Evaluation of CAM-CHEM VSL model performance during Southtrac campaign

Autores
Berná Peña, Lucas Luciano; Lopez Noreña, Ana Isabel; Puliafito, Salvador Enrique; Barreras, Javier Marcelo; Engel, Andreas; Jesswein, Markus; Cuevas, Carlos A.; Saiz Lopez, Alfonso; Fernandez, Rafael Pedro
Año de publicación
2021
Idioma
inglés
Tipo de recurso
documento de conferencia
Estado
versión publicada
Descripción
In the framework of the SouthTRAC Campaign (Transport and Composition of the Southern Hemisphere Upper Troposphere and Lower Stratosphere) based on Rio Grande, Argentina, a local research group from CONICET (Argentine National Research Council) joined the German consortium maintaining the HALO research aircraft (High-Altitude and LOng-range aircraft) to help with the flight planning and evaluation of the chemical composition of the upper troposphere and lower stratosphere within the ozone hole periphery. The SouthTRAC aircraft campaign was carried out in two phases which took place in September and November 2019, respectively. With the purpose of providing additional information of the atmospheric composition of brominated Very Short-Lived (VSLBr) species and compare with HALO observations during the transfer and campaign flights, a CAM-Chem (Community Atmosphere Model with Chemistry) global chemistry-climate simulation was conducted. The model setup used in the halogenated CAM-Chem simulation had a 1° x 1.25° lat-lon resolution, 56 hybrid vertical levels from the surface to the middle stratosphere and considered assimilated meteorology from MERRA, including an explicit treatment of VSLBr sources and chemistry. Model output of VSLBr, long-lived bromine and chlorine (LLBr and LLCl) species and ozone mixing ratios, as well as the main inorganic halogen reactive and reservoir species and gas/heterogeneous phase reaction rates affecting lowermost stratospheric ozone were analyzed in horizontal domains and vertical cross-sections across each flightpath. The model performance with respect to the HALO observations has a general good agreement, presenting better results for mid latitudes (between 30º S and 50º S) than for southern latitudes (>50º S). In particular, CAM-Chem timeseries consistently reproduced the spatio-temporal variation of the main VSLBr species (CH2Br2 and CHBr3), including the sharp variations observed across the tropopause. For both VSLBr as well as for LLCl compounds such as CFC-12, the Pearson correlation coefficient r obtained during each of the flights ranged between 0.7 and 0.9, while the Normalized Mean Bias (NMB) was smaller than 8% for almost every flight. Regarding LLBr CH3Br, the correlation with the aircraft observations is high (r>0.9) but the inter-hemispheric variability during transfer flights is not fully captured. For Ozone, the model presents mid to high correlation with respect to measures (0.5
Fil: Berná Peña, Lucas Luciano. Universidad Tecnológica Nacional. Facultad Regional de Mendoza; Argentina
Fil: Lopez Noreña, Ana Isabel. Universidad Tecnológica Nacional. Facultad Regional de Mendoza; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Mendoza; Argentina
Fil: Puliafito, Salvador Enrique. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Mendoza; Argentina. Universidad Tecnológica Nacional. Facultad Regional de Mendoza; Argentina
Fil: Barreras, Javier Marcelo. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Engel, Andreas. Goethe Universitat Frankfurt; Alemania
Fil: Jesswein, Markus. Goethe Universitat Frankfurt; Alemania
Fil: Cuevas, Carlos A.. Consejo Superior de Investigaciones Científicas. Instituto de Química Física; España
Fil: Saiz Lopez, Alfonso. Consejo Superior de Investigaciones Científicas. Instituto de Química Física; España
Fil: Fernandez, Rafael Pedro. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Mendoza. Instituto Interdisciplinario de Ciencias Básicas. - Universidad Nacional de Cuyo. Instituto Interdisciplinario de Ciencias Básicas; Argentina
EGU General Assembly 2021
Austria
European Geosciences Union
Materia
VERY SHORT LIVED POLLUTANT
MODEL
CAM-CHEM
SOUTHTRAC
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/175563
Acceder
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oai_identifier_str oai:ri.conicet.gov.ar:11336/175563
