Magnetic parameters as proxies for anthropogenic pollution in water reservoir sediments from Mexico: an interdisciplinary approach

Autores
Chaparro, Marcos Adrián Eduardo; Ramírez Ramírez, Margarita; Chaparro, Mauro Alejandro Eduardo; Miranda Avilés, Raúl; Puy Alquiza, María Jesús; Böhnel, Harald N.; Zanor, Gabriela Ana
Año de publicación
2020
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
We assess the element pollution level of water reservoir sediments using environmental magnetism techniques as a novel approach. Although “La Purísima” Water Reservoir is an important source for multiple activities (e.g. recreational, fishing and agricultural) in Guanajuato state, it has been receiving for the last centuries a high load of pollutants by mining extraction, urbanization and land-use change from the Guanajuato Hydrological Basin. The analyses of environmental magnetism, geochemistry, X-ray energy dispersive spectroscopy, scanning electron microscopy and multivariate methods were applied to study sediments from the reservoir and basin. Accordingly, they indicate the presence of iron oxides (magnetite and hematite) and iron sulfides (pyrite and greigite), which evidences relevant differences in particle size and concentration within the water reservoir (median mass-specific magnetic susceptibility χ = 23.2 × 10−8 m3/kg), as well as with respect to the river basin sediments (median χ = 88.8 × 10−8 m3/kg). The highest enrichment factor EF values (median values of EF = 2–10 for As, Co, Ba, Cu, Cd, Ni and EF > 20 for S) are mainly associated with historical mining activities that have led to an enrichment of potentially toxic elements on these water reservoir sediments. We propose the use of concentration and grain size dependent magnetic parameters, i.e. χ, remanent magnetizations and anhysteretic ratios ARM/SIRM and χARM/χ, as proxies for Ba, Co, Cr, Ni, P and Pb pollution in these river and water reservoir sediments. Such parameters allow to evaluate this sedimentary environment, and similar ones, through useful and convenient proxies.
Fil: Chaparro, Marcos Adrián Eduardo. Universidad Nacional del Centro de la Provincia de Buenos Aires. Centro de Investigaciones en Física e Ingeniería del Centro de la Provincia de Buenos Aires. - Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Tandil. Centro de Investigaciones en Física e Ingeniería del Centro de la Provincia de Buenos Aires. - Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas. Centro de Investigaciones en Física e Ingeniería del Centro de la Provincia de Buenos Aires; Argentina
Fil: Ramírez Ramírez, Margarita. Universidad de Guanajuato. División Ciencias de la Vida; México
Fil: Chaparro, Mauro Alejandro Eduardo. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Universidad Nacional de Mar del Plata. Facultad de Ciencias Exactas y Naturales. Departamento de Matemática; Argentina
Fil: Miranda Avilés, Raúl. Universidad de Guanajuato; México
Fil: Puy Alquiza, María Jesús. Universidad de Guanajuato; México
Fil: Böhnel, Harald N.. Universidad Nacional Autónoma de México. Centro de Geociencias; México
Fil: Zanor, Gabriela Ana. Universidad de Guanajuato. División Ciencias de la Vida; México
Materia
ENRICHMENT FACTOR EF
MAGNETIC PROXIES
MINING
MULTIVARIATE STATISTICS
RESERVOIR SEDIMENTS
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/105253
Acceder
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oai_identifier_str oai:ri.conicet.gov.ar:11336/105253
network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Magnetic parameters as proxies for anthropogenic pollution in water reservoir sediments from Mexico: an interdisciplinary approachChaparro, Marcos Adrián EduardoRamírez Ramírez, MargaritaChaparro, Mauro Alejandro EduardoMiranda Avilés, RaúlPuy Alquiza, María JesúsBöhnel, Harald N.Zanor, Gabriela AnaENRICHMENT FACTOR EFMAGNETIC PROXIESMININGMULTIVARIATE STATISTICSRESERVOIR SEDIMENTShttps://purl.org/becyt/ford/1.5https://purl.org/becyt/ford/1We assess the element pollution level of water reservoir sediments using environmental magnetism techniques as a novel approach. Although “La Purísima” Water Reservoir is an important source for multiple activities (e.g. recreational, fishing and agricultural) in Guanajuato state, it has been receiving for the last centuries a high load of pollutants by mining extraction, urbanization and land-use change from the Guanajuato Hydrological Basin. The analyses of environmental magnetism, geochemistry, X-ray energy dispersive spectroscopy, scanning electron microscopy and multivariate