Mixed Ionic and Electronic Conducting Eutectogels for 3D-Printable Wearable Sensors and Bioelectrodes

Autores
Picchio, Matías Luis; Gallastegui, Antonela; Casado, Nerea; Lopez Larrea, Naroa; Marchiori, Bastien; del Agua, Isabel; Criado Gonzalez, Miryam; Mantione, Daniele; Minari, Roque Javier; Mecerreyes, David
Año de publicación
2022
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
Eutectogels are a new class of soft ion conductive materials that are attracting attention as an alternative to conventional hydrogels and costly ionic liquid gels to build wearable sensors and bioelectrodes. Herein, the first example of mixed ionic and electronic conductive eutectogels showing high adhesion, flexibility, nonvolatility, and reversible low-temperature gel transition for 3D printing manufacturing is reporting. The eutectogels consist of choline chloride/glycerol deep eutectic solvent, poly(3,4-ethylenedioxythiophene): lignin sulfonate, and gelatin as the biocompatible polymer matrix. These soft materials are flexible and stretchable, show high ionic and electronic conductivities of 7.3 and 8.7 mS cm−1, respectively, and have high adhesion energy. Due to this unique combination of properties, they could be applied as strain sensors to precisely detect physical movements. Furthermore, these soft mixed ionic electronic conductors possess excellent capacity as conformal electrodes to record epidermal physiological signals, such as electrocardiograms and electromyograms, over a long time.
Fil: Picchio, Matías Luis. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Desarrollo Tecnológico para la Industria Química. Universidad Nacional del Litoral. Instituto de Desarrollo Tecnológico para la Industria Química; Argentina
Fil: Gallastegui, Antonela. Universidad del Pais Vasco. Polymat.; España
Fil: Casado, Nerea. Universidad del Pais Vasco. Polymat.; España
Fil: Lopez Larrea, Naroa. Universidad del Pais Vasco. Polymat.; España
Fil: Marchiori, Bastien. No especifíca;
Fil: del Agua, Isabel. No especifíca;
Fil: Criado Gonzalez, Miryam. Universidad del Pais Vasco. Polymat.; España
Fil: Mantione, Daniele. Universidad del Pais Vasco. Polymat.; España
Fil: Minari, Roque Javier. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Desarrollo Tecnológico para la Industria Química. Universidad Nacional del Litoral. Instituto de Desarrollo Tecnológico para la Industria Química; Argentina
Fil: Mecerreyes, David. Universidad del Pais Vasco. Polymat.; España
Materia
3D PRINTING
BODY SENSORS
DEEP EUTECTIC SOLVENTS
IONIC SOFT MATERIALS
PEDOT
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/216012
Acceder
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oai_identifier_str oai:ri.conicet.gov.ar:11336/216012
network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Mixed Ionic and Electronic Conducting Eutectogels for 3D-Printable Wearable Sensors and BioelectrodesPicchio, Matías LuisGallastegui, AntonelaCasado, NereaLopez Larrea, NaroaMarchiori, Bastiendel Agua, IsabelCriado Gonzalez, MiryamMantione, DanieleMinari, Roque JavierMecerreyes, David3D PRINTINGBODY SENSORSDEEP EUTECTIC SOLVENTSIONIC SOFT MATERIALSPEDOThttps://purl.org/becyt/ford/1.4https://purl.org/becyt/ford/1Eutectogels are a new class of soft ion conductive materials that are attracting attention as an alternative to conventional hydrogels and costly ionic liquid gels to build wearable sensors and bioelectrodes. Herein, the first example of mixed ionic and electronic conductive eutectogels showing high adhesion, flexibility, nonvolatility, and reversible low-temperature gel transition for 3D printing manufacturing is reporting. The eutectogels consist of choline chloride/glycerol deep eutectic solvent, poly(3,4-ethylenedioxythiophene): lignin sulfonate, and gelatin as the biocompatible polymer matrix. These soft materials are flexible and stretchable, show high ionic and electronic conductivities of 7.3 and 8.7 mS cm−1, respectively, and have high adhesion energy. Due to this unique combination of properties, they could be applied as strain sensors to precisely detect physical movements. Furthermore, these soft mixed ionic electronic conductors possess excellent capacity as conformal electrodes to record epidermal physiological signals, such as electrocardiograms and electromyograms, over a long time.Fil: Picchio, Matías Luis. