Autocatalysis and CO2: Carbon Capture and Utilization (CCU) Meets Natural Processes

Autores
Gastelu, Gabriela; Saha, Pritha; Dyson, Paul; Hulla, Martin; Uranga, Jorge Gustavo
Año de publicación
2023
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
Autocatalytic reactions were proposed to play a key role at the beginning of life starting from the first reduction of CO2 to formate, acetate and C1 C4 hydrocarbons. In carbon capture and utilization (CCU) processes, the same reactions were demonstrated to be autocatalytic and, in some cases, promoted by catalysts of the same composition. Through evolution, CO2 reduction then turned into complex autocatalytic networks such as photosynthesis, where CCU chemists found inspiration for the development of more advanced systems for the synthesis of value-added chemicals. Less evolved systems than photosynthesis, however, may be easier to emulate and provide valuable inspiration into CO2 reduction chemistry for CCU. Other synthetic systems were also demonstrated to be autocatalytic demonstrating that CO2 reactions and autocatalysis are closely connected. In this concept article, the relationship between natural, artificial and bio-inspired autocatalytic CO2 reduction processes is summarized and discussed. The accomplishments resulting from the integration of autocatalysis and CCU strategies, along with their inherent benefits and future prospectives are also outlined.
Fil: Gastelu, Gabriela. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; Argentina
Fil: Saha, Pritha. Charles University; República Checa
Fil: Dyson, Paul. École Polytechnique Fédérale de Lausanne; Suiza
Fil: Hulla, Martin. Charles University; República Checa
Fil: Uranga, Jorge Gustavo. Universidad Nacional de Córdoba; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; Argentina
Materia
AUTOCATALYSIS
BIOMIMETIC SYNTHESIS
CARBON CAPTURE AND UTILIZATION
CCU
CO2 UTILIZATION
HETEROGENEOUS CATALYSIS
ORGANOCATALYSIS
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/226803
Acceder
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oai_identifier_str oai:ri.conicet.gov.ar:11336/226803
network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Autocatalysis and CO2: Carbon Capture and Utilization (CCU) Meets Natural ProcessesGastelu, GabrielaSaha, PrithaDyson, PaulHulla, MartinUranga, Jorge GustavoAUTOCATALYSISBIOMIMETIC SYNTHESISCARBON CAPTURE AND UTILIZATIONCCUCO2 UTILIZATIONHETEROGENEOUS CATALYSISORGANOCATALYSIShttps://purl.org/becyt/ford/1.4https://purl.org/becyt/ford/1Autocatalytic reactions were proposed to play a key role at the beginning of life starting from the first reduction of CO2 to formate, acetate and C1 C4 hydrocarbons. In carbon capture and utilization (CCU) processes, the same reactions were demonstrated to be autocatalytic and, in some cases, promoted by catalysts of the same composition. Through evolution, CO2 reduction then turned into complex autocatalytic networks such as photosynthesis, where CCU chemists found inspiration for the development of more advanced systems for the synthesis of value-added chemicals. Less evolved systems than photosynthesis, however, may be easier to emulate and provide valuable inspiration into CO2 reduction chemistry for CCU. Other synthetic systems were also demonstrated to be autocatalytic demonstrating that CO2 reactions and autocatalysis are closely connected. In this concept article, the relationship between natural, artificial and bio-inspired autocatalytic CO2 reduction processes is summarized and discussed. The accomplishments resulting from the integration of autocatalysis and CCU strategies, along with their inherent benefits and future prospectives are also outlined.Fil: Gastelu, Gabriela. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; ArgentinaFil: Saha, Pritha. Charles University; República ChecaFil: Dyson, Paul. École Polytechnique Fédérale de Lausanne; SuizaFil: Hulla, Martin. Charles University; República ChecaFil: Uranga, Jorge Gustavo. Universidad Nacional de Córdoba; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; ArgentinaWiley VCH Verlag2023-11info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/226803Gastelu, Gabriela; Saha, Pritha; Dyson, Paul; Hulla, Martin; Uranga, Jorge Gustavo; Autocatalysis and CO2: Carbon Capture and Utilization (CCU) Meets Natural Processes; Wiley VCH Verlag; Chemcatchem; 15; 22; 11-2023; 1-61867-3880CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://doi.org/10.1002/cctc.202300905info:eu-repo/semantics/altIdentifier/doi/10.1002/cctc.202300905info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-nd/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-03T09:45:38Zoai:ri.conicet.gov.ar:11336/226803instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-03 09:45:38.6CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Autocatalysis and CO2: Carbon Capture and Utilization (CCU) Meets Natural Processes
title Autocatalysis and CO2: Carbon Capture and Utilization (CCU) Meets Natural Processes
spellingShingle Autocatalysis and CO2: Carbon Capture and Utilization (CCU) Meets Natural Processes
Gastelu, Gabriela
AUTOCATALYSIS
BIOMIMETIC SYNTHESIS
CARBON CAPTURE AND UTILIZATION
CCU
CO2 UTILIZATION
