Structural magnetic glassiness in the spin ice Dy 2 Ti 2 O 7

Autores
Samarakoon, Anjana M.; Sokolowski, André; Klemke, Bastian; Feyerherm, Ralf; Meissner, Michael; Borzi, Rodolfo Alberto; Ye, Feng; Zhang, Qiang; Dun, Zhiling; Zhou, Haidong; Egami, T.; Hallén, Jonathan N.; Jaubert, Ludovic; Castelnovo, Claudio; Moessner, Roderich; Grigera, Santiago Andrés; Tennant, D. Alan
Año de publicación
2022
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
The origin and nature of glassy dynamics presents one of the central enigmas of condensed-matter physics across a broad range of systems ranging from window glass to spin glasses. The spin-ice compound Dy2Ti2O7, which is perhaps best known as hosting a three-dimensional Coulomb spin liquid with magnetically charged monopole excitations, also falls out of equilibrium at low temperature. How and why it does so remains an open question. Based on an analysis of low-temperature diffuse neutron-scattering experiments employing different cooling protocols alongside recent magnetic noise studies, combined with extensive numerical modeling, we argue that upon cooling, the spins freeze into what may be termed a "structural magnetic glass,"without an a priori need for chemical or structural disorder. Specifically, our model indicates the presence of frustration on two levels, first producing a near-degenerate constrained manifold inside which phase ordering kinetics is in turn frustrated. A remarkable feature is that monopoles act as sole annealers of the spin network and their pathways and history encode the development of glass dynamics, allowing the glass formation to be visualized. Our results suggest that spin ice Dy2Ti2O7 provides one prototype of magnetic glass formation specifically and a setting for the study of kinetically constrained systems more generally.
Fil: Samarakoon, Anjana M.. Oak Ridge National Laboratory; Estados Unidos. Argonne National Laboratory; Estados Unidos
Fil: Sokolowski, André. Helmholtz-zentrum Berlin Für Materialien Und Energie; Alemania
Fil: Klemke, Bastian. Helmholtz-zentrum Berlin Für Materialien Und Energie; Alemania
Fil: Feyerherm, Ralf. Helmholtz-zentrum Berlin Für Materialien Und Energie; Alemania
Fil: Meissner, Michael. Helmholtz-zentrum Berlin Für Materialien Und Energie; Alemania
Fil: Borzi, Rodolfo Alberto. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Física de Líquidos y Sistemas Biológicos. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Física de Líquidos y Sistemas Biológicos; Argentina
Fil: Ye, Feng. Oak Ridge National Laboratory; Estados Unidos
Fil: Zhang, Qiang. Oak Ridge National Laboratory; Estados Unidos
Fil: Dun, Zhiling. University of Tennessee; Estados Unidos
Fil: Zhou, Haidong. University of Tennessee; Estados Unidos
Fil: Egami, T.. University of Tennessee; Estados Unidos. Oak Ridge National Laboratory; Alemania
Fil: Hallén, Jonathan N.. Max Planck Institute For The Physics Of Complex Systems; Alemania. University of Cambridge; Estados Unidos
Fil: Jaubert, Ludovic. Max Planck Institute For The Physics Of Complex Systems; Alemania
Fil: Castelnovo, Claudio. University of Cambridge; Estados Unidos
Fil: Moessner, Roderich. Max Planck Institute For The Physics Of Complex Systems; Alemania
Fil: Grigera, Santiago Andrés. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Física de Líquidos y Sistemas Biológicos. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Física de Líquidos y Sistemas Biológicos; Argentina
Fil: Tennant, D. Alan. University of Tennessee; Estados Unidos. Oak Ridge National Laboratory; Estados Unidos
Materia
magnetism
frustrated materials
glassiness
spin ice
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/212670
Acceder
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oai_identifier_str oai:ri.conicet.gov.ar:11336/212670
