Analysis of PM2.5 in Córdoba, Argentina under the effects of the El Niño Southern Oscillation
- Autores
- Lanzaco, Bethania Luz; Olcese, Luis Eduardo; Querol, Xavier; Toselli, Beatriz Margarita
- Año de publicación
- 2017
- Idioma
- inglés
- Tipo de recurso
- artículo
- Estado
- versión publicada
- Descripción
- In this work, PM2.5 samples were collected in the winter-spring months of 2014–2016 at an urban site in Córdoba. Córdoba is the second largest city in Argentina and is an important industrial and touristic center. The collected samples were individually analyzed for chemical composition using different techniques. The soluble inorganic ions and carbonaceous particles were determined from bulk aerosol samples for the first time in the city. The mass concentrations of PM2.5, organic carbon, elemental carbon, inorganic ions and metals were determined according to the mass balance. The dominant mass components were organic matter and elemental carbon (54.8%), mineral dust (6.1%), secondary inorganic aerosols (3.0%), and salt (1.2%). A principal component analysis was applied to the samples and resulted in five major factors that explained 79% of the variance in PM2.5. These factors represented combustion, industrial sources, soil dust, secondary inorganic aerosol, and salt, and each explained between 11% and 20% of the variance. A comparison with the results from a previous campaign (2010–2011) revealed appreciable changes in the PM2.5 chemical composition. These changes were attributed to the two extreme meteorological conditions that prevailed in the region. The years 2014–2016 were largely dominated by the warm phase of the El Niño–Southern Oscillation, which leads to humid and cold weather in the Córdoba region, while the samples from 2010 to 2011 were collected during the dry and hot years resulting from the La Niña regime.
Fil: Lanzaco, Bethania Luz. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; Argentina
Fil: Olcese, Luis Eduardo. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; Argentina
Fil: Querol, Xavier. Institute of Environmental Assessment and Water Research; España. Consejo Superior de Investigaciones Científicas; España
Fil: Toselli, Beatriz Margarita. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; Argentina - Materia
-
Argentina
Carbonaceous Particles
CÓRdoba
Fine Aerosol Chemical Speciation
Principal Component Analysis - Nivel de accesibilidad
- acceso abierto
- Condiciones de uso
- https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
- Repositorio
- Institución
- Consejo Nacional de Investigaciones Científicas y Técnicas
- OAI Identificador
- oai:ri.conicet.gov.ar:11336/64340
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Analysis of PM2.5 in Córdoba, Argentina under the effects of the El Niño Southern OscillationLanzaco, Bethania LuzOlcese, Luis EduardoQuerol, XavierToselli, Beatriz MargaritaArgentinaCarbonaceous ParticlesCÓRdobaFine Aerosol Chemical SpeciationPrincipal Component Analysishttps://purl.org/becyt/ford/1.5https://purl.org/becyt/ford/1In this work, PM2.5 samples were collected in the winter-spring months of 2014–2016 at an urban site in Córdoba. Córdoba is the second largest city in Argentina and is an important industrial and touristic center. The collected samples were individually analyzed for chemical composition using different techniques. The soluble inorganic ions and carbonaceous particles were determined from bulk aerosol samples for the first time in the city. The mass concentrations of PM2.5, organic carbon, elemental carbon, inorganic ions and metals were determined according to the mass balance. The dominant mass components were organic matter and elemental carbon (54.8%), mineral dust (6.1%), secondary inorganic aerosols (3.0%), and salt (1.2%). A principal component analysis was applied to the samples and resulted in five major factors that explained 79% of the variance in PM2.5. These factors represented combustion, industrial sources, soil dust, secondary inorganic aerosol, and salt, and each explained between 11% and 20% of the variance. A comparison with the results from a previous campaign (2010–2011) revealed appreciable changes in the PM2.5 chemical composition. These changes were attributed to the two extreme meteorological conditions that prevailed in the region. The years 2014–2016 were largely dominated by the warm phase of the El Niño–Southern Oscillation, which leads to humid and cold weather in the Córdoba region, while the samples from 2010 to 2011 were collected during the dry and hot years resulting from the La Niña regime.Fil: Lanzaco, Bethania Luz. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; ArgentinaFil: Olcese, Luis Eduardo. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; ArgentinaFil: Querol, Xavier. Institute of Environmental Assessment and Water Research; España. Consejo Superior de Investigaciones Científicas; EspañaFil: Toselli, Beatriz Margarita. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; ArgentinaPergamon-Elsevier Science Ltd2017-12info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/64340Lanzaco, Bethania Luz; Olcese, Luis Eduardo; Querol, Xavier; Toselli, Beatriz Margarita; Analysis of PM2.5 in Córdoba, Argentina under the effects of the El Niño Southern Oscillation; Pergamon-Elsevier Science Ltd; Atmospheric Environment; 171; 12-2017; 49-581352-2310CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/http://linkinghub.elsevier.com/retrieve/pii/S1352231017306623info:eu-repo/semantics/altIdentifier/doi/10.1016/j.atmosenv.2017.10.001info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-10T13:03:07Zoai:ri.conicet.gov.ar:11336/64340instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-10 13:03:07.869CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse |
dc.title.none.fl_str_mv |
Analysis of PM2.5 in Córdoba, Argentina under the effects of the El Niño Southern Oscillation |
title |
Analysis of PM2.5 in Córdoba, Argentina under the effects of the El Niño Southern Oscillation |
spellingShingle |
Analysis of PM2.5 in Córdoba, Argentina under the effects of the El Niño Southern Oscillation Lanzaco, Bethania Luz Argentina Carbonaceous Particles CÓRdoba Fine Aerosol Chemical Speciation Principal Component Analysis |
title_short |
Analysis of PM2.5 in Córdoba, Argentina under the effects of the El Niño Southern Oscillation |
title_full |
Analysis of PM2.5 in Córdoba, Argentina under the effects of the El Niño Southern Oscillation |
title_fullStr |
Analysis of PM2.5 in Córdoba, Argentina under the effects of the El Niño Southern Oscillation |
title_full_unstemmed |
Analysis of PM2.5 in Córdoba, Argentina under the effects of the El Niño Southern Oscillation |
title_sort |
Analysis of PM2.5 in Córdoba, Argentina under the effects of the El Niño Southern Oscillation |
dc.creator.none.fl_str_mv |
Lanzaco, Bethania Luz Olcese, Luis Eduardo Querol, Xavier Toselli, Beatriz Margarita |
author |
Lanzaco, Bethania Luz |
author_facet |
Lanzaco, Bethania Luz Olcese, Luis Eduardo Querol, Xavier Toselli, Beatriz Margarita |
author_role |
author |
author2 |
Olcese, Luis Eduardo Querol, Xavier Toselli, Beatriz Margarita |
author2_role |
author author author |
dc.subject.none.fl_str_mv |
Argentina Carbonaceous Particles CÓRdoba Fine Aerosol Chemical Speciation Principal Component Analysis |
topic |
Argentina Carbonaceous Particles CÓRdoba Fine Aerosol Chemical Speciation Principal Component Analysis |
purl_subject.fl_str_mv |
https://purl.org/becyt/ford/1.5 https://purl.org/becyt/ford/1 |
dc.description.none.fl_txt_mv |
In this work, PM2.5 samples were collected in the winter-spring months of 2014–2016 at an urban site in Córdoba. Córdoba is the second largest city in Argentina and is an important industrial and touristic center. The collected samples were individually analyzed for chemical composition using different techniques. The soluble inorganic ions and carbonaceous particles were determined from bulk aerosol samples for the first time in the city. The mass concentrations of PM2.5, organic carbon, elemental carbon, inorganic ions and metals were determined according to the mass balance. The dominant mass components were organic matter and elemental carbon (54.8%), mineral dust (6.1%), secondary inorganic aerosols (3.0%), and salt (1.2%). A principal component analysis was applied to the samples and resulted in five major factors that explained 79% of the variance in PM2.5. These factors represented combustion, industrial sources, soil dust, secondary inorganic aerosol, and salt, and each explained between 11% and 20% of the variance. A comparison with the results from a previous campaign (2010–2011) revealed appreciable changes in the PM2.5 chemical composition. These changes were attributed to the two extreme meteorological conditions that prevailed in the region. The years 2014–2016 were largely dominated by the warm phase of the El Niño–Southern Oscillation, which leads to humid and cold weather in the Córdoba region, while the samples from 2010 to 2011 were collected during the dry and hot years resulting from the La Niña regime. Fil: Lanzaco, Bethania Luz. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; Argentina Fil: Olcese, Luis Eduardo. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; Argentina Fil: Querol, Xavier. Institute of Environmental Assessment and Water Research; España. Consejo Superior de Investigaciones Científicas; España Fil: Toselli, Beatriz Margarita. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; Argentina |
