ODTMA+ and HDTMA+ organo-montmorillonites characterization: New insight byWAXS, SAXS and surface charge
- Autores
- Bianchi, Ana Elisa; Fernandez, Mariela Alejandra; Pantanetti, Mariano; Viña, Raul Oscar; Torriani, I.; Torres Sanchez, Rosa Maria; Punte, Graciela Maria
- Año de publicación
- 2013
- Idioma
- inglés
- Tipo de recurso
- artículo
- Estado
- versión publicada
- Descripción
- In this work we investigate the microstructure and properties of organo-montmorillonites (OMts) synthesized by intercalation of a Patagonian Mt with different surfactant/CEC ratios (0.5, 1 and 2) of octadecyl trimethylammonium (ODTMA+) and hexadecyl trimethylammonium (HDTMA+) cations. X-ray diffraction (XRD) patterns showed that
in all OMt samples d001 value increases with respect to raw Mt (1.258 nm). Small angle andwide angle X-ray scattering (SAXS andWAXS) curves, particle apparent diameters (determined by laser), zeta potential values and scanning electron microscopy (SEM) images, showed the presence of assorted d001 values (which depend on storage conditions), aggregate formation and charge reversal (which varied with loading and cation length) for samples obtained with 1 and 2 CEC. However, for samples intercalatedwith 0.5 CEC, we found evidence of smaller aggregate formation, no charge reversal, and similar d001 and zeta potential values (both higher than those of Mt). Findings reported here will help attain better conditions to functionalize highly charged Mt making them suitable to be used as nanocomposite precursors for different applications.
Fil: Bianchi, Ana Elisa. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Instituto de Física la Plata; Argentina. Universidad Nacional de La Plata. Facultad de Ingenieria; Argentina
Fil: Fernandez, Mariela Alejandra. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Centro Tecnológico de Recursos Minerales y Cerámica (i); Argentina. Universidad Nacional de La Plata. Facultad de Ingenieria; Argentina
Fil: Pantanetti, Mariano. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Centro Tecnológico de Recursos Minerales y Cerámica (i); Argentina
Fil: Viña, Raul Oscar. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Instituto de Física la Plata; Argentina
Fil: Torriani, I.. Universidade Estadual de Campinas. Departamento de Física da Matéria Condensada; Brasil
Fil: Torres Sanchez, Rosa Maria. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Centro Tecnológico de Recursos Minerales y Cerámica (i); Argentina
Fil: Punte, Graciela Maria. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Instituto de Física la Plata; Argentina - Materia
-
Montmorillonite
Organo-Montmorillonite
Saxs
Zeta Potential - Nivel de accesibilidad
- acceso abierto
- Condiciones de uso
- https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
- Repositorio
- Institución
- Consejo Nacional de Investigaciones Científicas y Técnicas
- OAI Identificador
- oai:ri.conicet.gov.ar:11336/5287
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ODTMA+ and HDTMA+ organo-montmorillonites characterization: New insight byWAXS, SAXS and surface chargeBianchi, Ana ElisaFernandez, Mariela AlejandraPantanetti, MarianoViña, Raul OscarTorriani, I.Torres Sanchez, Rosa MariaPunte, Graciela MariaMontmorilloniteOrgano-MontmorilloniteSaxsZeta Potentialhttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1In this work we investigate the microstructure and properties of organo-montmorillonites (OMts) synthesized by intercalation of a Patagonian Mt with different surfactant/CEC ratios (0.5, 1 and 2) of octadecyl trimethylammonium (ODTMA+) and hexadecyl trimethylammonium (HDTMA+) cations. X-ray diffraction (XRD) patterns showed that<br />in all OMt samples d001 value increases with respect to raw Mt (1.258 nm). Small angle andwide angle X-ray scattering (SAXS andWAXS) curves, particle apparent diameters (determined by laser), zeta potential values and scanning electron microscopy (SEM) images, showed the presence of assorted d001 values (which depend on storage conditions), aggregate formation and charge reversal (which varied with loading and cation length) for samples obtained with 1 and 2 CEC. However, for samples intercalatedwith 0.5 CEC, we found evidence of smaller aggregate formation, no charge reversal, and similar d001 and zeta potential values (both higher than those of Mt). Findings reported here will help attain better conditions to functionalize highly charged Mt making them suitable to be used as nanocomposite precursors for different applications.<br />Fil: Bianchi, Ana Elisa. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Instituto de Física la Plata; Argentina. Universidad Nacional de La Plata. Facultad de Ingenieria; ArgentinaFil: Fernandez, Mariela Alejandra. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Centro Tecnológico de Recursos Minerales y Cerámica (i); Argentina. Universidad Nacional de La Plata. Facultad de Ingenieria; ArgentinaFil: Pantanetti, Mariano. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Centro Tecnológico de Recursos Minerales y Cerámica (i); ArgentinaFil: Viña, Raul Oscar. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Instituto de Física la Plata; ArgentinaFil: Torriani, I.. Universidade Estadual de Campinas. Departamento de Física da Matéria Condensada; BrasilFil: Torres Sanchez, Rosa Maria. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Centro Tecnológico de Recursos Minerales y Cerámica (i); ArgentinaFil: Punte, Graciela Maria. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Instituto de Física la Plata; ArgentinaElsevier2013-09info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/5287Bianchi, Ana Elisa; Fernandez, Mariela Alejandra; Pantanetti, Mariano; Viña, Raul Oscar; Torriani, I.; et al.; ODTMA+ and HDTMA+ organo-montmorillonites characterization: New insight byWAXS, SAXS and surface charge; Elsevier; Applied Clay Science; 83-84; 9-2013; 280–2850169-1317enginfo:eu-repo/semantics/altIdentifier/doi/info:eu-repo/semantics/altIdentifier/url/http://www.sciencedirect.com/science/article/pii/S0169131713002779?np=yinfo:eu-repo/semantics/altIdentifier/doi/10.1016/j.clay.2013.08.032info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-nd/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T09:36:41Zoai:ri.conicet.gov.ar:11336/5287instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 09:36:42.184CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse |
dc.title.none.fl_str_mv |
ODTMA+ and HDTMA+ organo-montmorillonites characterization: New insight byWAXS, SAXS and surface charge |
title |
ODTMA+ and HDTMA+ organo-montmorillonites characterization: New insight byWAXS, SAXS and surface charge |
spellingShingle |
ODTMA+ and HDTMA+ organo-montmorillonites characterization: New insight byWAXS, SAXS and surface charge Bianchi, Ana Elisa Montmorillonite Organo-Montmorillonite Saxs Zeta Potential |
title_short |
ODTMA+ and HDTMA+ organo-montmorillonites characterization: New insight byWAXS, SAXS and surface charge |
title_full |
ODTMA+ and HDTMA+ organo-montmorillonites characterization: New insight byWAXS, SAXS and surface charge |
title_fullStr |
ODTMA+ and HDTMA+ organo-montmorillonites characterization: New insight byWAXS, SAXS and surface charge |
title_full_unstemmed |
ODTMA+ and HDTMA+ organo-montmorillonites characterization: New insight byWAXS, SAXS and surface charge |
title_sort |
ODTMA+ and HDTMA+ organo-montmorillonites characterization: New insight byWAXS, SAXS and surface charge |
dc.creator.none.fl_str_mv |
Bianchi, Ana Elisa Fernandez, Mariela Alejandra Pantanetti, Mariano Viña, Raul Oscar Torriani, I. Torres Sanchez, Rosa Maria Punte, Graciela Maria |
author |
Bianchi, Ana Elisa |
author_facet |
Bianchi, Ana Elisa Fernandez, Mariela Alejandra Pantanetti, Mariano Viña, Raul Oscar Torriani, I. Torres Sanchez, Rosa Maria Punte, Graciela Maria |
author_role |
author |
author2 |
Fernandez, Mariela Alejandra Pantanetti, Mariano Viña, Raul Oscar Torriani, I. Torres Sanchez, Rosa Maria Punte, Graciela Maria |
author2_role |
author author author author author author |
dc.subject.none.fl_str_mv |
Montmorillonite Organo-Montmorillonite Saxs Zeta Potential |
topic |
Montmorillonite Organo-Montmorillonite Saxs Zeta Potential |
purl_subject.fl_str_mv |
https://purl.org/becyt/ford/1.3 https://purl.org/becyt/ford/1 |
dc.description.none.fl_txt_mv |
In this work we investigate the microstructure and properties of organo-montmorillonites (OMts) synthesized by intercalation of a Patagonian Mt with different surfactant/CEC ratios (0.5, 1 and 2) of octadecyl trimethylammonium (ODTMA+) and hexadecyl trimethylammonium (HDTMA+) cations. X-ray diffraction (XRD) patterns showed that<br />in all OMt samples d001 value increases with respect to raw Mt (1.258 nm). Small angle andwide angle X-ray scattering (SAXS andWAXS) curves, particle apparent diameters (determined by laser), zeta potential values and scanning electron microscopy (SEM) images, showed the presence of assorted d001 values (which depend on storage conditions), aggregate formation and charge reversal (which varied with loading and cation length) for samples obtained with 1 and 2 CEC. However, for samples intercalatedwith 0.5 CEC, we found evidence of smaller aggregate formation, no charge reversal, and similar d001 and zeta potential values (both higher than those of Mt). Findings reported here will help attain better conditions to functionalize highly charged Mt making them suitable to be used as nanocomposite precursors for different applications.