Sustainable synergy: Valorisation of spent lithium-ion batteries and dry reforming of methane for a circular energy future

Autores
Dubois, Franco; Volpe Giangiordano, María Florencia; Pompeo, Francisco; Furlong, Octavio Javier; Nazzarro, Marcelo Sandro; Peluso, Miguel Andrés; Sambeth, Jorge Enrique
Año de publicación
2025
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
From the recovery of Ni, Co, and Mn from Li-ion batteries using the hydrometallurgical technique, two catalysts supported on γ-Al₂O₃ with different metal load concentrations were prepared. The catalysts were characterized using XRD, SEM, TPR, XPS and BET surface area measurements. These catalysts were studied in the dry reforming of methane reaction at 600 ◦C. The results showed that the solids prepared from a leach solution of lithium-ion batteries exhibit good catalytic activity in the DRM reaction at low temperatures (600 ◦C). The prepared catalysts demonstrated good performance, with conversion rates comparable to those in other studies and an H₂/CO ratio of 0.7–0.8, making them promising for catalytic applications aimed at reducing greenhouse gases and hazardous waste, such as those found in these batteries.
Planta Piloto Multipropósito - Laboratorio de Servicios a la Industria y al Sistema Científico
Centro de Investigación y Desarrollo en Criotecnología de Alimentos
Materia
Química
Li-ion batteries
Recycling
NiMnCo
Methane dry reforming
Nivel de accesibilidad
acceso abierto
Condiciones de uso
http://creativecommons.org/licenses/by/4.0/
Repositorio
SEDICI (UNLP)
Institución
Universidad Nacional de La Plata
OAI Identificador
oai:sedici.unlp.edu.ar:10915/182243
Acceder
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oai_identifier_str oai:sedici.unlp.edu.ar:10915/182243
network_acronym_str SEDICI
repository_id_str 1329
network_name_str SEDICI (UNLP)
spelling Sustainable synergy: Valorisation of spent lithium-ion batteries and dry reforming of methane for a circular energy futureDubois, FrancoVolpe Giangiordano, María FlorenciaPompeo, FranciscoFurlong, Octavio JavierNazzarro, Marcelo SandroPeluso, Miguel AndrésSambeth, Jorge EnriqueQuímicaLi-ion batteriesRecyclingNiMnCoMethane dry reformingFrom the recovery of Ni, Co, and Mn from Li-ion batteries using the hydrometallurgical technique, two catalysts supported on γ-Al₂O₃ with different metal load concentrations were prepared. The catalysts were characterized using XRD, SEM, TPR, XPS and BET surface area measurements. These catalysts were studied in the dry reforming of methane reaction at 600 ◦C. The results showed that the solids prepared from a leach solution of lithium-ion batteries exhibit good catalytic activity in the DRM reaction at low temperatures (600 ◦C). The prepared catalysts demonstrated good performance, with conversion rates comparable to those in other studies and an H₂/CO ratio of 0.7–0.8, making them promising for catalytic applications aimed at reducing greenhouse gases and hazardous waste, such as those found in these batteries.Planta Piloto Multipropósito - Laboratorio de Servicios a la Industria y al Sistema CientíficoCentro de Investigación y Desarrollo en Criotecnología de Alimentos2025-09info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionArticulohttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfhttp://sedici.unlp.edu.ar/handle/10915/182243enginfo:eu-repo/semantics/altIdentifier/issn/2950-6492info:eu-repo/semantics/altIdentifier/issn/2950-6484info:eu-repo/semantics/altIdentifier/doi/10.1016/j.apcato.2025.207061info:eu-repo/semantics/openAccesshttp://creativecommons.org/licenses/by/4.0/Creative Commons Attribution 4.0 International (CC BY 4.0)reponame:SEDICI (UNLP)instname:Universidad Nacional de La Platainstacron:UNLP2025-09-29T11:49:47Zoai:sedici.unlp.edu.ar:10915/182243Institucionalhttp://sedici.unlp.edu.ar/Universidad públicaNo correspondehttp://sedici.unlp.edu.ar/oai/snrdalira@sedici.unlp.edu.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:13292025-09-29 11:49:47.957SEDICI (UNLP) - Universidad Nacional de La Platafalse
dc.title.none.fl_str_mv Sustainable synergy: Valorisation of spent lithium-ion batteries and dry reforming of methane for a circular energy future
title Sustainable synergy: Valorisation of spent lithium-ion batteries and dry reforming of methane for a circular energy future
spellingShingle Sustainable synergy: Valorisation of spent lithium-ion batteries and dry reforming of methane for a circular energy future
Dubois, Franco
Química
Li-ion batteries
Recycling
NiMnCo
Methane dry reforming
