Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots
- Autores
- Alonso González, P.; Albella, P.; Schnell, M.; Chen, J.; Huth, F.; García Etxarri, A.; Casanova, F.; Golmar, Federico; Arzubiaga, L.; Hueso, L. E.; Aizpurua, J.; Hillenbrand, R.
- Año de publicación
- 2012
- Idioma
- inglés
- Tipo de recurso
- artículo
- Estado
- versión publicada
- Descripción
- Light scattering at nanoparticles and molecules can be dramatically enhanced in the 'hot spots' of optical antennas, where the incident light is highly concentrated. Although this effect is widely applied in surface-enhanced optical sensing, spectroscopy and microscopy, the underlying electromagnetic mechanism of the signal enhancement is challenging to trace experimentally. Here we study elastically scattered light from an individual object located in the well-defined hot spot of single antennas, as a new approach to resolve the role of the antenna in the scattering process. We provide experimental evidence that the intensity elastically scattered off the object scales with the fourth power of the local field enhancement provided by the antenna, and that the underlying electromagnetic mechanism is identical to the one commonly accepted in surface-enhanced Raman scattering. We also measure the phase shift of the scattered light, which provides a novel and unambiguous fingerprint of surface-enhanced light scattering.
Fil: Alonso González, P.. No especifíca;
Fil: Albella, P.. No especifíca;
Fil: Schnell, M.. No especifíca;
Fil: Chen, J.. No especifíca;
Fil: Huth, F.. No especifíca;
Fil: García Etxarri, A.. No especifíca;
Fil: Casanova, F.. No especifíca;
Fil: Golmar, Federico. Instituto Nacional de Tecnología Industrial; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Arzubiaga, L.. No especifíca;
Fil: Hueso, L. E.. No especifíca;
Fil: Aizpurua, J.. No especifíca;
Fil: Hillenbrand, R.. No especifíca; - Materia
- Light scattering
- Nivel de accesibilidad
- acceso abierto
- Condiciones de uso
- https://creativecommons.org/licenses/by/2.5/ar/
- Repositorio
- Institución
- Consejo Nacional de Investigaciones Científicas y Técnicas
- OAI Identificador
- oai:ri.conicet.gov.ar:11336/194670
Ver los metadatos del registro completo
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spelling |
Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spotsAlonso González, P.Albella, P.Schnell, M.Chen, J.Huth, F.García Etxarri, A.Casanova, F.Golmar, FedericoArzubiaga, L.Hueso, L. E.Aizpurua, J.Hillenbrand, R.Light scatteringhttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1Light scattering at nanoparticles and molecules can be dramatically enhanced in the 'hot spots' of optical antennas, where the incident light is highly concentrated. Although this effect is widely applied in surface-enhanced optical sensing, spectroscopy and microscopy, the underlying electromagnetic mechanism of the signal enhancement is challenging to trace experimentally. Here we study elastically scattered light from an individual object located in the well-defined hot spot of single antennas, as a new approach to resolve the role of the antenna in the scattering process. We provide experimental evidence that the intensity elastically scattered off the object scales with the fourth power of the local field enhancement provided by the antenna, and that the underlying electromagnetic mechanism is identical to the one commonly accepted in surface-enhanced Raman scattering. We also measure the phase shift of the scattered light, which provides a novel and unambiguous fingerprint of surface-enhanced light scattering.Fil: Alonso González, P.. No especifíca;Fil: Albella, P.. No especifíca;Fil: Schnell, M.. No especifíca;Fil: Chen, J.. No especifíca;Fil: Huth, F.. No especifíca;Fil: García Etxarri, A.. No especifíca;Fil: Casanova, F.. No especifíca;Fil: Golmar, Federico. Instituto Nacional de Tecnología Industrial; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaFil: Arzubiaga, L.. No especifíca;Fil: Hueso, L. E.. No especifíca;Fil: Aizpurua, J.. No especifíca;Fil: Hillenbrand, R.. No especifíca;Nature Publishing Group2012-02info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/194670Alonso González, P.; Albella, P.; Schnell, M.; Chen, J.; Huth, F.; et al.; Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots; Nature Publishing Group; Nature Communications; 3; 2-2012; 1-72041-1723CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/http://www.nature.com/ncomms/journal/v3/n2/full/ncomms1674.htmlinfo:eu-repo/semantics/altIdentifier/doi/10.1038/ncomms1674info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T10:18:04Zoai:ri.conicet.gov.ar:11336/194670instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 10:18:04.984CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse |
dc.title.none.fl_str_mv |
Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots |
title |
Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots |
spellingShingle |
Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots Alonso González, P. Light scattering |
title_short |
Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots |
title_full |
Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots |
title_fullStr |
Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots |
title_full_unstemmed |
Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots |
title_sort |
Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots |
dc.creator.none.fl_str_mv |
