Fragmented monopole crystal, dimer entropy, and Coulomb interactions in Dy2Ir2O 7
- Autores
- Cathelin, V.; Lefrançois, E.; Robert, J.; Guruciaga, Pamela Carolina; Paulsen, C.; Prabhakaran, D.; Lejay, P.; Damay, F.; Ollivier, J.; Fåk, B.; Chapon, L. C.; Ballou, Rafik; Simonet, V.; Holdsworth, P. C. W.; Lhotel, E.
- Año de publicación
- 2020
- Idioma
- inglés
- Tipo de recurso
- artículo
- Estado
- versión publicada
- Descripción
- Neutron scattering, specific-heat, and magnetization measurements on both powders and single crystals reveal that Dy2Ir2O7 realizes the fragmented monopole crystal state in which antiferromagnetic order and a Coulomb phase spin liquid coinhabit. The measured residual entropy is that of a hard-core dimer liquid, as predicted. Inclusion of Coulomb interactions allows for a quantitative description of both the thermodynamic data and the magnetization dynamics, with the energy scale given by deconfined defects in the emergent ionic crystal. Our data reveal low-energy excitations, as well as a large distribution of energy barriers down to low temperatures, while the magnetic response to an applied field suggests that domain wall pinning is important, results that call for further theoretical modeling.
Fil: Cathelin, V.. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; Francia
Fil: Lefrançois, E.. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; Francia. Institut Laue Langevin; Francia
Fil: Robert, J.. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; Francia
Fil: Guruciaga, Pamela Carolina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Patagonia Norte; Argentina. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina
Fil: Paulsen, C.. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; Francia
Fil: Prabhakaran, D.. University of Oxford. Department of Physics; Reino Unido
Fil: Lejay, P.. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; Francia
Fil: Damay, F.. Centre National de la Recherche Scientifique; Francia. Université Paris-saclay; Francia
Fil: Ollivier, J.. Institut Laue Langevin; Francia
Fil: Fåk, B.. Institut Laue Langevin; Francia. Diamond Light Source Limited. Harwell Science and Innovation Campus; Reino Unido
Fil: Chapon, L. C.. Institut Laue Langevin; Francia. Diamond Light Source Limited. Harwell Science and Innovation Campus; Reino Unido
Fil: Ballou, Rafik. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; Francia
Fil: Simonet, V.. Institut Néel; Francia. Universite Grenoble Alpes; Francia. Centre National de la Recherche Scientifique; Francia
Fil: Holdsworth, P. C. W.. Université Claude Bernard Lyon 1; Francia. Centre National de la Recherche Scientifique; Francia
Fil: Lhotel, E.. Institut Néel; Francia. Universite Grenoble Alpes; Francia. Centre National de la Recherche Scientifique; Francia - Materia
-
FRUSTRATED MAGNETIC SYSTEMS
COULOMB PHASE
SPIN LIQUID - Nivel de accesibilidad
- acceso abierto
- Condiciones de uso
- https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
- Repositorio
- Institución
- Consejo Nacional de Investigaciones Científicas y Técnicas
- OAI Identificador
- oai:ri.conicet.gov.ar:11336/140403
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Fragmented monopole crystal, dimer entropy, and Coulomb interactions in Dy2Ir2O 7Cathelin, V.Lefrançois, E.Robert, J.Guruciaga, Pamela CarolinaPaulsen, C.Prabhakaran, D.Lejay, P.Damay, F.Ollivier, J.Fåk, B.Chapon, L. C.Ballou, RafikSimonet, V.Holdsworth, P. C. W.Lhotel, E.FRUSTRATED MAGNETIC SYSTEMSCOULOMB PHASESPIN LIQUIDhttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1Neutron scattering, specific-heat, and magnetization measurements on both powders and single crystals reveal that Dy2Ir2O7 realizes the fragmented monopole crystal state in which antiferromagnetic order and a Coulomb phase spin liquid coinhabit. The measured residual entropy is that of a hard-core dimer liquid, as predicted. Inclusion of Coulomb interactions allows for a quantitative description of both the thermodynamic data and the magnetization dynamics, with the energy scale given by deconfined defects in the emergent ionic crystal. Our data reveal low-energy excitations, as well as a large distribution of energy barriers down to low temperatures, while the magnetic response to an applied field suggests that domain wall pinning is important, results that call for further theoretical modeling.Fil: Cathelin, V.. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; FranciaFil: Lefrançois, E.. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; Francia. Institut Laue Langevin; FranciaFil: Robert, J.. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; FranciaFil: Guruciaga, Pamela Carolina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Patagonia Norte; Argentina. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; ArgentinaFil: Paulsen, C.. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; FranciaFil: Prabhakaran, D.. University of Oxford. Department of Physics; Reino UnidoFil: Lejay, P.. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; FranciaFil: Damay, F.. Centre National de la Recherche Scientifique; Francia. Université Paris-saclay; FranciaFil: Ollivier, J.. Institut Laue Langevin; FranciaFil: Fåk, B.. Institut Laue Langevin; Francia. Diamond Light Source Limited. Harwell Science and Innovation Campus; Reino UnidoFil: Chapon, L. C.. Institut Laue Langevin; Francia. Diamond Light Source Limited. Harwell Science and Innovation Campus; Reino UnidoFil: Ballou, Rafik. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; FranciaFil: Simonet, V.. Institut Néel; Francia. Universite Grenoble Alpes; Francia. Centre National de la Recherche Scientifique; FranciaFil: Holdsworth, P. C. W.. Université Claude Bernard Lyon 1; Francia. Centre National de la Recherche Scientifique; FranciaFil: Lhotel, E.. Institut Néel; Francia. Universite Grenoble Alpes; Francia. Centre National de la Recherche Scientifique; FranciaAmerican Physical Society2020-09info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/140403Cathelin, V.; Lefrançois, E.; Robert, J.; Guruciaga, Pamela Carolina; Paulsen, C.; et al.; Fragmented monopole crystal, dimer entropy, and Coulomb interactions in Dy2Ir2O 7; American Physical Society; Physical Review Research; 2; 3; 9-2020; 1-62643-1564CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://link.aps.org/doi/10.1103/PhysRevResearch.2.032073info:eu-repo/semantics/altIdentifier/doi/10.1103/PhysRevResearch.2.032073info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T09:38:29Zoai:ri.conicet.gov.ar:11336/140403instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 09:38:29.845CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse |
dc.title.none.fl_str_mv |
Fragmented monopole crystal, dimer entropy, and Coulomb interactions in Dy2Ir2O 7 |
title |
Fragmented monopole crystal, dimer entropy, and Coulomb interactions in Dy2Ir2O 7 |
spellingShingle |
Fragmented monopole crystal, dimer entropy, and Coulomb interactions in Dy2Ir2O 7 Cathelin, V. FRUSTRATED MAGNETIC SYSTEMS COULOMB PHASE SPIN LIQUID |
title_short |
Fragmented monopole crystal, dimer entropy, and Coulomb interactions in Dy2Ir2O 7 |
title_full |
Fragmented monopole crystal, dimer entropy, and Coulomb interactions in Dy2Ir2O 7 |
title_fullStr |
Fragmented monopole crystal, dimer entropy, and Coulomb interactions in Dy2Ir2O 7 |
title_full_unstemmed |
Fragmented monopole crystal, dimer entropy, and Coulomb interactions in Dy2Ir2O 7 |
title_sort |
Fragmented monopole crystal, dimer entropy, and Coulomb interactions in Dy2Ir2O 7 |
dc.creator.none.fl_str_mv |
Cathelin, V. Lefrançois, E. Robert, J. Guruciaga, Pamela Carolina Paulsen, C. Prabhakaran, D. Lejay, P. Damay, F. Ollivier, J. Fåk, B. Chapon, L. C. Ballou, Rafik Simonet, V. Holdsworth, P. C. W. Lhotel, E. |
author |
Cathelin, V. |
author_facet |
Cathelin, V. Lefrançois, E. Robert, J. Guruciaga, Pamela Carolina Paulsen, C. Prabhakaran, D. Lejay, P. Damay, F. Ollivier, J. Fåk, B. Chapon, L. C. Ballou, Rafik Simonet, V. Holdsworth, P. C. W. Lhotel, E. |
author_role |
author |
author2 |
Lefrançois, E. Robert, J. Guruciaga, Pamela Carolina Paulsen, C. Prabhakaran, D. Lejay, P. Damay, F. Ollivier, J. Fåk, B. Chapon, L. C. Ballou, Rafik Simonet, V. Holdsworth, P. C. W. Lhotel, E. |
author2_role |
author author author author author author author author author author author author author author |
dc.subject.none.fl_str_mv |
FRUSTRATED MAGNETIC SYSTEMS COULOMB PHASE SPIN LIQUID |
topic |
FRUSTRATED MAGNETIC SYSTEMS COULOMB PHASE SPIN LIQUID |
purl_subject.fl_str_mv |
https://purl.org/becyt/ford/1.3 https://purl.org/becyt/ford/1 |
dc.description.none.fl_txt_mv |
Neutron scattering, specific-heat, and magnetization measurements on both powders and single crystals reveal that Dy2Ir2O7 realizes the fragmented monopole crystal state in which antiferromagnetic order and a Coulomb phase spin liquid coinhabit. The measured residual entropy is that of a hard-core dimer liquid, as predicted. Inclusion of Coulomb interactions allows for a quantitative description of both the thermodynamic data and the magnetization dynamics, with the energy scale given by deconfined defects in the emergent ionic crystal. Our data reveal low-energy excitations, as well as a large distribution of energy barriers down to low temperatures, while the magnetic response to an applied field suggests that domain wall pinning is important, results that call for further theoretical modeling. Fil: Cathelin, V.. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; Francia Fil: Lefrançois, E.. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; Francia. Institut Laue Langevin; Francia Fil: Robert, J.. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; Francia Fil: Guruciaga, Pamela Carolina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Patagonia Norte; Argentina. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina Fil: Paulsen, C.. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; Francia Fil: Prabhakaran, D.. University of Oxford. Department of Physics; Reino Unido Fil: Lejay, P.. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; Francia Fil: Damay, F.. Centre National de la Recherche Scientifique; Francia. Université Paris-saclay; Francia Fil: Ollivier, J.. Institut Laue Langevin; Francia Fil: Fåk, B.. Institut Laue Langevin; Francia. Diamond Light Source Limited. Harwell Science and Innovation Campus; Reino Unido Fil: Chapon, L. C.. Institut Laue Langevin; Francia. Diamond Light Source Limited. Harwell Science and Innovation Campus; Reino Unido Fil: Ballou, Rafik. Centre National de la Recherche Scientifique; Francia. Universite Grenoble Alpes; Francia. Institut Néel; Francia Fil: Simonet, V.. Institut Néel; Francia. Universite Grenoble Alpes; Francia. Centre National de la Recherche Scientifique; Francia Fil: Holdsworth, P. C. W.. Université Claude Bernard Lyon 1; Francia. Centre National de la Recherche Scientifique; Francia Fil: Lhotel, E.. Institut Néel; Francia. Universite Grenoble Alpes; Francia. Centre National de la Recherche Scientifique; Francia |
description |
Neutron scattering, specific-heat, and magnetization measurements on both powders and single crystals reveal that Dy2Ir2O7 realizes the fragmented monopole crystal state in which antiferromagnetic order and a Coulomb phase spin liquid coinhabit. The measured residual entropy is that of a hard-core dimer liquid, as predicted. Inclusion of Coulomb interactions allows for a quantitative description of both the thermodynamic data and the magnetization dynamics, with the energy scale given by deconfined defects in the emergent ionic crystal. Our data reveal low-energy excitations, as well as a large distribution of energy barriers down to low temperatures, while the magnetic response to an applied field suggests that domain wall pinning is important, results that call for further theoretical modeling. |
publishDate |
2020 |
dc.date.none.fl_str_mv |
2020-09 |
dc.type.none.fl_str_mv |
info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion http://purl.org/coar/resource_type/c_6501 info:ar-repo/semantics/articulo |
format |
article |
status_str |
publishedVersion |
dc.identifier.none.fl_str_mv |
http://hdl.handle.net/11336/140403 Cathelin, V.; Lefrançois, E.; Robert, J.; Guruciaga, Pamela Carolina; Paulsen, C.; et al.; Fragmented monopole crystal, dimer entropy, and Coulomb interactions in Dy2Ir2O 7; American Physical Society; Physical Review Research; 2; 3; 9-2020; 1-6 2643-1564 CONICET Digital CONICET |
url |
http://hdl.handle.net/11336/140403 |
identifier_str_mv |
Cathelin, V.; Lefrançois, E.; Robert, J.; Guruciaga, Pamela Carolina; Paulsen, C.; et al.; Fragmented monopole crystal, dimer entropy, and Coulomb interactions in Dy2Ir2O 7; American Physical Society; Physical Review Research; 2; 3; 9-2020; 1-6 2643-1564 CONICET Digital CONICET |
dc.language.none.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
info:eu-repo/semantics/altIdentifier/url/https://link.aps.org/doi/10.1103/PhysRevResearch.2.032073 info:eu-repo/semantics/altIdentifier/doi/10.1103/PhysRevResearch.2.032073 |
dc.rights.none.fl_str_mv |
info:eu-repo/semantics/openAccess https://creativecommons.org/licenses/by-nc-sa/2.5/ar/ |
eu_rights_str_mv |
openAccess |
rights_invalid_str_mv |
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/ |
dc.format.none.fl_str_mv |
application/pdf application/pdf |
dc.publisher.none.fl_str_mv |
American Physical Society |
publisher.none.fl_str_mv |
American Physical Society |
dc.source.none.fl_str_mv |
reponame:CONICET Digital (CONICET) instname:Consejo Nacional de Investigaciones Científicas y Técnicas |
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CONICET Digital (CONICET) |
collection |
CONICET Digital (CONICET) |
instname_str |
Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.name.fl_str_mv |
CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.mail.fl_str_mv |
dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar |
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1844613216452214784 |
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13.070432 |