Dynamic response of an irreversible reaction system to a pulsed perturbation
- Autores
- Albano, Ezequiel Vicente
- Año de publicación
- 1999
- Idioma
- inglés
- Tipo de recurso
- artículo
- Estado
- versión publicada
- Descripción
- The dynamic response of the ZGB surface reaction lattice gas model, for the catalyzed reaction, is studied by means of Monte-Carlo simulations in the neighborhood of its second order irreversible phase transition (IPT). It is found that shortly after driving a stationary configuration into the absorbing state, the relaxation of the system can be well described by a stretched exponential behavior. The dependence of the relaxation characteristic time and the induced changes on the coverage of the reactants, on both, the intensity and the period of the pulsed perturbation, are systematically investigated. The obtained insights can straightforwardly be extended to a wide variety of irreversible systems exhibiting second order IPT's, such as directed percolation, forest fire models, the contact process, branching annihilating walkers, catalyzed reactions, etc.
Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas - Materia
-
Física
Química
ZGB
IPT - Nivel de accesibilidad
- acceso abierto
- Condiciones de uso
- http://creativecommons.org/licenses/by/4.0/
- Repositorio
- Institución
- Universidad Nacional de La Plata
- OAI Identificador
- oai:sedici.unlp.edu.ar:10915/134087
Ver los metadatos del registro completo
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Dynamic response of an irreversible reaction system to a pulsed perturbationAlbano, Ezequiel VicenteFísicaQuímicaZGBIPTThe dynamic response of the ZGB surface reaction lattice gas model, for the catalyzed reaction, is studied by means of Monte-Carlo simulations in the neighborhood of its second order irreversible phase transition (IPT). It is found that shortly after driving a stationary configuration into the absorbing state, the relaxation of the system can be well described by a stretched exponential behavior. The dependence of the relaxation characteristic time and the induced changes on the coverage of the reactants, on both, the intensity and the period of the pulsed perturbation, are systematically investigated. The obtained insights can straightforwardly be extended to a wide variety of irreversible systems exhibiting second order IPT's, such as directed percolation, forest fire models, the contact process, branching annihilating walkers, catalyzed reactions, etc.Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas1999info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionArticulohttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdf685-690http://sedici.unlp.edu.ar/handle/10915/134087enginfo:eu-repo/semantics/altIdentifier/issn/1434-6028info:eu-repo/semantics/altIdentifier/issn/1434-6036info:eu-repo/semantics/altIdentifier/doi/10.1007/s100510050813info:eu-repo/semantics/openAccesshttp://creativecommons.org/licenses/by/4.0/Creative Commons Attribution 4.0 International (CC BY 4.0)reponame:SEDICI (UNLP)instname:Universidad Nacional de La Platainstacron:UNLP2025-09-29T11:31:48Zoai:sedici.unlp.edu.ar:10915/134087Institucionalhttp://sedici.unlp.edu.ar/Universidad públicaNo correspondehttp://sedici.unlp.edu.ar/oai/snrdalira@sedici.unlp.edu.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:13292025-09-29 11:31:48.44SEDICI (UNLP) - Universidad Nacional de La Platafalse |
dc.title.none.fl_str_mv |
Dynamic response of an irreversible reaction system to a pulsed perturbation |
title |
Dynamic response of an irreversible reaction system to a pulsed perturbation |
spellingShingle |
Dynamic response of an irreversible reaction system to a pulsed perturbation Albano, Ezequiel Vicente Física Química ZGB IPT |
title_short |
Dynamic response of an irreversible reaction system to a pulsed perturbation |
title_full |
Dynamic response of an irreversible reaction system to a pulsed perturbation |
title_fullStr |
Dynamic response of an irreversible reaction system to a pulsed perturbation |
title_full_unstemmed |
Dynamic response of an irreversible reaction system to a pulsed perturbation |
title_sort |
Dynamic response of an irreversible reaction system to a pulsed perturbation |
dc.creator.none.fl_str_mv |
Albano, Ezequiel Vicente |
author |
Albano, Ezequiel Vicente |
author_facet |
Albano, Ezequiel Vicente |
author_role |
author |
dc.subject.none.fl_str_mv |
Física Química ZGB IPT |
topic |
Física Química ZGB IPT |
dc.description.none.fl_txt_mv |
The dynamic response of the ZGB surface reaction lattice gas model, for the catalyzed reaction, is studied by means of Monte-Carlo simulations in the neighborhood of its second order irreversible phase transition (IPT). It is found that shortly after driving a stationary configuration into the absorbing state, the relaxation of the system can be well described by a stretched exponential behavior. The dependence of the relaxation characteristic time and the induced changes on the coverage of the reactants, on both, the intensity and the period of the pulsed perturbation, are systematically investigated. The obtained insights can straightforwardly be extended to a wide variety of irreversible systems exhibiting second order IPT's, such as directed percolation, forest fire models, the contact process, branching annihilating walkers, catalyzed reactions, etc. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas |
description |
The dynamic response of the ZGB surface reaction lattice gas model, for the catalyzed reaction, is studied by means of Monte-Carlo simulations in the neighborhood of its second order irreversible phase transition (IPT). It is found that shortly after driving a stationary configuration into the absorbing state, the relaxation of the system can be well described by a stretched exponential behavior. The dependence of the relaxation characteristic time and the induced changes on the coverage of the reactants, on both, the intensity and the period of the pulsed perturbation, are systematically investigated. The obtained insights can straightforwardly be extended to a wide variety of irreversible systems exhibiting second order IPT's, such as directed percolation, forest fire models, the contact process, branching annihilating walkers, catalyzed reactions, etc. |
publishDate |
1999 |
dc.date.none.fl_str_mv |
1999 |
dc.type.none.fl_str_mv |
info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion Articulo http://purl.org/coar/resource_type/c_6501 info:ar-repo/semantics/articulo |
format |
article |
status_str |
publishedVersion |
dc.identifier.none.fl_str_mv |
http://sedici.unlp.edu.ar/handle/10915/134087 |
url |
http://sedici.unlp.edu.ar/handle/10915/134087 |
dc.language.none.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
info:eu-repo/semantics/altIdentifier/issn/1434-6028 info:eu-repo/semantics/altIdentifier/issn/1434-6036 info:eu-repo/semantics/altIdentifier/doi/10.1007/s100510050813 |
dc.rights.none.fl_str_mv |
info:eu-repo/semantics/openAccess http://creativecommons.org/licenses/by/4.0/ Creative Commons Attribution 4.0 International (CC BY 4.0) |
eu_rights_str_mv |
openAccess |
rights_invalid_str_mv |
http://creativecommons.org/licenses/by/4.0/ Creative Commons Attribution 4.0 International (CC BY 4.0) |
dc.format.none.fl_str_mv |
application/pdf 685-690 |
dc.source.none.fl_str_mv |
reponame:SEDICI (UNLP) instname:Universidad Nacional de La Plata instacron:UNLP |
reponame_str |
SEDICI (UNLP) |
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SEDICI (UNLP) |
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Universidad Nacional de La Plata |
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UNLP |
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UNLP |
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SEDICI (UNLP) - Universidad Nacional de La Plata |
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13.070432 |