Quantum transport through single and multilayer icosahedral fullerenes

Autores
Lovey, Daniel Adrián; Romero, Rodolfo Horacio
Año de publicación
2013
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
We use a tight-binding Hamiltonian and Green functions methods to calculate the quantum transmission through single-wall fullerenes and bilayered and trilayered onions of icosahedral symmetry attached to metallic leads. The electronic structure of the onion-like fullerenes takes into account the curvature and finite size of the fullerenes layers as well as the strength of the intershell interactions depending on to the number of interacting atom pairs belonging to adjacent shells.  
Misalignment of the symmetry axes of the concentric iscosahedral shells produces breaking of the level degeneracies of the individual shells, giving rise some narrow quasi-continuum bands instead of the localized discrete peaks of the individual fullerenes. As a result, the transmission function for non symmetrical onions are rapidly varying functions of the Fermi energy. Furthermore, we found that most of the features of the transmission through the onions are due to the electronic structure of the outer shell with additional Fano-like antiresonances arising from coupling with or between the inner shells.
Fil: Lovey, Daniel Adrián. Universidad Nacional del Nordeste. Facultad de Cs.exactas Naturales y Agrimensura. Departamento de Fisica; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Nordeste. Instituto de Modelado E Innovación Tecnológica; Argentina
Fil: Romero, Rodolfo Horacio. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Nordeste. Instituto de Modelado E Innovación Tecnológica; Argentina. Universidad Nacional del Nordeste. Facultad de Cs.exactas Naturales y Agrimensura. Departamento de Fisica; Argentina
Materia
Quantum Transmission
Buckyonions
Tight Binding
Fullerenes
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/2427
Acceder
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network_name_str CONICET Digital (CONICET)
spelling Quantum transport through single and multilayer icosahedral fullerenesLovey, Daniel AdriánRomero, Rodolfo HoracioQuantum TransmissionBuckyonionsTight BindingFullereneshttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1We use a tight-binding Hamiltonian and Green functions methods to calculate the quantum transmission through single-wall fullerenes and bilayered and trilayered onions of icosahedral symmetry attached to metallic leads. The electronic structure of the onion-like fullerenes takes into account the curvature and finite size of the fullerenes layers as well as the strength of the intershell interactions depending on to the number of interacting atom pairs belonging to adjacent shells.  <br />Misalignment of the symmetry axes of the concentric iscosahedral shells produces breaking of the level degeneracies of the individual shells, giving rise some narrow quasi-continuum bands instead of the localized discrete peaks of the individual fullerenes. As a result, the transmission function for non symmetrical onions are rapidly varying functions of the Fermi energy. Furthermore, we found that most of the features of the transmission through the onions are due to the electronic structure of the outer shell with additional Fano-like antiresonances arising from coupling with or between the inner shells.Fil: Lovey, Daniel Adrián. Universidad Nacional del Nordeste. Facultad de Cs.exactas Naturales y Agrimensura. Departamento de Fisica; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Nordeste. Instituto de Modelado E Innovación Tecnológica; ArgentinaFil: Romero, Rodolfo Horacio. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Nordeste. Instituto de Modelado E Innovación Tecnológica; Argentina. Universidad Nacional del Nordeste. Facultad de Cs.exactas Naturales y Agrimensura. Departamento de Fisica; ArgentinaAmerican Institute of Physics2013-10-10info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/2427Lovey, Daniel Adrián; Romero, Rodolfo Horacio; Quantum transport through single and multilayer icosahedral fullerenes; American Institute of Physics; Journal of Applied Physics; 114; 10-10-2013; 144305-1443110021-8979enginfo:eu-repo/semantics/altIdentifier/doi/10.1063/1.4824460info:eu-repo/semantics/altIdentifier/url/http://scitation.aip.org/content/aip/journal/jap/114/14/10.1063/1.4824460info:eu-repo/semantics/altIdentifier/url/http://jap.aip.org/resource/1/japiau/v114/i14/p144305_s1?isAuthorized=noinfo:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-10-22T11:08:27Zoai:ri.conicet.gov.ar:11336/2427instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-10-22 11:08:28.403CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Quantum transport through single and multilayer icosahedral fullerenes
title Quantum transport through single and multilayer icosahedral fullerenes