network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Evaluation of CAM-CHEM VSL model performance during Southtrac campaignBerná Peña, Lucas LucianoLopez Noreña, Ana IsabelPuliafito, Salvador EnriqueBarreras, Javier MarceloEngel, AndreasJesswein, MarkusCuevas, Carlos A.Saiz Lopez, AlfonsoFernandez, Rafael PedroVERY SHORT LIVED POLLUTANTMODELCAM-CHEMSOUTHTRAChttps://purl.org/becyt/ford/1.5https://purl.org/becyt/ford/1In the framework of the SouthTRAC Campaign (Transport and Composition of the Southern Hemisphere Upper Troposphere and Lower Stratosphere) based on Rio Grande, Argentina, a local research group from CONICET (Argentine National Research Council) joined the German consortium maintaining the HALO research aircraft (High-Altitude and LOng-range aircraft) to help with the flight planning and evaluation of the chemical composition of the upper troposphere and lower stratosphere within the ozone hole periphery. The SouthTRAC aircraft campaign was carried out in two phases which took place in September and November 2019, respectively. With the purpose of providing additional information of the atmospheric composition of brominated Very Short-Lived (VSLBr) species and compare with HALO observations during the transfer and campaign flights, a CAM-Chem (Community Atmosphere Model with Chemistry) global chemistry-climate simulation was conducted. The model setup used in the halogenated CAM-Chem simulation had a 1° x 1.25° lat-lon resolution, 56 hybrid vertical levels from the surface to the middle stratosphere and considered assimilated meteorology from MERRA, including an explicit treatment of VSLBr sources and chemistry. Model output of VSLBr, long-lived bromine and chlorine (LLBr and LLCl) species and ozone mixing ratios, as well as the main inorganic halogen reactive and reservoir species and gas/heterogeneous phase reaction rates affecting lowermost stratospheric ozone were analyzed in horizontal domains and vertical cross-sections across each flightpath. The model performance with respect to the HALO observations has a general good agreement, presenting better results for mid latitudes (between 30º S and 50º S) than for southern latitudes (>50º S). In particular, CAM-Chem timeseries consistently reproduced the spatio-temporal variation of the main VSLBr species (CH2Br2 and CHBr3), including the sharp variations observed across the tropopause. For both VSLBr as well as for LLCl compounds such as CFC-12, the Pearson correlation coefficient r obtained during each of the flights ranged between 0.7 and 0.9, while the Normalized Mean Bias (NMB) was smaller than 8% for almost every flight. Regarding LLBr CH3Br, the correlation with the aircraft observations is high (r>0.9) but the inter-hemispheric variability during transfer flights is not fully captured. For Ozone, the model presents mid to high correlation with respect to measures (0.5Fil: Berná Peña, Lucas Luciano. Universidad Tecnológica Nacional. Facultad Regional de Mendoza; ArgentinaFil: Lopez Noreña, Ana Isabel. Universidad Tecnológica Nacional. Facultad Regional de Mendoza; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Mendoza; ArgentinaFil: Puliafito, Salvador Enrique. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Mendoza; Argentina. Universidad Tecnológica Nacional. Facultad Regional de Mendoza; ArgentinaFil: Barreras, Javier Marcelo. Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaFil: Engel, Andreas. Goethe Universitat Frankfurt; AlemaniaFil: Jesswein, Markus. Goethe Universitat Frankfurt; AlemaniaFil: Cuevas, Carlos A.. Consejo Superior de Investigaciones Científicas. Instituto de Química Física; EspañaFil: Saiz Lopez, Alfonso. Consejo Superior de Investigaciones Científicas. Instituto de Química Física; EspañaFil: Fernandez, Rafael Pedro. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Mendoza. Instituto Interdisciplinario de Ciencias Básicas. - Universidad Nacional de Cuyo. Instituto Interdisciplinario de Ciencias Básicas; ArgentinaEGU General Assembly 2021AustriaEuropean Geosciences UnionCopernicus Publications2021info:eu-repo/semantics/publishedVersioninfo:eu-repo/semantics/conferenceObjectCongresoJournalhttp://purl.org/coar/resource_type/c_5794info:ar-repo/semantics/documentoDeConferenciaapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/175563Evaluation of CAM-CHEM VSL model performance during Southtrac campaign; EGU General Assembly 2021; Austria; 2021; 1-2CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://doi.org/10.5194/egusphere-egu21-2298Internacionalinfo:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-10-15T15:28:30Zoai:ri.conicet.gov.ar:11336/175563instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-10-15 15:28:30.995CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Evaluation of CAM-CHEM VSL model performance during Southtrac campaign
title Evaluation of CAM-CHEM VSL model performance during Southtrac campaign
spellingShingle Evaluation of CAM-CHEM VSL model performance during Southtrac campaign
Berná Peña, Lucas Luciano
VERY SHORT LIVED POLLUTANT
MODEL
CAM-CHEM
SOUTHTRAC
title_short Evaluation of CAM-CHEM VSL model performance during Southtrac campaign
title_full Evaluation of CAM-CHEM VSL model performance during Southtrac campaign
title_fullStr Evaluation of CAM-CHEM VSL model performance during Southtrac campaign
title_full_unstemmed Evaluation of CAM-CHEM VSL model performance during Southtrac campaign
title_sort Evaluation of CAM-CHEM VSL model performance during Southtrac campaign
dc.creator.none.fl_str_mv Berná Peña, Lucas Luciano
Lopez Noreña, Ana Isabel
Puliafito, Salvador Enrique
Barreras, Javier Marcelo
Engel, Andreas
Jesswein, Markus
Cuevas, Carlos A.