<br /> Fil: Bianchi, Ana Elisa. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Instituto de Física la Plata; Argentina. Universidad Nacional de La Plata. Facultad de Ingenieria; Argentina Fil: Fernandez, Mariela Alejandra. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Centro Tecnológico de Recursos Minerales y Cerámica (i); Argentina. Universidad Nacional de La Plata. Facultad de Ingenieria; Argentina Fil: Pantanetti, Mariano. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Centro Tecnológico de Recursos Minerales y Cerámica (i); Argentina Fil: Viña, Raul Oscar. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Instituto de Física la Plata; Argentina Fil: Torriani, I.. Universidade Estadual de Campinas. Departamento de Física da Matéria Condensada; Brasil Fil: Torres Sanchez, Rosa Maria. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Centro Tecnológico de Recursos Minerales y Cerámica (i); Argentina Fil: Punte, Graciela Maria. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Instituto de Física la Plata; Argentina |
description |
In this work we investigate the microstructure and properties of organo-montmorillonites (OMts) synthesized by intercalation of a Patagonian Mt with different surfactant/CEC ratios (0.5, 1 and 2) of octadecyl trimethylammonium (ODTMA+) and hexadecyl trimethylammonium (HDTMA+) cations. X-ray diffraction (XRD) patterns showed that<br />in all OMt samples d001 value increases with respect to raw Mt (1.258 nm). Small angle andwide angle X-ray scattering (SAXS andWAXS) curves, particle apparent diameters (determined by laser), zeta potential values and scanning electron microscopy (SEM) images, showed the presence of assorted d001 values (which depend on storage conditions), aggregate formation and charge reversal (which varied with loading and cation length) for samples obtained with 1 and 2 CEC. However, for samples intercalatedwith 0.5 CEC, we found evidence of smaller aggregate formation, no charge reversal, and similar d001 and zeta potential values (both higher than those of Mt). Findings reported here will help attain better conditions to functionalize highly charged Mt making them suitable to be used as nanocomposite precursors for different applications.<br /> |
publishDate |
2013 |
dc.date.none.fl_str_mv |
2013-09 |
dc.type.none.fl_str_mv |
info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion http://purl.org/coar/resource_type/c_6501 info:ar-repo/semantics/articulo |
format |
article |
status_str |
publishedVersion |
dc.identifier.none.fl_str_mv |
http://hdl.handle.net/11336/5287 Bianchi, Ana Elisa; Fernandez, Mariela Alejandra; Pantanetti, Mariano; Viña, Raul Oscar; Torriani, I.; et al.; ODTMA+ and HDTMA+ organo-montmorillonites characterization: New insight byWAXS, SAXS and surface charge; Elsevier; Applied Clay Science; 83-84; 9-2013; 280–285 0169-1317 |
url |
http://hdl.handle.net/11336/5287 |
identifier_str_mv |
Bianchi, Ana Elisa; Fernandez, Mariela Alejandra; Pantanetti, Mariano; Viña, Raul Oscar; Torriani, I.; et al.; ODTMA+ and HDTMA+ organo-montmorillonites characterization: New insight byWAXS, SAXS and surface charge; Elsevier; Applied Clay Science; 83-84; 9-2013; 280–285 0169-1317 |
dc.language.none.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
info:eu-repo/semantics/altIdentifier/doi/ info:eu-repo/semantics/altIdentifier/url/http://www.sciencedirect.com/science/article/pii/S0169131713002779?np=y info:eu-repo/semantics/altIdentifier/doi/10.1016/j.clay.2013.08.032 |
dc.rights.none.fl_str_mv |
info:eu-repo/semantics/openAccess https://creativecommons.org/licenses/by-nc-nd/2.5/ar/ |
eu_rights_str_mv |
openAccess |
rights_invalid_str_mv |
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/ |
dc.format.none.fl_str_mv |
application/pdf application/pdf application/pdf application/pdf |
dc.publisher.none.fl_str_mv |
Elsevier |
publisher.none.fl_str_mv |
Elsevier |
dc.source.none.fl_str_mv |
reponame:CONICET Digital (CONICET) instname:Consejo Nacional de Investigaciones Científicas y Técnicas |
reponame_str |
CONICET Digital (CONICET) |
collection |
CONICET Digital (CONICET) |
instname_str |
Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.name.fl_str_mv |
CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.mail.fl_str_mv |
dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar |
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1844613152794214400 |
score |
13.070432 |