Structure, configuration, and sizing of Ni nanoparticles generated by ultrafast laser ablation in different media

Autores
Muñetón Arboleda, David; Santillán, Jesica María José; Mendoza Herrera, Luis Joaquin; Fernandez Van Raap, Marcela Beatriz; Muraca, Diego; Schinca, D. C.; Scaffardi, Lucia Beatriz
Año de publicación
2015
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
In recent years, nickel nanoparticles (NPs) have increased scientific interest because of their extensive prospects in catalysts, information storage, large-scale batteries and biomedicine. Several works on Ni NPs generation by laser ablation have appeared in the literature in the last years, using different pulsed laser regimes and different media have been published recently. In this work we analyze the characteristics of species, structure (bare core or core-shell), configuration and size distribution of NPs generated by fs pulse laser ablation over a Ni solid target in n-heptane and water. We explore the presence of NiO-Ni core-shell and hollow Ni (or air-Ni) NPs in the colloids obtained. These were experimentally characterized using AFM and TEM microscopy, as well as Optical Extinction Spectroscopy (OES). Extinction spectra were modeled using Mie theory through an appropriate modification of the complex experimental dielectric function, taking into account a size-dependent corrective term for each free and bound electron contribution. Experimental UVvisible-NIR spectra were reproduced considering a size distribution of bare core, hollow and core-shell structures NPs. In both media, Ni NPs shape and size distribution agrees with that derived from TEM and AFM analysis.
Fil: Muñetón Arboleda, David. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Centro de Investigaciones Opticas (i); Argentina. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas; Argentina
Fil: Santillán, Jesica María José. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Centro de Investigaciones Opticas (i); Argentina. Universidad Nacional de Catamarca. Facultad de Ciencias Exactas y Naturales; Argentina. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas; Argentina
Fil: Mendoza Herrera, Luis Joaquin. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Centro de Investigaciones Opticas (i); Argentina. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas; Argentina
Fil: Fernandez Van Raap, Marcela Beatriz. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Instituto de Física La Plata; Argentina. Universidad Nacional de la Plata. Facultad de Ciencias Exactas. Departamento de Física; Argentina
Fil: Muraca, Diego. Universidade Estadual de Campinas; Brasil. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Schinca, D. C.. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Centro de Investigaciones Opticas (i); Argentina. Universidad Nacional de La Plata. Facultad de Ingenieria; Argentina. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas; Argentina
Fil: Scaffardi, Lucia Beatriz. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Centro de Investigaciones Opticas (i); Argentina. Universidad Nacional de La Plata. Facultad de Ingenieria; Argentina. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas; Argentina
Materia
Nickel Colloidal Suspensions
Nickel Dielectric Function
Optical Extinction Spectroscopy
Femtosecond Pulse Laser Ablation
Hollow Nanoparticles
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/11883
Acceder
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repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Structure, configuration, and sizing of Ni nanoparticles generated by ultrafast laser ablation in different mediaMuñetón Arboleda, DavidSantillán, Jesica María JoséMendoza Herrera, Luis JoaquinFernandez Van Raap, Marcela BeatrizMuraca, DiegoSchinca, D. C.Scaffardi, Lucia BeatrizNickel Colloidal SuspensionsNickel Dielectric FunctionOptical Extinction SpectroscopyFemtosecond Pulse Laser AblationHollow Nanoparticleshttps://purl.org/becyt/ford/2.10https://purl.org/becyt/ford/2In recent years, nickel nanoparticles (NPs) have increased scientific interest because of their extensive prospects in catalysts, information storage, large-scale batteries and biomedicine. Several works on Ni NPs generation by laser ablation have appeared in the literature in the last years, using different pulsed laser regimes and different media have been published recently. In this work we analyze the characteristics of species, structure (bare core or core-shell), configuration and size distribution of NPs generated by fs pulse laser ablation over a Ni solid target in n-heptane and water. We explore the presence of NiO-Ni core-shell and hollow Ni (or air-Ni) NPs in the colloids obtained. These were experimentally characterized using AFM and TEM microscopy, as well as Optical Extinction Spectroscopy (OES). Extinction spectra were modeled using Mie theory through an appropriate modification of the complex experimental dielectric function, taking into account a size-dependent corrective term for each free and bound electron contribution. Experimental UVvisible-NIR spectra were reproduced considering a size distribution of bare core, hollow and core-shell structures NPs. In both media, Ni NPs shape and size distribution agrees with that derived from TEM and AFM analysis.Fil: Muñetón Arboleda, David. