Efficient ultrafast all-optical modulation in a nonlinear crystalline gallium phosphide nanodisk at the anapole excitation

Autores
Grinblat, Gustavo Sergio; Zhang, Haizhong; Nielsen, Michael P.; Krivitsky, Leonid; Berté, Rodrigo; Li, Yi; Tilmann, Benjamin; Cortés, Emiliano; Oulton, Rupert F.; Kuznetsov, Arseniy I.; Maier, Stefan A.
Año de publicación
2020
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
High-refractive index nanostructured dielectrics have the ability to locally enhance electromagnetic fields with low losses while presenting high third-order nonlinearities. In this work, we exploit these characteristics to achieve efficient ultrafast all-optical modulation in a crystalline gallium phosphide (GaP) nanoantenna through the optical Kerr effect (OKE) and two-photon absorption (TPA) in the visible/near-infrared range. We show that an individual GaP nanodisk can yield differential reflectivity modulations of up to -40%, with characteristic modulation times between 14 and 66 fs, when probed at the anapole excitation (AE). Numerical simulations reveal that the AE represents a unique condition where both the OKE and TPA contribute with the same modulation sign, maximizing the response. These findings highly outperform previous reports on sub-100-fs all-optical switching from resonant nanoscale dielectrics, which have demonstrated modulation depths no larger than 0.5%, placing GaP nanoantennas as a promising choice for ultrafast all-optical modulation at the nanometer scale.
Fil: Grinblat, Gustavo Sergio. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; Argentina
Fil: Zhang, Haizhong. Institute of Materials Research and Engineering; Singapur
Fil: Nielsen, Michael P.. University of New South Wales; Australia
Fil: Krivitsky, Leonid. Institute of Materials Research and Engineering; Singapur
Fil: Berté, Rodrigo. Ludwig Maximilians Universitat; Alemania
Fil: Li, Yi. Ludwig Maximilians Universitat; Alemania
Fil: Tilmann, Benjamin. Ludwig Maximilians Universitat; Alemania
Fil: Cortés, Emiliano. Ludwig Maximilians Universitat; Alemania
Fil: Oulton, Rupert F.. Imperial College London; Reino Unido
Fil: Kuznetsov, Arseniy I.. Institute of Materials Research and Engineering; Singapur
Fil: Maier, Stefan A.. Ludwig Maximilians Universitat; Alemania
Materia
Nanoantenas ópticas dieléctricas
Conmutación óptica
Efecto Kerr óptico
Absorción de dos fotones
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/146133
Acceder
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oai_identifier_str oai:ri.conicet.gov.ar:11336/146133
network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Efficient ultrafast all-optical modulation in a nonlinear crystalline gallium phosphide nanodisk at the anapole excitationGrinblat, Gustavo SergioZhang, HaizhongNielsen, Michael P.Krivitsky, LeonidBerté, RodrigoLi, YiTilmann, BenjaminCortés, EmilianoOulton, Rupert F.Kuznetsov, Arseniy I.Maier, Stefan A.Nanoantenas ópticas dieléctricasConmutación ópticaEfecto Kerr ópticoAbsorción de dos fotoneshttps://purl.org/becyt/ford/2.10https://purl.org/becyt/ford/2High-refractive index nanostructured dielectrics have the ability to locally enhance electromagnetic fields with low losses while presenting high third-order nonlinearities. In this work, we exploit these characteristics to achieve efficient ultrafast all-optical modulation in a crystalline gallium phosphide (GaP) nanoantenna through the optical Kerr effect (OKE) and two-photon absorption (TPA) in the visible/near-infrared range. We show that an individual GaP nanodisk can yield differential reflectivity modulations of up to -40%, with characteristic modulation times between 14 and 66 fs, when probed at the anapole excitation (AE). Numerical simulations reveal that the AE represents a unique condition where both the OKE and TPA contribute with the same modulation sign, maximizing the response. These findings highly outperform previous reports on sub-100-fs all-optical switching from resonant nanoscale dielectrics, which have demonstrated modulation depths no larger than 0.5%, placing GaP nanoantennas as a promising choice for ultrafast all-optical modulation at the nanometer scale.Fil: Grinblat, Gustavo Sergio. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; ArgentinaFil: Zhang, Haizhong. Institute of Materials Research and Engineering; SingapurFil: Nielsen, Michael P.. University of New South Wales; AustraliaFil: Krivitsky, Leonid. Institute of Materials Research and Engineering; SingapurFil: Berté, Rodrigo. Ludwig Maximilians Universitat; AlemaniaFil: Li, Yi. Ludwig Maximilians Universitat; AlemaniaFil: Tilmann, Benjamin. Ludwig Maximilians Universitat; AlemaniaFil: Cortés, Emiliano. Ludwig Maximilians Universitat; AlemaniaFil: Oulton, Rupert F.. Imperial College London; Reino UnidoFil: Kuznetsov, Arseniy I.. Institute of Materials Research and Engineering; SingapurFil: Maier, Stefan A.. Ludwig Maximilians Universitat; AlemaniaScience Advances is the American Association for the Advancement of Science2020-08info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/146133Grinblat, Gustavo Sergio; Zhang, Haizhong; Nielsen, Michael P.; Krivitsky, Leonid; Berté, Rodrigo; et al.; Efficient ultrafast all-optical modulation in a nonlinear crystalline gallium phosphide nanodisk at the anapole excitation; Science Advances is the American Association for the Advancement of Science; Science Advances; 6; 34; 8-2020; 1-72375-2548CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://advances.sciencemag.org/lookup/doi/10.1126/sciadv.abb3123info:eu-repo/semantics/altIdentifier/doi/10.1126/sciadv.abb3123info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T09:39:47Zoai:ri.conicet.gov.ar:11336/146133instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 09:39:48.059CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Efficient ultrafast all-optical modulation in a nonlinear crystalline gallium phosphide nanodisk at the anapole excitation
title Efficient ultrafast all-optical modulation in a nonlinear crystalline gallium phosphide nanodisk at the anapole excitation
spellingShingle Efficient ultrafast all-optical modulation in a nonlinear crystalline gallium phosphide nanodisk at the anapole excitation
Grinblat, Gustavo Sergio
Nanoantenas ópticas dieléctricas
Conmutación óptica
Efecto Kerr óptico
Absorción de dos fotones
title_short Efficient ultrafast all-optical modulation in a nonlinear crystalline gallium phosphide nanodisk at the anapole excitation
title_full Efficient ultrafast all-optical modulation in a nonlinear crystalline gallium phosphide nanodisk at the anapole excitation
title_fullStr Efficient ultrafast all-optical modulation in a nonlinear crystalline gallium phosphide nanodisk at the anapole excitation
title_full_unstemmed Efficient ultrafast all-optical modulation in a nonlinear crystalline gallium phosphide nanodisk at the anapole excitation
title_sort Efficient ultrafast all-optical modulation in a nonlinear crystalline gallium phosphide nanodisk at the anapole excitation
dc.creator.none.fl_str_mv Grinblat, Gustavo Sergio
Zhang, Haizhong
Nielsen, Michael P.
Krivitsky, Leonid
Berté, Rodrigo
Li, Yi
Tilmann, Benjamin
Cortés, Emiliano
Oulton, Rupert F.
Kuznetsov, Arseniy I.
Maier, Stefan A.
author Grinblat, Gustavo Sergio
author_facet Grinblat, Gustavo Sergio
Zhang, Haizhong
Nielsen, Michael P.
Krivitsky, Leonid
Berté, Rodrigo
Li, Yi
Tilmann, Benjamin
Cortés, Emiliano
Oulton, Rupert F.
Kuznetsov, Arseniy I.
Maier, Stefan A.
author_role author
author2 Zhang, Haizhong
Nielsen, Michael P.
Krivitsky, Leonid
Berté, Rodrigo
Li, Yi
Tilmann, Benjamin
Cortés, Emiliano
Oulton, Rupert F.
Kuznetsov, Arseniy I.