Saiz Lopez, Alfonso
Fernandez, Rafael Pedro
author Berná Peña, Lucas Luciano
author_facet Berná Peña, Lucas Luciano
Lopez Noreña, Ana Isabel
Puliafito, Salvador Enrique
Barreras, Javier Marcelo
Engel, Andreas
Jesswein, Markus
Cuevas, Carlos A.
Saiz Lopez, Alfonso
Fernandez, Rafael Pedro
author_role author
author2 Lopez Noreña, Ana Isabel
Puliafito, Salvador Enrique
Barreras, Javier Marcelo
Engel, Andreas
Jesswein, Markus
Cuevas, Carlos A.
Saiz Lopez, Alfonso
Fernandez, Rafael Pedro
author2_role author
author
author
author
author
author
author
author
dc.subject.none.fl_str_mv VERY SHORT LIVED POLLUTANT
MODEL
CAM-CHEM
SOUTHTRAC
topic VERY SHORT LIVED POLLUTANT
MODEL
CAM-CHEM
SOUTHTRAC
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.5
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv In the framework of the SouthTRAC Campaign (Transport and Composition of the Southern Hemisphere Upper Troposphere and Lower Stratosphere) based on Rio Grande, Argentina, a local research group from CONICET (Argentine National Research Council) joined the German consortium maintaining the HALO research aircraft (High-Altitude and LOng-range aircraft) to help with the flight planning and evaluation of the chemical composition of the upper troposphere and lower stratosphere within the ozone hole periphery. The SouthTRAC aircraft campaign was carried out in two phases which took place in September and November 2019, respectively. With the purpose of providing additional information of the atmospheric composition of brominated Very Short-Lived (VSLBr) species and compare with HALO observations during the transfer and campaign flights, a CAM-Chem (Community Atmosphere Model with Chemistry) global chemistry-climate simulation was conducted. The model setup used in the halogenated CAM-Chem simulation had a 1° x 1.25° lat-lon resolution, 56 hybrid vertical levels from the surface to the middle stratosphere and considered assimilated meteorology from MERRA, including an explicit treatment of VSLBr sources and chemistry. Model output of VSLBr, long-lived bromine and chlorine (LLBr and LLCl) species and ozone mixing ratios, as well as the main inorganic halogen reactive and reservoir species and gas/heterogeneous phase reaction rates affecting lowermost stratospheric ozone were analyzed in horizontal domains and vertical cross-sections across each flightpath. The model performance with respect to the HALO observations has a general good agreement, presenting better results for mid latitudes (between 30º S and 50º S) than for southern latitudes (>50º S). In particular, CAM-Chem timeseries consistently reproduced the spatio-temporal variation of the main VSLBr species (CH2Br2 and CHBr3), including the sharp variations observed across the tropopause. For both VSLBr as well as for LLCl compounds such as CFC-12, the Pearson correlation coefficient r obtained during each of the flights ranged between 0.7 and 0.9, while the Normalized Mean Bias (NMB) was smaller than 8% for almost every flight. Regarding LLBr CH3Br, the correlation with the aircraft observations is high (r>0.9) but the inter-hemispheric variability during transfer flights is not fully captured. For Ozone, the model presents mid to high correlation with respect to measures (0.5
Fil: Berná Peña, Lucas Luciano. Universidad Tecnológica Nacional. Facultad Regional de Mendoza; Argentina
Fil: Lopez Noreña, Ana Isabel. Universidad Tecnológica Nacional. Facultad Regional de Mendoza; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Mendoza; Argentina
Fil: Puliafito, Salvador Enrique. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Mendoza; Argentina. Universidad Tecnológica Nacional. Facultad Regional de Mendoza; Argentina
Fil: Barreras, Javier Marcelo. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Engel, Andreas. Goethe Universitat Frankfurt; Alemania
Fil: Jesswein, Markus. Goethe Universitat Frankfurt; Alemania
Fil: Cuevas, Carlos A.. Consejo Superior de Investigaciones Científicas. Instituto de Química Física; España