description |
In this work, PM2.5 samples were collected in the winter-spring months of 2014–2016 at an urban site in Córdoba. Córdoba is the second largest city in Argentina and is an important industrial and touristic center. The collected samples were individually analyzed for chemical composition using different techniques. The soluble inorganic ions and carbonaceous particles were determined from bulk aerosol samples for the first time in the city. The mass concentrations of PM2.5, organic carbon, elemental carbon, inorganic ions and metals were determined according to the mass balance. The dominant mass components were organic matter and elemental carbon (54.8%), mineral dust (6.1%), secondary inorganic aerosols (3.0%), and salt (1.2%). A principal component analysis was applied to the samples and resulted in five major factors that explained 79% of the variance in PM2.5. These factors represented combustion, industrial sources, soil dust, secondary inorganic aerosol, and salt, and each explained between 11% and 20% of the variance. A comparison with the results from a previous campaign (2010–2011) revealed appreciable changes in the PM2.5 chemical composition. These changes were attributed to the two extreme meteorological conditions that prevailed in the region. The years 2014–2016 were largely dominated by the warm phase of the El Niño–Southern Oscillation, which leads to humid and cold weather in the Córdoba region, while the samples from 2010 to 2011 were collected during the dry and hot years resulting from the La Niña regime. |
publishDate |
2017 |
dc.date.none.fl_str_mv |
2017-12 |
dc.type.none.fl_str_mv |
info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion http://purl.org/coar/resource_type/c_6501 info:ar-repo/semantics/articulo |
format |
article |
status_str |
publishedVersion |
dc.identifier.none.fl_str_mv |
http://hdl.handle.net/11336/64340 Lanzaco, Bethania Luz; Olcese, Luis Eduardo; Querol, Xavier; Toselli, Beatriz Margarita; Analysis of PM2.5 in Córdoba, Argentina under the effects of the El Niño Southern Oscillation; Pergamon-Elsevier Science Ltd; Atmospheric Environment; 171; 12-2017; 49-58 1352-2310 CONICET Digital CONICET |
url |
http://hdl.handle.net/11336/64340 |
identifier_str_mv |
Lanzaco, Bethania Luz; Olcese, Luis Eduardo; Querol, Xavier; Toselli, Beatriz Margarita; Analysis of PM2.5 in Córdoba, Argentina under the effects of the El Niño Southern Oscillation; Pergamon-Elsevier Science Ltd; Atmospheric Environment; 171; 12-2017; 49-58 1352-2310 CONICET Digital CONICET |
dc.language.none.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
info:eu-repo/semantics/altIdentifier/url/http://linkinghub.elsevier.com/retrieve/pii/S1352231017306623 info:eu-repo/semantics/altIdentifier/doi/10.1016/j.atmosenv.2017.10.001 |
dc.rights.none.fl_str_mv |
info:eu-repo/semantics/openAccess https://creativecommons.org/licenses/by-nc-sa/2.5/ar/ |
eu_rights_str_mv |
openAccess |
rights_invalid_str_mv |
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/ |
dc.format.none.fl_str_mv |
application/pdf application/pdf application/pdf |
dc.publisher.none.fl_str_mv |
Pergamon-Elsevier Science Ltd |
publisher.none.fl_str_mv |
Pergamon-Elsevier Science Ltd |
dc.source.none.fl_str_mv |
reponame:CONICET Digital (CONICET) instname:Consejo Nacional de Investigaciones Científicas y Técnicas |
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CONICET Digital (CONICET) |
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CONICET Digital (CONICET) |
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Consejo Nacional de Investigaciones Científicas y Técnicas |
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CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.mail.fl_str_mv |
dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar |
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1842980061816291328 |
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13.004268 |