Quantum transport through single and multilayer icosahedral fullerenes
- Autores
- Lovey, Daniel Adrián; Romero, Rodolfo Horacio
- Año de publicación
- 2013
- Idioma
- inglés
- Tipo de recurso
- artículo
- Estado
- versión publicada
- Descripción
- We use a tight-binding Hamiltonian and Green functions methods to calculate the quantum transmission through single-wall fullerenes and bilayered and trilayered onions of icosahedral symmetry attached to metallic leads. The electronic structure of the onion-like fullerenes takes into account the curvature and finite size of the fullerenes layers as well as the strength of the intershell interactions depending on to the number of interacting atom pairs belonging to adjacent shells.
Misalignment of the symmetry axes of the concentric iscosahedral shells produces breaking of the level degeneracies of the individual shells, giving rise some narrow quasi-continuum bands instead of the localized discrete peaks of the individual fullerenes. As a result, the transmission function for non symmetrical onions are rapidly varying functions of the Fermi energy. Furthermore, we found that most of the features of the transmission through the onions are due to the electronic structure of the outer shell with additional Fano-like antiresonances arising from coupling with or between the inner shells.
Fil: Lovey, Daniel Adrián. Universidad Nacional del Nordeste. Facultad de Cs.exactas Naturales y Agrimensura. Departamento de Fisica; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Nordeste. Instituto de Modelado E Innovación Tecnológica; Argentina
Fil: Romero, Rodolfo Horacio. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Nordeste. Instituto de Modelado E Innovación Tecnológica; Argentina. Universidad Nacional del Nordeste. Facultad de Cs.exactas Naturales y Agrimensura. Departamento de Fisica; Argentina - Materia
-
Quantum Transmission
Buckyonions
Tight Binding
Fullerenes - Nivel de accesibilidad
- acceso abierto
- Condiciones de uso
- https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
- Repositorio
- Institución
- Consejo Nacional de Investigaciones Científicas y Técnicas
- OAI Identificador
- oai:ri.conicet.gov.ar:11336/2427
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Quantum transport through single and multilayer icosahedral fullerenesLovey, Daniel AdriánRomero, Rodolfo HoracioQuantum TransmissionBuckyonionsTight BindingFullereneshttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1We use a tight-binding Hamiltonian and Green functions methods to calculate the quantum transmission through single-wall fullerenes and bilayered and trilayered onions of icosahedral symmetry attached to metallic leads. The electronic structure of the onion-like fullerenes takes into account the curvature and finite size of the fullerenes layers as well as the strength of the intershell interactions depending on to the number of interacting atom pairs belonging to adjacent shells. <br />Misalignment of the symmetry axes of the concentric iscosahedral shells produces breaking of the level degeneracies of the individual shells, giving rise some narrow quasi-continuum bands instead of the localized discrete peaks of the individual fullerenes. As a result, the transmission function for non symmetrical onions are rapidly varying functions of the Fermi energy. Furthermore, we found that most of the features of the transmission through the onions are due to the electronic structure of the outer shell with additional Fano-like antiresonances arising from coupling with or between the inner shells.Fil: Lovey, Daniel Adrián. Universidad Nacional del Nordeste. Facultad de Cs.exactas Naturales y Agrimensura. Departamento de Fisica; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Nordeste. Instituto de Modelado E Innovación Tecnológica; ArgentinaFil: Romero, Rodolfo Horacio. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Nordeste. Instituto de Modelado E Innovación Tecnológica; Argentina. Universidad Nacional del Nordeste. Facultad de Cs.exactas Naturales y Agrimensura. Departamento de Fisica; ArgentinaAmerican Institute of Physics2013-10-10info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/2427Lovey, Daniel Adrián; Romero, Rodolfo Horacio; Quantum transport through single and multilayer icosahedral fullerenes; American Institute of Physics; Journal of Applied Physics; 114; 10-10-2013; 144305-1443110021-8979enginfo:eu-repo/semantics/altIdentifier/doi/10.1063/1.4824460info:eu-repo/semantics/altIdentifier/url/http://scitation.aip.org/content/aip/journal/jap/114/14/10.1063/1.4824460info:eu-repo/semantics/altIdentifier/url/http://jap.aip.org/resource/1/japiau/v114/i14/p144305_s1?isAuthorized=noinfo:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T09:40:03Zoai:ri.conicet.gov.ar:11336/2427instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 09:40:03.274CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse |
dc.title.none.fl_str_mv |
Quantum transport through single and multilayer icosahedral fullerenes |
title |
Quantum transport through single and multilayer icosahedral fullerenes |
spellingShingle |
Quantum transport through single and multilayer icosahedral fullerenes Lovey, Daniel Adrián Quantum Transmission Buckyonions Tight Binding Fullerenes |
title_short |
Quantum transport through single and multilayer icosahedral fullerenes |
title_full |
Quantum transport through single and multilayer icosahedral fullerenes |
title_fullStr |
Quantum transport through single and multilayer icosahedral fullerenes |
title_full_unstemmed |