methods were applied to study sediments from the reservoir and basin. Accordingly, they indicate the presence of iron oxides (magnetite and hematite) and iron sulfides (pyrite and greigite), which evidences relevant differences in particle size and concentration within the water reservoir (median mass-specific magnetic susceptibility χ = 23.2 × 10−8 m3/kg), as well as with respect to the river basin sediments (median χ = 88.8 × 10−8 m3/kg). The highest enrichment factor EF values (median values of EF = 2–10 for As, Co, Ba, Cu, Cd, Ni and EF > 20 for S) are mainly associated with historical mining activities that have led to an enrichment of potentially toxic elements on these water reservoir sediments. We propose the use of concentration and grain size dependent magnetic parameters, i.e. χ, remanent magnetizations and anhysteretic ratios ARM/SIRM and χARM/χ, as proxies for Ba, Co, Cr, Ni, P and Pb pollution in these river and water reservoir sediments. Such parameters allow to evaluate this sedimentary environment, and similar ones, through useful and convenient proxies.Fil: Chaparro, Marcos Adrián Eduardo. Universidad Nacional del Centro de la Provincia de Buenos Aires. Centro de Investigaciones en Física e Ingeniería del Centro de la Provincia de Buenos Aires. - Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Tandil. Centro de Investigaciones en Física e Ingeniería del Centro de la Provincia de Buenos Aires. - Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas. Centro de Investigaciones en Física e Ingeniería del Centro de la Provincia de Buenos Aires; ArgentinaFil: Ramírez Ramírez, Margarita. Universidad de Guanajuato. División Ciencias de la Vida; MéxicoFil: Chaparro, Mauro Alejandro Eduardo. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Universidad Nacional de Mar del Plata. Facultad de Ciencias Exactas y Naturales. Departamento de Matemática; ArgentinaFil: Miranda Avilés, Raúl. Universidad de Guanajuato; MéxicoFil: Puy Alquiza, María Jesús. Universidad de Guanajuato; MéxicoFil: Böhnel, Harald N.. Universidad Nacional Autónoma de México. Centro de Geociencias; MéxicoFil: Zanor, Gabriela Ana. Universidad de Guanajuato. División Ciencias de la Vida; MéxicoElsevier2020-01info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/105253Chaparro, Marcos Adrián Eduardo; Ramírez Ramírez, Margarita; Chaparro, Mauro Alejandro Eduardo; Miranda Avilés, Raúl; Puy Alquiza, María Jesús; et al.; Magnetic parameters as proxies for anthropogenic pollution in water reservoir sediments from Mexico: an interdisciplinary approach; Elsevier; Science of the Total Environment; 700; 1-2020; 1-400048-96971879-1026CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://linkinghub.elsevier.com/retrieve/pii/S0048969719343347info:eu-repo/semantics/altIdentifier/doi/10.1016/j.scitotenv.2019.134343info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-nd/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T10:23:23Zoai:ri.conicet.gov.ar:11336/105253instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 10:23:23.454CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Magnetic parameters as proxies for anthropogenic pollution in water reservoir sediments from Mexico: an interdisciplinary approach
title Magnetic parameters as proxies for anthropogenic pollution in water reservoir sediments from Mexico: an interdisciplinary approach
spellingShingle Magnetic parameters as proxies for anthropogenic pollution in water reservoir sediments from Mexico: an interdisciplinary approach
Chaparro, Marcos Adrián Eduardo
ENRICHMENT FACTOR EF
MAGNETIC PROXIES
MINING
MULTIVARIATE STATISTICS
RESERVOIR SEDIMENTS
title_short Magnetic parameters as proxies for anthropogenic pollution in water reservoir sediments from Mexico: an interdisciplinary approach
title_full Magnetic parameters as proxies for anthropogenic pollution in water reservoir sediments from Mexico: an interdisciplinary approach
title_fullStr Magnetic parameters as proxies for anthropogenic pollution in water reservoir sediments from Mexico: an interdisciplinary approach
title_full_unstemmed Magnetic parameters as proxies for anthropogenic pollution in water reservoir sediments from Mexico: an interdisciplinary approach
title_sort Magnetic parameters as proxies for anthropogenic pollution in water reservoir sediments from Mexico: an interdisciplinary approach
dc.creator.none.fl_str_mv Chaparro, Marcos Adrián Eduardo
Ramírez Ramírez, Margarita
Chaparro, Mauro Alejandro Eduardo
Miranda Avilés, Raúl
Puy Alquiza, María Jesús
Böhnel, Harald N.
