Collision of protons with carbon atoms of a graphene surface in the presence of adsorbed potassium

Autores
Iglesias García, Adalberto de Jesús; Romero, M. A.; García, Evelina Andrea; Goldberg, Edith Catalina
Año de publicación
2020
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
In this work we study the frontal collision of protons with the carbon atoms of a graphene surface with a low coverage of adsorbed potassium. It is aimed at the analysis of the effect of the adsorbates in both charge exchange and electron emission processes, when the binary collision occurs between the proton and a carbon atom of the surface. The frontal collision with the K adsorbate, already analyzed and discussed in a previous work, is compared with the frontal collision with different carbon neighbors. In the present work we studied the signals, due to the localized structures in the density matrix of the composed graphene plus potassium surface, that can be distinguished when the collision occurs either with the adsorbate, a nearby carbon atom, or a carbon atom that does not feel the presence of the adsorbate. The interacting system is described by the Anderson Hamiltonian which takes into account the electronic repulsion on the projectile site; the charge fractions, the energy distribution of electrons in the solid, and the electron emission after the collision are calculated by using the nonequilibrium Green-Keldysh functions formalism solved by the equation of motion method. In the binary collision with a carbon atom, the extended features of the band structure of graphene smooth the dependence of the projectile charge fractions on the incoming energy and notably decrease the negative ions formation. The localized structures of the density of matrix caused by the presence of the adsorbate are perceptible for scattered carbon atoms close to K. The intense emission of low energy electrons obtained in the case of the scattering by potassium is fundamentally associated with the very localized K-4s empty band. This characteristic, although less marked, remain in the scattering by nearby carbon atoms, due to both the interaction with K along the projectile trajectory and the perturbed local density of states on the carbon atoms due to the adsorbate presence. In addition, the extended nature of the electronic structure of graphene allows for the emission of more energetic electrons.
Fil: Iglesias García, Adalberto de Jesús. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Física del Litoral. Universidad Nacional del Litoral. Instituto de Física del Litoral; Argentina
Fil: Romero, M. A.. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Física del Litoral. Universidad Nacional del Litoral. Instituto de Física del Litoral; Argentina
Fil: García, Evelina Andrea. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Física del Litoral. Universidad Nacional del Litoral. Instituto de Física del Litoral; Argentina
Fil: Goldberg, Edith Catalina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Física del Litoral. Universidad Nacional del Litoral. Instituto de Física del Litoral; Argentina
Materia
ALKALI-GRAPHENE
CHARGE EXCHANGE
EMISSION PROCESSES
GREEN-KELDYSH FUNCTION
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/141877
Acceder
id CONICETDig_7c6f120edbf0f875de2933ea9917ad61
oai_identifier_str oai:ri.conicet.gov.ar:11336/141877
network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Collision of protons with carbon atoms of a graphene surface in the presence of adsorbed potassiumIglesias García, Adalberto de JesúsRomero, M. A.García, Evelina AndreaGoldberg, Edith CatalinaALKALI-GRAPHENECHARGE EXCHANGEEMISSION PROCESSESGREEN-KELDYSH FUNCTIONhttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1In this work we study the frontal collision of protons with the carbon atoms of a graphene surface with a low coverage of adsorbed potassium. It is aimed at the analysis of the effect of the adsorbates in both charge exchange and electron emission processes, when the binary collision occurs between the proton and a carbon atom of the surface. The frontal collision with the K adsorbate, already analyzed and discussed in a previous work, is compared with the frontal collision with different carbon neighbors. In the present work we studied the signals, due to the localized structures in the density matrix of the composed graphene plus potassium surface, that can be distinguished when the collision occurs either with the adsorbate, a nearby carbon atom, or a carbon atom that does not feel the presence of the adsorbate. The interacting system is described by the Anderson Hamiltonian which takes into account the electronic repulsion on the projectile site; the charge fractions, the energy distribution of electrons in the solid, and the electron emission after the collision are calculated by using the nonequilibrium Green-Keldysh functions formalism solved by the equation of motion method. In the binary collision with a carbon atom, the extended features of the band structure of graphene smooth the dependence of the projectile charge fractions on the incoming energy and notably decrease the negative ions formation. The localized structures of the density of matrix caused by the presence of the adsorbate are perceptible for scattered carbon atoms close to K. The intense emission of low energy electrons obtained in the case of the scattering by potassium is fundamentally associated with the very localized K-4s empty band. This characteristic, although less marked, remain in the scattering by nearby carbon atoms, due to both the interaction with K along the projectile trajectory and the perturbed local density of states on the carbon atoms due to the adsorbate presence. In addition, the extended nature of the electronic structure of graphene allows for the emission of more energetic electrons.Fil: Iglesias García, Adalberto de Jesús. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Física del Litoral. Universidad Nacional del Litoral. Instituto de Física del Litoral; ArgentinaFil: Romero, M. A.. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Física del Litoral. Universidad Nacional del Litoral. Instituto de Física del Litoral; ArgentinaFil: García, Evelina Andrea. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Física del Litoral. Universidad Nacional del Litoral. Instituto de Física del Litoral; ArgentinaFil: Goldberg, Edith Catalina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Física del Litoral. Universidad Nacional del Litoral. Instituto de Física del Litoral; ArgentinaAmerican Physical Society2020-09info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/141877Iglesias García, Adalberto de Jesús; Romero, M. A.; García, Evelina Andrea; Goldberg, Edith Catalina; Collision of protons with carbon atoms of a graphene surface in the presence of adsorbed potassium; American Physical Society; Physical Review B; 102; 9-20201098-0121CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://link.aps.org/doi/10.1103/PhysRevB.102.115406info:eu-repo/semantics/altIdentifier/doi/10.1103/PhysRevB.102.115406info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-03T10:06:27Zoai:ri.conicet.gov.ar:11336/141877instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-03 10:06:27.483CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Collision of protons with carbon atoms of a graphene surface in the presence of adsorbed potassium
title Collision of protons with carbon atoms of a graphene surface in the presence of adsorbed potassium
spellingShingle Collision of protons with carbon atoms of a graphene surface in the presence of adsorbed potassium
Iglesias García, Adalberto de Jesús
ALKALI-GRAPHENE
CHARGE EXCHANGE
EMISSION PROCESSES
GREEN-KELDYSH FUNCTION
title_short Collision of protons with carbon atoms of a graphene surface in the presence of adsorbed potassium
title_full Collision of protons with carbon atoms of a graphene surface in the presence of adsorbed potassium
title_fullStr Collision of protons with carbon atoms of a graphene surface in the presence of adsorbed potassium
title_full_unstemmed Collision of protons with carbon atoms of a graphene surface in the presence of adsorbed potassium
title_sort Collision of protons with carbon atoms of a graphene surface in the presence of adsorbed potassium
dc.creator.none.fl_str_mv Iglesias García, Adalberto de Jesús
Romero, M. A.
García, Evelina Andrea
Goldberg, Edith Catalina
author Iglesias García, Adalberto de Jesús
author_facet Iglesias García, Adalberto de Jesús
Romero, M. A.
García, Evelina Andrea
Goldberg, Edith Catalina
author_role author
author2 Romero, M. A.
García, Evelina Andrea
Goldberg, Edith Catalina
author2_role author
author
author
dc.subject.none.fl_str_mv ALKALI-GRAPHENE
CHARGE EXCHANGE
EMISSION PROCESSES
GREEN-KELDYSH FUNCTION
topic ALKALI-GRAPHENE
CHARGE EXCHANGE
EMISSION PROCESSES
GREEN-KELDYSH FUNCTION
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv In this work we study the frontal collision of protons with the carbon atoms of a graphene surface with a low coverage of adsorbed potassium. It is aimed at the analysis of the effect of the adsorbates in both charge exchange and electron emission processes, when the binary collision occurs between the proton and a carbon atom of the surface. The frontal collision with the K adsorbate, already analyzed and discussed in a previous work, is compared with the frontal collision with different carbon neighbors. In the present work we studied the signals, due to the localized structures in the density matrix of the composed graphene plus potassium surface, that can be distinguished when the collision occurs either with the adsorbate, a nearby carbon atom, or a carbon atom that does not feel the presence of the adsorbate. The interacting system is described by the Anderson Hamiltonian which takes into account the electronic repulsion on the projectile site; the charge fractions, the energy distribution of electrons in the solid, and the electron emission after the collision are calculated by using the nonequilibrium Green-Keldysh functions formalism solved by the equation of motion method. In the binary collision with a carbon atom, the extended features of the band structure of graphene smooth the dependence of the projectile charge fractions on the incoming energy and notably decrease the negative ions formation. The localized structures of the density of matrix caused by the presence of the adsorbate are perceptible for scattered carbon atoms close to K. The intense emission of low energy electrons obtained in the case of the scattering by potassium is fundamentally associated with the very localized K-4s empty band. This characteristic, although less marked, remain in the scattering by nearby carbon atoms, due to both the interaction with K along the projectile trajectory and the perturbed local density of states on the carbon atoms due to the adsorbate presence. In addition, the extended nature of the electronic structure of graphene allows for the emission of more energetic electrons.
