Printing of In Situ Functionalized Mesoporous Silica with Digital Light Processing for Combinatorial Sensing

Autores
Zhao, Lucy; Spiehl, Dieter; Kohnen, Marion C.; Ceolin, Marcelo Raul; Mikolei, Joanna J.; Pardehkhorram, Raheleh; Andrieu Brunsen, Annette
Año de publicación
2024
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
Combinatorial sensing is especially important in the context of modern drug development to enable fast screening of large data sets. Mesoporous silica materials offer high surface area and a wide range of functionalization possibilities. By adding structural control, the combination of structural and functional control along all length scales opens a new pathway that permits larger amounts of analytes being tested simultaneously for complex sensing tasks. This study presents a fast and simple way to produce mesoporoussilica in various shapes and sizes between 0.27–6 mm by using light-induced sol-gel chemistry and digital light processing (DLP). Shape-selective functionalization of mesoporous silica is successfully carried out either after printing using organosilanes or in situ while printing through the use of functional mesopore template for the in situ functionalization approach. Shape-selective adsorption of dyes is shown as a demonstrator toward shape selective screening of potential analytes.
Fil: Zhao, Lucy. Universitat Technische Darmstadt; Alemania
Fil: Spiehl, Dieter. Universitat Technische Darmstadt; Alemania
Fil: Kohnen, Marion C.. Universitat Technische Darmstadt; Alemania
Fil: Ceolin, Marcelo Raul. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; Argentina
Fil: Mikolei, Joanna J.. Universitat Technische Darmstadt; Alemania
Fil: Pardehkhorram, Raheleh. Universitat Technische Darmstadt; Alemania
Fil: Andrieu Brunsen, Annette. Universitat Technische Darmstadt; Alemania
Materia
PRINTING
MESOPOROUS
LIGHT PROCESSING
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/262276
Acceder
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network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Printing of In Situ Functionalized Mesoporous Silica with Digital Light Processing for Combinatorial SensingZhao, LucySpiehl, DieterKohnen, Marion C.Ceolin, Marcelo RaulMikolei, Joanna J.Pardehkhorram, RahelehAndrieu Brunsen, AnnettePRINTINGMESOPOROUSLIGHT PROCESSINGhttps://purl.org/becyt/ford/1.4https://purl.org/becyt/ford/1Combinatorial sensing is especially important in the context of modern drug development to enable fast screening of large data sets. Mesoporous silica materials offer high surface area and a wide range of functionalization possibilities. By adding structural control, the combination of structural and functional control along all length scales opens a new pathway that permits larger amounts of analytes being tested simultaneously for complex sensing tasks. This study presents a fast and simple way to produce mesoporoussilica in various shapes and sizes between 0.27–6 mm by using light-induced sol-gel chemistry and digital light processing (DLP). Shape-selective functionalization of mesoporous silica is successfully carried out either after printing using organosilanes or in situ while printing through the use of functional mesopore template for the in situ functionalization approach. Shape-selective adsorption of dyes is shown as a demonstrator toward shape selective screening of potential analytes.Fil: Zhao, Lucy. Universitat Technische Darmstadt; AlemaniaFil: Spiehl, Dieter. Universitat Technische Darmstadt; AlemaniaFil: Kohnen, Marion C.. Universitat Technische Darmstadt; AlemaniaFil: Ceolin, Marcelo Raul. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; ArgentinaFil: Mikolei, Joanna J.. Universitat Technische Darmstadt; AlemaniaFil: Pardehkhorram, Raheleh. Universitat Technische Darmstadt; AlemaniaFil: Andrieu Brunsen, Annette. Universitat Technische Darmstadt; AlemaniaWiley VCH Verlag2024-02info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/262276Zhao, Lucy; Spiehl, Dieter; Kohnen, Marion C.; Ceolin, Marcelo Raul; Mikolei, Joanna J.; et al.; Printing of In Situ Functionalized Mesoporous Silica with Digital Light Processing for Combinatorial Sensing; Wiley VCH Verlag; Small; 20; 28; 2-2024; 1-91613-6810CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://onlinelibrary.wiley.com/doi/10.1002/smll.202311121info:eu-repo/semantics/altIdentifier/doi/10.1002/smll.202311121info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-nd/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T09:52:34Zoai:ri.conicet.gov.ar:11336/262276instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 09:52:35.028CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Printing of In Situ Functionalized Mesoporous Silica with Digital Light Processing for Combinatorial Sensing
title Printing of In Situ Functionalized Mesoporous Silica with Digital Light Processing for Combinatorial Sensing
spellingShingle Printing of In Situ Functionalized Mesoporous Silica with Digital Light Processing for Combinatorial Sensing
Zhao, Lucy
PRINTING
MESOPOROUS
LIGHT PROCESSING
title_short Printing of In Situ Functionalized Mesoporous Silica with Digital Light Processing for Combinatorial Sensing
title_full Printing of In Situ Functionalized Mesoporous Silica with Digital Light Processing for Combinatorial Sensing
title_fullStr Printing of In Situ Functionalized Mesoporous Silica with Digital Light Processing for Combinatorial Sensing
title_full_unstemmed Printing of In Situ Functionalized Mesoporous Silica with Digital Light Processing for Combinatorial Sensing
title_sort Printing of In Situ Functionalized Mesoporous Silica with Digital Light Processing for Combinatorial Sensing
dc.creator.none.fl_str_mv Zhao, Lucy
Spiehl, Dieter
Kohnen, Marion C.
