“On the fly” characterization of YbIII:ErIII co-doped upconversion nanoparticle nonlinear optical response from single-particle trajectories

Autores
Cavalcante, Isabela N.; Marchi, María Claudia; Sigoli, Fernando A.; de Sousa Filho, Paulo C.; Barja, Beatriz Carmen; Nome, René A.
Año de publicación
2021
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
Spectroscopic characterization of individual nanoparticles is essential for understanding their structure-property relationship and for applications. Upconversion nanoparticles (UCNPs) in condensed phases can undergo both nonlinear optical and stochastic dynamics when interacting with near-infrared sources. By integrating optical trapping microspectroscopy, stochastic dynamics and light-matter interactions experiments and simulations, in the present work we study how individual trajectories of YbIII:ErIII co-doped UCNPs can be used to perform “on the fly” characterization of their nonlinear optical power-law response upon near-infrared excitation. We illustrate the methodology in the case of freely diffusing and optically trapped UCNPs as well as with particles bound to the substrate. The approach presented in this work can be applied to UCNPs with varying composition and morphological features, particularly in single-particle studies.
Fil: Cavalcante, Isabela N.. Universidade Estadual de Campinas; Brasil
Fil: Marchi, María Claudia. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Química, Física de los Materiales, Medioambiente y Energía. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Química, Física de los Materiales, Medioambiente y Energía; Argentina. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Centro de Microscopías Avanzadas; Argentina
Fil: Sigoli, Fernando A.. Universidade Estadual de Campinas; Brasil
Fil: de Sousa Filho, Paulo C.. Universidade Estadual de Campinas; Brasil
Fil: Barja, Beatriz Carmen. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Química, Física de los Materiales, Medioambiente y Energía. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Química, Física de los Materiales, Medioambiente y Energía; Argentina
Fil: Nome, René A.. Universidade Estadual de Campinas; Brasil
Materia
UPCONVERSION NANOPARTICLE
NONLINEAR OPTICAL RESPONSE
SINGLE-PARTICLE TRAJECTORIES
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/182060
Acceder
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network_name_str CONICET Digital (CONICET)
spelling “On the fly” characterization of YbIII:ErIII co-doped upconversion nanoparticle nonlinear optical response from single-particle trajectoriesCavalcante, Isabela N.Marchi, María ClaudiaSigoli, Fernando A.de Sousa Filho, Paulo C.Barja, Beatriz CarmenNome, René A.UPCONVERSION NANOPARTICLENONLINEAR OPTICAL RESPONSESINGLE-PARTICLE TRAJECTORIEShttps://purl.org/becyt/ford/2.10https://purl.org/becyt/ford/2Spectroscopic characterization of individual nanoparticles is essential for understanding their structure-property relationship and for applications. Upconversion nanoparticles (UCNPs) in condensed phases can undergo both nonlinear optical and stochastic dynamics when interacting with near-infrared sources. By integrating optical trapping microspectroscopy, stochastic dynamics and light-matter interactions experiments and simulations, in the present work we study how individual trajectories of YbIII:ErIII co-doped UCNPs can be used to perform “on the fly” characterization of their nonlinear optical power-law response upon near-infrared excitation. We illustrate the methodology in the case of freely diffusing and optically trapped UCNPs as well as with particles bound to the substrate. The approach presented in this work can be applied to UCNPs with varying composition and morphological features, particularly in single-particle studies.Fil: Cavalcante, Isabela N.. Universidade Estadual de Campinas; BrasilFil: Marchi, María Claudia. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Química, Física de los Materiales, Medioambiente y Energía. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Química, Física de los Materiales, Medioambiente y Energía; Argentina. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Centro de Microscopías Avanzadas; ArgentinaFil: Sigoli, Fernando A.. Universidade Estadual de Campinas; BrasilFil: de Sousa Filho, Paulo C.. Universidade Estadual de Campinas; BrasilFil: Barja, Beatriz Carmen. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Química, Física de los Materiales, Medioambiente y Energía. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Química, Física de los Materiales, Medioambiente y Energía; ArgentinaFil: Nome, René A.. Universidade Estadual de Campinas; BrasilChemRxiv2021-05info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/182060Cavalcante, Isabela N.; Marchi, María Claudia; Sigoli, Fernando A.; de Sousa Filho, Paulo C.; Barja, Beatriz Carmen; et al.; “On the fly” characterization of YbIII:ErIII co-doped upconversion nanoparticle nonlinear optical response from single-particle trajectories; ChemRxiv; ChemRxiv; 5-2021; 1-162573-2293CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/doi/10.26434/chemrxiv.14609985info:eu-repo/semantics/altIdentifier/url/https://chemrxiv.org/engage/chemrxiv/article-details/60c758cf567dfe0f75ec6900info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-nd/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T09:32:56Zoai:ri.conicet.gov.ar:11336/182060instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 09:32:57.215CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv “On the fly” characterization of YbIII:ErIII co-doped upconversion nanoparticle nonlinear optical response from single-particle trajectories
title “On the fly” characterization of YbIII:ErIII co-doped upconversion nanoparticle nonlinear optical response from single-particle trajectories
spellingShingle “On the fly” characterization of YbIII:ErIII co-doped upconversion nanoparticle nonlinear optical response from single-particle trajectories
Cavalcante, Isabela N.
