Aging and crystallization in a lattice glass model

Autores
Seif, Alejandro; Loscar, Ernesto Selim; Grigera, Tomas Sebastian
Año de publicación
2015
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
We have studied the three-dimensional lattice glass of Pica Ciamarra et al. [Phys. Rev. E 67, 057105 (2003)], which has been shown to reproduce several features of the structural glass phenomenology, such as the cage effect, exponential increase of relaxation times, and aging. We show, using short-time dynamics, that the metastability limit is above the estimated Kauzmann temperature. We also find that in the region where the metastable liquid exists the aging exponent is lower than 0.5, indicating that equilibrium is reached relatively quickly. We conclude that the usefulness of this model to study the deeply supercooled regime is rather limited.
Fil: Seif, Alejandro. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; Argentina
Fil: Loscar, Ernesto Selim. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; Argentina
Fil: Grigera, Tomas Sebastian. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; Argentina
Materia
Aging
Short Time Dynamics
Lattice Model
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/48019
Acceder
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spelling Aging and crystallization in a lattice glass modelSeif, AlejandroLoscar, Ernesto SelimGrigera, Tomas SebastianAgingShort Time DynamicsLattice Modelhttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1We have studied the three-dimensional lattice glass of Pica Ciamarra et al. [Phys. Rev. E 67, 057105 (2003)], which has been shown to reproduce several features of the structural glass phenomenology, such as the cage effect, exponential increase of relaxation times, and aging. We show, using short-time dynamics, that the metastability limit is above the estimated Kauzmann temperature. We also find that in the region where the metastable liquid exists the aging exponent is lower than 0.5, indicating that equilibrium is reached relatively quickly. We conclude that the usefulness of this model to study the deeply supercooled regime is rather limited.Fil: Seif, Alejandro. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; ArgentinaFil: Loscar, Ernesto Selim. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; ArgentinaFil: Grigera, Tomas Sebastian. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; ArgentinaAmerican Physical Society2015-04info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/48019Seif, Alejandro; Loscar, Ernesto Selim; Grigera, Tomas Sebastian; Aging and crystallization in a lattice glass model; American Physical Society; Physical Review E: Statistical, Nonlinear and Soft Matter Physics; 91; 4; 4-2015; 1-6; 0423021539-3755CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/doi/10.1103/PhysRevE.91.042302info:eu-repo/semantics/altIdentifier/url/https://journals.aps.org/pre/abstract/10.1103/PhysRevE.91.042302info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T09:47:45Zoai:ri.conicet.gov.ar:11336/48019instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 09:47:46.09CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Aging and crystallization in a lattice glass model
title Aging and crystallization in a lattice glass model
spellingShingle Aging and crystallization in a lattice glass model
Seif, Alejandro
Aging
Short Time Dynamics
Lattice Model
title_short Aging and crystallization in a lattice glass model
title_full Aging and crystallization in a lattice glass model
title_fullStr Aging and crystallization in a lattice glass model
title_full_unstemmed Aging and crystallization in a lattice glass model
title_sort Aging and crystallization in a lattice glass model
dc.creator.none.fl_str_mv Seif, Alejandro
Loscar, Ernesto Selim
Grigera, Tomas Sebastian
author Seif, Alejandro
author_facet Seif, Alejandro
Loscar, Ernesto Selim
Grigera, Tomas Sebastian
author_role author
author2 Loscar, Ernesto Selim
Grigera, Tomas Sebastian
author2_role author
author
dc.subject.none.fl_str_mv Aging
Short Time Dynamics
Lattice Model
topic Aging
Short Time Dynamics
Lattice Model
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv We have studied the three-dimensional lattice glass of Pica Ciamarra et al. [Phys. Rev. E 67, 057105 (2003)], which has been shown to reproduce several features of the structural glass phenomenology, such as the cage effect, exponential increase of relaxation times, and aging. We show, using short-time dynamics, that the metastability limit is above the estimated Kauzmann temperature. We also find that in the region where the metastable liquid exists the aging exponent is lower than 0.5, indicating that equilibrium is reached relatively quickly. We conclude that the usefulness of this model to study the deeply supercooled regime is rather limited.
Fil: Seif, Alejandro. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; Argentina
Fil: Loscar, Ernesto Selim. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; Argentina
Fil: Grigera, Tomas Sebastian. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; Argentina
description We have studied the three-dimensional lattice glass of Pica Ciamarra et al. [Phys. Rev. E 67, 057105 (2003)], which has been shown to reproduce several features of the structural glass phenomenology, such as the cage effect, exponential increase of relaxation times, and aging. We show, using short-time dynamics, that the metastability limit is above the estimated Kauzmann temperature. We also find that in the region where the metastable liquid exists the aging exponent is lower than 0.5, indicating that equilibrium is reached relatively quickly. We conclude that the usefulness of this model to study the deeply supercooled regime is rather limited.
publishDate 2015
dc.date.none.fl_str_mv 2015-04
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/48019
Seif, Alejandro; Loscar, Ernesto Selim; Grigera, Tomas Sebastian; Aging and crystallization in a lattice glass model; American Physical Society; Physical Review E: Statistical, Nonlinear and Soft Matter Physics; 91; 4; 4-2015; 1-6; 042302
1539-3755
CONICET Digital
CONICET
url http://hdl.handle.net/11336/48019
identifier_str_mv Seif, Alejandro; Loscar, Ernesto Selim; Grigera, Tomas Sebastian; Aging and crystallization in a lattice glass model; American Physical Society; Physical Review E: Statistical, Nonlinear and Soft Matter Physics; 91; 4; 4-2015; 1-6; 042302
1539-3755
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/doi/10.1103/PhysRevE.91.042302
info:eu-repo/semantics/altIdentifier/url/https://journals.aps.org/pre/abstract/10.1103/PhysRevE.91.042302
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
application/pdf
dc.publisher.none.fl_str_mv American Physical Society
publisher.none.fl_str_mv American Physical Society
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 13.070432

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