network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Structural magnetic glassiness in the spin ice Dy 2 Ti 2 O 7Samarakoon, Anjana M.Sokolowski, AndréKlemke, BastianFeyerherm, RalfMeissner, MichaelBorzi, Rodolfo AlbertoYe, FengZhang, QiangDun, ZhilingZhou, HaidongEgami, T.Hallén, Jonathan N.Jaubert, LudovicCastelnovo, ClaudioMoessner, RoderichGrigera, Santiago AndrésTennant, D. Alanmagnetismfrustrated materialsglassinessspin icehttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1The origin and nature of glassy dynamics presents one of the central enigmas of condensed-matter physics across a broad range of systems ranging from window glass to spin glasses. The spin-ice compound Dy2Ti2O7, which is perhaps best known as hosting a three-dimensional Coulomb spin liquid with magnetically charged monopole excitations, also falls out of equilibrium at low temperature. How and why it does so remains an open question. Based on an analysis of low-temperature diffuse neutron-scattering experiments employing different cooling protocols alongside recent magnetic noise studies, combined with extensive numerical modeling, we argue that upon cooling, the spins freeze into what may be termed a "structural magnetic glass,"without an a priori need for chemical or structural disorder. Specifically, our model indicates the presence of frustration on two levels, first producing a near-degenerate constrained manifold inside which phase ordering kinetics is in turn frustrated. A remarkable feature is that monopoles act as sole annealers of the spin network and their pathways and history encode the development of glass dynamics, allowing the glass formation to be visualized. Our results suggest that spin ice Dy2Ti2O7 provides one prototype of magnetic glass formation specifically and a setting for the study of kinetically constrained systems more generally.Fil: Samarakoon, Anjana M.. Oak Ridge National Laboratory; Estados Unidos. Argonne National Laboratory; Estados UnidosFil: Sokolowski, André. Helmholtz-zentrum Berlin Für Materialien Und Energie; AlemaniaFil: Klemke, Bastian. Helmholtz-zentrum Berlin Für Materialien Und Energie; AlemaniaFil: Feyerherm, Ralf. Helmholtz-zentrum Berlin Für Materialien Und Energie; AlemaniaFil: Meissner, Michael. Helmholtz-zentrum Berlin Für Materialien Und Energie; AlemaniaFil: Borzi, Rodolfo Alberto. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Física de Líquidos y Sistemas Biológicos. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Física de Líquidos y Sistemas Biológicos; ArgentinaFil: Ye, Feng. Oak Ridge National Laboratory; Estados UnidosFil: Zhang, Qiang. Oak Ridge National Laboratory; Estados UnidosFil: Dun, Zhiling. University of Tennessee; Estados UnidosFil: Zhou, Haidong. University of Tennessee; Estados UnidosFil: Egami, T.. University of Tennessee; Estados Unidos. Oak Ridge National Laboratory; AlemaniaFil: Hallén, Jonathan N.. Max Planck Institute For The Physics Of Complex Systems; Alemania. University of Cambridge; Estados UnidosFil: Jaubert, Ludovic. Max Planck Institute For The Physics Of Complex Systems; AlemaniaFil: Castelnovo, Claudio. University of Cambridge; Estados UnidosFil: Moessner, Roderich. Max Planck Institute For The Physics Of Complex Systems; AlemaniaFil: Grigera, Santiago Andrés. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Física de Líquidos y Sistemas Biológicos. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Física de Líquidos y Sistemas Biológicos; ArgentinaFil: Tennant, D. Alan. University of Tennessee; Estados Unidos. Oak Ridge National Laboratory; Estados UnidosAmerican Physical Society2022-08info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/212670Samarakoon, Anjana M.; Sokolowski, André; Klemke, Bastian; Feyerherm, Ralf; Meissner, Michael; et al.; Structural magnetic glassiness in the spin ice Dy 2 Ti 2 O 7; American Physical Society; Physical Review Research; 4; 3; 8-2022; 1-82643-1564CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://link.aps.org/doi/10.1103/PhysRevResearch.4.033159info:eu-repo/semantics/altIdentifier/doi/10.1103/PhysRevResearch.4.033159info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T09:34:25Zoai:ri.conicet.gov.ar:11336/212670instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 09:34:26.185CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Structural magnetic glassiness in the spin ice Dy 2 Ti 2 O 7
title Structural magnetic glassiness in the spin ice Dy 2 Ti 2 O 7
spellingShingle Structural magnetic glassiness in the spin ice Dy 2 Ti 2 O 7
Samarakoon, Anjana M.