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Centro de Investigaciones Opticas (i); Argentina. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas; ArgentinaFil: Santillán, Jesica María José. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Centro de Investigaciones Opticas (i); Argentina. Universidad Nacional de Catamarca. Facultad de Ciencias Exactas y Naturales; Argentina. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas; ArgentinaFil: Mendoza Herrera, Luis Joaquin. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Centro de Investigaciones Opticas (i); Argentina. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas; ArgentinaFil: Fernandez Van Raap, Marcela Beatriz. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Instituto de Física La Plata; Argentina. Universidad Nacional de la Plata. Facultad de Ciencias Exactas. Departamento de Física; ArgentinaFil: Muraca, Diego. Universidade Estadual de Campinas; Brasil. Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaFil: Schinca, D. C.. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Centro de Investigaciones Opticas (i); Argentina. Universidad Nacional de La Plata. Facultad de Ingenieria; Argentina. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas; ArgentinaFil: Scaffardi, Lucia Beatriz. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Centro de Investigaciones Opticas (i); Argentina. Universidad Nacional de La Plata. Facultad de Ingenieria; Argentina. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas; ArgentinaSpie2015-08info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/11883Muñetón Arboleda, David; Santillán, Jesica María José; Mendoza Herrera, Luis Joaquin; Fernandez Van Raap, Marcela Beatriz; Muraca, Diego; et al.; Structure, configuration, and sizing of Ni nanoparticles generated by ultrafast laser ablation in different media; Spie; Spie; 9547; 8-2015; 1-9; 95473J-10277-786Xenginfo:eu-repo/semantics/altIdentifier/url/http://dx.doi.org/10.1117/12.2190421info:eu-repo/semantics/altIdentifier/url/http://proceedings.spiedigitallibrary.org/proceeding.aspx?articleid=2432871info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-03T09:44:58Zoai:ri.conicet.gov.ar:11336/11883instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-03 09:44:58.541CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Structure, configuration, and sizing of Ni nanoparticles generated by ultrafast laser ablation in different media
title Structure, configuration, and sizing of Ni nanoparticles generated by ultrafast laser ablation in different media
spellingShingle Structure, configuration, and sizing of Ni nanoparticles generated by ultrafast laser ablation in different media
Muñetón Arboleda, David
Nickel Colloidal Suspensions
Nickel Dielectric Function
Optical Extinction Spectroscopy
Femtosecond Pulse Laser Ablation
Hollow Nanoparticles
title_short Structure, configuration, and sizing of Ni nanoparticles generated by ultrafast laser ablation in different media
title_full Structure, configuration, and sizing of Ni nanoparticles generated by ultrafast laser ablation in different media
title_fullStr Structure, configuration, and sizing of Ni nanoparticles generated by ultrafast laser ablation in different media
title_full_unstemmed Structure, configuration, and sizing of Ni nanoparticles generated by ultrafast laser ablation in different media
title_sort Structure, configuration, and sizing of Ni nanoparticles generated by ultrafast laser ablation in different media
dc.creator.none.fl_str_mv Muñetón Arboleda, David
Santillán, Jesica María José
Mendoza Herrera, Luis Joaquin
Fernandez Van Raap, Marcela Beatriz
Muraca, Diego
Schinca, D. C.
Scaffardi, Lucia Beatriz
author Muñetón Arboleda, David
author_facet Muñetón Arboleda, David
Santillán, Jesica María José
Mendoza Herrera, Luis Joaquin
Fernandez Van Raap, Marcela Beatriz
Muraca, Diego
Schinca, D. C.
Scaffardi, Lucia Beatriz
author_role author
author2 Santillán, Jesica María José
Mendoza Herrera, Luis Joaquin
Fernandez Van Raap, Marcela Beatriz
Muraca, Diego
Schinca, D. C.
