to a wide variety of irreversible systems exhibiting second order IPT's, such as directed percolation, forest fire models, the contact process, branching annihilating walkers, catalyzed reactions, etc.Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas1999info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionArticulohttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdf685-690http://sedici.unlp.edu.ar/handle/10915/134087enginfo:eu-repo/semantics/altIdentifier/issn/1434-6028info:eu-repo/semantics/altIdentifier/issn/1434-6036info:eu-repo/semantics/altIdentifier/doi/10.1007/s100510050813info:eu-repo/semantics/openAccesshttp://creativecommons.org/licenses/by/4.0/Creative Commons Attribution 4.0 International (CC BY 4.0)reponame:SEDICI (UNLP)instname:Universidad Nacional de La Platainstacron:UNLP2025-10-22T17:12:46Zoai:sedici.unlp.edu.ar:10915/134087Institucionalhttp://sedici.unlp.edu.ar/Universidad públicaNo correspondehttp://sedici.unlp.edu.ar/oai/snrdalira@sedici.unlp.edu.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:13292025-10-22 17:12:46.543SEDICI (UNLP) - Universidad Nacional de La Platafalse
dc.title.none.fl_str_mv Dynamic response of an irreversible reaction system to a pulsed perturbation
title Dynamic response of an irreversible reaction system to a pulsed perturbation
spellingShingle Dynamic response of an irreversible reaction system to a pulsed perturbation
Albano, Ezequiel Vicente
Física
Química
ZGB
IPT
title_short Dynamic response of an irreversible reaction system to a pulsed perturbation
title_full Dynamic response of an irreversible reaction system to a pulsed perturbation
title_fullStr Dynamic response of an irreversible reaction system to a pulsed perturbation
title_full_unstemmed Dynamic response of an irreversible reaction system to a pulsed perturbation
title_sort Dynamic response of an irreversible reaction system to a pulsed perturbation
dc.creator.none.fl_str_mv Albano, Ezequiel Vicente
author Albano, Ezequiel Vicente
author_facet Albano, Ezequiel Vicente
author_role author
dc.subject.none.fl_str_mv Física
Química
ZGB
IPT
topic Física
Química
ZGB
IPT
dc.description.none.fl_txt_mv The dynamic response of the ZGB surface reaction lattice gas model, for the catalyzed reaction, is studied by means of Monte-Carlo simulations in the neighborhood of its second order irreversible phase transition (IPT). It is found that shortly after driving a stationary configuration into the absorbing state, the relaxation of the system can be well described by a stretched exponential behavior. The dependence of the relaxation characteristic time and the induced changes on the coverage of the reactants, on both, the intensity and the period of the pulsed perturbation, are systematically investigated. The obtained insights can straightforwardly be extended to a wide variety of irreversible systems exhibiting second order IPT's, such as directed percolation, forest fire models, the contact process, branching annihilating walkers, catalyzed reactions, etc.
Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas
description The dynamic response of the ZGB surface reaction lattice gas model, for the catalyzed reaction, is studied by means of Monte-Carlo simulations in the neighborhood of its second order irreversible phase transition (IPT). It is found that shortly after driving a stationary configuration into the absorbing state, the relaxation of the system can be well described by a stretched exponential behavior. The dependence of the relaxation characteristic time and the induced changes on the coverage of the reactants, on both, the intensity and the period of the pulsed perturbation, are systematically investigated. The obtained insights can straightforwardly be extended to a wide variety of irreversible systems exhibiting second order IPT's, such as directed percolation, forest fire models, the contact process, branching annihilating walkers, catalyzed reactions, etc.
publishDate 1999
dc.date.none.fl_str_mv 1999
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
Articulo
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://sedici.unlp.edu.ar/handle/10915/134087
url http://sedici.unlp.edu.ar/handle/10915/134087
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/issn/1434-6028
info:eu-repo/semantics/altIdentifier/issn/1434-6036
info:eu-repo/semantics/altIdentifier/doi/10.1007/s100510050813
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
http://creativecommons.org/licenses/by/4.0/
Creative Commons Attribution 4.0 International (CC BY 4.0)
eu_rights_str_mv openAccess
rights_invalid_str_mv http://creativecommons.org/licenses/by/4.0/
Creative Commons Attribution 4.0 International (CC BY 4.0)
dc.format.none.fl_str_mv application/pdf
685-690
dc.source.none.fl_str_mv reponame:SEDICI (UNLP)
instname:Universidad Nacional de La Plata
instacron:UNLP
reponame_str SEDICI (UNLP)
collection SEDICI (UNLP)
instname_str Universidad Nacional de La Plata
instacron_str UNLP
institution UNLP
repository.name.fl_str_mv SEDICI (UNLP) - Universidad Nacional de La Plata
repository.mail.fl_str_mv alira@sedici.unlp.edu.ar
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score 12.982451

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