HETEROGENEOUS CATALYSIS
ORGANOCATALYSIS
title_short Autocatalysis and CO2: Carbon Capture and Utilization (CCU) Meets Natural Processes
title_full Autocatalysis and CO2: Carbon Capture and Utilization (CCU) Meets Natural Processes
title_fullStr Autocatalysis and CO2: Carbon Capture and Utilization (CCU) Meets Natural Processes
title_full_unstemmed Autocatalysis and CO2: Carbon Capture and Utilization (CCU) Meets Natural Processes
title_sort Autocatalysis and CO2: Carbon Capture and Utilization (CCU) Meets Natural Processes
dc.creator.none.fl_str_mv Gastelu, Gabriela
Saha, Pritha
Dyson, Paul
Hulla, Martin
Uranga, Jorge Gustavo
author Gastelu, Gabriela
author_facet Gastelu, Gabriela
Saha, Pritha
Dyson, Paul
Hulla, Martin
Uranga, Jorge Gustavo
author_role author
author2 Saha, Pritha
Dyson, Paul
Hulla, Martin
Uranga, Jorge Gustavo
author2_role author
author
author
author
dc.subject.none.fl_str_mv AUTOCATALYSIS
BIOMIMETIC SYNTHESIS
CARBON CAPTURE AND UTILIZATION
CCU
CO2 UTILIZATION
HETEROGENEOUS CATALYSIS
ORGANOCATALYSIS
topic AUTOCATALYSIS
BIOMIMETIC SYNTHESIS
CARBON CAPTURE AND UTILIZATION
CCU
CO2 UTILIZATION
HETEROGENEOUS CATALYSIS
ORGANOCATALYSIS
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv Autocatalytic reactions were proposed to play a key role at the beginning of life starting from the first reduction of CO2 to formate, acetate and C1 C4 hydrocarbons. In carbon capture and utilization (CCU) processes, the same reactions were demonstrated to be autocatalytic and, in some cases, promoted by catalysts of the same composition. Through evolution, CO2 reduction then turned into complex autocatalytic networks such as photosynthesis, where CCU chemists found inspiration for the development of more advanced systems for the synthesis of value-added chemicals. Less evolved systems than photosynthesis, however, may be easier to emulate and provide valuable inspiration into CO2 reduction chemistry for CCU. Other synthetic systems were also demonstrated to be autocatalytic demonstrating that CO2 reactions and autocatalysis are closely connected. In this concept article, the relationship between natural, artificial and bio-inspired autocatalytic CO2 reduction processes is summarized and discussed. The accomplishments resulting from the integration of autocatalysis and CCU strategies, along with their inherent benefits and future prospectives are also outlined.
Fil: Gastelu, Gabriela. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; Argentina
Fil: Saha, Pritha. Charles University; República Checa
Fil: Dyson, Paul. École Polytechnique Fédérale de Lausanne; Suiza
Fil: Hulla, Martin. Charles University; República Checa
Fil: Uranga, Jorge Gustavo. Universidad Nacional de Córdoba; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Córdoba. Instituto de Investigaciones en Físico-química de Córdoba. Universidad Nacional de Córdoba. Facultad de Ciencias Químicas. Instituto de Investigaciones en Físico-química de Córdoba; Argentina
description Autocatalytic reactions were proposed to play a key role at the beginning of life starting from the first reduction of CO2 to formate, acetate and C1 C4 hydrocarbons. In carbon capture and utilization (CCU) processes, the same reactions were demonstrated to be autocatalytic and, in some cases, promoted by catalysts of the same composition. Through evolution, CO2 reduction then turned into complex autocatalytic networks such as photosynthesis, where CCU chemists found inspiration for the development of more advanced systems for the synthesis of value-added chemicals. Less evolved systems than photosynthesis, however, may be easier to emulate and provide valuable inspiration into CO2 reduction chemistry for CCU. Other synthetic systems were also demonstrated to be autocatalytic demonstrating that CO2 reactions and autocatalysis are closely connected. In this concept article, the relationship between natural, artificial and bio-inspired autocatalytic CO2 reduction processes is summarized and discussed. The accomplishments resulting from the integration of autocatalysis and CCU strategies, along with their inherent benefits and future prospectives are also outlined.
publishDate 2023
dc.date.none.fl_str_mv 2023-11
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/226803
Gastelu, Gabriela; Saha, Pritha; Dyson, Paul; Hulla, Martin; Uranga, Jorge Gustavo; Autocatalysis and CO2: Carbon Capture and Utilization (CCU) Meets Natural Processes; Wiley VCH Verlag; Chemcatchem; 15; 22; 11-2023; 1-6
1867-3880
CONICET Digital
CONICET
url http://hdl.handle.net/11336/226803
identifier_str_mv Gastelu, Gabriela; Saha, Pritha; Dyson, Paul; Hulla, Martin; Uranga, Jorge Gustavo; Autocatalysis and CO2: Carbon Capture and Utilization (CCU) Meets Natural Processes; Wiley VCH Verlag; Chemcatchem; 15; 22; 11-2023; 1-6
1867-3880
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://doi.org/10.1002/cctc.202300905
info:eu-repo/semantics/altIdentifier/doi/10.1002/cctc.202300905
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv Wiley VCH Verlag
publisher.none.fl_str_mv Wiley VCH Verlag
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
_version_ 1842268745256402944
score 13.13397

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