UPCONVERSION NANOPARTICLE
NONLINEAR OPTICAL RESPONSE
SINGLE-PARTICLE TRAJECTORIES
title_short “On the fly” characterization of YbIII:ErIII co-doped upconversion nanoparticle nonlinear optical response from single-particle trajectories
title_full “On the fly” characterization of YbIII:ErIII co-doped upconversion nanoparticle nonlinear optical response from single-particle trajectories
title_fullStr “On the fly” characterization of YbIII:ErIII co-doped upconversion nanoparticle nonlinear optical response from single-particle trajectories
title_full_unstemmed “On the fly” characterization of YbIII:ErIII co-doped upconversion nanoparticle nonlinear optical response from single-particle trajectories
title_sort “On the fly” characterization of YbIII:ErIII co-doped upconversion nanoparticle nonlinear optical response from single-particle trajectories
dc.creator.none.fl_str_mv Cavalcante, Isabela N.
Marchi, María Claudia
Sigoli, Fernando A.
de Sousa Filho, Paulo C.
Barja, Beatriz Carmen
Nome, René A.
author Cavalcante, Isabela N.
author_facet Cavalcante, Isabela N.
Marchi, María Claudia
Sigoli, Fernando A.
de Sousa Filho, Paulo C.
Barja, Beatriz Carmen
Nome, René A.
author_role author
author2 Marchi, María Claudia
Sigoli, Fernando A.
de Sousa Filho, Paulo C.
Barja, Beatriz Carmen
Nome, René A.
author2_role author
author
author
author
author
dc.subject.none.fl_str_mv UPCONVERSION NANOPARTICLE
NONLINEAR OPTICAL RESPONSE
SINGLE-PARTICLE TRAJECTORIES
topic UPCONVERSION NANOPARTICLE
NONLINEAR OPTICAL RESPONSE
SINGLE-PARTICLE TRAJECTORIES
purl_subject.fl_str_mv https://purl.org/becyt/ford/2.10
https://purl.org/becyt/ford/2
dc.description.none.fl_txt_mv Spectroscopic characterization of individual nanoparticles is essential for understanding their structure-property relationship and for applications. Upconversion nanoparticles (UCNPs) in condensed phases can undergo both nonlinear optical and stochastic dynamics when interacting with near-infrared sources. By integrating optical trapping microspectroscopy, stochastic dynamics and light-matter interactions experiments and simulations, in the present work we study how individual trajectories of YbIII:ErIII co-doped UCNPs can be used to perform “on the fly” characterization of their nonlinear optical power-law response upon near-infrared excitation. We illustrate the methodology in the case of freely diffusing and optically trapped UCNPs as well as with particles bound to the substrate. The approach presented in this work can be applied to UCNPs with varying composition and morphological features, particularly in single-particle studies.
Fil: Cavalcante, Isabela N.. Universidade Estadual de Campinas; Brasil
Fil: Marchi, María Claudia. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Química, Física de los Materiales, Medioambiente y Energía. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Química, Física de los Materiales, Medioambiente y Energía; Argentina. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Centro de Microscopías Avanzadas; Argentina
Fil: Sigoli, Fernando A.. Universidade Estadual de Campinas; Brasil
Fil: de Sousa Filho, Paulo C.. Universidade Estadual de Campinas; Brasil
Fil: Barja, Beatriz Carmen. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Química, Física de los Materiales, Medioambiente y Energía. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Química, Física de los Materiales, Medioambiente y Energía; Argentina
Fil: Nome, René A.. Universidade Estadual de Campinas; Brasil
description Spectroscopic characterization of individual nanoparticles is essential for understanding their structure-property relationship and for applications. Upconversion nanoparticles (UCNPs) in condensed phases can undergo both nonlinear optical and stochastic dynamics when interacting with near-infrared sources. By integrating optical trapping microspectroscopy, stochastic dynamics and light-matter interactions experiments and simulations, in the present work we study how individual trajectories of YbIII:ErIII co-doped UCNPs can be used to perform “on the fly” characterization of their nonlinear optical power-law response upon near-infrared excitation. We illustrate the methodology in the case of freely diffusing and optically trapped UCNPs as well as with particles bound to the substrate. The approach presented in this work can be applied to UCNPs with varying composition and morphological features, particularly in single-particle studies.
publishDate 2021
dc.date.none.fl_str_mv 2021-05
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/182060
Cavalcante, Isabela N.; Marchi, María Claudia; Sigoli, Fernando A.; de Sousa Filho, Paulo C.; Barja, Beatriz Carmen; et al.; “On the fly” characterization of YbIII:ErIII co-doped upconversion nanoparticle nonlinear optical response from single-particle trajectories; ChemRxiv; ChemRxiv; 5-2021; 1-16
2573-2293
CONICET Digital
CONICET
url http://hdl.handle.net/11336/182060
identifier_str_mv Cavalcante, Isabela N.; Marchi, María Claudia; Sigoli, Fernando A.; de Sousa Filho, Paulo C.; Barja, Beatriz Carmen; et al.; “On the fly” characterization of YbIII:ErIII co-doped upconversion nanoparticle nonlinear optical response from single-particle trajectories; ChemRxiv; ChemRxiv; 5-2021; 1-16
2573-2293
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/doi/10.26434/chemrxiv.14609985
info:eu-repo/semantics/altIdentifier/url/https://chemrxiv.org/engage/chemrxiv/article-details/60c758cf567dfe0f75ec6900
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv ChemRxiv
publisher.none.fl_str_mv ChemRxiv
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 13.070432

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