Monitoring the photothermal reshaping of individual plasmonic nanorods with coherent mechanical oscillations

Autores
Della Picca, Fabricio Leandro; Gutiérrez, Marina V.; Bragas, Andrea Veronica; Scarpettini, Alberto Franco
Año de publicación
2018
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
Light absorption in gold nanoparticles leads to metal heating that induces photothermal reshaping because of atomic surface diffusion at temperatures well below the gold melting point. In this work, we perform time-resolved experiments to measure the frequencies of the extensional coherent mechanical mode in single gold nanorods, as a monitor of the changes in their aspect ratio produced by this photoinduced reshaping. We show that photothermal reshaping always occurs in typical pump-probe experiments conducted in air even at low-excitation light irradiance and usually long measuring times. The reshaping effect can be reduced by a polymer coating, which allows faster heat dissipation from the nanoparticle to the environment.
Fil: Della Picca, Fabricio Leandro. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Departamento de Física; Argentina
Fil: Gutiérrez, Marina V.. Universidad Tecnológica Nacional. Facultad Regional Delta; Argentina
Fil: Bragas, Andrea Veronica. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Departamento de Física; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; Argentina
Fil: Scarpettini, Alberto Franco. Universidad Tecnológica Nacional. Facultad Regional Delta; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Materia
NANOANTENAS
PLASMONICA
CALOR
OSCILACIONES MECANICAS
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/147749
Acceder
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network_name_str CONICET Digital (CONICET)
spelling Monitoring the photothermal reshaping of individual plasmonic nanorods with coherent mechanical oscillationsDella Picca, Fabricio LeandroGutiérrez, Marina V.Bragas, Andrea VeronicaScarpettini, Alberto FrancoNANOANTENASPLASMONICACALOROSCILACIONES MECANICAShttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1Light absorption in gold nanoparticles leads to metal heating that induces photothermal reshaping because of atomic surface diffusion at temperatures well below the gold melting point. In this work, we perform time-resolved experiments to measure the frequencies of the extensional coherent mechanical mode in single gold nanorods, as a monitor of the changes in their aspect ratio produced by this photoinduced reshaping. We show that photothermal reshaping always occurs in typical pump-probe experiments conducted in air even at low-excitation light irradiance and usually long measuring times. The reshaping effect can be reduced by a polymer coating, which allows faster heat dissipation from the nanoparticle to the environment.Fil: Della Picca, Fabricio Leandro. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Departamento de Física; ArgentinaFil: Gutiérrez, Marina V.. Universidad Tecnológica Nacional. Facultad Regional Delta; ArgentinaFil: Bragas, Andrea Veronica. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Departamento de Física; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; ArgentinaFil: Scarpettini, Alberto Franco. Universidad Tecnológica Nacional. Facultad Regional Delta; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaAmerican Chemical Society2018-12-03info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/147749Della Picca, Fabricio Leandro; Gutiérrez, Marina V.; Bragas, Andrea Veronica; Scarpettini, Alberto Franco; Monitoring the photothermal reshaping of individual plasmonic nanorods with coherent mechanical oscillations; American Chemical Society; Journal of Physical Chemistry C; 122; 51; 03-12-2018; 29598-296061932-74471932-7455CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://pubs.acs.org/doi/10.1021/acs.jpcc.8b09458info:eu-repo/semantics/altIdentifier/doi/10.1021/acs.jpcc.8b09458info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T09:32:23Zoai:ri.conicet.gov.ar:11336/147749instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 09:32:23.519CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Monitoring the photothermal reshaping of individual plasmonic nanorods with coherent mechanical oscillations
title Monitoring the photothermal reshaping of individual plasmonic nanorods with coherent mechanical oscillations
spellingShingle Monitoring the photothermal reshaping of individual plasmonic nanorods with coherent mechanical oscillations
Della Picca, Fabricio Leandro
NANOANTENAS
PLASMONICA
CALOR
OSCILACIONES MECANICAS
title_short Monitoring the photothermal reshaping of individual plasmonic nanorods with coherent mechanical oscillations
title_full Monitoring the photothermal reshaping of individual plasmonic nanorods with coherent mechanical oscillations
title_fullStr Monitoring the photothermal reshaping of individual plasmonic nanorods with coherent mechanical oscillations
title_full_unstemmed Monitoring the photothermal reshaping of individual plasmonic nanorods with coherent mechanical oscillations
title_sort Monitoring the photothermal reshaping of individual plasmonic nanorods with coherent mechanical oscillations
dc.creator.none.fl_str_mv Della Picca, Fabricio Leandro
Gutiérrez, Marina V.