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Desarrollo Tecnológico para la Industria Química. Universidad Nacional del Litoral. Instituto de Desarrollo Tecnológico para la Industria Química; ArgentinaFil: Gallastegui, Antonela. Universidad del Pais Vasco. Polymat.; EspañaFil: Casado, Nerea. Universidad del Pais Vasco. Polymat.; EspañaFil: Lopez Larrea, Naroa. Universidad del Pais Vasco. Polymat.; EspañaFil: Marchiori, Bastien. No especifíca;Fil: del Agua, Isabel. No especifíca;Fil: Criado Gonzalez, Miryam. Universidad del Pais Vasco. Polymat.; EspañaFil: Mantione, Daniele. Universidad del Pais Vasco. Polymat.; EspañaFil: Minari, Roque Javier. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Desarrollo Tecnológico para la Industria Química. Universidad Nacional del Litoral. Instituto de Desarrollo Tecnológico para la Industria Química; ArgentinaFil: Mecerreyes, David. Universidad del Pais Vasco. Polymat.; EspañaWiley2022-03info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/216012Picchio, Matías Luis; Gallastegui, Antonela; Casado, Nerea; Lopez Larrea, Naroa; Marchiori, Bastien; et al.; Mixed Ionic and Electronic Conducting Eutectogels for 3D-Printable Wearable Sensors and Bioelectrodes; Wiley; Advanced Materials Technologies; 7; 10; 3-2022; 1-82365-709XCONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://onlinelibrary.wiley.com/doi/10.1002/admt.202101680info:eu-repo/semantics/altIdentifier/doi/10.1002/admt.202101680info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-10T13:07:19Zoai:ri.conicet.gov.ar:11336/216012instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-10 13:07:19.531CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Mixed Ionic and Electronic Conducting Eutectogels for 3D-Printable Wearable Sensors and Bioelectrodes
title Mixed Ionic and Electronic Conducting Eutectogels for 3D-Printable Wearable Sensors and Bioelectrodes
spellingShingle Mixed Ionic and Electronic Conducting Eutectogels for 3D-Printable Wearable Sensors and Bioelectrodes
Picchio, Matías Luis
3D PRINTING
BODY SENSORS
DEEP EUTECTIC SOLVENTS
IONIC SOFT MATERIALS
PEDOT
title_short Mixed Ionic and Electronic Conducting Eutectogels for 3D-Printable Wearable Sensors and Bioelectrodes
title_full Mixed Ionic and Electronic Conducting Eutectogels for 3D-Printable Wearable Sensors and Bioelectrodes
title_fullStr Mixed Ionic and Electronic Conducting Eutectogels for 3D-Printable Wearable Sensors and Bioelectrodes
title_full_unstemmed Mixed Ionic and Electronic Conducting Eutectogels for 3D-Printable Wearable Sensors and Bioelectrodes
title_sort Mixed Ionic and Electronic Conducting Eutectogels for 3D-Printable Wearable Sensors and Bioelectrodes
dc.creator.none.fl_str_mv Picchio, Matías Luis
Gallastegui, Antonela
Casado, Nerea
Lopez Larrea, Naroa
Marchiori, Bastien
del Agua, Isabel
Criado Gonzalez, Miryam
Mantione, Daniele
Minari, Roque Javier
Mecerreyes, David
author Picchio, Matías Luis
author_facet Picchio, Matías Luis
Gallastegui, Antonela
Casado, Nerea
Lopez Larrea, Naroa
Marchiori, Bastien
del Agua, Isabel
Criado Gonzalez, Miryam
Mantione, Daniele
Minari, Roque Javier
Mecerreyes, David
author_role author
author2 Gallastegui, Antonela
Casado, Nerea
Lopez Larrea, Naroa
Marchiori, Bastien
del Agua, Isabel
Criado Gonzalez, Miryam
Mantione, Daniele
Minari, Roque Javier
Mecerreyes, David
author2_role author
author
author
author
author
author
author
author
author
dc.subject.none.fl_str_mv 3D PRINTING
BODY SENSORS
DEEP EUTECTIC SOLVENTS
IONIC SOFT MATERIALS
PEDOT
topic 3D PRINTING
BODY SENSORS
DEEP EUTECTIC SOLVENTS
IONIC SOFT MATERIALS
PEDOT
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv Eutectogels are a new class of soft ion conductive materials that are attracting attention as an alternative to conventional hydrogels and costly ionic liquid gels to build wearable sensors and bioelectrodes. Herein, the first example of mixed ionic and electronic conductive eutectogels showing high adhesion, flexibility, nonvolatility, and reversible low-temperature gel transition for 3D printing manufacturing is reporting. The eutectogels consist of choline chloride/glycerol deep eutectic solvent, poly(3,4-ethylenedioxythiophene): lignin sulfonate, and gelatin as the biocompatible polymer matrix. These soft materials are flexible and stretchable, show high ionic and electronic conductivities of 7.3 and 8.7 mS cm−1, respectively, and have high adhesion energy. Due to this unique combination of properties, they could be applied as strain sensors to precisely detect physical movements. Furthermore, these soft mixed ionic electronic conductors possess excellent capacity as conformal electrodes to record epidermal physiological signals, such as electrocardiograms and electromyograms, over a long time.