Maier, Stefan A.
author2_role author
author
author
author
author
author
author
author
author
author
dc.subject.none.fl_str_mv Nanoantenas ópticas dieléctricas
Conmutación óptica
Efecto Kerr óptico
Absorción de dos fotones
topic Nanoantenas ópticas dieléctricas
Conmutación óptica
Efecto Kerr óptico
Absorción de dos fotones
purl_subject.fl_str_mv https://purl.org/becyt/ford/2.10
https://purl.org/becyt/ford/2
dc.description.none.fl_txt_mv High-refractive index nanostructured dielectrics have the ability to locally enhance electromagnetic fields with low losses while presenting high third-order nonlinearities. In this work, we exploit these characteristics to achieve efficient ultrafast all-optical modulation in a crystalline gallium phosphide (GaP) nanoantenna through the optical Kerr effect (OKE) and two-photon absorption (TPA) in the visible/near-infrared range. We show that an individual GaP nanodisk can yield differential reflectivity modulations of up to -40%, with characteristic modulation times between 14 and 66 fs, when probed at the anapole excitation (AE). Numerical simulations reveal that the AE represents a unique condition where both the OKE and TPA contribute with the same modulation sign, maximizing the response. These findings highly outperform previous reports on sub-100-fs all-optical switching from resonant nanoscale dielectrics, which have demonstrated modulation depths no larger than 0.5%, placing GaP nanoantennas as a promising choice for ultrafast all-optical modulation at the nanometer scale.
Fil: Grinblat, Gustavo Sergio. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; Argentina
Fil: Zhang, Haizhong. Institute of Materials Research and Engineering; Singapur
Fil: Nielsen, Michael P.. University of New South Wales; Australia
Fil: Krivitsky, Leonid. Institute of Materials Research and Engineering; Singapur
Fil: Berté, Rodrigo. Ludwig Maximilians Universitat; Alemania
Fil: Li, Yi. Ludwig Maximilians Universitat; Alemania
Fil: Tilmann, Benjamin. Ludwig Maximilians Universitat; Alemania
Fil: Cortés, Emiliano. Ludwig Maximilians Universitat; Alemania
Fil: Oulton, Rupert F.. Imperial College London; Reino Unido
Fil: Kuznetsov, Arseniy I.. Institute of Materials Research and Engineering; Singapur
Fil: Maier, Stefan A.. Ludwig Maximilians Universitat; Alemania
description High-refractive index nanostructured dielectrics have the ability to locally enhance electromagnetic fields with low losses while presenting high third-order nonlinearities. In this work, we exploit these characteristics to achieve efficient ultrafast all-optical modulation in a crystalline gallium phosphide (GaP) nanoantenna through the optical Kerr effect (OKE) and two-photon absorption (TPA) in the visible/near-infrared range. We show that an individual GaP nanodisk can yield differential reflectivity modulations of up to -40%, with characteristic modulation times between 14 and 66 fs, when probed at the anapole excitation (AE). Numerical simulations reveal that the AE represents a unique condition where both the OKE and TPA contribute with the same modulation sign, maximizing the response. These findings highly outperform previous reports on sub-100-fs all-optical switching from resonant nanoscale dielectrics, which have demonstrated modulation depths no larger than 0.5%, placing GaP nanoantennas as a promising choice for ultrafast all-optical modulation at the nanometer scale.
publishDate 2020
dc.date.none.fl_str_mv 2020-08
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/146133
Grinblat, Gustavo Sergio; Zhang, Haizhong; Nielsen, Michael P.; Krivitsky, Leonid; Berté, Rodrigo; et al.; Efficient ultrafast all-optical modulation in a nonlinear crystalline gallium phosphide nanodisk at the anapole excitation; Science Advances is the American Association for the Advancement of Science; Science Advances; 6; 34; 8-2020; 1-7
2375-2548
CONICET Digital
CONICET
url http://hdl.handle.net/11336/146133
identifier_str_mv Grinblat, Gustavo Sergio; Zhang, Haizhong; Nielsen, Michael P.; Krivitsky, Leonid; Berté, Rodrigo; et al.; Efficient ultrafast all-optical modulation in a nonlinear crystalline gallium phosphide nanodisk at the anapole excitation; Science Advances is the American Association for the Advancement of Science; Science Advances; 6; 34; 8-2020; 1-7
2375-2548
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://advances.sciencemag.org/lookup/doi/10.1126/sciadv.abb3123
info:eu-repo/semantics/altIdentifier/doi/10.1126/sciadv.abb3123
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv Science Advances is the American Association for the Advancement of Science
publisher.none.fl_str_mv Science Advances is the American Association for the Advancement of Science
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 13.070432

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