Bragas, Andrea Veronica
Scarpettini, Alberto Franco
author Della Picca, Fabricio Leandro
author_facet Della Picca, Fabricio Leandro
Gutiérrez, Marina V.
Bragas, Andrea Veronica
Scarpettini, Alberto Franco
author_role author
author2 Gutiérrez, Marina V.
Bragas, Andrea Veronica
Scarpettini, Alberto Franco
author2_role author
author
author
dc.subject.none.fl_str_mv NANOANTENAS
PLASMONICA
CALOR
OSCILACIONES MECANICAS
topic NANOANTENAS
PLASMONICA
CALOR
OSCILACIONES MECANICAS
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv Light absorption in gold nanoparticles leads to metal heating that induces photothermal reshaping because of atomic surface diffusion at temperatures well below the gold melting point. In this work, we perform time-resolved experiments to measure the frequencies of the extensional coherent mechanical mode in single gold nanorods, as a monitor of the changes in their aspect ratio produced by this photoinduced reshaping. We show that photothermal reshaping always occurs in typical pump-probe experiments conducted in air even at low-excitation light irradiance and usually long measuring times. The reshaping effect can be reduced by a polymer coating, which allows faster heat dissipation from the nanoparticle to the environment.
Fil: Della Picca, Fabricio Leandro. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Departamento de Física; Argentina
Fil: Gutiérrez, Marina V.. Universidad Tecnológica Nacional. Facultad Regional Delta; Argentina
Fil: Bragas, Andrea Veronica. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Departamento de Física; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; Argentina
Fil: Scarpettini, Alberto Franco. Universidad Tecnológica Nacional. Facultad Regional Delta; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
description Light absorption in gold nanoparticles leads to metal heating that induces photothermal reshaping because of atomic surface diffusion at temperatures well below the gold melting point. In this work, we perform time-resolved experiments to measure the frequencies of the extensional coherent mechanical mode in single gold nanorods, as a monitor of the changes in their aspect ratio produced by this photoinduced reshaping. We show that photothermal reshaping always occurs in typical pump-probe experiments conducted in air even at low-excitation light irradiance and usually long measuring times. The reshaping effect can be reduced by a polymer coating, which allows faster heat dissipation from the nanoparticle to the environment.
publishDate 2018
dc.date.none.fl_str_mv 2018-12-03
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/147749
Della Picca, Fabricio Leandro; Gutiérrez, Marina V.; Bragas, Andrea Veronica; Scarpettini, Alberto Franco; Monitoring the photothermal reshaping of individual plasmonic nanorods with coherent mechanical oscillations; American Chemical Society; Journal of Physical Chemistry C; 122; 51; 03-12-2018; 29598-29606
1932-7447
1932-7455
CONICET Digital
CONICET
url http://hdl.handle.net/11336/147749
identifier_str_mv Della Picca, Fabricio Leandro; Gutiérrez, Marina V.; Bragas, Andrea Veronica; Scarpettini, Alberto Franco; Monitoring the photothermal reshaping of individual plasmonic nanorods with coherent mechanical oscillations; American Chemical Society; Journal of Physical Chemistry C; 122; 51; 03-12-2018; 29598-29606
1932-7447
1932-7455
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://pubs.acs.org/doi/10.1021/acs.jpcc.8b09458
info:eu-repo/semantics/altIdentifier/doi/10.1021/acs.jpcc.8b09458
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
application/pdf
dc.publisher.none.fl_str_mv American Chemical Society
publisher.none.fl_str_mv American Chemical Society
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 13.070432

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