Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)]
- Autores
- Gradenigo, Giacomo; Trozzo, Roberto; Cavagna, Andrea; Grigera, Tomás Sebastián
- Año de publicación
- 2016
- Idioma
- inglés
- Tipo de recurso
- artículo
- Estado
- versión publicada
- Descripción
- The point-to-set correlation function has proved to be a very valuable tool to probe structural correlations in disordered systems, but more than that, its detailed behavior has been used to try to draw information on the mechanisms leading to glassy behavior in supercooled liquids. For this reason it is of primary importance to discern which of those details are peculiar to glassy systems, and which are general features of confinement. Thus the concerns raised in Ref. 1 definitely need to meet an answer. The Comment proposes an alternative analysis of the numerical data presented in Ref. 2, according to which the behaviour of the point-to-set correlation function can be interpreted as a linear superposition of boundary effects, rather than the effect of non-trivial thermodynamics. We believe this alternative explanation is not compelling.
Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas - Materia
- Química
- Nivel de accesibilidad
- acceso abierto
- Condiciones de uso
- http://creativecommons.org/licenses/by-nc-sa/4.0/
- Repositorio
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- Institución
- Universidad Nacional de La Plata
- OAI Identificador
- oai:sedici.unlp.edu.ar:10915/87064
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Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)]Gradenigo, GiacomoTrozzo, RobertoCavagna, AndreaGrigera, Tomás SebastiánQuímicaThe point-to-set correlation function has proved to be a very valuable tool to probe structural correlations in disordered systems, but more than that, its detailed behavior has been used to try to draw information on the mechanisms leading to glassy behavior in supercooled liquids. For this reason it is of primary importance to discern which of those details are peculiar to glassy systems, and which are general features of confinement. Thus the concerns raised in Ref. 1 definitely need to meet an answer. The Comment proposes an alternative analysis of the numerical data presented in Ref. 2, according to which the behaviour of the point-to-set correlation function can be interpreted as a linear superposition of boundary effects, rather than the effect of non-trivial thermodynamics. We believe this alternative explanation is not compelling.Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas2016info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionArticulohttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfhttp://sedici.unlp.edu.ar/handle/10915/87064enginfo:eu-repo/semantics/altIdentifier/issn/0021-9606info:eu-repo/semantics/altIdentifier/doi/10.1063/1.4953615info:eu-repo/semantics/openAccesshttp://creativecommons.org/licenses/by-nc-sa/4.0/Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International (CC BY-NC-SA 4.0)reponame:SEDICI (UNLP)instname:Universidad Nacional de La Platainstacron:UNLP2025-11-12T10:41:06Zoai:sedici.unlp.edu.ar:10915/87064Institucionalhttp://sedici.unlp.edu.ar/Universidad públicaNo correspondehttp://sedici.unlp.edu.ar/oai/snrdalira@sedici.unlp.edu.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:13292025-11-12 10:41:06.582SEDICI (UNLP) - Universidad Nacional de La Platafalse |
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Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)] |
| title |
Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)] |
| spellingShingle |
Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)] Gradenigo, Giacomo Química |
| title_short |
Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)] |
| title_full |
Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)] |
| title_fullStr |
Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)] |
| title_full_unstemmed |
Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)] |
| title_sort |
Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)] |
| dc.creator.none.fl_str_mv |
Gradenigo, Giacomo Trozzo, Roberto Cavagna, Andrea Grigera, Tomás Sebastián |
| author |
Gradenigo, Giacomo |
| author_facet |
Gradenigo, Giacomo Trozzo, Roberto Cavagna, Andrea Grigera, Tomás Sebastián |
| author_role |
author |
| author2 |
Trozzo, Roberto Cavagna, Andrea Grigera, Tomás Sebastián |
| author2_role |
author author author |
| dc.subject.none.fl_str_mv |
Química |
| topic |
Química |
| dc.description.none.fl_txt_mv |
The point-to-set correlation function has proved to be a very valuable tool to probe structural correlations in disordered systems, but more than that, its detailed behavior has been used to try to draw information on the mechanisms leading to glassy behavior in supercooled liquids. For this reason it is of primary importance to discern which of those details are peculiar to glassy systems, and which are general features of confinement. Thus the concerns raised in Ref. 1 definitely need to meet an answer. The Comment proposes an alternative analysis of the numerical data presented in Ref. 2, according to which the behaviour of the point-to-set correlation function can be interpreted as a linear superposition of boundary effects, rather than the effect of non-trivial thermodynamics. We believe this alternative explanation is not compelling. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas |
| description |
The point-to-set correlation function has proved to be a very valuable tool to probe structural correlations in disordered systems, but more than that, its detailed behavior has been used to try to draw information on the mechanisms leading to glassy behavior in supercooled liquids. For this reason it is of primary importance to discern which of those details are peculiar to glassy systems, and which are general features of confinement. Thus the concerns raised in Ref. 1 definitely need to meet an answer. The Comment proposes an alternative analysis of the numerical data presented in Ref. 2, according to which the behaviour of the point-to-set correlation function can be interpreted as a linear superposition of boundary effects, rather than the effect of non-trivial thermodynamics. We believe this alternative explanation is not compelling. |
| publishDate |
2016 |
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2016 |
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