Application of ETS-10 microporous titanosilicate as support of Ru nanoparticles for hydrogen production

Autores
Faroldi, Betina María Cecilia; Lombardo, Eduardo Agustin; Cornaglia, Laura Maria; Irusta, S.
Año de publicación
2012
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
Supported ruthenium catalysts have been shown to be effective for the dry reforming of methane.Besides, ETS-10 titanosilicate has properties able to disperse Ru species. In this work,  microporous ETS-10 titanosilicate was synthesized by hydrothermal synthesis employing anatase as Ti source. Ru was incorporated using three different methods: by incipient wetness impregnation (RuH), by ion exchange (RuI) and by adding Ru to the gel synthesis (RuG). The species present in the solids were characterized by XRD, N2 adsorption, ICP, SEM, TEM, EDX, TGA, TPR, UV?vis and XPS.RuH and RuI catalysts were found to be active and stable for the dry reforming of methane. These results show the potential application of ETS-10 as support of Ru catalysts for the production of hydrogen.
Fil: Faroldi, Betina María Cecilia. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera". Universidad Nacional del Litoral. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera"; Argentina
Fil: Lombardo, Eduardo Agustin. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera". Universidad Nacional del Litoral. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera"; Argentina
Fil: Cornaglia, Laura Maria. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera". Universidad Nacional del Litoral. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera"; Argentina
Fil: Irusta, S.. Universidad de Zaragoza. Instituto de Nanociencia de Aragón; España
Materia
Methane reforming
ETS-10
Ru
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/268911

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spelling Application of ETS-10 microporous titanosilicate as support of Ru nanoparticles for hydrogen productionFaroldi, Betina María CeciliaLombardo, Eduardo AgustinCornaglia, Laura MariaIrusta, S.Methane reformingETS-10Ruhttps://purl.org/becyt/ford/2.4https://purl.org/becyt/ford/2Supported ruthenium catalysts have been shown to be effective for the dry reforming of methane.Besides, ETS-10 titanosilicate has properties able to disperse Ru species. In this work,  microporous ETS-10 titanosilicate was synthesized by hydrothermal synthesis employing anatase as Ti source. Ru was incorporated using three different methods: by incipient wetness impregnation (RuH), by ion exchange (RuI) and by adding Ru to the gel synthesis (RuG). The species present in the solids were characterized by XRD, N2 adsorption, ICP, SEM, TEM, EDX, TGA, TPR, UV?vis and XPS.RuH and RuI catalysts were found to be active and stable for the dry reforming of methane. These results show the potential application of ETS-10 as support of Ru catalysts for the production of hydrogen.Fil: Faroldi, Betina María Cecilia. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera". Universidad Nacional del Litoral. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera"; ArgentinaFil: Lombardo, Eduardo Agustin. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera". Universidad Nacional del Litoral. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera"; ArgentinaFil: Cornaglia, Laura Maria. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera". Universidad Nacional del Litoral. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera"; ArgentinaFil: Irusta, S.. Universidad de Zaragoza. Instituto de Nanociencia de Aragón; EspañaElsevier Science2012-02info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/268911Faroldi, Betina María Cecilia; Lombardo, Eduardo Agustin; Cornaglia, Laura Maria; Irusta, S.; Application of ETS-10 microporous titanosilicate as support of Ru nanoparticles for hydrogen production; Elsevier Science; Applied Catalysis A: General; 417-418; 2-2012; 43-520926-860XCONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://www.sciencedirect.com/science/article/abs/pii/S0926860X11007411info:eu-repo/semantics/altIdentifier/doi/10.1016/j.apcata.2011.12.023info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T09:33:11Zoai:ri.conicet.gov.ar:11336/268911instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 09:33:12.191CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Application of ETS-10 microporous titanosilicate as support of Ru nanoparticles for hydrogen production
title Application of ETS-10 microporous titanosilicate as support of Ru nanoparticles for hydrogen production
spellingShingle Application of ETS-10 microporous titanosilicate as support of Ru nanoparticles for hydrogen production
Faroldi, Betina María Cecilia
Methane reforming
ETS-10
Ru
title_short Application of ETS-10 microporous titanosilicate as support of Ru nanoparticles for hydrogen production
title_full Application of ETS-10 microporous titanosilicate as support of Ru nanoparticles for hydrogen production
title_fullStr Application of ETS-10 microporous titanosilicate as support of Ru nanoparticles for hydrogen production
title_full_unstemmed Application of ETS-10 microporous titanosilicate as support of Ru nanoparticles for hydrogen production
title_sort Application of ETS-10 microporous titanosilicate as support of Ru nanoparticles for hydrogen production
dc.creator.none.fl_str_mv Faroldi, Betina María Cecilia
Lombardo, Eduardo Agustin
Cornaglia, Laura Maria
Irusta, S.