title_short Sustainable synergy: Valorisation of spent lithium-ion batteries and dry reforming of methane for a circular energy future
title_full Sustainable synergy: Valorisation of spent lithium-ion batteries and dry reforming of methane for a circular energy future
title_fullStr Sustainable synergy: Valorisation of spent lithium-ion batteries and dry reforming of methane for a circular energy future
title_full_unstemmed Sustainable synergy: Valorisation of spent lithium-ion batteries and dry reforming of methane for a circular energy future
title_sort Sustainable synergy: Valorisation of spent lithium-ion batteries and dry reforming of methane for a circular energy future
dc.creator.none.fl_str_mv Dubois, Franco
Volpe Giangiordano, María Florencia
Pompeo, Francisco
Furlong, Octavio Javier
Nazzarro, Marcelo Sandro
Peluso, Miguel Andrés
Sambeth, Jorge Enrique
author Dubois, Franco
author_facet Dubois, Franco
Volpe Giangiordano, María Florencia
Pompeo, Francisco
Furlong, Octavio Javier
Nazzarro, Marcelo Sandro
Peluso, Miguel Andrés
Sambeth, Jorge Enrique
author_role author
author2 Volpe Giangiordano, María Florencia
Pompeo, Francisco
Furlong, Octavio Javier
Nazzarro, Marcelo Sandro
Peluso, Miguel Andrés
Sambeth, Jorge Enrique
author2_role author
author
author
author
author
author
dc.subject.none.fl_str_mv Química
Li-ion batteries
Recycling
NiMnCo
Methane dry reforming
topic Química
Li-ion batteries
Recycling
NiMnCo
Methane dry reforming
dc.description.none.fl_txt_mv From the recovery of Ni, Co, and Mn from Li-ion batteries using the hydrometallurgical technique, two catalysts supported on γ-Al₂O₃ with different metal load concentrations were prepared. The catalysts were characterized using XRD, SEM, TPR, XPS and BET surface area measurements. These catalysts were studied in the dry reforming of methane reaction at 600 ◦C. The results showed that the solids prepared from a leach solution of lithium-ion batteries exhibit good catalytic activity in the DRM reaction at low temperatures (600 ◦C). The prepared catalysts demonstrated good performance, with conversion rates comparable to those in other studies and an H₂/CO ratio of 0.7–0.8, making them promising for catalytic applications aimed at reducing greenhouse gases and hazardous waste, such as those found in these batteries.
Planta Piloto Multipropósito - Laboratorio de Servicios a la Industria y al Sistema Científico
Centro de Investigación y Desarrollo en Criotecnología de Alimentos
description From the recovery of Ni, Co, and Mn from Li-ion batteries using the hydrometallurgical technique, two catalysts supported on γ-Al₂O₃ with different metal load concentrations were prepared. The catalysts were characterized using XRD, SEM, TPR, XPS and BET surface area measurements. These catalysts were studied in the dry reforming of methane reaction at 600 ◦C. The results showed that the solids prepared from a leach solution of lithium-ion batteries exhibit good catalytic activity in the DRM reaction at low temperatures (600 ◦C). The prepared catalysts demonstrated good performance, with conversion rates comparable to those in other studies and an H₂/CO ratio of 0.7–0.8, making them promising for catalytic applications aimed at reducing greenhouse gases and hazardous waste, such as those found in these batteries.
publishDate 2025
dc.date.none.fl_str_mv 2025-09
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
Articulo
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://sedici.unlp.edu.ar/handle/10915/182243
url http://sedici.unlp.edu.ar/handle/10915/182243
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/issn/2950-6492
info:eu-repo/semantics/altIdentifier/issn/2950-6484
info:eu-repo/semantics/altIdentifier/doi/10.1016/j.apcato.2025.207061
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
http://creativecommons.org/licenses/by/4.0/
Creative Commons Attribution 4.0 International (CC BY 4.0)
eu_rights_str_mv openAccess
rights_invalid_str_mv http://creativecommons.org/licenses/by/4.0/
Creative Commons Attribution 4.0 International (CC BY 4.0)
dc.format.none.fl_str_mv application/pdf
dc.source.none.fl_str_mv reponame:SEDICI (UNLP)
instname:Universidad Nacional de La Plata
instacron:UNLP
reponame_str SEDICI (UNLP)
collection SEDICI (UNLP)
instname_str Universidad Nacional de La Plata
instacron_str UNLP
institution UNLP
repository.name.fl_str_mv SEDICI (UNLP) - Universidad Nacional de La Plata
repository.mail.fl_str_mv alira@sedici.unlp.edu.ar
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score 13.070432

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