Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots

Autores
Alonso González, P.; Albella, P.; Schnell, M.; Chen, J.; Huth, F.; García Etxarri, A.; Casanova, F.; Golmar, Federico; Arzubiaga, L.; Hueso, L. E.; Aizpurua, J.; Hillenbrand, R.
Año de publicación
2012
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
Light scattering at nanoparticles and molecules can be dramatically enhanced in the 'hot spots' of optical antennas, where the incident light is highly concentrated. Although this effect is widely applied in surface-enhanced optical sensing, spectroscopy and microscopy, the underlying electromagnetic mechanism of the signal enhancement is challenging to trace experimentally. Here we study elastically scattered light from an individual object located in the well-defined hot spot of single antennas, as a new approach to resolve the role of the antenna in the scattering process. We provide experimental evidence that the intensity elastically scattered off the object scales with the fourth power of the local field enhancement provided by the antenna, and that the underlying electromagnetic mechanism is identical to the one commonly accepted in surface-enhanced Raman scattering. We also measure the phase shift of the scattered light, which provides a novel and unambiguous fingerprint of surface-enhanced light scattering.
Fil: Alonso González, P.. No especifíca;
Fil: Albella, P.. No especifíca;
Fil: Schnell, M.. No especifíca;
Fil: Chen, J.. No especifíca;
Fil: Huth, F.. No especifíca;
Fil: García Etxarri, A.. No especifíca;
Fil: Casanova, F.. No especifíca;
Fil: Golmar, Federico. Instituto Nacional de Tecnología Industrial; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Arzubiaga, L.. No especifíca;
Fil: Hueso, L. E.. No especifíca;
Fil: Aizpurua, J.. No especifíca;
Fil: Hillenbrand, R.. No especifíca;
Materia
Light scattering
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/194670
Acceder
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oai_identifier_str oai:ri.conicet.gov.ar:11336/194670
network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spotsAlonso González, P.Albella, P.Schnell, M.Chen, J.Huth, F.García Etxarri, A.Casanova, F.Golmar, FedericoArzubiaga, L.Hueso, L. E.Aizpurua, J.Hillenbrand, R.Light scatteringhttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1Light scattering at nanoparticles and molecules can be dramatically enhanced in the 'hot spots' of optical antennas, where the incident light is highly concentrated. Although this effect is widely applied in surface-enhanced optical sensing, spectroscopy and microscopy, the underlying electromagnetic mechanism of the signal enhancement is challenging to trace experimentally. Here we study elastically scattered light from an individual object located in the well-defined hot spot of single antennas, as a new approach to resolve the role of the antenna in the scattering process. We provide experimental evidence that the intensity elastically scattered off the object scales with the fourth power of the local field enhancement provided by the antenna, and that the underlying electromagnetic mechanism is identical to the one commonly accepted in surface-enhanced Raman scattering. We also measure the phase shift of the scattered light, which provides a novel and unambiguous fingerprint of surface-enhanced light scattering.Fil: Alonso González, P.. No especifíca;Fil: Albella, P.. No especifíca;Fil: Schnell, M.. No especifíca;Fil: Chen, J.. No especifíca;Fil: Huth, F.. No especifíca;Fil: García Etxarri, A.. No especifíca;Fil: Casanova, F.. No especifíca;Fil: Golmar, Federico. Instituto Nacional de Tecnología Industrial; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaFil: Arzubiaga, L.. No especifíca;Fil: Hueso, L. E.. No especifíca;Fil: Aizpurua, J.. No especifíca;Fil: Hillenbrand, R.. No especifíca;Nature Publishing Group2012-02info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/194670Alonso González, P.; Albella, P.; Schnell, M.; Chen, J.; Huth, F.; et al.; Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots; Nature Publishing Group; Nature Communications; 3; 2-2012; 1-72041-1723CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/http://www.nature.com/ncomms/journal/v3/n2/full/ncomms1674.htmlinfo:eu-repo/semantics/altIdentifier/doi/10.1038/ncomms1674info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-10-15T15:15:16Zoai:ri.conicet.gov.ar:11336/194670instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-10-15 15:15:17.185CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots
title Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots
spellingShingle Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots
Alonso González, P.
