Aging and crystallization in a lattice glass model

Autores
Seif, Alejandro; Loscar, Ernesto Selim; Grigera, Tomás Sebastián
Año de publicación
2015
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
We have studied the three-dimensional lattice glass of Pica Ciamarra et al. [Phys. Rev. E 67, 057105 (2003)], which has been shown to reproduce several features of the structural glass phenomenology, such as the cage effect, exponential increase of relaxation times, and aging. We show, using short-time dynamics, that the metastability limit is above the estimated Kauzmann temperature. We also find that in the region where the metastable liquid exists the aging exponent is lower than 0.5, indicating that equilibrium is reached relatively quickly. We conclude that the usefulness of this model to study the deeply supercooled regime is rather limited.
Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas
Materia
Física
Supercooling
Lattice (order)
Exponential function
Materials science
Crystallization
Condensed matter physics
Cage effect
Exponent
Metastability
Nivel de accesibilidad
acceso abierto
Condiciones de uso
http://creativecommons.org/licenses/by-nc-sa/4.0/
Repositorio
SEDICI (UNLP)
Institución
Universidad Nacional de La Plata
OAI Identificador
oai:sedici.unlp.edu.ar:10915/126045
Acceder
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oai_identifier_str oai:sedici.unlp.edu.ar:10915/126045
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network_name_str SEDICI (UNLP)
spelling Aging and crystallization in a lattice glass modelSeif, AlejandroLoscar, Ernesto SelimGrigera, Tomás SebastiánFísicaSupercoolingLattice (order)Exponential functionMaterials scienceCrystallizationCondensed matter physicsCage effectExponentMetastabilityWe have studied the three-dimensional lattice glass of Pica Ciamarra et al. [Phys. Rev. E 67, 057105 (2003)], which has been shown to reproduce several features of the structural glass phenomenology, such as the cage effect, exponential increase of relaxation times, and aging. We show, using short-time dynamics, that the metastability limit is above the estimated Kauzmann temperature. We also find that in the region where the metastable liquid exists the aging exponent is lower than 0.5, indicating that equilibrium is reached relatively quickly. We conclude that the usefulness of this model to study the deeply supercooled regime is rather limited.Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas2015-04-03info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionArticulohttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfhttp://sedici.unlp.edu.ar/handle/10915/126045enginfo:eu-repo/semantics/altIdentifier/issn/1550-2376info:eu-repo/semantics/altIdentifier/issn/1539-3755info:eu-repo/semantics/altIdentifier/arxiv/1412.4744info:eu-repo/semantics/altIdentifier/pmid/25974486info:eu-repo/semantics/altIdentifier/doi/10.1103/physreve.91.042302info:eu-repo/semantics/openAccesshttp://creativecommons.org/licenses/by-nc-sa/4.0/Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International (CC BY-NC-SA 4.0)reponame:SEDICI (UNLP)instname:Universidad Nacional de La Platainstacron:UNLP2025-09-29T11:30:18Zoai:sedici.unlp.edu.ar:10915/126045Institucionalhttp://sedici.unlp.edu.ar/Universidad públicaNo correspondehttp://sedici.unlp.edu.ar/oai/snrdalira@sedici.unlp.edu.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:13292025-09-29 11:30:19.175SEDICI (UNLP) - Universidad Nacional de La Platafalse
dc.title.none.fl_str_mv Aging and crystallization in a lattice glass model
title Aging and crystallization in a lattice glass model
spellingShingle Aging and crystallization in a lattice glass model
Seif, Alejandro
Física
Supercooling
Lattice (order)
Exponential function
Materials science
Crystallization
Condensed matter physics
Cage effect
Exponent
Metastability
title_short Aging and crystallization in a lattice glass model
title_full Aging and crystallization in a lattice glass model
title_fullStr Aging and crystallization in a lattice glass model
title_full_unstemmed Aging and crystallization in a lattice glass model
title_sort Aging and crystallization in a lattice glass model
dc.creator.none.fl_str_mv Seif, Alejandro
Loscar, Ernesto Selim
Grigera, Tomás Sebastián
author Seif, Alejandro
author_facet Seif, Alejandro
Loscar, Ernesto Selim
Grigera, Tomás Sebastián
author_role author
author2 Loscar, Ernesto Selim
Grigera, Tomás Sebastián
author2_role author
author
dc.subject.none.fl_str_mv Física
Supercooling
Lattice (order)
Exponential function
Materials science
Crystallization
Condensed matter physics
Cage effect
Exponent
Metastability
topic Física
Supercooling
Lattice (order)
Exponential function
Materials science
Crystallization
Condensed matter physics
Cage effect
Exponent
Metastability
dc.description.none.fl_txt_mv We have studied the three-dimensional lattice glass of Pica Ciamarra et al. [Phys. Rev. E 67, 057105 (2003)], which has been shown to reproduce several features of the structural glass phenomenology, such as the cage effect, exponential increase of relaxation times, and aging. We show, using short-time dynamics, that the metastability limit is above the estimated Kauzmann temperature. We also find that in the region where the metastable liquid exists the aging exponent is lower than 0.5, indicating that equilibrium is reached relatively quickly. We conclude that the usefulness of this model to study the deeply supercooled regime is rather limited.
Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas
description We have studied the three-dimensional lattice glass of Pica Ciamarra et al. [Phys. Rev. E 67, 057105 (2003)], which has been shown to reproduce several features of the structural glass phenomenology, such as the cage effect, exponential increase of relaxation times, and aging. We show, using short-time dynamics, that the metastability limit is above the estimated Kauzmann temperature. We also find that in the region where the metastable liquid exists the aging exponent is lower than 0.5, indicating that equilibrium is reached relatively quickly. We conclude that the usefulness of this model to study the deeply supercooled regime is rather limited.
publishDate 2015
dc.date.none.fl_str_mv 2015-04-03
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
Articulo
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info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://sedici.unlp.edu.ar/handle/10915/126045
url http://sedici.unlp.edu.ar/handle/10915/126045
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/issn/1550-2376
info:eu-repo/semantics/altIdentifier/issn/1539-3755
info:eu-repo/semantics/altIdentifier/arxiv/1412.4744
info:eu-repo/semantics/altIdentifier/pmid/25974486
info:eu-repo/semantics/altIdentifier/doi/10.1103/physreve.91.042302
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
http://creativecommons.org/licenses/by-nc-sa/4.0/
Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International (CC BY-NC-SA 4.0)
eu_rights_str_mv openAccess
rights_invalid_str_mv http://creativecommons.org/licenses/by-nc-sa/4.0/
Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International (CC BY-NC-SA 4.0)
dc.format.none.fl_str_mv application/pdf
dc.source.none.fl_str_mv reponame:SEDICI (UNLP)
instname:Universidad Nacional de La Plata
instacron:UNLP
reponame_str SEDICI (UNLP)
collection SEDICI (UNLP)
instname_str Universidad Nacional de La Plata
instacron_str UNLP
institution UNLP
repository.name.fl_str_mv SEDICI (UNLP) - Universidad Nacional de La Plata
repository.mail.fl_str_mv alira@sedici.unlp.edu.ar
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