Scaffardi, Lucia Beatriz
author2_role author
author
author
author
author
author
dc.subject.none.fl_str_mv Nickel Colloidal Suspensions
Nickel Dielectric Function
Optical Extinction Spectroscopy
Femtosecond Pulse Laser Ablation
Hollow Nanoparticles
topic Nickel Colloidal Suspensions
Nickel Dielectric Function
Optical Extinction Spectroscopy
Femtosecond Pulse Laser Ablation
Hollow Nanoparticles
purl_subject.fl_str_mv https://purl.org/becyt/ford/2.10
https://purl.org/becyt/ford/2
dc.description.none.fl_txt_mv In recent years, nickel nanoparticles (NPs) have increased scientific interest because of their extensive prospects in catalysts, information storage, large-scale batteries and biomedicine. Several works on Ni NPs generation by laser ablation have appeared in the literature in the last years, using different pulsed laser regimes and different media have been published recently. In this work we analyze the characteristics of species, structure (bare core or core-shell), configuration and size distribution of NPs generated by fs pulse laser ablation over a Ni solid target in n-heptane and water. We explore the presence of NiO-Ni core-shell and hollow Ni (or air-Ni) NPs in the colloids obtained. These were experimentally characterized using AFM and TEM microscopy, as well as Optical Extinction Spectroscopy (OES). Extinction spectra were modeled using Mie theory through an appropriate modification of the complex experimental dielectric function, taking into account a size-dependent corrective term for each free and bound electron contribution. Experimental UVvisible-NIR spectra were reproduced considering a size distribution of bare core, hollow and core-shell structures NPs. In both media, Ni NPs shape and size distribution agrees with that derived from TEM and AFM analysis.
Fil: Muñetón Arboleda, David. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Centro de Investigaciones Opticas (i); Argentina. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas; Argentina
Fil: Santillán, Jesica María José. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Centro de Investigaciones Opticas (i); Argentina. Universidad Nacional de Catamarca. Facultad de Ciencias Exactas y Naturales; Argentina. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas; Argentina
Fil: Mendoza Herrera, Luis Joaquin. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Centro de Investigaciones Opticas (i); Argentina. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas; Argentina
Fil: Fernandez Van Raap, Marcela Beatriz. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Instituto de Física La Plata; Argentina. Universidad Nacional de la Plata. Facultad de Ciencias Exactas. Departamento de Física; Argentina
Fil: Muraca, Diego. Universidade Estadual de Campinas; Brasil. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Schinca, D. C.. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Centro de Investigaciones Opticas (i); Argentina. Universidad Nacional de La Plata. Facultad de Ingenieria; Argentina. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas; Argentina
Fil: Scaffardi, Lucia Beatriz. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico La Plata. Centro de Investigaciones Opticas (i); Argentina. Universidad Nacional de La Plata. Facultad de Ingenieria; Argentina. Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas; Argentina
description In recent years, nickel nanoparticles (NPs) have increased scientific interest because of their extensive prospects in catalysts, information storage, large-scale batteries and biomedicine. Several works on Ni NPs generation by laser ablation have appeared in the literature in the last years, using different pulsed laser regimes and different media have been published recently. In this work we analyze the characteristics of species, structure (bare core or core-shell), configuration and size distribution of NPs generated by fs pulse laser ablation over a Ni solid target in n-heptane and water. We explore the presence of NiO-Ni core-shell and hollow Ni (or air-Ni) NPs in the colloids obtained. These were experimentally characterized using AFM and TEM microscopy, as well as Optical Extinction Spectroscopy (OES). Extinction spectra were modeled using Mie theory through an appropriate modification of the complex experimental dielectric function, taking into account a size-dependent corrective term for each free and bound electron contribution. Experimental UVvisible-NIR spectra were reproduced considering a size distribution of bare core, hollow and core-shell structures NPs. In both media, Ni NPs shape and size distribution agrees with that derived from TEM and AFM analysis.
publishDate 2015
dc.date.none.fl_str_mv 2015-08
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/11883
Muñetón Arboleda, David; Santillán, Jesica María José; Mendoza Herrera, Luis Joaquin; Fernandez Van Raap, Marcela Beatriz; Muraca, Diego; et al.; Structure, configuration, and sizing of Ni nanoparticles generated by ultrafast laser ablation in different media; Spie; Spie; 9547; 8-2015; 1-9; 95473J-1
0277-786X
url http://hdl.handle.net/11336/11883
identifier_str_mv Muñetón Arboleda, David; Santillán, Jesica María José; Mendoza Herrera, Luis Joaquin; Fernandez Van Raap, Marcela Beatriz; Muraca, Diego; et al.; Structure, configuration, and sizing of Ni nanoparticles generated by ultrafast laser ablation in different media; Spie; Spie; 9547; 8-2015; 1-9; 95473J-1
0277-786X
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/http://dx.doi.org/10.1117/12.2190421
info:eu-repo/semantics/altIdentifier/url/http://proceedings.spiedigitallibrary.org/proceeding.aspx?articleid=2432871
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
application/pdf
application/pdf
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dc.publisher.none.fl_str_mv Spie
publisher.none.fl_str_mv Spie
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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