Membrane-based processes: Optimization of hydrogen separation by minimization of power, membrane area, and cost

Autores
Mores, Patricia Liliana; Arias, Ana Marisa; Scenna, Nicolas Jose; Caballero, José A.; Mussati, Sergio Fabian; Mussati, Miguel Ceferino
Año de publicación
2018
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
This work deals with the optimization of two-stage membrane systems for H2 separation from off-gases in hydrocarbons processing plants to simultaneously attain high values of both H2 recovery and H2 product purity. First, for a given H2 recovery level of 90%, optimizations of the total annual cost (TAC) are performed for desired H2 product purity values ranging between 0.90 and 0.95 mole fraction. One of the results showed that the contribution of the operating expenditures is more significant than the contribution of the annualized capital expenditures (approximately 62% and 38%, respectively). In addition, it was found that the optimal trade-offs existing between process variables (such as total membrane area and total electric power) depend on the specified H2 product purity level. Second, the minimization of the total power demand and the minimization of the total membrane area were performed for H2 recovery of 90% and H2 product purity of 0.90. The TAC values obtained in the first and second cases increased by 19.9% and 4.9%, respectively, with respect to that obtained by cost minimization. Finally, by analyzing and comparing the three optimal solutions, a strategy to systematically and rationally provide 'good' lower and upper bounds for model variables and initial guess values to solve the cost minimization problem by means of global optimization algorithms is proposed, which can be straightforward applied to other processes.
Fil: Mores, Patricia Liliana. Universidad Tecnológica Nacional; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario; Argentina
Fil: Arias, Ana Marisa. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario; Argentina. Universidad Tecnológica Nacional; Argentina
Fil: Scenna, Nicolas Jose. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario; Argentina. Universidad Tecnológica Nacional; Argentina
Fil: Caballero, José A.. Universidad de Alicante; España
Fil: Mussati, Sergio Fabian. Universidad Tecnológica Nacional; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Desarrollo y Diseño. Universidad Tecnológica Nacional. Facultad Regional Santa Fe. Instituto de Desarrollo y Diseño; Argentina
Fil: Mussati, Miguel Ceferino. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Desarrollo y Diseño. Universidad Tecnológica Nacional. Facultad Regional Santa Fe. Instituto de Desarrollo y Diseño; Argentina
Materia
COST
DESIGN
ENERGY
GAMS
H2 SEPARATION
MATHEMATICAL PROGRAMMING
MEMBRANE AREA
MEMBRANES
MULTI-STAGE PROCESS
NLP
OPERATION
OPTIMIZATION
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/91826
Acceder
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oai_identifier_str oai:ri.conicet.gov.ar:11336/91826
network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Membrane-based processes: Optimization of hydrogen separation by minimization of power, membrane area, and costMores, Patricia LilianaArias, Ana MarisaScenna, Nicolas JoseCaballero, José A.Mussati, Sergio FabianMussati, Miguel CeferinoCOSTDESIGNENERGYGAMSH2 SEPARATIONMATHEMATICAL PROGRAMMINGMEMBRANE AREAMEMBRANESMULTI-STAGE PROCESSNLPOPERATIONOPTIMIZATIONhttps://purl.org/becyt/ford/2.4https://purl.org/becyt/ford/2This work deals with the optimization of two-stage membrane systems for H2 separation from off-gases in hydrocarbons processing plants to simultaneously attain high values of both H2 recovery and H2 product purity. First, for a given H2 recovery level of 90%, optimizations of the total annual cost (TAC) are performed for desired H2 product purity values ranging between 0.90 and 0.95 mole fraction. One of the results showed that the contribution of the operating expenditures is more significant than the contribution of the annualized capital expenditures (approximately 