Zanor, Gabriela Ana
author Chaparro, Marcos Adrián Eduardo
author_facet Chaparro, Marcos Adrián Eduardo
Ramírez Ramírez, Margarita
Chaparro, Mauro Alejandro Eduardo
Miranda Avilés, Raúl
Puy Alquiza, María Jesús
Böhnel, Harald N.
Zanor, Gabriela Ana
author_role author
author2 Ramírez Ramírez, Margarita
Chaparro, Mauro Alejandro Eduardo
Miranda Avilés, Raúl
Puy Alquiza, María Jesús
Böhnel, Harald N.
Zanor, Gabriela Ana
author2_role author
author
author
author
author
author
dc.subject.none.fl_str_mv ENRICHMENT FACTOR EF
MAGNETIC PROXIES
MINING
MULTIVARIATE STATISTICS
RESERVOIR SEDIMENTS
topic ENRICHMENT FACTOR EF
MAGNETIC PROXIES
MINING
MULTIVARIATE STATISTICS
RESERVOIR SEDIMENTS
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.5
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv We assess the element pollution level of water reservoir sediments using environmental magnetism techniques as a novel approach. Although “La Purísima” Water Reservoir is an important source for multiple activities (e.g. recreational, fishing and agricultural) in Guanajuato state, it has been receiving for the last centuries a high load of pollutants by mining extraction, urbanization and land-use change from the Guanajuato Hydrological Basin. The analyses of environmental magnetism, geochemistry, X-ray energy dispersive spectroscopy, scanning electron microscopy and multivariate methods were applied to study sediments from the reservoir and basin. Accordingly, they indicate the presence of iron oxides (magnetite and hematite) and iron sulfides (pyrite and greigite), which evidences relevant differences in particle size and concentration within the water reservoir (median mass-specific magnetic susceptibility χ = 23.2 × 10−8 m3/kg), as well as with respect to the river basin sediments (median χ = 88.8 × 10−8 m3/kg). The highest enrichment factor EF values (median values of EF = 2–10 for As, Co, Ba, Cu, Cd, Ni and EF > 20 for S) are mainly associated with historical mining activities that have led to an enrichment of potentially toxic elements on these water reservoir sediments. We propose the use of concentration and grain size dependent magnetic parameters, i.e. χ, remanent magnetizations and anhysteretic ratios ARM/SIRM and χARM/χ, as proxies for Ba, Co, Cr, Ni, P and Pb pollution in these river and water reservoir sediments. Such parameters allow to evaluate this sedimentary environment, and similar ones, through useful and convenient proxies.