magnetism
frustrated materials
glassiness
spin ice
title_short Structural magnetic glassiness in the spin ice Dy 2 Ti 2 O 7
title_full Structural magnetic glassiness in the spin ice Dy 2 Ti 2 O 7
title_fullStr Structural magnetic glassiness in the spin ice Dy 2 Ti 2 O 7
title_full_unstemmed Structural magnetic glassiness in the spin ice Dy 2 Ti 2 O 7
title_sort Structural magnetic glassiness in the spin ice Dy 2 Ti 2 O 7
dc.creator.none.fl_str_mv Samarakoon, Anjana M.
Sokolowski, André
Klemke, Bastian
Feyerherm, Ralf
Meissner, Michael
Borzi, Rodolfo Alberto
Ye, Feng
Zhang, Qiang
Dun, Zhiling
Zhou, Haidong
Egami, T.
Hallén, Jonathan N.
Jaubert, Ludovic
Castelnovo, Claudio
Moessner, Roderich
Grigera, Santiago Andrés
Tennant, D. Alan
author Samarakoon, Anjana M.
author_facet Samarakoon, Anjana M.
Sokolowski, André
Klemke, Bastian
Feyerherm, Ralf
Meissner, Michael
Borzi, Rodolfo Alberto
Ye, Feng
Zhang, Qiang
Dun, Zhiling
Zhou, Haidong
Egami, T.
Hallén, Jonathan N.
Jaubert, Ludovic
Castelnovo, Claudio
Moessner, Roderich
Grigera, Santiago Andrés
Tennant, D. Alan
author_role author
author2 Sokolowski, André
Klemke, Bastian
Feyerherm, Ralf
Meissner, Michael
Borzi, Rodolfo Alberto
Ye, Feng
Zhang, Qiang
Dun, Zhiling
Zhou, Haidong
Egami, T.
Hallén, Jonathan N.
Jaubert, Ludovic
Castelnovo, Claudio
Moessner, Roderich
Grigera, Santiago Andrés
Tennant, D. Alan
author2_role author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
author
dc.subject.none.fl_str_mv magnetism
frustrated materials
glassiness
spin ice
topic magnetism
frustrated materials
glassiness
spin ice
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv The origin and nature of glassy dynamics presents one of the central enigmas of condensed-matter physics across a broad range of systems ranging from window glass to spin glasses. The spin-ice compound Dy2Ti2O7, which is perhaps best known as hosting a three-dimensional Coulomb spin liquid with magnetically charged monopole excitations, also falls out of equilibrium at low temperature. How and why it does so remains an open question. Based on an analysis of low-temperature diffuse neutron-scattering experiments employing different cooling protocols alongside recent magnetic noise studies, combined with extensive numerical modeling, we argue that upon cooling, the spins freeze into what may be termed a "structural magnetic glass,"without an a priori need for chemical or structural disorder. Specifically, our model indicates the presence of frustration on two levels, first producing a near-degenerate constrained manifold inside which phase ordering kinetics is in turn frustrated. A remarkable feature is that monopoles act as sole annealers of the spin network and their pathways and history encode the development of glass dynamics, allowing the glass formation to be visualized. Our results suggest that spin ice Dy2Ti2O7 provides one prototype of magnetic glass formation specifically and a setting for the study of kinetically constrained systems more generally.
