Effect of Water Content in the Gas Diffusion Layer of H<SUB>2</SUB>/O<SUB>2</SUB> PEM Fuel Cell

Autores
Cespedes, Germán; Asteazaran, Mariano; Castro Luna Berenguer, Ana María del Carmen
Año de publicación
2016
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
The heart of a fuel cell is the membrane-electrode assembly consisting of two porous electrodes, where the electrochemical reactions take place, and the ionomer conductive membrane, which allows the proton exchange from the anode to the cathode. The porosity of the electrodes plays an important role in the fuel cell performance. One of the drawbacks presented by the porous electrodes is the accumulation of water in their structure, which implies a hindrance for the reactive gas transport to reach the catalytic reactive sites. In this paper, a mathematical model of a porous electrode, assuming single pores with uniform distribution, is introduced to determine the influence of water accumulation in the electrode on the fuel cell performance under different operating conditions. It is demonstrated that at low current densities, water accumulation has no effect in the fuel cell behavior, whereas at high current densities its performance is severely affected.
Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas
Materia
Química
Fuel cells
porous-electrodes
electrode flooding
Nivel de accesibilidad
acceso abierto
Condiciones de uso
http://creativecommons.org/licenses/by-nc-sa/4.0/
Repositorio
SEDICI (UNLP)
Institución
Universidad Nacional de La Plata
OAI Identificador
oai:sedici.unlp.edu.ar:10915/108950

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spelling Effect of Water Content in the Gas Diffusion Layer of H<SUB>2</SUB>/O<SUB>2</SUB> PEM Fuel CellCespedes, GermánAsteazaran, MarianoCastro Luna Berenguer, Ana María del CarmenQuímicaFuel cellsporous-electrodeselectrode floodingThe heart of a fuel cell is the membrane-electrode assembly consisting of two porous electrodes, where the electrochemical reactions take place, and the ionomer conductive membrane, which allows the proton exchange from the anode to the cathode. The porosity of the electrodes plays an important role in the fuel cell performance. One of the drawbacks presented by the porous electrodes is the accumulation of water in their structure, which implies a hindrance for the reactive gas transport to reach the catalytic reactive sites. In this paper, a mathematical model of a porous electrode, assuming single pores with uniform distribution, is introduced to determine the influence of water accumulation in the electrode on the fuel cell performance under different operating conditions. It is demonstrated that at low current densities, water accumulation has no effect in the fuel cell behavior, whereas at high current densities its performance is severely affected.Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas2016info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionArticulohttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdf213-221http://sedici.unlp.edu.ar/handle/10915/108950enginfo:eu-repo/semantics/altIdentifier/issn/2161-6213info:eu-repo/semantics/altIdentifier/doi/10.17265/2161-6213/2016.7-8.004info:eu-repo/semantics/openAccesshttp://creativecommons.org/licenses/by-nc-sa/4.0/Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International (CC BY-NC-SA 4.0)reponame:SEDICI (UNLP)instname:Universidad Nacional de La Platainstacron:UNLP2025-10-15T11:16:34Zoai:sedici.unlp.edu.ar:10915/108950Institucionalhttp://sedici.unlp.edu.ar/Universidad públicaNo correspondehttp://sedici.unlp.edu.ar/oai/snrdalira@sedici.unlp.edu.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:13292025-10-15 11:16:34.334SEDICI (UNLP) - Universidad Nacional de La Platafalse
dc.title.none.fl_str_mv Effect of Water Content in the Gas Diffusion Layer of H<SUB>2</SUB>/O<SUB>2</SUB> PEM Fuel Cell
title Effect of Water Content in the Gas Diffusion Layer of H<SUB>2</SUB>/O<SUB>2</SUB> PEM Fuel Cell
spellingShingle Effect of Water Content in the Gas Diffusion Layer of H<SUB>2</SUB>/O<SUB>2</SUB> PEM Fuel Cell
Cespedes, Germán
Química
Fuel cells
porous-electrodes
electrode flooding
title_short Effect of Water Content in the Gas Diffusion Layer of H<SUB>2</SUB>/O<SUB>2</SUB> PEM Fuel Cell