62% and 38%, respectively). In addition, it was found that the optimal trade-offs existing between process variables (such as total membrane area and total electric power) depend on the specified H2 product purity level. Second, the minimization of the total power demand and the minimization of the total membrane area were performed for H2 recovery of 90% and H2 product purity of 0.90. The TAC values obtained in the first and second cases increased by 19.9% and 4.9%, respectively, with respect to that obtained by cost minimization. Finally, by analyzing and comparing the three optimal solutions, a strategy to systematically and rationally provide 'good' lower and upper bounds for model variables and initial guess values to solve the cost minimization problem by means of global optimization algorithms is proposed, which can be straightforward applied to other processes.Fil: Mores, Patricia Liliana. Universidad Tecnológica Nacional; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario; ArgentinaFil: Arias, Ana Marisa. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario; Argentina. Universidad Tecnológica Nacional; ArgentinaFil: Scenna, Nicolas Jose. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario; Argentina. Universidad Tecnológica Nacional; ArgentinaFil: Caballero, José A.. Universidad de Alicante; EspañaFil: Mussati, Sergio Fabian. Universidad Tecnológica Nacional; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Desarrollo y Diseño. Universidad Tecnológica Nacional. Facultad Regional Santa Fe. Instituto de Desarrollo y Diseño; ArgentinaFil: Mussati, Miguel Ceferino. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Desarrollo y Diseño. Universidad Tecnológica Nacional. Facultad Regional Santa Fe. Instituto de Desarrollo y Diseño; ArgentinaMDPI2018-11info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/91826Mores, Patricia Liliana; Arias, Ana Marisa; Scenna, Nicolas Jose; Caballero, José A.; Mussati, Sergio Fabian; et al.; Membrane-based processes: Optimization of hydrogen separation by minimization of power, membrane area, and cost; MDPI; Processes; 6; 11; 11-2018; 1-202227-9717CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/http://www.mdpi.com/2227-9717/6/11/221info:eu-repo/semantics/altIdentifier/doi/10.3390/pr6110221info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T10:24:47Zoai:ri.conicet.gov.ar:11336/91826instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 10:24:47.53CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Membrane-based processes: Optimization of hydrogen separation by minimization of power, membrane area, and cost
title Membrane-based processes: Optimization of hydrogen separation by minimization of power, membrane area, and cost
spellingShingle Membrane-based processes: Optimization of hydrogen separation by minimization of power, membrane area, and cost
Mores, Patricia Liliana
COST
DESIGN
ENERGY
GAMS
H2 SEPARATION
MATHEMATICAL PROGRAMMING
MEMBRANE AREA
MEMBRANES
MULTI-STAGE PROCESS
NLP
OPERATION
OPTIMIZATION
title_short Membrane-based processes: Optimization of hydrogen separation by minimization of power, membrane area, and cost
title_full Membrane-based processes: Optimization of hydrogen separation by minimization of power, membrane area, and cost
title_fullStr Membrane-based processes: Optimization of hydrogen separation by minimization of power, membrane area, and cost
title_full_unstemmed Membrane-based processes: Optimization of hydrogen separation by minimization of power, membrane area, and cost
title_sort Membrane-based processes: Optimization of hydrogen separation by minimization of power, membrane area, and cost
dc.creator.none.fl_str_mv Mores, Patricia Liliana
Arias, Ana Marisa
Scenna, Nicolas Jose
Caballero, José A.
Mussati, Sergio Fabian
Mussati, Miguel Ceferino
author Mores, Patricia Liliana
author_facet Mores, Patricia Liliana
Arias, Ana Marisa
Scenna, Nicolas Jose
Caballero, José A.
Mussati, Sergio Fabian
Mussati, Miguel Ceferino
author_role author
author2 Arias, Ana Marisa
Scenna, Nicolas Jose
Caballero, José A.