Fil: Samarakoon, Anjana M.. Oak Ridge National Laboratory; Estados Unidos. Argonne National Laboratory; Estados Unidos
Fil: Sokolowski, André. Helmholtz-zentrum Berlin Für Materialien Und Energie; Alemania
Fil: Klemke, Bastian. Helmholtz-zentrum Berlin Für Materialien Und Energie; Alemania
Fil: Feyerherm, Ralf. Helmholtz-zentrum Berlin Für Materialien Und Energie; Alemania
Fil: Meissner, Michael. Helmholtz-zentrum Berlin Für Materialien Und Energie; Alemania
Fil: Borzi, Rodolfo Alberto. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Física de Líquidos y Sistemas Biológicos. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Física de Líquidos y Sistemas Biológicos; Argentina
Fil: Ye, Feng. Oak Ridge National Laboratory; Estados Unidos
Fil: Zhang, Qiang. Oak Ridge National Laboratory; Estados Unidos
Fil: Dun, Zhiling. University of Tennessee; Estados Unidos
Fil: Zhou, Haidong. University of Tennessee; Estados Unidos
Fil: Egami, T.. University of Tennessee; Estados Unidos. Oak Ridge National Laboratory; Alemania
Fil: Hallén, Jonathan N.. Max Planck Institute For The Physics Of Complex Systems; Alemania. University of Cambridge; Estados Unidos
Fil: Jaubert, Ludovic. Max Planck Institute For The Physics Of Complex Systems; Alemania
Fil: Castelnovo, Claudio. University of Cambridge; Estados Unidos
Fil: Moessner, Roderich. Max Planck Institute For The Physics Of Complex Systems; Alemania
Fil: Grigera, Santiago Andrés. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Física de Líquidos y Sistemas Biológicos. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Física de Líquidos y Sistemas Biológicos; Argentina
Fil: Tennant, D. Alan. University of Tennessee; Estados Unidos. Oak Ridge National Laboratory; Estados Unidos
description The origin and nature of glassy dynamics presents one of the central enigmas of condensed-matter physics across a broad range of systems ranging from window glass to spin glasses. The spin-ice compound Dy2Ti2O7, which is perhaps best known as hosting a three-dimensional Coulomb spin liquid with magnetically charged monopole excitations, also falls out of equilibrium at low temperature. How and why it does so remains an open question. Based on an analysis of low-temperature diffuse neutron-scattering experiments employing different cooling protocols alongside recent magnetic noise studies, combined with extensive numerical modeling, we argue that upon cooling, the spins freeze into what may be termed a "structural magnetic glass,"without an a priori need for chemical or structural disorder. Specifically, our model indicates the presence of frustration on two levels, first producing a near-degenerate constrained manifold inside which phase ordering kinetics is in turn frustrated. A remarkable feature is that monopoles act as sole annealers of the spin network and their pathways and history encode the development of glass dynamics, allowing the glass formation to be visualized. Our results suggest that spin ice Dy2Ti2O7 provides one prototype of magnetic glass formation specifically and a setting for the study of kinetically constrained systems more generally.
publishDate 2022
dc.date.none.fl_str_mv 2022-08
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/212670
Samarakoon, Anjana M.; Sokolowski, André; Klemke, Bastian; Feyerherm, Ralf; Meissner, Michael; et al.; Structural magnetic glassiness in the spin ice Dy 2 Ti 2 O 7; American Physical Society; Physical Review Research; 4; 3; 8-2022; 1-8
2643-1564
CONICET Digital
CONICET
url http://hdl.handle.net/11336/212670
identifier_str_mv Samarakoon, Anjana M.; Sokolowski, André; Klemke, Bastian; Feyerherm, Ralf; Meissner, Michael; et al.; Structural magnetic glassiness in the spin ice Dy 2 Ti 2 O 7; American Physical Society; Physical Review Research; 4; 3; 8-2022; 1-8
2643-1564
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://link.aps.org/doi/10.1103/PhysRevResearch.4.033159
info:eu-repo/semantics/altIdentifier/doi/10.1103/PhysRevResearch.4.033159
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
application/pdf
dc.publisher.none.fl_str_mv American Physical Society
publisher.none.fl_str_mv American Physical Society
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 13.070432

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