Light scattering
title_short Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots
title_full Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots
title_fullStr Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots
title_full_unstemmed Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots
title_sort Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots
dc.creator.none.fl_str_mv Alonso González, P.
Albella, P.
Schnell, M.
Chen, J.
Huth, F.
García Etxarri, A.
Casanova, F.
Golmar, Federico
Arzubiaga, L.
Hueso, L. E.
Aizpurua, J.
Hillenbrand, R.
author Alonso González, P.
author_facet Alonso González, P.
Albella, P.
Schnell, M.
Chen, J.
Huth, F.
García Etxarri, A.
Casanova, F.
Golmar, Federico
Arzubiaga, L.
Hueso, L. E.
Aizpurua, J.
Hillenbrand, R.
author_role author
author2 Albella, P.
Schnell, M.
Chen, J.
Huth, F.
García Etxarri, A.
Casanova, F.
Golmar, Federico
Arzubiaga, L.
Hueso, L. E.
Aizpurua, J.
Hillenbrand, R.
author2_role author
author
author
author
author
author
author
author
author
author
author
dc.subject.none.fl_str_mv Light scattering
topic Light scattering
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv Light scattering at nanoparticles and molecules can be dramatically enhanced in the 'hot spots' of optical antennas, where the incident light is highly concentrated. Although this effect is widely applied in surface-enhanced optical sensing, spectroscopy and microscopy, the underlying electromagnetic mechanism of the signal enhancement is challenging to trace experimentally. Here we study elastically scattered light from an individual object located in the well-defined hot spot of single antennas, as a new approach to resolve the role of the antenna in the scattering process. We provide experimental evidence that the intensity elastically scattered off the object scales with the fourth power of the local field enhancement provided by the antenna, and that the underlying electromagnetic mechanism is identical to the one commonly accepted in surface-enhanced Raman scattering. We also measure the phase shift of the scattered light, which provides a novel and unambiguous fingerprint of surface-enhanced light scattering.
Fil: Alonso González, P.. No especifíca;
Fil: Albella, P.. No especifíca;
Fil: Schnell, M.. No especifíca;
Fil: Chen, J.. No especifíca;
Fil: Huth, F.. No especifíca;
Fil: García Etxarri, A.. No especifíca;
Fil: Casanova, F.. No especifíca;
Fil: Golmar, Federico. Instituto Nacional de Tecnología Industrial; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Arzubiaga, L.. No especifíca;
Fil: Hueso, L. E.. No especifíca;
Fil: Aizpurua, J.. No especifíca;
Fil: Hillenbrand, R.. No especifíca;
description Light scattering at nanoparticles and molecules can be dramatically enhanced in the 'hot spots' of optical antennas, where the incident light is highly concentrated. Although this effect is widely applied in surface-enhanced optical sensing, spectroscopy and microscopy, the underlying electromagnetic mechanism of the signal enhancement is challenging to trace experimentally. Here we study elastically scattered light from an individual object located in the well-defined hot spot of single antennas, as a new approach to resolve the role of the antenna in the scattering process. We provide experimental evidence that the intensity elastically scattered off the object scales with the fourth power of the local field enhancement provided by the antenna, and that the underlying electromagnetic mechanism is identical to the one commonly accepted in surface-enhanced Raman scattering. We also measure the phase shift of the scattered light, which provides a novel and unambiguous fingerprint of surface-enhanced light scattering.
publishDate 2012
dc.date.none.fl_str_mv 2012-02
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/194670
Alonso González, P.; Albella, P.; Schnell, M.; Chen, J.; Huth, F.; et al.; Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots; Nature Publishing Group; Nature Communications; 3; 2-2012; 1-7
2041-1723
CONICET Digital
CONICET
url http://hdl.handle.net/11336/194670
identifier_str_mv Alonso González, P.; Albella, P.; Schnell, M.; Chen, J.; Huth, F.; et al.; Resolving the electromagnetic mechanism of surface-enhanced light scattering at single hot spots; Nature Publishing Group; Nature Communications; 3; 2-2012; 1-7
2041-1723
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/http://www.nature.com/ncomms/journal/v3/n2/full/ncomms1674.html
info:eu-repo/semantics/altIdentifier/doi/10.1038/ncomms1674
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv Nature Publishing Group
publisher.none.fl_str_mv Nature Publishing Group
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
_version_ 1846083300623384576
score 13.22299

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