Hyperfine interaction of individual atoms on a surface

Autores
Willke, Philip; Bae, Yujeong; Yang, Kai; Lado, Jose Luis; Ferrón, Alejandro; Choi, Taeyoung; Ardavan, Arzhang; Fernandez Rossier, Joaquín; Heinrich, Andreas; Lutz, Christopher
Año de publicación
2018
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
Taking advantage of nuclear spins for electronic structure analysis, magnetic resonance imaging, and quantum devices hinges on knowledge and control of the surrounding atomic-scale environment. We measured and manipulated the hyperfine interaction of individual iron and titanium atoms placed on a magnesium oxide surface by using spin-polarized scanning tunneling microscopy in combination with single-atom electron spin resonance. Using atom manipulation to move single atoms, we found that the hyperfine interaction strongly depended on the binding configuration of the atom. We could extract atom- and position-dependent information about the electronic ground state, the state mixing with neighboring atoms, and properties of the nuclear spin. Thus, the hyperfine spectrum becomes a powerful probe of the chemical environment of individual atoms and nanostructures.
Fil: Willke, Philip. Ewha Womans University; Corea del Norte. IBM Almaden Research Center; Estados Unidos. Institute for Basic Science; Corea del Norte
Fil: Bae, Yujeong. Ewha Womans University; Estados Unidos. Institute for Basic Science; Corea del Norte. IBM Almaden Research Center; Estados Unidos
Fil: Yang, Kai. IBM Almaden Research Center; Estados Unidos
Fil: Lado, Jose Luis. International Iberian Nanotechnology Laboratory; Portugal. Universitat Zurich; Suiza
Fil: Ferrón, Alejandro. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Nordeste. Instituto de Modelado e Innovación Tecnológica. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas Naturales y Agrimensura. Instituto de Modelado e Innovación Tecnológica; Argentina. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas y Naturales y Agrimensura. Departamento de Física; Argentina
Fil: Choi, Taeyoung. Seoul National University; Corea del Sur. Ewha Womans University; Estados Unidos
Fil: Ardavan, Arzhang. University of Oxford; Reino Unido
Fil: Fernandez Rossier, Joaquín. International Iberian Nanotechnology Laboratory; Portugal
Fil: Heinrich, Andreas. Seoul National University; Corea del Sur. Ewha Womans University; Estados Unidos
Fil: Lutz, Christopher. IBM Almaden Research Center; Estados Unidos
Materia
HYPERFINE
STM
DFT
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/86793
Acceder
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spelling Hyperfine interaction of individual atoms on a surfaceWillke, PhilipBae, YujeongYang, KaiLado, Jose LuisFerrón, AlejandroChoi, TaeyoungArdavan, ArzhangFernandez Rossier, JoaquínHeinrich, AndreasLutz, ChristopherHYPERFINESTMDFThttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1Taking advantage of nuclear spins for electronic structure analysis, magnetic resonance imaging, and quantum devices hinges on knowledge and control of the surrounding atomic-scale environment. We measured and manipulated the hyperfine interaction of individual iron and titanium atoms placed on a magnesium oxide surface by using spin-polarized scanning tunneling microscopy in combination with single-atom electron spin resonance. Using atom manipulation to move single atoms, we found that the hyperfine interaction strongly depended on the binding configuration of the atom. We could extract atom- and position-dependent information about the electronic ground state, the state mixing with neighboring atoms, and properties of the nuclear spin. Thus, the hyperfine spectrum becomes a powerful probe of the chemical environment of individual atoms and nanostructures.Fil: Willke, Philip. Ewha Womans University; Corea del Norte. IBM Almaden Research Center; Estados Unidos. Institute for Basic Science; Corea del NorteFil: Bae, Yujeong. Ewha Womans University; Estados Unidos. Institute for Basic Science; Corea del Norte. IBM Almaden Research Center; Estados UnidosFil: Yang, Kai. IBM Almaden Research Center; Estados UnidosFil: Lado, Jose Luis. International Iberian Nanotechnology Laboratory; Portugal. Universitat Zurich; SuizaFil: Ferrón, Alejandro. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Nordeste. Instituto de Modelado e Innovación Tecnológica. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas Naturales y Agrimensura. Instituto de Modelado e Innovación Tecnológica; Argentina. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas y Naturales y Agrimensura. Departamento de Física; ArgentinaFil: Choi, Taeyoung. Seoul National University; Corea del Sur. Ewha Womans University; Estados UnidosFil: Ardavan, Arzhang. University of Oxford; Reino UnidoFil: Fernandez Rossier, Joaquín. International Iberian Nanotechnology Laboratory; PortugalFil: Heinrich, Andreas. Seoul National University; Corea del Sur. Ewha Womans University; Estados UnidosFil: Lutz, Christopher. IBM Almaden Research Center; Estados UnidosAmerican Association for the Advancement of Science2018-10info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/86793Willke, Philip; Bae, Yujeong; Yang, Kai; Lado, Jose Luis; Ferrón, Alejandro; et al.; Hyperfine interaction of individual atoms on a surface; American Association for the Advancement of Science; Science; 362; 6412; 10-2018; 336-3390036-80751095-9203CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/http://science.sciencemag.org/content/362/6412/336info:eu-repo/semantics/altIdentifier/doi/10.1126/science.aat7047info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-10-22T11:44:25Zoai:ri.conicet.gov.ar:11336/86793instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-10-22 11:44:25.651CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Hyperfine interaction of individual atoms on a surface
