Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays
- Autores
- Ezendam, Simone; Nan, Lin; Violi, Ianina Lucila; Maier, Stefan A.; Cortés, Emiliano; Baffou, Guillaume; Gargiulo, Julian
- Año de publicación
- 2023
- Idioma
- inglés
- Tipo de recurso
- artículo
- Estado
- versión publicada
- Descripción
- Metallic nanoparticles possess strong photothermal responses, especially when illuminated as ensembles due to collective effects. However, accurately quantifying the temperature increase remains a significant challenge, impeding progress in several applications. Anti Stokes thermometry offers a promising solution by enabling direct and non-invasive temperature measurements of the metal without the need for labeling or prior calibration. While Anti Stokes thermometry is successfully applied to individual nanoparticles, its potential to study light-to-heat conversion with plasmonic ensembles remains unexplored. In this study, the theoretical framework and the conditions that must be fulfilled for applying Anti Stokes thermometry to ensembles of nanoparticles are discussed. Then, this technique is implemented to measure the light-induced heating of square arrays of Au nanodisks. The obtained temperature measurements are validated using wavefront microscopy, demonstrating excellent agreement between the two thermometry methods. These results showcase the extension of Anti Stokes thermometry to plasmonic ensembles, highlighting its potential for implementation in the diverse photothermal applications involving these systems.
Fil: Ezendam, Simone. Ludwig Maximilians Universitat; Alemania
Fil: Nan, Lin. Ludwig Maximilians Universitat; Alemania
Fil: Violi, Ianina Lucila. Universidad Nacional de San Martin. Instituto de Nanosistemas; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Maier, Stefan A.. Imperial College London; Reino Unido. Monash University; Australia. Ludwig Maximilians Universitat; Alemania
Fil: Cortés, Emiliano. Ludwig Maximilians Universitat; Alemania. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Baffou, Guillaume. Centre National de la Recherche Scientifique; Francia
Fil: Gargiulo, Julian. Ludwig Maximilians Universitat; Alemania. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina - Materia
-
ANTI STOKES PHOTOLUMINESCENCE
NANOTHERMOMETRY
PHOTOTHERMAL EFFECT
THERMOPLASMONICS - Nivel de accesibilidad
- acceso abierto
- Condiciones de uso
- https://creativecommons.org/licenses/by/2.5/ar/
- Repositorio
- Institución
- Consejo Nacional de Investigaciones Científicas y Técnicas
- OAI Identificador
- oai:ri.conicet.gov.ar:11336/220002
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Anti Stokes Thermometry of Plasmonic Nanoparticle ArraysEzendam, SimoneNan, LinVioli, Ianina LucilaMaier, Stefan A.Cortés, EmilianoBaffou, GuillaumeGargiulo, JulianANTI STOKES PHOTOLUMINESCENCENANOTHERMOMETRYPHOTOTHERMAL EFFECTTHERMOPLASMONICShttps://purl.org/becyt/ford/2.10https://purl.org/becyt/ford/2Metallic nanoparticles possess strong photothermal responses, especially when illuminated as ensembles due to collective effects. However, accurately quantifying the temperature increase remains a significant challenge, impeding progress in several applications. Anti Stokes thermometry offers a promising solution by enabling direct and non-invasive temperature measurements of the metal without the need for labeling or prior calibration. While Anti Stokes thermometry is successfully applied to individual nanoparticles, its potential to study light-to-heat conversion with plasmonic ensembles remains unexplored. In this study, the theoretical framework and the conditions that must be fulfilled for applying Anti Stokes thermometry to ensembles of nanoparticles are discussed. Then, this technique is implemented to measure the light-induced heating of square arrays of Au nanodisks. The obtained temperature measurements are validated using wavefront microscopy, demonstrating excellent agreement between the two thermometry methods. These results showcase the extension of Anti Stokes thermometry to plasmonic ensembles, highlighting its potential for implementation in the diverse photothermal applications involving these systems.Fil: Ezendam, Simone. Ludwig Maximilians Universitat; AlemaniaFil: Nan, Lin. Ludwig Maximilians Universitat; AlemaniaFil: Violi, Ianina Lucila. Universidad Nacional de San Martin. Instituto de Nanosistemas; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaFil: Maier, Stefan A.. Imperial College London; Reino Unido. Monash University; Australia. Ludwig Maximilians Universitat; AlemaniaFil: Cortés, Emiliano. Ludwig Maximilians Universitat; Alemania. Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaFil: Baffou, Guillaume. Centre National de la Recherche Scientifique; FranciaFil: Gargiulo, Julian. Ludwig Maximilians Universitat; Alemania. Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaWiley2023-09info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/220002Ezendam, Simone; Nan, Lin; Violi, Ianina Lucila; Maier, Stefan A.; Cortés, Emiliano; et al.; Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays; Wiley; Advanced Optical Materials; 9-2023; 1-82195-1071CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://onlinelibrary.wiley.com/doi/10.1002/adom.202301496info:eu-repo/semantics/altIdentifier/doi/10.1002/adom.202301496info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T10:37:42Zoai:ri.conicet.gov.ar:11336/220002instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 10:37:42.878CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse |
dc.title.none.fl_str_mv |
Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays |
title |
Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays |
spellingShingle |
Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays Ezendam, Simone ANTI STOKES PHOTOLUMINESCENCE NANOTHERMOMETRY PHOTOTHERMAL EFFECT THERMOPLASMONICS |
title_short |
Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays |
title_full |
Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays |
title_fullStr |
Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays |
title_full_unstemmed |
Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays |
title_sort |
Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays |
dc.creator.none.fl_str_mv |
Ezendam, Simone Nan, Lin Violi, Ianina Lucila Maier, Stefan A. Cortés, Emiliano Baffou, Guillaume Gargiulo, Julian |
author |
Ezendam, Simone |
author_facet |
Ezendam, Simone Nan, Lin Violi, Ianina Lucila Maier, Stefan A. Cortés, Emiliano Baffou, Guillaume Gargiulo, Julian |
author_role |
author |
author2 |
Nan, Lin Violi, Ianina Lucila Maier, Stefan A. Cortés, Emiliano Baffou, Guillaume Gargiulo, Julian |
author2_role |
author author author author author author |
dc.subject.none.fl_str_mv |
ANTI STOKES PHOTOLUMINESCENCE NANOTHERMOMETRY PHOTOTHERMAL EFFECT THERMOPLASMONICS |
topic |
ANTI STOKES PHOTOLUMINESCENCE NANOTHERMOMETRY PHOTOTHERMAL EFFECT THERMOPLASMONICS |
purl_subject.fl_str_mv |
https://purl.org/becyt/ford/2.10 https://purl.org/becyt/ford/2 |
dc.description.none.fl_txt_mv |
Metallic nanoparticles possess strong photothermal responses, especially when illuminated as ensembles due to collective effects. However, accurately quantifying the temperature increase remains a significant challenge, impeding progress in several applications. Anti Stokes thermometry offers a promising solution by enabling direct and non-invasive temperature measurements of the metal without the need for labeling or prior calibration. While Anti Stokes thermometry is successfully applied to individual nanoparticles, its potential to study light-to-heat conversion with plasmonic ensembles remains unexplored. In this study, the theoretical framework and the conditions that must be fulfilled for applying Anti Stokes thermometry to ensembles of nanoparticles are discussed. Then, this technique is implemented to measure the light-induced heating of square arrays of Au nanodisks. The obtained temperature measurements are validated using wavefront microscopy, demonstrating excellent agreement between the two thermometry methods. These results showcase the extension of Anti Stokes thermometry to plasmonic ensembles, highlighting its potential for implementation in the diverse photothermal applications involving these systems. Fil: Ezendam, Simone. Ludwig Maximilians Universitat; Alemania Fil: Nan, Lin. Ludwig Maximilians Universitat; Alemania Fil: Violi, Ianina Lucila. Universidad Nacional de San Martin. Instituto de Nanosistemas; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina Fil: Maier, Stefan A.. Imperial College London; Reino Unido. Monash University; Australia. Ludwig Maximilians Universitat; Alemania Fil: Cortés, Emiliano. Ludwig Maximilians Universitat; Alemania. