Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays

Autores
Ezendam, Simone; Nan, Lin; Violi, Ianina Lucila; Maier, Stefan A.; Cortés, Emiliano; Baffou, Guillaume; Gargiulo, Julian
Año de publicación
2023
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
Metallic nanoparticles possess strong photothermal responses, especially when illuminated as ensembles due to collective effects. However, accurately quantifying the temperature increase remains a significant challenge, impeding progress in several applications. Anti Stokes thermometry offers a promising solution by enabling direct and non-invasive temperature measurements of the metal without the need for labeling or prior calibration. While Anti Stokes thermometry is successfully applied to individual nanoparticles, its potential to study light-to-heat conversion with plasmonic ensembles remains unexplored. In this study, the theoretical framework and the conditions that must be fulfilled for applying Anti Stokes thermometry to ensembles of nanoparticles are discussed. Then, this technique is implemented to measure the light-induced heating of square arrays of Au nanodisks. The obtained temperature measurements are validated using wavefront microscopy, demonstrating excellent agreement between the two thermometry methods. These results showcase the extension of Anti Stokes thermometry to plasmonic ensembles, highlighting its potential for implementation in the diverse photothermal applications involving these systems.
Fil: Ezendam, Simone. Ludwig Maximilians Universitat; Alemania
Fil: Nan, Lin. Ludwig Maximilians Universitat; Alemania
Fil: Violi, Ianina Lucila. Universidad Nacional de San Martin. Instituto de Nanosistemas; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Maier, Stefan A.. Imperial College London; Reino Unido. Monash University; Australia. Ludwig Maximilians Universitat; Alemania
Fil: Cortés, Emiliano. Ludwig Maximilians Universitat; Alemania. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Baffou, Guillaume. Centre National de la Recherche Scientifique; Francia
Fil: Gargiulo, Julian. Ludwig Maximilians Universitat; Alemania. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Materia
ANTI STOKES PHOTOLUMINESCENCE
NANOTHERMOMETRY
PHOTOTHERMAL EFFECT
THERMOPLASMONICS
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/220002
Acceder
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network_name_str CONICET Digital (CONICET)
spelling Anti Stokes Thermometry of Plasmonic Nanoparticle ArraysEzendam, SimoneNan, LinVioli, Ianina LucilaMaier, Stefan A.Cortés, EmilianoBaffou, GuillaumeGargiulo, JulianANTI STOKES PHOTOLUMINESCENCENANOTHERMOMETRYPHOTOTHERMAL EFFECTTHERMOPLASMONICShttps://purl.org/becyt/ford/2.10https://purl.org/becyt/ford/2Metallic nanoparticles possess strong photothermal responses, especially when illuminated as ensembles due to collective effects. However, accurately quantifying the temperature increase remains a significant challenge, impeding progress in several applications. Anti Stokes thermometry offers a promising solution by enabling direct and non-invasive temperature measurements of the metal without the need for labeling or prior calibration. While Anti Stokes thermometry is successfully applied to individual nanoparticles, its potential to study light-to-heat conversion with plasmonic ensembles remains unexplored. In this study, the theoretical framework and the conditions that must be fulfilled for applying Anti Stokes thermometry to ensembles of nanoparticles are discussed. Then, this technique is implemented to measure the light-induced heating of square arrays of Au nanodisks. The obtained temperature measurements are validated using wavefront microscopy, demonstrating excellent agreement between the two thermometry methods. These results showcase the extension of Anti Stokes thermometry to plasmonic ensembles, highlighting its potential for implementation in the diverse photothermal applications involving these systems.Fil: Ezendam, Simone. Ludwig Maximilians Universitat; AlemaniaFil: Nan, Lin. Ludwig Maximilians Universitat; AlemaniaFil: Violi, Ianina Lucila. Universidad Nacional de San Martin. Instituto de Nanosistemas; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaFil: Maier, Stefan A.. Imperial College London; Reino Unido. Monash University; Australia. Ludwig Maximilians Universitat; AlemaniaFil: Cortés, Emiliano. Ludwig Maximilians Universitat; Alemania. Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaFil: Baffou, Guillaume. Centre National de la Recherche Scientifique; FranciaFil: Gargiulo, Julian. Ludwig Maximilians Universitat; Alemania. Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaWiley2023-09info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/220002Ezendam, Simone; Nan, Lin; Violi, Ianina Lucila; Maier, Stefan A.; Cortés, Emiliano; et al.; Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays; Wiley; Advanced Optical Materials; 9-2023; 1-82195-1071CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://onlinelibrary.wiley.com/doi/10.1002/adom.202301496info:eu-repo/semantics/altIdentifier/doi/10.1002/adom.202301496info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-10-22T12:09:51Zoai:ri.conicet.gov.ar:11336/220002instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-10-22 12:09:51.388CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays
title Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays
spellingShingle Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays
Ezendam, Simone
ANTI STOKES PHOTOLUMINESCENCE
NANOTHERMOMETRY
PHOTOTHERMAL EFFECT
THERMOPLASMONICS
title_short Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays
title_full Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays
title_fullStr Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays
title_full_unstemmed Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays
title_sort Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays
dc.creator.none.fl_str_mv Ezendam, Simone
Nan, Lin
Violi, Ianina Lucila
Maier, Stefan A.