spellingShingle Quantum transport through single and multilayer icosahedral fullerenes
Lovey, Daniel Adrián
Quantum Transmission
Buckyonions
Tight Binding
Fullerenes
title_short Quantum transport through single and multilayer icosahedral fullerenes
title_full Quantum transport through single and multilayer icosahedral fullerenes
title_fullStr Quantum transport through single and multilayer icosahedral fullerenes
title_full_unstemmed Quantum transport through single and multilayer icosahedral fullerenes
title_sort Quantum transport through single and multilayer icosahedral fullerenes
dc.creator.none.fl_str_mv Lovey, Daniel Adrián
Romero, Rodolfo Horacio
author Lovey, Daniel Adrián
author_facet Lovey, Daniel Adrián
Romero, Rodolfo Horacio
author_role author
author2 Romero, Rodolfo Horacio
author2_role author
dc.subject.none.fl_str_mv Quantum Transmission
Buckyonions
Tight Binding
Fullerenes
topic Quantum Transmission
Buckyonions
Tight Binding
Fullerenes
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv We use a tight-binding Hamiltonian and Green functions methods to calculate the quantum transmission through single-wall fullerenes and bilayered and trilayered onions of icosahedral symmetry attached to metallic leads. The electronic structure of the onion-like fullerenes takes into account the curvature and finite size of the fullerenes layers as well as the strength of the intershell interactions depending on to the number of interacting atom pairs belonging to adjacent shells.  <br />Misalignment of the symmetry axes of the concentric iscosahedral shells produces breaking of the level degeneracies of the individual shells, giving rise some narrow quasi-continuum bands instead of the localized discrete peaks of the individual fullerenes. As a result, the transmission function for non symmetrical onions are rapidly varying functions of the Fermi energy. Furthermore, we found that most of the features of the transmission through the onions are due to the electronic structure of the outer shell with additional Fano-like antiresonances arising from coupling with or between the inner shells.
Fil: Lovey, Daniel Adrián. Universidad Nacional del Nordeste. Facultad de Cs.exactas Naturales y Agrimensura. Departamento de Fisica; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Nordeste. Instituto de Modelado E Innovación Tecnológica; Argentina
Fil: Romero, Rodolfo Horacio. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Nordeste. Instituto de Modelado E Innovación Tecnológica; Argentina. Universidad Nacional del Nordeste. Facultad de Cs.exactas Naturales y Agrimensura. Departamento de Fisica; Argentina
description We use a tight-binding Hamiltonian and Green functions methods to calculate the quantum transmission through single-wall fullerenes and bilayered and trilayered onions of icosahedral symmetry attached to metallic leads. The electronic structure of the onion-like fullerenes takes into account the curvature and finite size of the fullerenes layers as well as the strength of the intershell interactions depending on to the number of interacting atom pairs belonging to adjacent shells.  <br />Misalignment of the symmetry axes of the concentric iscosahedral shells produces breaking of the level degeneracies of the individual shells, giving rise some narrow quasi-continuum bands instead of the localized discrete peaks of the individual fullerenes. As a result, the transmission function for non symmetrical onions are rapidly varying functions of the Fermi energy. Furthermore, we found that most of the features of the transmission through the onions are due to the electronic structure of the outer shell with additional Fano-like antiresonances arising from coupling with or between the inner shells.
publishDate 2013
dc.date.none.fl_str_mv 2013-10-10
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/2427
Lovey, Daniel Adrián; Romero, Rodolfo Horacio; Quantum transport through single and multilayer icosahedral fullerenes; American Institute of Physics; Journal of Applied Physics; 114; 10-10-2013; 144305-144311
0021-8979
url http://hdl.handle.net/11336/2427
identifier_str_mv Lovey, Daniel Adrián; Romero, Rodolfo Horacio; Quantum transport through single and multilayer icosahedral fullerenes; American Institute of Physics; Journal of Applied Physics; 114; 10-10-2013; 144305-144311
0021-8979
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/doi/10.1063/1.4824460
info:eu-repo/semantics/altIdentifier/url/http://scitation.aip.org/content/aip/journal/jap/114/14/10.1063/1.4824460
info:eu-repo/semantics/altIdentifier/url/http://jap.aip.org/resource/1/japiau/v114/i14/p144305_s1?isAuthorized=no
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv American Institute of Physics
publisher.none.fl_str_mv American Institute of Physics
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 12.982451

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