Kondo physics of magnetic adatoms on metallic surfaces when the onset of the surface conduction density of states crosses the Fermi level

Autores
Fernández, Joaquín; Roura Bas, Pablo Gines
Año de publicación
2019
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
We study the role of the onset of Shockley states Ds belonging to (111) surfaces of Cu, Ag, and Au in the Kondo effect when a magnetic impurity is deposited on them. When Ds approaches the Fermi level EF, which can be done by compressing (stretching) the metallic sample, we find that most of the thermodynamic and dynamic properties of the impurity are affected in a nontrivial way. We model the system by a generic Anderson impurity model and solve it by using the numerical renormalization group technique. In particular, the impurity contribution to magnetic susceptibility and entropy as a function of temperature exhibit negative values and go to zero slowly in a logarithmic shape. Furthermore, we found suppression of the spectral density weight at the Fermi level when Ds∼EF even in the Kondo regime. As a consequence, the conductance through the impurity is strongly reduced by nearly 25% of the unitary value 2e2/h. Finally, we analyze these features in realistic systems like Co on Ag(111) reported in the literature.
Fil: Fernández, Joaquín. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Patagonia Norte; Argentina
Fil: Roura Bas, Pablo Gines. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Patagonia Norte; Argentina
Materia
surface states
magnetic impurity
Kondo
NRG
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/123503
Acceder
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oai_identifier_str oai:ri.conicet.gov.ar:11336/123503
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network_name_str CONICET Digital (CONICET)
spelling Kondo physics of magnetic adatoms on metallic surfaces when the onset of the surface conduction density of states crosses the Fermi levelFernández, JoaquínRoura Bas, Pablo Ginessurface statesmagnetic impurityKondoNRGhttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1We study the role of the onset of Shockley states Ds belonging to (111) surfaces of Cu, Ag, and Au in the Kondo effect when a magnetic impurity is deposited on them. When Ds approaches the Fermi level EF, which can be done by compressing (stretching) the metallic sample, we find that most of the thermodynamic and dynamic properties of the impurity are affected in a nontrivial way. We model the system by a generic Anderson impurity model and solve it by using the numerical renormalization group technique. In particular, the impurity contribution to magnetic susceptibility and entropy as a function of temperature exhibit negative values and go to zero slowly in a logarithmic shape. Furthermore, we found suppression of the spectral density weight at the Fermi level when Ds∼EF even in the Kondo regime. As a consequence, the conductance through the impurity is strongly reduced by nearly 25% of the unitary value 2e2/h. Finally, we analyze these features in realistic systems like Co on Ag(111) reported in the literature.Fil: Fernández, Joaquín. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Patagonia Norte; ArgentinaFil: Roura Bas, Pablo Gines. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Patagonia Norte; ArgentinaAmerican Physical Society2019-10info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/123503Fernández, Joaquín; Roura Bas, Pablo Gines; Kondo physics of magnetic adatoms on metallic surfaces when the onset of the surface conduction density of states crosses the Fermi level; American Physical Society; Physical Review B; 100; 16; 10-2019; 165139-1651502469-99502469-9969CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://link.aps.org/doi/10.1103/PhysRevB.100.165139info:eu-repo/semantics/altIdentifier/doi/10.1103/PhysRevB.100.165139info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T09:55:38Zoai:ri.conicet.gov.ar:11336/123503instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 09:55:38.759CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Kondo physics of magnetic adatoms on metallic surfaces when the onset of the surface conduction density of states crosses the Fermi level
title Kondo physics of magnetic adatoms on metallic surfaces when the onset of the surface conduction density of states crosses the Fermi level
spellingShingle Kondo physics of magnetic adatoms on metallic surfaces when the onset of the surface conduction density of states crosses the Fermi level
Fernández, Joaquín
surface states
magnetic impurity
Kondo
NRG