Fil: Picchio, Matías Luis. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Desarrollo Tecnológico para la Industria Química. Universidad Nacional del Litoral. Instituto de Desarrollo Tecnológico para la Industria Química; Argentina
Fil: Gallastegui, Antonela. Universidad del Pais Vasco. Polymat.; España
Fil: Casado, Nerea. Universidad del Pais Vasco. Polymat.; España
Fil: Lopez Larrea, Naroa. Universidad del Pais Vasco. Polymat.; España
Fil: Marchiori, Bastien. No especifíca;
Fil: del Agua, Isabel. No especifíca;
Fil: Criado Gonzalez, Miryam. Universidad del Pais Vasco. Polymat.; España
Fil: Mantione, Daniele. Universidad del Pais Vasco. Polymat.; España
Fil: Minari, Roque Javier. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Desarrollo Tecnológico para la Industria Química. Universidad Nacional del Litoral. Instituto de Desarrollo Tecnológico para la Industria Química; Argentina
Fil: Mecerreyes, David. Universidad del Pais Vasco. Polymat.; España
description Eutectogels are a new class of soft ion conductive materials that are attracting attention as an alternative to conventional hydrogels and costly ionic liquid gels to build wearable sensors and bioelectrodes. Herein, the first example of mixed ionic and electronic conductive eutectogels showing high adhesion, flexibility, nonvolatility, and reversible low-temperature gel transition for 3D printing manufacturing is reporting. The eutectogels consist of choline chloride/glycerol deep eutectic solvent, poly(3,4-ethylenedioxythiophene): lignin sulfonate, and gelatin as the biocompatible polymer matrix. These soft materials are flexible and stretchable, show high ionic and electronic conductivities of 7.3 and 8.7 mS cm−1, respectively, and have high adhesion energy. Due to this unique combination of properties, they could be applied as strain sensors to precisely detect physical movements. Furthermore, these soft mixed ionic electronic conductors possess excellent capacity as conformal electrodes to record epidermal physiological signals, such as electrocardiograms and electromyograms, over a long time.
publishDate 2022
dc.date.none.fl_str_mv 2022-03
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/216012
Picchio, Matías Luis; Gallastegui, Antonela; Casado, Nerea; Lopez Larrea, Naroa; Marchiori, Bastien; et al.; Mixed Ionic and Electronic Conducting Eutectogels for 3D-Printable Wearable Sensors and Bioelectrodes; Wiley; Advanced Materials Technologies; 7; 10; 3-2022; 1-8
2365-709X
CONICET Digital
CONICET
url http://hdl.handle.net/11336/216012
identifier_str_mv Picchio, Matías Luis; Gallastegui, Antonela; Casado, Nerea; Lopez Larrea, Naroa; Marchiori, Bastien; et al.; Mixed Ionic and Electronic Conducting Eutectogels for 3D-Printable Wearable Sensors and Bioelectrodes; Wiley; Advanced Materials Technologies; 7; 10; 3-2022; 1-8
2365-709X
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://onlinelibrary.wiley.com/doi/10.1002/admt.202101680
info:eu-repo/semantics/altIdentifier/doi/10.1002/admt.202101680
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv Wiley
publisher.none.fl_str_mv Wiley
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 12.993085

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