Ceolin, Marcelo Raul
Mikolei, Joanna J.
Pardehkhorram, Raheleh
Andrieu Brunsen, Annette
author Zhao, Lucy
author_facet Zhao, Lucy
Spiehl, Dieter
Kohnen, Marion C.
Ceolin, Marcelo Raul
Mikolei, Joanna J.
Pardehkhorram, Raheleh
Andrieu Brunsen, Annette
author_role author
author2 Spiehl, Dieter
Kohnen, Marion C.
Ceolin, Marcelo Raul
Mikolei, Joanna J.
Pardehkhorram, Raheleh
Andrieu Brunsen, Annette
author2_role author
author
author
author
author
author
dc.subject.none.fl_str_mv PRINTING
MESOPOROUS
LIGHT PROCESSING
topic PRINTING
MESOPOROUS
LIGHT PROCESSING
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.4
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv Combinatorial sensing is especially important in the context of modern drug development to enable fast screening of large data sets. Mesoporous silica materials offer high surface area and a wide range of functionalization possibilities. By adding structural control, the combination of structural and functional control along all length scales opens a new pathway that permits larger amounts of analytes being tested simultaneously for complex sensing tasks. This study presents a fast and simple way to produce mesoporoussilica in various shapes and sizes between 0.27–6 mm by using light-induced sol-gel chemistry and digital light processing (DLP). Shape-selective functionalization of mesoporous silica is successfully carried out either after printing using organosilanes or in situ while printing through the use of functional mesopore template for the in situ functionalization approach. Shape-selective adsorption of dyes is shown as a demonstrator toward shape selective screening of potential analytes.
Fil: Zhao, Lucy. Universitat Technische Darmstadt; Alemania
Fil: Spiehl, Dieter. Universitat Technische Darmstadt; Alemania
Fil: Kohnen, Marion C.. Universitat Technische Darmstadt; Alemania
Fil: Ceolin, Marcelo Raul. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; Argentina
Fil: Mikolei, Joanna J.. Universitat Technische Darmstadt; Alemania
Fil: Pardehkhorram, Raheleh. Universitat Technische Darmstadt; Alemania
Fil: Andrieu Brunsen, Annette. Universitat Technische Darmstadt; Alemania
description Combinatorial sensing is especially important in the context of modern drug development to enable fast screening of large data sets. Mesoporous silica materials offer high surface area and a wide range of functionalization possibilities. By adding structural control, the combination of structural and functional control along all length scales opens a new pathway that permits larger amounts of analytes being tested simultaneously for complex sensing tasks. This study presents a fast and simple way to produce mesoporoussilica in various shapes and sizes between 0.27–6 mm by using light-induced sol-gel chemistry and digital light processing (DLP). Shape-selective functionalization of mesoporous silica is successfully carried out either after printing using organosilanes or in situ while printing through the use of functional mesopore template for the in situ functionalization approach. Shape-selective adsorption of dyes is shown as a demonstrator toward shape selective screening of potential analytes.
publishDate 2024
dc.date.none.fl_str_mv 2024-02
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/262276
Zhao, Lucy; Spiehl, Dieter; Kohnen, Marion C.; Ceolin, Marcelo Raul; Mikolei, Joanna J.; et al.; Printing of In Situ Functionalized Mesoporous Silica with Digital Light Processing for Combinatorial Sensing; Wiley VCH Verlag; Small; 20; 28; 2-2024; 1-9
1613-6810
CONICET Digital
CONICET
url http://hdl.handle.net/11336/262276
identifier_str_mv Zhao, Lucy; Spiehl, Dieter; Kohnen, Marion C.; Ceolin, Marcelo Raul; Mikolei, Joanna J.; et al.; Printing of In Situ Functionalized Mesoporous Silica with Digital Light Processing for Combinatorial Sensing; Wiley VCH Verlag; Small; 20; 28; 2-2024; 1-9
1613-6810
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://onlinelibrary.wiley.com/doi/10.1002/smll.202311121
info:eu-repo/semantics/altIdentifier/doi/10.1002/smll.202311121
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv Wiley VCH Verlag
publisher.none.fl_str_mv Wiley VCH Verlag
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
_version_ 1844613612641976320
score 13.070432

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