Cortés, Emiliano
Baffou, Guillaume
Gargiulo, Julian
author Ezendam, Simone
author_facet Ezendam, Simone
Nan, Lin
Violi, Ianina Lucila
Maier, Stefan A.
Cortés, Emiliano
Baffou, Guillaume
Gargiulo, Julian
author_role author
author2 Nan, Lin
Violi, Ianina Lucila
Maier, Stefan A.
Cortés, Emiliano
Baffou, Guillaume
Gargiulo, Julian
author2_role author
author
author
author
author
author
dc.subject.none.fl_str_mv ANTI STOKES PHOTOLUMINESCENCE
NANOTHERMOMETRY
PHOTOTHERMAL EFFECT
THERMOPLASMONICS
topic ANTI STOKES PHOTOLUMINESCENCE
NANOTHERMOMETRY
PHOTOTHERMAL EFFECT
THERMOPLASMONICS
purl_subject.fl_str_mv https://purl.org/becyt/ford/2.10
https://purl.org/becyt/ford/2
dc.description.none.fl_txt_mv Metallic nanoparticles possess strong photothermal responses, especially when illuminated as ensembles due to collective effects. However, accurately quantifying the temperature increase remains a significant challenge, impeding progress in several applications. Anti Stokes thermometry offers a promising solution by enabling direct and non-invasive temperature measurements of the metal without the need for labeling or prior calibration. While Anti Stokes thermometry is successfully applied to individual nanoparticles, its potential to study light-to-heat conversion with plasmonic ensembles remains unexplored. In this study, the theoretical framework and the conditions that must be fulfilled for applying Anti Stokes thermometry to ensembles of nanoparticles are discussed. Then, this technique is implemented to measure the light-induced heating of square arrays of Au nanodisks. The obtained temperature measurements are validated using wavefront microscopy, demonstrating excellent agreement between the two thermometry methods. These results showcase the extension of Anti Stokes thermometry to plasmonic ensembles, highlighting its potential for implementation in the diverse photothermal applications involving these systems.
Fil: Ezendam, Simone. Ludwig Maximilians Universitat; Alemania
Fil: Nan, Lin. Ludwig Maximilians Universitat; Alemania
Fil: Violi, Ianina Lucila. Universidad Nacional de San Martin. Instituto de Nanosistemas; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Maier, Stefan A.. Imperial College London; Reino Unido. Monash University; Australia. Ludwig Maximilians Universitat; Alemania
Fil: Cortés, Emiliano. Ludwig Maximilians Universitat; Alemania. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Baffou, Guillaume. Centre National de la Recherche Scientifique; Francia
Fil: Gargiulo, Julian. Ludwig Maximilians Universitat; Alemania. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
description Metallic nanoparticles possess strong photothermal responses, especially when illuminated as ensembles due to collective effects. However, accurately quantifying the temperature increase remains a significant challenge, impeding progress in several applications. Anti Stokes thermometry offers a promising solution by enabling direct and non-invasive temperature measurements of the metal without the need for labeling or prior calibration. While Anti Stokes thermometry is successfully applied to individual nanoparticles, its potential to study light-to-heat conversion with plasmonic ensembles remains unexplored. In this study, the theoretical framework and the conditions that must be fulfilled for applying Anti Stokes thermometry to ensembles of nanoparticles are discussed. Then, this technique is implemented to measure the light-induced heating of square arrays of Au nanodisks. The obtained temperature measurements are validated using wavefront microscopy, demonstrating excellent agreement between the two thermometry methods. These results showcase the extension of Anti Stokes thermometry to plasmonic ensembles, highlighting its potential for implementation in the diverse photothermal applications involving these systems.
publishDate 2023
dc.date.none.fl_str_mv 2023-09
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/220002
Ezendam, Simone; Nan, Lin; Violi, Ianina Lucila; Maier, Stefan A.; Cortés, Emiliano; et al.; Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays; Wiley; Advanced Optical Materials; 9-2023; 1-8
2195-1071
CONICET Digital
CONICET
url http://hdl.handle.net/11336/220002
identifier_str_mv Ezendam, Simone; Nan, Lin; Violi, Ianina Lucila; Maier, Stefan A.; Cortés, Emiliano; et al.; Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays; Wiley; Advanced Optical Materials; 9-2023; 1-8
2195-1071
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://onlinelibrary.wiley.com/doi/10.1002/adom.202301496
info:eu-repo/semantics/altIdentifier/doi/10.1002/adom.202301496
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
application/pdf
dc.publisher.none.fl_str_mv Wiley
publisher.none.fl_str_mv Wiley
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 12.982451

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