Quantum transport through single and multilayer icosahedral fullerenes |
title_sort |
Quantum transport through single and multilayer icosahedral fullerenes |
dc.creator.none.fl_str_mv |
Lovey, Daniel Adrián Romero, Rodolfo Horacio |
author |
Lovey, Daniel Adrián |
author_facet |
Lovey, Daniel Adrián Romero, Rodolfo Horacio |
author_role |
author |
author2 |
Romero, Rodolfo Horacio |
author2_role |
author |
dc.subject.none.fl_str_mv |
Quantum Transmission Buckyonions Tight Binding Fullerenes |
topic |
Quantum Transmission Buckyonions Tight Binding Fullerenes |
purl_subject.fl_str_mv |
https://purl.org/becyt/ford/1.3 https://purl.org/becyt/ford/1 |
dc.description.none.fl_txt_mv |
We use a tight-binding Hamiltonian and Green functions methods to calculate the quantum transmission through single-wall fullerenes and bilayered and trilayered onions of icosahedral symmetry attached to metallic leads. The electronic structure of the onion-like fullerenes takes into account the curvature and finite size of the fullerenes layers as well as the strength of the intershell interactions depending on to the number of interacting atom pairs belonging to adjacent shells. <br />Misalignment of the symmetry axes of the concentric iscosahedral shells produces breaking of the level degeneracies of the individual shells, giving rise some narrow quasi-continuum bands instead of the localized discrete peaks of the individual fullerenes. As a result, the transmission function for non symmetrical onions are rapidly varying functions of the Fermi energy. Furthermore, we found that most of the features of the transmission through the onions are due to the electronic structure of the outer shell with additional Fano-like antiresonances arising from coupling with or between the inner shells. Fil: Lovey, Daniel Adrián. Universidad Nacional del Nordeste. Facultad de Cs.exactas Naturales y Agrimensura. Departamento de Fisica; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Nordeste. Instituto de Modelado E Innovación Tecnológica; Argentina Fil: Romero, Rodolfo Horacio. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Nordeste. Instituto de Modelado E Innovación Tecnológica; Argentina. Universidad Nacional del Nordeste. Facultad de Cs.exactas Naturales y Agrimensura. Departamento de Fisica; Argentina |
description |
We use a tight-binding Hamiltonian and Green functions methods to calculate the quantum transmission through single-wall fullerenes and bilayered and trilayered onions of icosahedral symmetry attached to metallic leads. The electronic structure of the onion-like fullerenes takes into account the curvature and finite size of the fullerenes layers as well as the strength of the intershell interactions depending on to the number of interacting atom pairs belonging to adjacent shells. <br />Misalignment of the symmetry axes of the concentric iscosahedral shells produces breaking of the level degeneracies of the individual shells, giving rise some narrow quasi-continuum bands instead of the localized discrete peaks of the individual fullerenes. As a result, the transmission function for non symmetrical onions are rapidly varying functions of the Fermi energy. Furthermore, we found that most of the features of the transmission through the onions are due to the electronic structure of the outer shell with additional Fano-like antiresonances arising from coupling with or between the inner shells. |
publishDate |
2013 |
dc.date.none.fl_str_mv |
2013-10-10 |
dc.type.none.fl_str_mv |
info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion http://purl.org/coar/resource_type/c_6501 info:ar-repo/semantics/articulo |
format |
article |
status_str |
publishedVersion |
dc.identifier.none.fl_str_mv |
http://hdl.handle.net/11336/2427 Lovey, Daniel Adrián; Romero, Rodolfo Horacio; Quantum transport through single and multilayer icosahedral fullerenes; American Institute of Physics; Journal of Applied Physics; 114; 10-10-2013; 144305-144311 0021-8979 |
url |
http://hdl.handle.net/11336/2427 |
identifier_str_mv |
Lovey, Daniel Adrián; Romero, Rodolfo Horacio; Quantum transport through single and multilayer icosahedral fullerenes; American Institute of Physics; Journal of Applied Physics; 114; 10-10-2013; 144305-144311 0021-8979 |
dc.language.none.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
info:eu-repo/semantics/altIdentifier/doi/10.1063/1.4824460 info:eu-repo/semantics/altIdentifier/url/http://scitation.aip.org/content/aip/journal/jap/114/14/10.1063/1.4824460 info:eu-repo/semantics/altIdentifier/url/http://jap.aip.org/resource/1/japiau/v114/i14/p144305_s1?isAuthorized=no |
dc.rights.none.fl_str_mv |
info:eu-repo/semantics/openAccess https://creativecommons.org/licenses/by-nc-sa/2.5/ar/ |
eu_rights_str_mv |
openAccess |
rights_invalid_str_mv |
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/ |
dc.format.none.fl_str_mv |
application/pdf application/pdf |
dc.publisher.none.fl_str_mv |
American Institute of Physics |
publisher.none.fl_str_mv |
American Institute of Physics |
dc.source.none.fl_str_mv |
reponame:CONICET Digital (CONICET) instname:Consejo Nacional de Investigaciones Científicas y Técnicas |
reponame_str |
CONICET Digital (CONICET) |
collection |
CONICET Digital (CONICET) |
instname_str |
Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.name.fl_str_mv |
CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.mail.fl_str_mv |
dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar |
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1844613266272157696 |
score |
13.070432 |