Mussati, Sergio Fabian
Mussati, Miguel Ceferino
author2_role author
author
author
author
author
dc.subject.none.fl_str_mv COST
DESIGN
ENERGY
GAMS
H2 SEPARATION
MATHEMATICAL PROGRAMMING
MEMBRANE AREA
MEMBRANES
MULTI-STAGE PROCESS
NLP
OPERATION
OPTIMIZATION
topic COST
DESIGN
ENERGY
GAMS
H2 SEPARATION
MATHEMATICAL PROGRAMMING
MEMBRANE AREA
MEMBRANES
MULTI-STAGE PROCESS
NLP
OPERATION
OPTIMIZATION
purl_subject.fl_str_mv https://purl.org/becyt/ford/2.4
https://purl.org/becyt/ford/2
dc.description.none.fl_txt_mv This work deals with the optimization of two-stage membrane systems for H2 separation from off-gases in hydrocarbons processing plants to simultaneously attain high values of both H2 recovery and H2 product purity. First, for a given H2 recovery level of 90%, optimizations of the total annual cost (TAC) are performed for desired H2 product purity values ranging between 0.90 and 0.95 mole fraction. One of the results showed that the contribution of the operating expenditures is more significant than the contribution of the annualized capital expenditures (approximately 62% and 38%, respectively). In addition, it was found that the optimal trade-offs existing between process variables (such as total membrane area and total electric power) depend on the specified H2 product purity level. Second, the minimization of the total power demand and the minimization of the total membrane area were performed for H2 recovery of 90% and H2 product purity of 0.90. The TAC values obtained in the first and second cases increased by 19.9% and 4.9%, respectively, with respect to that obtained by cost minimization. Finally, by analyzing and comparing the three optimal solutions, a strategy to systematically and rationally provide 'good' lower and upper bounds for model variables and initial guess values to solve the cost minimization problem by means of global optimization algorithms is proposed, which can be straightforward applied to other processes.
Fil: Mores, Patricia Liliana. Universidad Tecnológica Nacional; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario; Argentina
Fil: Arias, Ana Marisa. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario; Argentina. Universidad Tecnológica Nacional; Argentina
Fil: Scenna, Nicolas Jose. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario; Argentina. Universidad Tecnológica Nacional; Argentina
Fil: Caballero, José A.. Universidad de Alicante; España
Fil: Mussati, Sergio Fabian. Universidad Tecnológica Nacional; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Desarrollo y Diseño. Universidad Tecnológica Nacional. Facultad Regional Santa Fe. Instituto de Desarrollo y Diseño; Argentina
Fil: Mussati, Miguel Ceferino. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Desarrollo y Diseño. Universidad Tecnológica Nacional. Facultad Regional Santa Fe. Instituto de Desarrollo y Diseño; Argentina
description This work deals with the optimization of two-stage membrane systems for H2 separation from off-gases in hydrocarbons processing plants to simultaneously attain high values of both H2 recovery and H2 product purity. First, for a given H2 recovery level of 90%, optimizations of the total annual cost (TAC) are performed for desired H2 product purity values ranging between 0.90 and 0.95 mole fraction. One of the results showed that the contribution of the operating expenditures is more significant than the contribution of the annualized capital expenditures (approximately 62% and 38%, respectively). In addition, it was found that the optimal trade-offs existing between process variables (such as total membrane area and total electric power) depend on the specified H2 product purity level. Second, the minimization of the total power demand and the minimization of the total membrane area were performed for H2 recovery of 90% and H2 product purity of 0.90. The TAC values obtained in the first and second cases increased by 19.9% and 4.9%, respectively, with respect to that obtained by cost minimization. Finally, by analyzing and comparing the three optimal solutions, a strategy to systematically and rationally provide 'good' lower and upper bounds for model variables and initial guess values to solve the cost minimization problem by means of global optimization algorithms is proposed, which can be straightforward applied to other processes.
publishDate 2018
dc.date.none.fl_str_mv 2018-11
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/91826
Mores, Patricia Liliana; Arias, Ana Marisa; Scenna, Nicolas Jose; Caballero, José A.; Mussati, Sergio Fabian; et al.; Membrane-based processes: Optimization of hydrogen separation by minimization of power, membrane area, and cost; MDPI; Processes; 6; 11; 11-2018; 1-20
2227-9717
CONICET Digital
CONICET
url http://hdl.handle.net/11336/91826
identifier_str_mv Mores, Patricia Liliana; Arias, Ana Marisa; Scenna, Nicolas Jose; Caballero, José A.; Mussati, Sergio Fabian; et al.; Membrane-based processes: Optimization of hydrogen separation by minimization of power, membrane area, and cost; MDPI; Processes; 6; 11; 11-2018; 1-20
2227-9717
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/http://www.mdpi.com/2227-9717/6/11/221
info:eu-repo/semantics/altIdentifier/doi/10.3390/pr6110221
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
application/pdf
application/pdf
application/pdf
application/pdf
dc.publisher.none.fl_str_mv MDPI
publisher.none.fl_str_mv MDPI
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 13.070432

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