Fil: Iglesias García, Adalberto de Jesús. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Física del Litoral. Universidad Nacional del Litoral. Instituto de Física del Litoral; Argentina
Fil: Romero, M. A.. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Física del Litoral. Universidad Nacional del Litoral. Instituto de Física del Litoral; Argentina
Fil: García, Evelina Andrea. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Física del Litoral. Universidad Nacional del Litoral. Instituto de Física del Litoral; Argentina
Fil: Goldberg, Edith Catalina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Física del Litoral. Universidad Nacional del Litoral. Instituto de Física del Litoral; Argentina
description In this work we study the frontal collision of protons with the carbon atoms of a graphene surface with a low coverage of adsorbed potassium. It is aimed at the analysis of the effect of the adsorbates in both charge exchange and electron emission processes, when the binary collision occurs between the proton and a carbon atom of the surface. The frontal collision with the K adsorbate, already analyzed and discussed in a previous work, is compared with the frontal collision with different carbon neighbors. In the present work we studied the signals, due to the localized structures in the density matrix of the composed graphene plus potassium surface, that can be distinguished when the collision occurs either with the adsorbate, a nearby carbon atom, or a carbon atom that does not feel the presence of the adsorbate. The interacting system is described by the Anderson Hamiltonian which takes into account the electronic repulsion on the projectile site; the charge fractions, the energy distribution of electrons in the solid, and the electron emission after the collision are calculated by using the nonequilibrium Green-Keldysh functions formalism solved by the equation of motion method. In the binary collision with a carbon atom, the extended features of the band structure of graphene smooth the dependence of the projectile charge fractions on the incoming energy and notably decrease the negative ions formation. The localized structures of the density of matrix caused by the presence of the adsorbate are perceptible for scattered carbon atoms close to K. The intense emission of low energy electrons obtained in the case of the scattering by potassium is fundamentally associated with the very localized K-4s empty band. This characteristic, although less marked, remain in the scattering by nearby carbon atoms, due to both the interaction with K along the projectile trajectory and the perturbed local density of states on the carbon atoms due to the adsorbate presence. In addition, the extended nature of the electronic structure of graphene allows for the emission of more energetic electrons.
publishDate 2020
dc.date.none.fl_str_mv 2020-09
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/141877
Iglesias García, Adalberto de Jesús; Romero, M. A.; García, Evelina Andrea; Goldberg, Edith Catalina; Collision of protons with carbon atoms of a graphene surface in the presence of adsorbed potassium; American Physical Society; Physical Review B; 102; 9-2020
1098-0121
CONICET Digital
CONICET
url http://hdl.handle.net/11336/141877
identifier_str_mv Iglesias García, Adalberto de Jesús; Romero, M. A.; García, Evelina Andrea; Goldberg, Edith Catalina; Collision of protons with carbon atoms of a graphene surface in the presence of adsorbed potassium; American Physical Society; Physical Review B; 102; 9-2020
1098-0121
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://link.aps.org/doi/10.1103/PhysRevB.102.115406
info:eu-repo/semantics/altIdentifier/doi/10.1103/PhysRevB.102.115406
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
application/pdf
dc.publisher.none.fl_str_mv American Physical Society
publisher.none.fl_str_mv American Physical Society
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
_version_ 1842269959086931968
score 13.13397

Publicaciones similares