Alonso González, P. Albella, P. Schnell, M. Chen, J. Huth, F. García Etxarri, A. Casanova, F. Golmar, Federico Arzubiaga, L. Hueso, L. E. Aizpurua, J. Hillenbrand, R. |
author |
Alonso González, P. |
author_facet |
Alonso González, P. Albella, P. Schnell, M. Chen, J. Huth, F. García Etxarri, A. Casanova, F. Golmar, Federico Arzubiaga, L. Hueso, L. E. Aizpurua, J. Hillenbrand, R. |
author_role |
author |
author2 |
Albella, P. Schnell, M. Chen, J. Huth, F. García Etxarri, A. Casanova, F. Golmar, Federico Arzubiaga, L. Hueso, L. E. Aizpurua, J. Hillenbrand, R. |
author2_role |
author author author author author author author author author author author |
dc.subject.none.fl_str_mv |
Light scattering |
topic |
Light scattering |
purl_subject.fl_str_mv |
https://purl.org/becyt/ford/1.3 https://purl.org/becyt/ford/1 |
dc.description.none.fl_txt_mv |
Light scattering at nanoparticles and molecules can be dramatically enhanced in the 'hot spots' of optical antennas, where the incident light is highly concentrated. Although this effect is widely applied in surface-enhanced optical sensing, spectroscopy and microscopy, the underlying electromagnetic mechanism of the signal enhancement is challenging to trace experimentally. Here we study elastically scattered light from an individual object located in the well-defined hot spot of single antennas, as a new approach to resolve the role of the antenna in the scattering process. We provide experimental evidence that the intensity elastically scattered off the object scales with the fourth power of the local field enhancement provided by the antenna, and that the underlying electromagnetic mechanism is identical to the one commonly accepted in surface-enhanced Raman scattering. We also measure the phase shift of the scattered light, which provides a novel and unambiguous fingerprint of surface-enhanced light scattering. Fil: Alonso González, P.. No especifíca; Fil: Albella, P.. No especifíca; Fil: Schnell, M.. No especifíca; Fil: Chen, J.. No especifíca; Fil: Huth, F.. No especifíca; Fil: García Etxarri, A.. No especifíca; Fil: Casanova, F.. No especifíca; Fil: Golmar, Federico. Instituto Nacional de Tecnología Industrial; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina Fil: Arzubiaga, L.. No especifíca; Fil: Hueso, L. E.. No especifíca; Fil: Aizpurua, J.. No especifíca; Fil: Hillenbrand, R.. No especifíca; |
description |
Light scattering at nanoparticles and molecules can be dramatically enhanced in the 'hot spots' of optical antennas, where the incident light is highly concentrated. Although this effect is widely applied in surface-enhanced optical sensing, spectroscopy and microscopy, the underlying electromagnetic mechanism of the signal enhancement is challenging to trace experimentally. Here we study elastically scattered light from an individual object located in the well-defined hot spot of single antennas, as a new approach to resolve the role of the antenna in the scattering process. We provide experimental evidence that the intensity elastically scattered off the object scales with the fourth power of the local field enhancement provided by the antenna, and that the underlying electromagnetic mechanism is identical to the one commonly accepted in surface-enhanced Raman scattering. We also measure the phase shift of the scattered light, which provides a novel and unambiguous fingerprint of surface-enhanced light scattering. |
publishDate |
2012 |
dc.date.none.fl_str_mv |
2012-02 |
dc.type.none.fl_str_mv |
info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion http://purl.org/coar/resource_type/c_6501 info:ar-repo/semantics/articulo |
format |
article |
status_str |
publishedVersion |
dc.identifier.none.fl_str_mv |
http://hdl.handle.net/11336/194670 Alonso González, P.; Albella, P.; Schnell, M.; Chen, J.; Huth, F.; et al.; Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots; Nature Publishing Group; Nature Communications; 3; 2-2012; 1-7 2041-1723 CONICET Digital CONICET |
url |
http://hdl.handle.net/11336/194670 |
identifier_str_mv |
Alonso González, P.; Albella, P.; Schnell, M.; Chen, J.; Huth, F.; et al.; Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots; Nature Publishing Group; Nature Communications; 3; 2-2012; 1-7 2041-1723 CONICET Digital CONICET |
dc.language.none.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
info:eu-repo/semantics/altIdentifier/url/http://www.nature.com/ncomms/journal/v3/n2/full/ncomms1674.html info:eu-repo/semantics/altIdentifier/doi/10.1038/ncomms1674 |
dc.rights.none.fl_str_mv |
info:eu-repo/semantics/openAccess https://creativecommons.org/licenses/by/2.5/ar/ |
eu_rights_str_mv |
openAccess |
rights_invalid_str_mv |
https://creativecommons.org/licenses/by/2.5/ar/ |
dc.format.none.fl_str_mv |
application/pdf application/pdf |
dc.publisher.none.fl_str_mv |
Nature Publishing Group |
publisher.none.fl_str_mv |
Nature Publishing Group |
dc.source.none.fl_str_mv |
reponame:CONICET Digital (CONICET) instname:Consejo Nacional de Investigaciones Científicas y Técnicas |
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CONICET Digital (CONICET) |
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CONICET Digital (CONICET) |
instname_str |
Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.name.fl_str_mv |
CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.mail.fl_str_mv |
dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar |
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1844614138972602368 |
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13.070432 |