title Hyperfine interaction of individual atoms on a surface
spellingShingle Hyperfine interaction of individual atoms on a surface
Willke, Philip
HYPERFINE
STM
DFT
title_short Hyperfine interaction of individual atoms on a surface
title_full Hyperfine interaction of individual atoms on a surface
title_fullStr Hyperfine interaction of individual atoms on a surface
title_full_unstemmed Hyperfine interaction of individual atoms on a surface
title_sort Hyperfine interaction of individual atoms on a surface
dc.creator.none.fl_str_mv Willke, Philip
Bae, Yujeong
Yang, Kai
Lado, Jose Luis
Ferrón, Alejandro
Choi, Taeyoung
Ardavan, Arzhang
Fernandez Rossier, Joaquín
Heinrich, Andreas
Lutz, Christopher
author Willke, Philip
author_facet Willke, Philip
Bae, Yujeong
Yang, Kai
Lado, Jose Luis
Ferrón, Alejandro
Choi, Taeyoung
Ardavan, Arzhang
Fernandez Rossier, Joaquín
Heinrich, Andreas
Lutz, Christopher
author_role author
author2 Bae, Yujeong
Yang, Kai
Lado, Jose Luis
Ferrón, Alejandro
Choi, Taeyoung
Ardavan, Arzhang
Fernandez Rossier, Joaquín
Heinrich, Andreas
Lutz, Christopher
author2_role author
author
author
author
author
author
author
author
author
dc.subject.none.fl_str_mv HYPERFINE
STM
DFT
topic HYPERFINE
STM
DFT
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv Taking advantage of nuclear spins for electronic structure analysis, magnetic resonance imaging, and quantum devices hinges on knowledge and control of the surrounding atomic-scale environment. We measured and manipulated the hyperfine interaction of individual iron and titanium atoms placed on a magnesium oxide surface by using spin-polarized scanning tunneling microscopy in combination with single-atom electron spin resonance. Using atom manipulation to move single atoms, we found that the hyperfine interaction strongly depended on the binding configuration of the atom. We could extract atom- and position-dependent information about the electronic ground state, the state mixing with neighboring atoms, and properties of the nuclear spin. Thus, the hyperfine spectrum becomes a powerful probe of the chemical environment of individual atoms and nanostructures.
Fil: Willke, Philip. Ewha Womans University; Corea del Norte. IBM Almaden Research Center; Estados Unidos. Institute for Basic Science; Corea del Norte
Fil: Bae, Yujeong. Ewha Womans University; Estados Unidos. Institute for Basic Science; Corea del Norte. IBM Almaden Research Center; Estados Unidos
Fil: Yang, Kai. IBM Almaden Research Center; Estados Unidos
Fil: Lado, Jose Luis. International Iberian Nanotechnology Laboratory; Portugal. Universitat Zurich; Suiza
Fil: Ferrón, Alejandro. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Nordeste. Instituto de Modelado e Innovación Tecnológica. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas Naturales y Agrimensura. Instituto de Modelado e Innovación Tecnológica; Argentina. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas y Naturales y Agrimensura. Departamento de Física; Argentina
Fil: Choi, Taeyoung. Seoul National University; Corea del Sur. Ewha Womans University; Estados Unidos
Fil: Ardavan, Arzhang. University of Oxford; Reino Unido
Fil: Fernandez Rossier, Joaquín. International Iberian Nanotechnology Laboratory; Portugal
Fil: Heinrich, Andreas. Seoul National University; Corea del Sur. Ewha Womans University; Estados Unidos
Fil: Lutz, Christopher. IBM Almaden Research Center; Estados Unidos
description Taking advantage of nuclear spins for electronic structure analysis, magnetic resonance imaging, and quantum devices hinges on knowledge and control of the surrounding atomic-scale environment. We measured and manipulated the hyperfine interaction of individual iron and titanium atoms placed on a magnesium oxide surface by using spin-polarized scanning tunneling microscopy in combination with single-atom electron spin resonance. Using atom manipulation to move single atoms, we found that the hyperfine interaction strongly depended on the binding configuration of the atom. We could extract atom- and position-dependent information about the electronic ground state, the state mixing with neighboring atoms, and properties of the nuclear spin. Thus, the hyperfine spectrum becomes a powerful probe of the chemical environment of individual atoms and nanostructures.
publishDate 2018
dc.date.none.fl_str_mv 2018-10
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/86793
Willke, Philip; Bae, Yujeong; Yang, Kai; Lado, Jose Luis; Ferrón, Alejandro; et al.; Hyperfine interaction of individual atoms on a surface; American Association for the Advancement of Science; Science; 362; 6412; 10-2018; 336-339
0036-8075
1095-9203
CONICET Digital
CONICET
url http://hdl.handle.net/11336/86793
identifier_str_mv Willke, Philip; Bae, Yujeong; Yang, Kai; Lado, Jose Luis; Ferrón, Alejandro; et al.; Hyperfine interaction of individual atoms on a surface; American Association for the Advancement of Science; Science; 362; 6412; 10-2018; 336-339
0036-8075
1095-9203
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/http://science.sciencemag.org/content/362/6412/336
info:eu-repo/semantics/altIdentifier/doi/10.1126/science.aat7047
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv American Association for the Advancement of Science
publisher.none.fl_str_mv American Association for the Advancement of Science
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
_version_ 1846782138657013760
score 12.982451

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