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina Fil: Baffou, Guillaume. Centre National de la Recherche Scientifique; Francia Fil: Gargiulo, Julian. Ludwig Maximilians Universitat; Alemania. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina |
description |
Metallic nanoparticles possess strong photothermal responses, especially when illuminated as ensembles due to collective effects. However, accurately quantifying the temperature increase remains a significant challenge, impeding progress in several applications. Anti Stokes thermometry offers a promising solution by enabling direct and non-invasive temperature measurements of the metal without the need for labeling or prior calibration. While Anti Stokes thermometry is successfully applied to individual nanoparticles, its potential to study light-to-heat conversion with plasmonic ensembles remains unexplored. In this study, the theoretical framework and the conditions that must be fulfilled for applying Anti Stokes thermometry to ensembles of nanoparticles are discussed. Then, this technique is implemented to measure the light-induced heating of square arrays of Au nanodisks. The obtained temperature measurements are validated using wavefront microscopy, demonstrating excellent agreement between the two thermometry methods. These results showcase the extension of Anti Stokes thermometry to plasmonic ensembles, highlighting its potential for implementation in the diverse photothermal applications involving these systems. |
publishDate |
2023 |
dc.date.none.fl_str_mv |
2023-09 |
dc.type.none.fl_str_mv |
info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion http://purl.org/coar/resource_type/c_6501 info:ar-repo/semantics/articulo |
format |
article |
status_str |
publishedVersion |
dc.identifier.none.fl_str_mv |
http://hdl.handle.net/11336/220002 Ezendam, Simone; Nan, Lin; Violi, Ianina Lucila; Maier, Stefan A.; Cortés, Emiliano; et al.; Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays; Wiley; Advanced Optical Materials; 9-2023; 1-8 2195-1071 CONICET Digital CONICET |
url |
http://hdl.handle.net/11336/220002 |
identifier_str_mv |
Ezendam, Simone; Nan, Lin; Violi, Ianina Lucila; Maier, Stefan A.; Cortés, Emiliano; et al.; Anti Stokes Thermometry of Plasmonic Nanoparticle Arrays; Wiley; Advanced Optical Materials; 9-2023; 1-8 2195-1071 CONICET Digital CONICET |
dc.language.none.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
info:eu-repo/semantics/altIdentifier/url/https://onlinelibrary.wiley.com/doi/10.1002/adom.202301496 info:eu-repo/semantics/altIdentifier/doi/10.1002/adom.202301496 |
dc.rights.none.fl_str_mv |
info:eu-repo/semantics/openAccess https://creativecommons.org/licenses/by/2.5/ar/ |
eu_rights_str_mv |
openAccess |
rights_invalid_str_mv |
https://creativecommons.org/licenses/by/2.5/ar/ |
dc.format.none.fl_str_mv |
application/pdf application/pdf application/pdf |
dc.publisher.none.fl_str_mv |
Wiley |
publisher.none.fl_str_mv |
Wiley |
dc.source.none.fl_str_mv |
reponame:CONICET Digital (CONICET) instname:Consejo Nacional de Investigaciones Científicas y Técnicas |
reponame_str |
CONICET Digital (CONICET) |
collection |
CONICET Digital (CONICET) |
instname_str |
Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.name.fl_str_mv |
CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.mail.fl_str_mv |
dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar |
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1844614397899571200 |
score |
13.070432 |