Ion implantation in nanodiamonds: Size effect and energy dependence

Autores
Shiryaev, Andrey A.; Hinks, Jonathan A.; Marks, Nigel A.; Greaves, Graeme; Valencia, Felipe J.; Donnelly, Stephen E.; González, Rafael I.; Kiwi, Miguel; Trigub, Alexander L.; Bringa, Eduardo Marcial; Fogg, Jason L.; Vlasov, Igor I.
Año de publicación
2018
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
Nanoparticles are ubiquitous in nature and are increasingly important for technology. They are subject to bombardment by ionizing radiation in a diverse range of environments. In particular, nanodiamonds represent a variety of nanoparticles of significant fundamental and applied interest. Here we present a combined experimental and computational study of the behaviour of nanodiamonds under irradiation by xenon ions. Unexpectedly, we observed a pronounced size effect on the radiation resistance of the nanodiamonds: particles larger than 8 nm behave similarly to macroscopic diamond (i.e. characterized by high radiation resistance) whereas smaller particles can be completely destroyed by a single impact from an ion in a defined energy range. This latter observation is explained by extreme heating of the nanodiamonds by the penetrating ion. The obtained results are not limited to nanodiamonds, making them of interest for several fields, putting constraints on processes for the controlled modification of nanodiamonds, on the survival of dust in astrophysical environments, and on the behaviour of actinides released from nuclear waste into the environment.
Fil: Shiryaev, Andrey A.. Moscow State University; Rusia. Frumkin Institute of Physical Chemistry and Electrochemistry Ram; Rusia
Fil: Hinks, Jonathan A.. University of Huddersfeld; Reino Unido
Fil: Marks, Nigel A.. Curtin University; Australia
Fil: Greaves, Graeme. University of Huddersfeld; Reino Unido
Fil: Valencia, Felipe J.. Centro Para El Desarrollo de la Nanociencia y Nanotecnología; Chile. Universidad de Chile; Chile. Universidad Mayor; Chile
Fil: Donnelly, Stephen E.. University of Huddersfeld; Reino Unido
Fil: González, Rafael I.. Universidad Mayor; Chile. Centro Para El Desarrollo de la Nanociencia y Nanotecnología; Chile
Fil: Kiwi, Miguel. Universidad de Chile; Chile. Centro Para El Desarrollo de la Nanociencia y Nanotecnología; Chile
Fil: Trigub, Alexander L.. Instituto Kurchátov; Rusia
Fil: Bringa, Eduardo Marcial. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Mendoza; Argentina. Universidad Nacional de Cuyo. Facultad de Ciencias Exactas y Naturales; Argentina
Fil: Fogg, Jason L.. Curtin University; Australia
Fil: Vlasov, Igor I.. National Research Nuclear University; Rusia
Materia
DIAMOND
IRRADIATION
SIMULATION
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/100431
Acceder
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network_name_str CONICET Digital (CONICET)
spelling Ion implantation in nanodiamonds: Size effect and energy dependenceShiryaev, Andrey A.Hinks, Jonathan A.Marks, Nigel A.Greaves, GraemeValencia, Felipe J.Donnelly, Stephen E.González, Rafael I.Kiwi, MiguelTrigub, Alexander L.Bringa, Eduardo MarcialFogg, Jason L.Vlasov, Igor I.DIAMONDIRRADIATIONSIMULATIONhttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1Nanoparticles are ubiquitous in nature and are increasingly important for technology. They are subject to bombardment by ionizing radiation in a diverse range of environments. In particular, nanodiamonds represent a variety of nanoparticles of significant fundamental and applied interest. Here we present a combined experimental and computational study of the behaviour of nanodiamonds under irradiation by xenon ions. Unexpectedly, we observed a pronounced size effect on the radiation resistance of the nanodiamonds: particles larger than 8 nm behave similarly to macroscopic diamond (i.e. characterized by high radiation resistance) whereas smaller particles can be completely destroyed by a single impact from an ion in a defined energy range. This latter observation is explained by extreme heating of the nanodiamonds by the penetrating ion. The obtained results are not limited to nanodiamonds, making them of interest for several fields, putting constraints on processes for the controlled modification of nanodiamonds, on the survival of dust in astrophysical environments, and on the behaviour of actinides released from nuclear waste into the environment.Fil: Shiryaev, Andrey A.. Moscow State University; Rusia. Frumkin Institute of Physical Chemistry and Electrochemistry Ram; RusiaFil: Hinks, Jonathan A.. University of Huddersfeld; Reino UnidoFil: Marks, Nigel A.. Curtin University; AustraliaFil: Greaves, Graeme. University of Huddersfeld; Reino UnidoFil: Valencia, Felipe J.. Centro Para El Desarrollo de la Nanociencia y Nanotecnología; Chile. Universidad de Chile; Chile. Universidad Mayor; ChileFil: Donnelly, Stephen E.. University of Huddersfeld; Reino UnidoFil: González, Rafael I.. Universidad Mayor; Chile. Centro Para El Desarrollo de la Nanociencia y Nanotecnología; ChileFil: Kiwi, Miguel. Universidad de Chile; Chile. Centro Para El Desarrollo de la Nanociencia y Nanotecnología; ChileFil: Trigub, Alexander L.. Instituto Kurchátov; RusiaFil: Bringa, Eduardo Marcial. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Mendoza; Argentina. Universidad Nacional de Cuyo. Facultad de Ciencias Exactas y Naturales; ArgentinaFil: Fogg, Jason L.. Curtin University; AustraliaFil: Vlasov, Igor I.. National Research Nuclear University; RusiaNature Publishing Group2018-12info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/100431Shiryaev, Andrey A.; Hinks, Jonathan A.; Marks, Nigel A.; Greaves, Graeme; Valencia, Felipe J.; et al.; Ion implantation in nanodiamonds: Size effect and energy dependence; Nature Publishing Group; Scientific Reports; 8; 1; 12-2018; 1-92045-2322CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/doi/10.1038/s41598-018-23434-yinfo:eu-repo/semantics/altIdentifier/url/https://www.nature.com/articles/s41598-018-23434-yinfo:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T09:48:06Zoai:ri.conicet.gov.ar:11336/100431instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 09:48:06.455CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Ion implantation in nanodiamonds: Size effect and energy dependence
title Ion implantation in nanodiamonds: Size effect and energy dependence
spellingShingle Ion implantation in nanodiamonds: Size effect and energy dependence
Shiryaev, Andrey A.
DIAMOND
IRRADIATION
SIMULATION
title_short Ion implantation in nanodiamonds: Size effect and energy dependence
title_full Ion implantation in nanodiamonds: Size effect and energy dependence
title_fullStr Ion implantation in nanodiamonds: Size effect and energy dependence
title_full_unstemmed Ion implantation in nanodiamonds: Size effect and energy dependence
title_sort Ion implantation in nanodiamonds: Size effect and energy dependence
dc.creator.none.fl_str_mv Shiryaev, Andrey A.
Hinks, Jonathan A.
Marks, Nigel A.
Greaves, Graeme
Valencia, Felipe J.
Donnelly, Stephen E.
González, Rafael I.
Kiwi, Miguel
Trigub, Alexander L.
Bringa, Eduardo Marcial
Fogg, Jason L.
Vlasov, Igor I.
author Shiryaev, Andrey A.
author_facet Shiryaev, Andrey A.
Hinks, Jonathan A.
Marks, Nigel A.
Greaves, Graeme
Valencia, Felipe J.
Donnelly, Stephen E.
González, Rafael I.
Kiwi, Miguel
Trigub, Alexander L.
Bringa, Eduardo Marcial
Fogg, Jason L.
Vlasov, Igor I.
author_role author
author2 Hinks, Jonathan A.
Marks, Nigel A.
Greaves, Graeme
Valencia, Felipe J.
Donnelly, Stephen E.
González, Rafael I.
Kiwi, Miguel
Trigub, Alexander L.
Bringa, Eduardo Marcial
Fogg, Jason L.
