Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)]

Autores
Gradenigo, Giacomo; Trozzo, Roberto; Cavagna, Andrea; Grigera, Tomás Sebastián
Año de publicación
2016
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
The point-to-set correlation function has proved to be a very valuable tool to probe structural correlations in disordered systems, but more than that, its detailed behavior has been used to try to draw information on the mechanisms leading to glassy behavior in supercooled liquids. For this reason it is of primary importance to discern which of those details are peculiar to glassy systems, and which are general features of confinement. Thus the concerns raised in Ref. 1 definitely need to meet an answer. The Comment proposes an alternative analysis of the numerical data presented in Ref. 2, according to which the behaviour of the point-to-set correlation function can be interpreted as a linear superposition of boundary effects, rather than the effect of non-trivial thermodynamics. We believe this alternative explanation is not compelling.
Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas
Materia
Química
Nivel de accesibilidad
acceso abierto
Condiciones de uso
http://creativecommons.org/licenses/by-nc-sa/4.0/
Repositorio
SEDICI (UNLP)
Institución
Universidad Nacional de La Plata
OAI Identificador
oai:sedici.unlp.edu.ar:10915/87064

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spelling Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)]Gradenigo, GiacomoTrozzo, RobertoCavagna, AndreaGrigera, Tomás SebastiánQuímicaThe point-to-set correlation function has proved to be a very valuable tool to probe structural correlations in disordered systems, but more than that, its detailed behavior has been used to try to draw information on the mechanisms leading to glassy behavior in supercooled liquids. For this reason it is of primary importance to discern which of those details are peculiar to glassy systems, and which are general features of confinement. Thus the concerns raised in Ref. 1 definitely need to meet an answer. The Comment proposes an alternative analysis of the numerical data presented in Ref. 2, according to which the behaviour of the point-to-set correlation function can be interpreted as a linear superposition of boundary effects, rather than the effect of non-trivial thermodynamics. We believe this alternative explanation is not compelling.Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas2016info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionArticulohttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfhttp://sedici.unlp.edu.ar/handle/10915/87064enginfo:eu-repo/semantics/altIdentifier/issn/0021-9606info:eu-repo/semantics/altIdentifier/doi/10.1063/1.4953615info:eu-repo/semantics/openAccesshttp://creativecommons.org/licenses/by-nc-sa/4.0/Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International (CC BY-NC-SA 4.0)reponame:SEDICI (UNLP)instname:Universidad Nacional de La Platainstacron:UNLP2025-11-12T10:41:06Zoai:sedici.unlp.edu.ar:10915/87064Institucionalhttp://sedici.unlp.edu.ar/Universidad públicaNo correspondehttp://sedici.unlp.edu.ar/oai/snrdalira@sedici.unlp.edu.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:13292025-11-12 10:41:06.582SEDICI (UNLP) - Universidad Nacional de La Platafalse
dc.title.none.fl_str_mv Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)]
title Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)]
spellingShingle Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)]
Gradenigo, Giacomo
Química
title_short Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)]
title_full Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)]
title_fullStr Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)]
title_full_unstemmed Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)]
title_sort Response to “Comment on ‘Static correlations functions and domain walls in glass-forming liquids: The case of a sandwich geometry”’ [J. Chem. Phys. 144, 227101 (2016)]
dc.creator.none.fl_str_mv Gradenigo, Giacomo
Trozzo, Roberto
Cavagna, Andrea
Grigera, Tomás Sebastián
author Gradenigo, Giacomo
author_facet Gradenigo, Giacomo
Trozzo, Roberto
Cavagna, Andrea
Grigera, Tomás Sebastián
author_role author
author2 Trozzo, Roberto
Cavagna, Andrea
Grigera, Tomás Sebastián
author2_role author
author
author
dc.subject.none.fl_str_mv Química
topic Química
dc.description.none.fl_txt_mv The point-to-set correlation function has proved to be a very valuable tool to probe structural correlations in disordered systems, but more than that, its detailed behavior has been used to try to draw information on the mechanisms leading to glassy behavior in supercooled liquids. For this reason it is of primary importance to discern which of those details are peculiar to glassy systems, and which are general features of confinement. Thus the concerns raised in Ref. 1 definitely need to meet an answer. The Comment proposes an alternative analysis of the numerical data presented in Ref. 2, according to which the behaviour of the point-to-set correlation function can be interpreted as a linear superposition of boundary effects, rather than the effect of non-trivial thermodynamics. We believe this alternative explanation is not compelling.
Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas
description The point-to-set correlation function has proved to be a very valuable tool to probe structural correlations in disordered systems, but more than that, its detailed behavior has been used to try to draw information on the mechanisms leading to glassy behavior in supercooled liquids. For this reason it is of primary importance to discern which of those details are peculiar to glassy systems, and which are general features of confinement. Thus the concerns raised in Ref. 1 definitely need to meet an answer. The Comment proposes an alternative analysis of the numerical data presented in Ref. 2, according to which the behaviour of the point-to-set correlation function can be interpreted as a linear superposition of boundary effects, rather than the effect of non-trivial thermodynamics. We believe this alternative explanation is not compelling.
publishDate 2016
dc.date.none.fl_str_mv 2016
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Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International (CC BY-NC-SA 4.0)
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