title_full Effect of Water Content in the Gas Diffusion Layer of H<SUB>2</SUB>/O<SUB>2</SUB> PEM Fuel Cell
title_fullStr Effect of Water Content in the Gas Diffusion Layer of H<SUB>2</SUB>/O<SUB>2</SUB> PEM Fuel Cell
title_full_unstemmed Effect of Water Content in the Gas Diffusion Layer of H<SUB>2</SUB>/O<SUB>2</SUB> PEM Fuel Cell
title_sort Effect of Water Content in the Gas Diffusion Layer of H<SUB>2</SUB>/O<SUB>2</SUB> PEM Fuel Cell
dc.creator.none.fl_str_mv Cespedes, Germán
Asteazaran, Mariano
Castro Luna Berenguer, Ana María del Carmen
author Cespedes, Germán
author_facet Cespedes, Germán
Asteazaran, Mariano
Castro Luna Berenguer, Ana María del Carmen
author_role author
author2 Asteazaran, Mariano
Castro Luna Berenguer, Ana María del Carmen
author2_role author
author
dc.subject.none.fl_str_mv Química
Fuel cells
porous-electrodes
electrode flooding
topic Química
Fuel cells
porous-electrodes
electrode flooding
dc.description.none.fl_txt_mv The heart of a fuel cell is the membrane-electrode assembly consisting of two porous electrodes, where the electrochemical reactions take place, and the ionomer conductive membrane, which allows the proton exchange from the anode to the cathode. The porosity of the electrodes plays an important role in the fuel cell performance. One of the drawbacks presented by the porous electrodes is the accumulation of water in their structure, which implies a hindrance for the reactive gas transport to reach the catalytic reactive sites. In this paper, a mathematical model of a porous electrode, assuming single pores with uniform distribution, is introduced to determine the influence of water accumulation in the electrode on the fuel cell performance under different operating conditions. It is demonstrated that at low current densities, water accumulation has no effect in the fuel cell behavior, whereas at high current densities its performance is severely affected.
Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas
description The heart of a fuel cell is the membrane-electrode assembly consisting of two porous electrodes, where the electrochemical reactions take place, and the ionomer conductive membrane, which allows the proton exchange from the anode to the cathode. The porosity of the electrodes plays an important role in the fuel cell performance. One of the drawbacks presented by the porous electrodes is the accumulation of water in their structure, which implies a hindrance for the reactive gas transport to reach the catalytic reactive sites. In this paper, a mathematical model of a porous electrode, assuming single pores with uniform distribution, is introduced to determine the influence of water accumulation in the electrode on the fuel cell performance under different operating conditions. It is demonstrated that at low current densities, water accumulation has no effect in the fuel cell behavior, whereas at high current densities its performance is severely affected.
publishDate 2016
dc.date.none.fl_str_mv 2016
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
Articulo
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://sedici.unlp.edu.ar/handle/10915/108950
url http://sedici.unlp.edu.ar/handle/10915/108950
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/issn/2161-6213
info:eu-repo/semantics/altIdentifier/doi/10.17265/2161-6213/2016.7-8.004
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
http://creativecommons.org/licenses/by-nc-sa/4.0/
Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International (CC BY-NC-SA 4.0)
eu_rights_str_mv openAccess
rights_invalid_str_mv http://creativecommons.org/licenses/by-nc-sa/4.0/
Creative Commons Attribution-NonCommercial-ShareAlike 4.0 International (CC BY-NC-SA 4.0)
dc.format.none.fl_str_mv application/pdf
213-221
dc.source.none.fl_str_mv reponame:SEDICI (UNLP)
instname:Universidad Nacional de La Plata
instacron:UNLP
reponame_str SEDICI (UNLP)
collection SEDICI (UNLP)
instname_str Universidad Nacional de La Plata
instacron_str UNLP
institution UNLP
repository.name.fl_str_mv SEDICI (UNLP) - Universidad Nacional de La Plata
repository.mail.fl_str_mv alira@sedici.unlp.edu.ar
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