Vlasov, Igor I.
author2_role author
author
author
author
author
author
author
author
author
author
author
dc.subject.none.fl_str_mv DIAMOND
IRRADIATION
SIMULATION
topic DIAMOND
IRRADIATION
SIMULATION
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv Nanoparticles are ubiquitous in nature and are increasingly important for technology. They are subject to bombardment by ionizing radiation in a diverse range of environments. In particular, nanodiamonds represent a variety of nanoparticles of significant fundamental and applied interest. Here we present a combined experimental and computational study of the behaviour of nanodiamonds under irradiation by xenon ions. Unexpectedly, we observed a pronounced size effect on the radiation resistance of the nanodiamonds: particles larger than 8 nm behave similarly to macroscopic diamond (i.e. characterized by high radiation resistance) whereas smaller particles can be completely destroyed by a single impact from an ion in a defined energy range. This latter observation is explained by extreme heating of the nanodiamonds by the penetrating ion. The obtained results are not limited to nanodiamonds, making them of interest for several fields, putting constraints on processes for the controlled modification of nanodiamonds, on the survival of dust in astrophysical environments, and on the behaviour of actinides released from nuclear waste into the environment.
Fil: Shiryaev, Andrey A.. Moscow State University; Rusia. Frumkin Institute of Physical Chemistry and Electrochemistry Ram; Rusia
Fil: Hinks, Jonathan A.. University of Huddersfeld; Reino Unido
Fil: Marks, Nigel A.. Curtin University; Australia
Fil: Greaves, Graeme. University of Huddersfeld; Reino Unido
Fil: Valencia, Felipe J.. Centro Para El Desarrollo de la Nanociencia y Nanotecnología; Chile. Universidad de Chile; Chile. Universidad Mayor; Chile
Fil: Donnelly, Stephen E.. University of Huddersfeld; Reino Unido
Fil: González, Rafael I.. Universidad Mayor; Chile. Centro Para El Desarrollo de la Nanociencia y Nanotecnología; Chile
Fil: Kiwi, Miguel. Universidad de Chile; Chile. Centro Para El Desarrollo de la Nanociencia y Nanotecnología; Chile
Fil: Trigub, Alexander L.. Instituto Kurchátov; Rusia
Fil: Bringa, Eduardo Marcial. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Mendoza; Argentina. Universidad Nacional de Cuyo. Facultad de Ciencias Exactas y Naturales; Argentina
Fil: Fogg, Jason L.. Curtin University; Australia
Fil: Vlasov, Igor I.. National Research Nuclear University; Rusia
description Nanoparticles are ubiquitous in nature and are increasingly important for technology. They are subject to bombardment by ionizing radiation in a diverse range of environments. In particular, nanodiamonds represent a variety of nanoparticles of significant fundamental and applied interest. Here we present a combined experimental and computational study of the behaviour of nanodiamonds under irradiation by xenon ions. Unexpectedly, we observed a pronounced size effect on the radiation resistance of the nanodiamonds: particles larger than 8 nm behave similarly to macroscopic diamond (i.e. characterized by high radiation resistance) whereas smaller particles can be completely destroyed by a single impact from an ion in a defined energy range. This latter observation is explained by extreme heating of the nanodiamonds by the penetrating ion. The obtained results are not limited to nanodiamonds, making them of interest for several fields, putting constraints on processes for the controlled modification of nanodiamonds, on the survival of dust in astrophysical environments, and on the behaviour of actinides released from nuclear waste into the environment.
publishDate 2018
dc.date.none.fl_str_mv 2018-12
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/100431
Shiryaev, Andrey A.; Hinks, Jonathan A.; Marks, Nigel A.; Greaves, Graeme; Valencia, Felipe J.; et al.; Ion implantation in nanodiamonds: Size effect and energy dependence; Nature Publishing Group; Scientific Reports; 8; 1; 12-2018; 1-9
2045-2322
CONICET Digital
CONICET
url http://hdl.handle.net/11336/100431
identifier_str_mv Shiryaev, Andrey A.; Hinks, Jonathan A.; Marks, Nigel A.; Greaves, Graeme; Valencia, Felipe J.; et al.; Ion implantation in nanodiamonds: Size effect and energy dependence; Nature Publishing Group; Scientific Reports; 8; 1; 12-2018; 1-9
2045-2322
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/doi/10.1038/s41598-018-23434-y
info:eu-repo/semantics/altIdentifier/url/https://www.nature.com/articles/s41598-018-23434-y
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv Nature Publishing Group
publisher.none.fl_str_mv Nature Publishing Group
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 13.070432

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