Fil: Chaparro, Marcos Adrián Eduardo. Universidad Nacional del Centro de la Provincia de Buenos Aires. Centro de Investigaciones en Física e Ingeniería del Centro de la Provincia de Buenos Aires. - Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Tandil. Centro de Investigaciones en Física e Ingeniería del Centro de la Provincia de Buenos Aires. - Provincia de Buenos Aires. Gobernación. Comisión de Investigaciones Científicas. Centro de Investigaciones en Física e Ingeniería del Centro de la Provincia de Buenos Aires; Argentina
Fil: Ramírez Ramírez, Margarita. Universidad de Guanajuato. División Ciencias de la Vida; México
Fil: Chaparro, Mauro Alejandro Eduardo. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Universidad Nacional de Mar del Plata. Facultad de Ciencias Exactas y Naturales. Departamento de Matemática; Argentina
Fil: Miranda Avilés, Raúl. Universidad de Guanajuato; México
Fil: Puy Alquiza, María Jesús. Universidad de Guanajuato; México
Fil: Böhnel, Harald N.. Universidad Nacional Autónoma de México. Centro de Geociencias; México
Fil: Zanor, Gabriela Ana. Universidad de Guanajuato. División Ciencias de la Vida; México
description We assess the element pollution level of water reservoir sediments using environmental magnetism techniques as a novel approach. Although “La Purísima” Water Reservoir is an important source for multiple activities (e.g. recreational, fishing and agricultural) in Guanajuato state, it has been receiving for the last centuries a high load of pollutants by mining extraction, urbanization and land-use change from the Guanajuato Hydrological Basin. The analyses of environmental magnetism, geochemistry, X-ray energy dispersive spectroscopy, scanning electron microscopy and multivariate methods were applied to study sediments from the reservoir and basin. Accordingly, they indicate the presence of iron oxides (magnetite and hematite) and iron sulfides (pyrite and greigite), which evidences relevant differences in particle size and concentration within the water reservoir (median mass-specific magnetic susceptibility χ = 23.2 × 10−8 m3/kg), as well as with respect to the river basin sediments (median χ = 88.8 × 10−8 m3/kg). The highest enrichment factor EF values (median values of EF = 2–10 for As, Co, Ba, Cu, Cd, Ni and EF > 20 for S) are mainly associated with historical mining activities that have led to an enrichment of potentially toxic elements on these water reservoir sediments. We propose the use of concentration and grain size dependent magnetic parameters, i.e. χ, remanent magnetizations and anhysteretic ratios ARM/SIRM and χARM/χ, as proxies for Ba, Co, Cr, Ni, P and Pb pollution in these river and water reservoir sediments. Such parameters allow to evaluate this sedimentary environment, and similar ones, through useful and convenient proxies.
publishDate 2020
dc.date.none.fl_str_mv 2020-01
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/105253
Chaparro, Marcos Adrián Eduardo; Ramírez Ramírez, Margarita; Chaparro, Mauro Alejandro Eduardo; Miranda Avilés, Raúl; Puy Alquiza, María Jesús; et al.; Magnetic parameters as proxies for anthropogenic pollution in water reservoir sediments from Mexico: an interdisciplinary approach; Elsevier; Science of the Total Environment; 700; 1-2020; 1-40
0048-9697
1879-1026
CONICET Digital
CONICET
url http://hdl.handle.net/11336/105253
identifier_str_mv Chaparro, Marcos Adrián Eduardo; Ramírez Ramírez, Margarita; Chaparro, Mauro Alejandro Eduardo; Miranda Avilés, Raúl; Puy Alquiza, María Jesús; et al.; Magnetic parameters as proxies for anthropogenic pollution in water reservoir sediments from Mexico: an interdisciplinary approach; Elsevier; Science of the Total Environment; 700; 1-2020; 1-40
0048-9697
1879-1026
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://linkinghub.elsevier.com/retrieve/pii/S0048969719343347
info:eu-repo/semantics/altIdentifier/doi/10.1016/j.scitotenv.2019.134343
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv Elsevier
publisher.none.fl_str_mv Elsevier
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 13.070432

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