author Faroldi, Betina María Cecilia
author_facet Faroldi, Betina María Cecilia
Lombardo, Eduardo Agustin
Cornaglia, Laura Maria
Irusta, S.
author_role author
author2 Lombardo, Eduardo Agustin
Cornaglia, Laura Maria
Irusta, S.
author2_role author
author
author
dc.subject.none.fl_str_mv Methane reforming
ETS-10
Ru
topic Methane reforming
ETS-10
Ru
purl_subject.fl_str_mv https://purl.org/becyt/ford/2.4
https://purl.org/becyt/ford/2
dc.description.none.fl_txt_mv Supported ruthenium catalysts have been shown to be effective for the dry reforming of methane.Besides, ETS-10 titanosilicate has properties able to disperse Ru species. In this work,  microporous ETS-10 titanosilicate was synthesized by hydrothermal synthesis employing anatase as Ti source. Ru was incorporated using three different methods: by incipient wetness impregnation (RuH), by ion exchange (RuI) and by adding Ru to the gel synthesis (RuG). The species present in the solids were characterized by XRD, N2 adsorption, ICP, SEM, TEM, EDX, TGA, TPR, UV?vis and XPS.RuH and RuI catalysts were found to be active and stable for the dry reforming of methane. These results show the potential application of ETS-10 as support of Ru catalysts for the production of hydrogen.
Fil: Faroldi, Betina María Cecilia. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera". Universidad Nacional del Litoral. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera"; Argentina
Fil: Lombardo, Eduardo Agustin. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera". Universidad Nacional del Litoral. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera"; Argentina
Fil: Cornaglia, Laura Maria. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera". Universidad Nacional del Litoral. Instituto de Investigaciones en Catálisis y Petroquímica "Ing. José Miguel Parera"; Argentina
Fil: Irusta, S.. Universidad de Zaragoza. Instituto de Nanociencia de Aragón; España
description Supported ruthenium catalysts have been shown to be effective for the dry reforming of methane.Besides, ETS-10 titanosilicate has properties able to disperse Ru species. In this work,  microporous ETS-10 titanosilicate was synthesized by hydrothermal synthesis employing anatase as Ti source. Ru was incorporated using three different methods: by incipient wetness impregnation (RuH), by ion exchange (RuI) and by adding Ru to the gel synthesis (RuG). The species present in the solids were characterized by XRD, N2 adsorption, ICP, SEM, TEM, EDX, TGA, TPR, UV?vis and XPS.RuH and RuI catalysts were found to be active and stable for the dry reforming of methane. These results show the potential application of ETS-10 as support of Ru catalysts for the production of hydrogen.
publishDate 2012
dc.date.none.fl_str_mv 2012-02
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/268911
Faroldi, Betina María Cecilia; Lombardo, Eduardo Agustin; Cornaglia, Laura Maria; Irusta, S.; Application of ETS-10 microporous titanosilicate as support of Ru nanoparticles for hydrogen production; Elsevier Science; Applied Catalysis A: General; 417-418; 2-2012; 43-52
0926-860X
CONICET Digital
CONICET
url http://hdl.handle.net/11336/268911
identifier_str_mv Faroldi, Betina María Cecilia; Lombardo, Eduardo Agustin; Cornaglia, Laura Maria; Irusta, S.; Application of ETS-10 microporous titanosilicate as support of Ru nanoparticles for hydrogen production; Elsevier Science; Applied Catalysis A: General; 417-418; 2-2012; 43-52
0926-860X
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://www.sciencedirect.com/science/article/abs/pii/S0926860X11007411
info:eu-repo/semantics/altIdentifier/doi/10.1016/j.apcata.2011.12.023
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
application/pdf
application/pdf
dc.publisher.none.fl_str_mv Elsevier Science
publisher.none.fl_str_mv Elsevier Science
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
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repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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