title_short Kondo physics of magnetic adatoms on metallic surfaces when the onset of the surface conduction density of states crosses the Fermi level
title_full Kondo physics of magnetic adatoms on metallic surfaces when the onset of the surface conduction density of states crosses the Fermi level
title_fullStr Kondo physics of magnetic adatoms on metallic surfaces when the onset of the surface conduction density of states crosses the Fermi level
title_full_unstemmed Kondo physics of magnetic adatoms on metallic surfaces when the onset of the surface conduction density of states crosses the Fermi level
title_sort Kondo physics of magnetic adatoms on metallic surfaces when the onset of the surface conduction density of states crosses the Fermi level
dc.creator.none.fl_str_mv Fernández, Joaquín
Roura Bas, Pablo Gines
author Fernández, Joaquín
author_facet Fernández, Joaquín
Roura Bas, Pablo Gines
author_role author
author2 Roura Bas, Pablo Gines
author2_role author
dc.subject.none.fl_str_mv surface states
magnetic impurity
Kondo
NRG
topic surface states
magnetic impurity
Kondo
NRG
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv We study the role of the onset of Shockley states Ds belonging to (111) surfaces of Cu, Ag, and Au in the Kondo effect when a magnetic impurity is deposited on them. When Ds approaches the Fermi level EF, which can be done by compressing (stretching) the metallic sample, we find that most of the thermodynamic and dynamic properties of the impurity are affected in a nontrivial way. We model the system by a generic Anderson impurity model and solve it by using the numerical renormalization group technique. In particular, the impurity contribution to magnetic susceptibility and entropy as a function of temperature exhibit negative values and go to zero slowly in a logarithmic shape. Furthermore, we found suppression of the spectral density weight at the Fermi level when Ds∼EF even in the Kondo regime. As a consequence, the conductance through the impurity is strongly reduced by nearly 25% of the unitary value 2e2/h. Finally, we analyze these features in realistic systems like Co on Ag(111) reported in the literature.
Fil: Fernández, Joaquín. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Patagonia Norte; Argentina
Fil: Roura Bas, Pablo Gines. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Patagonia Norte; Argentina
description We study the role of the onset of Shockley states Ds belonging to (111) surfaces of Cu, Ag, and Au in the Kondo effect when a magnetic impurity is deposited on them. When Ds approaches the Fermi level EF, which can be done by compressing (stretching) the metallic sample, we find that most of the thermodynamic and dynamic properties of the impurity are affected in a nontrivial way. We model the system by a generic Anderson impurity model and solve it by using the numerical renormalization group technique. In particular, the impurity contribution to magnetic susceptibility and entropy as a function of temperature exhibit negative values and go to zero slowly in a logarithmic shape. Furthermore, we found suppression of the spectral density weight at the Fermi level when Ds∼EF even in the Kondo regime. As a consequence, the conductance through the impurity is strongly reduced by nearly 25% of the unitary value 2e2/h. Finally, we analyze these features in realistic systems like Co on Ag(111) reported in the literature.
publishDate 2019
dc.date.none.fl_str_mv 2019-10
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/123503
Fernández, Joaquín; Roura Bas, Pablo Gines; Kondo physics of magnetic adatoms on metallic surfaces when the onset of the surface conduction density of states crosses the Fermi level; American Physical Society; Physical Review B; 100; 16; 10-2019; 165139-165150
2469-9950
2469-9969
CONICET Digital
CONICET
url http://hdl.handle.net/11336/123503
identifier_str_mv Fernández, Joaquín; Roura Bas, Pablo Gines; Kondo physics of magnetic adatoms on metallic surfaces when the onset of the surface conduction density of states crosses the Fermi level; American Physical Society; Physical Review B; 100; 16; 10-2019; 165139-165150
2469-9950
2469-9969
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://link.aps.org/doi/10.1103/PhysRevB.100.165139
info:eu-repo/semantics/altIdentifier/doi/10.1103/PhysRevB.100.165139
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
application/pdf
dc.publisher.none.fl_str_mv American Physical Society
publisher.none.fl_str_mv American Physical Society
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
_version_ 1844613675964432384
score 13.070432

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