Ce-Mn mixed oxides as supports of copper- and nickel-based catalysts for water-gas shift reaction
- Autores
- Poggio Fraccari, Eduardo Arístides; D'alessandro, Oriana; Sambeth, Jorge Enrique; Baronetti, Graciela Teresita; Mariño, Fernando Javier
- Año de publicación
- 2014
- Idioma
- inglés
- Tipo de recurso
- artículo
- Estado
- versión publicada
- Descripción
- Cerium-manganese mixed oxides with different composition were prepared by co-precipitation, characterized and evaluated for the water–gas shift (WGS) reaction. Base metal (5 wt.% Cu and 5 wt.% Ni) catalysts supported on Ce–Mn mixed oxides were also tested for the WGS reaction. The activity of the bare supports is higher in the mixed samples than in pure ceria or manganese oxide. This result can be explained by a combination of greater reducibility and surface area in the mixed samples. Addition of base metals produces superior WGS catalysts. Particularly, nickel catalysts tested are able to reduce typical CO concentrations entering the WGS process to the CO levels tolerated by phosphoric acid fuel cells in a single unit operated at 400 °C.
Fil: Poggio Fraccari, Eduardo Arístides. Universidad de Buenos Aires. Facultad de Ingenieria. Departamento de Ingenieria Quimica. Laboratorio de Procesos Cataliticos; Argentina
Fil: D'alessandro, Oriana. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Centro de Investigación y Desarrollo En Ciencias Aplicadas; Argentina
Fil: Sambeth, Jorge Enrique. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Centro de Investigación y Desarrollo En Ciencias Aplicadas; Argentina
Fil: Baronetti, Graciela Teresita. Universidad de Buenos Aires. Facultad de Ingenieria. Departamento de Ingenieria Quimica. Laboratorio de Procesos Cataliticos; Argentina
Fil: Mariño, Fernando Javier. Universidad de Buenos Aires. Facultad de Ingenieria. Departamento de Ingenieria Quimica. Laboratorio de Procesos Cataliticos; Argentina - Materia
-
Watergas Shift Reaction
Copper
Nickel
Cerium
Manganese
Fuel Cells - Nivel de accesibilidad
- acceso abierto
- Condiciones de uso
- https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
- Repositorio
- Institución
- Consejo Nacional de Investigaciones Científicas y Técnicas
- OAI Identificador
- oai:ri.conicet.gov.ar:11336/5266
Ver los metadatos del registro completo
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spelling |
Ce-Mn mixed oxides as supports of copper- and nickel-based catalysts for water-gas shift reactionPoggio Fraccari, Eduardo ArístidesD'alessandro, OrianaSambeth, Jorge EnriqueBaronetti, Graciela TeresitaMariño, Fernando JavierWatergas Shift ReactionCopperNickelCeriumManganeseFuel Cellshttps://purl.org/becyt/ford/2.4https://purl.org/becyt/ford/2Cerium-manganese mixed oxides with different composition were prepared by co-precipitation, characterized and evaluated for the water–gas shift (WGS) reaction. Base metal (5 wt.% Cu and 5 wt.% Ni) catalysts supported on Ce–Mn mixed oxides were also tested for the WGS reaction. The activity of the bare supports is higher in the mixed samples than in pure ceria or manganese oxide. This result can be explained by a combination of greater reducibility and surface area in the mixed samples. Addition of base metals produces superior WGS catalysts. Particularly, nickel catalysts tested are able to reduce typical CO concentrations entering the WGS process to the CO levels tolerated by phosphoric acid fuel cells in a single unit operated at 400 °C.Fil: Poggio Fraccari, Eduardo Arístides. Universidad de Buenos Aires. Facultad de Ingenieria. Departamento de Ingenieria Quimica. Laboratorio de Procesos Cataliticos; ArgentinaFil: D'alessandro, Oriana. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Centro de Investigación y Desarrollo En Ciencias Aplicadas; ArgentinaFil: Sambeth, Jorge Enrique. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Centro de Investigación y Desarrollo En Ciencias Aplicadas; ArgentinaFil: Baronetti, Graciela Teresita. Universidad de Buenos Aires. Facultad de Ingenieria. Departamento de Ingenieria Quimica. Laboratorio de Procesos Cataliticos; ArgentinaFil: Mariño, Fernando Javier. Universidad de Buenos Aires. Facultad de Ingenieria. Departamento de Ingenieria Quimica. Laboratorio de Procesos Cataliticos; ArgentinaElsevier2014-03info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfapplication/pdfapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/5266Poggio Fraccari, Eduardo Arístides; D'alessandro, Oriana; Sambeth, Jorge Enrique; Baronetti, Graciela Teresita; Mariño, Fernando Javier; Ce-Mn mixed oxides as supports of copper- and nickel-based catalysts for water-gas shift reaction; Elsevier; Fuel Processing Technology; 119; 3-2014; 67-730378-3820enginfo:eu-repo/semantics/altIdentifier/url/http://www.sciencedirect.com/science/article/pii/S0378382013003263info:eu-repo/semantics/altIdentifier/doi/10.1016/j.fuproc.2013.10.012info:eu-repo/semantics/altIdentifier/doi/info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-nd/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T10:41:53Zoai:ri.conicet.gov.ar:11336/5266instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 10:41:53.812CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse |
dc.title.none.fl_str_mv |
Ce-Mn mixed oxides as supports of copper- and nickel-based catalysts for water-gas shift reaction |
title |
Ce-Mn mixed oxides as supports of copper- and nickel-based catalysts for water-gas shift reaction |
spellingShingle |
Ce-Mn mixed oxides as supports of copper- and nickel-based catalysts for water-gas shift reaction Poggio Fraccari, Eduardo Arístides Watergas Shift Reaction Copper Nickel Cerium Manganese Fuel Cells |
title_short |
Ce-Mn mixed oxides as supports of copper- and nickel-based catalysts for water-gas shift reaction |
title_full |
Ce-Mn mixed oxides as supports of copper- and nickel-based catalysts for water-gas shift reaction |
title_fullStr |
Ce-Mn mixed oxides as supports of copper- and nickel-based catalysts for water-gas shift reaction |
title_full_unstemmed |
Ce-Mn mixed oxides as supports of copper- and nickel-based catalysts for water-gas shift reaction |
title_sort |
Ce-Mn mixed oxides as supports of copper- and nickel-based catalysts for water-gas shift reaction |
dc.creator.none.fl_str_mv |
Poggio Fraccari, Eduardo Arístides D'alessandro, Oriana Sambeth, Jorge Enrique Baronetti, Graciela Teresita Mariño, Fernando Javier |
author |
Poggio Fraccari, Eduardo Arístides |
author_facet |
Poggio Fraccari, Eduardo Arístides D'alessandro, Oriana Sambeth, Jorge Enrique Baronetti, Graciela Teresita Mariño, Fernando Javier |
author_role |
author |
author2 |
D'alessandro, Oriana Sambeth, Jorge Enrique Baronetti, Graciela Teresita Mariño, Fernando Javier |
author2_role |
author author author author |
dc.subject.none.fl_str_mv |
Watergas Shift Reaction Copper Nickel Cerium Manganese Fuel Cells |
topic |
Watergas Shift Reaction Copper Nickel Cerium Manganese Fuel Cells |
purl_subject.fl_str_mv |
https://purl.org/becyt/ford/2.4 https://purl.org/becyt/ford/2 |
dc.description.none.fl_txt_mv |
Cerium-manganese mixed oxides with different composition were prepared by co-precipitation, characterized and evaluated for the water–gas shift (WGS) reaction. Base metal (5 wt.% Cu and 5 wt.% Ni) catalysts supported on Ce–Mn mixed oxides were also tested for the WGS reaction. The activity of the bare supports is higher in the mixed samples than in pure ceria or manganese oxide. This result can be explained by a combination of greater reducibility and surface area in the mixed samples. Addition of base metals produces superior WGS catalysts. Particularly, nickel catalysts tested are able to reduce typical CO concentrations entering the WGS process to the CO levels tolerated by phosphoric acid fuel cells in a single unit operated at 400 °C. Fil: Poggio Fraccari, Eduardo Arístides. Universidad de Buenos Aires. Facultad de Ingenieria. Departamento de Ingenieria Quimica. Laboratorio de Procesos Cataliticos; Argentina Fil: D'alessandro, Oriana. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Centro de Investigación y Desarrollo En Ciencias Aplicadas; Argentina Fil: Sambeth, Jorge Enrique. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico la Plata. Centro de Investigación y Desarrollo En Ciencias Aplicadas; Argentina Fil: Baronetti, Graciela Teresita. Universidad de Buenos Aires. Facultad de Ingenieria. Departamento de Ingenieria Quimica. Laboratorio de Procesos Cataliticos; Argentina Fil: Mariño, Fernando Javier. Universidad de Buenos Aires. Facultad de Ingenieria. Departamento de Ingenieria Quimica. Laboratorio de Procesos Cataliticos; Argentina |
description |
Cerium-manganese mixed oxides with different composition were prepared by co-precipitation, characterized and evaluated for the water–gas shift (WGS) reaction. Base metal (5 wt.% Cu and 5 wt.% Ni) catalysts supported on Ce–Mn mixed oxides were also tested for the WGS reaction. The activity of the bare supports is higher in the mixed samples than in pure ceria or manganese oxide. This result can be explained by a combination of greater reducibility and surface area in the mixed samples. Addition of base metals produces superior WGS catalysts. Particularly, nickel catalysts tested are able to reduce typical CO concentrations entering the WGS process to the CO levels tolerated by phosphoric acid fuel cells in a single unit operated at 400 °C. |
publishDate |
2014 |
dc.date.none.fl_str_mv |
2014-03 |
dc.type.none.fl_str_mv |
info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion http://purl.org/coar/resource_type/c_6501 info:ar-repo/semantics/articulo |
format |
article |
status_str |
publishedVersion |
dc.identifier.none.fl_str_mv |
http://hdl.handle.net/11336/5266 Poggio Fraccari, Eduardo Arístides; D'alessandro, Oriana; Sambeth, Jorge Enrique; Baronetti, Graciela Teresita; Mariño, Fernando Javier; Ce-Mn mixed oxides as supports of copper- and nickel-based catalysts for water-gas shift reaction; Elsevier; Fuel Processing Technology; 119; 3-2014; 67-73 0378-3820 |
url |
http://hdl.handle.net/11336/5266 |
identifier_str_mv |
Poggio Fraccari, Eduardo Arístides; D'alessandro, Oriana; Sambeth, Jorge Enrique; Baronetti, Graciela Teresita; Mariño, Fernando Javier; Ce-Mn mixed oxides as supports of copper- and nickel-based catalysts for water-gas shift reaction; Elsevier; Fuel Processing Technology; 119; 3-2014; 67-73 0378-3820 |
dc.language.none.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
info:eu-repo/semantics/altIdentifier/url/http://www.sciencedirect.com/science/article/pii/S0378382013003263 info:eu-repo/semantics/altIdentifier/doi/10.1016/j.fuproc.2013.10.012 info:eu-repo/semantics/altIdentifier/doi/ |
dc.rights.none.fl_str_mv |
info:eu-repo/semantics/openAccess https://creativecommons.org/licenses/by-nc-nd/2.5/ar/ |
eu_rights_str_mv |
openAccess |
rights_invalid_str_mv |
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/ |
dc.format.none.fl_str_mv |
application/pdf application/pdf application/pdf application/pdf application/pdf application/pdf application/pdf |
dc.publisher.none.fl_str_mv |
Elsevier |
publisher.none.fl_str_mv |
Elsevier |
dc.source.none.fl_str_mv |
reponame:CONICET Digital (CONICET) instname:Consejo Nacional de Investigaciones Científicas y Técnicas |
reponame_str |
CONICET Digital (CONICET) |
collection |
CONICET Digital (CONICET) |
instname_str |
Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.name.fl_str_mv |
CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.mail.fl_str_mv |
dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar |
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1844614450772967424 |
score |
13.070432 |