Fil: Saiz Lopez, Alfonso. Consejo Superior de Investigaciones Científicas. Instituto de Química Física; España
Fil: Fernandez, Rafael Pedro. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Mendoza. Instituto Interdisciplinario de Ciencias Básicas. - Universidad Nacional de Cuyo. Instituto Interdisciplinario de Ciencias Básicas; Argentina
EGU General Assembly 2021
Austria
European Geosciences Union
description In the framework of the SouthTRAC Campaign (Transport and Composition of the Southern Hemisphere Upper Troposphere and Lower Stratosphere) based on Rio Grande, Argentina, a local research group from CONICET (Argentine National Research Council) joined the German consortium maintaining the HALO research aircraft (High-Altitude and LOng-range aircraft) to help with the flight planning and evaluation of the chemical composition of the upper troposphere and lower stratosphere within the ozone hole periphery. The SouthTRAC aircraft campaign was carried out in two phases which took place in September and November 2019, respectively. With the purpose of providing additional information of the atmospheric composition of brominated Very Short-Lived (VSLBr) species and compare with HALO observations during the transfer and campaign flights, a CAM-Chem (Community Atmosphere Model with Chemistry) global chemistry-climate simulation was conducted. The model setup used in the halogenated CAM-Chem simulation had a 1° x 1.25° lat-lon resolution, 56 hybrid vertical levels from the surface to the middle stratosphere and considered assimilated meteorology from MERRA, including an explicit treatment of VSLBr sources and chemistry. Model output of VSLBr, long-lived bromine and chlorine (LLBr and LLCl) species and ozone mixing ratios, as well as the main inorganic halogen reactive and reservoir species and gas/heterogeneous phase reaction rates affecting lowermost stratospheric ozone were analyzed in horizontal domains and vertical cross-sections across each flightpath. The model performance with respect to the HALO observations has a general good agreement, presenting better results for mid latitudes (between 30º S and 50º S) than for southern latitudes (>50º S). In particular, CAM-Chem timeseries consistently reproduced the spatio-temporal variation of the main VSLBr species (CH2Br2 and CHBr3), including the sharp variations observed across the tropopause. For both VSLBr as well as for LLCl compounds such as CFC-12, the Pearson correlation coefficient r obtained during each of the flights ranged between 0.7 and 0.9, while the Normalized Mean Bias (NMB) was smaller than 8% for almost every flight. Regarding LLBr CH3Br, the correlation with the aircraft observations is high (r>0.9) but the inter-hemispheric variability during transfer flights is not fully captured. For Ozone, the model presents mid to high correlation with respect to measures (0.5
publishDate 2021
dc.date.none.fl_str_mv 2021
dc.type.none.fl_str_mv info:eu-repo/semantics/publishedVersion
info:eu-repo/semantics/conferenceObject
Congreso
Journal
http://purl.org/coar/resource_type/c_5794
info:ar-repo/semantics/documentoDeConferencia
status_str publishedVersion
format conferenceObject
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/175563
Evaluation of CAM-CHEM VSL model performance during Southtrac campaign; EGU General Assembly 2021; Austria; 2021; 1-2
CONICET Digital
CONICET
url http://hdl.handle.net/11336/175563
identifier_str_mv Evaluation of CAM-CHEM VSL model performance during Southtrac campaign; EGU General Assembly 2021; Austria; 2021; 1-2
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://doi.org/10.5194/egusphere-egu21-2298
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.coverage.none.fl_str_mv Internacional
dc.publisher.none.fl_str_mv Copernicus Publications
publisher.none.fl_str_mv Copernicus Publications
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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