Magnetic field frustration of the metal-insulator transition in V2 O3

Autores
Trastoy, J.; Camjayi, Alberto; Del Valle, J.; Kalcheim, Y.; Crocombette, J. P.; Gilbert, D.A.; Borchers, J.A.; Villegas, J.E.; Ravelosona, D.; Rozenberg, M.J.; Schuller, Ivan K.
Año de publicación
2020
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
Despite decades of efforts, the origin of metal-insulator transitions (MITs) in strongly correlated materials remains one of the main long-standing problems in condensed-matter physics. An archetypal example is V2O3, which undergoes simultaneous electronic, structural, and magnetic phase transitions. This remarkable feature highlights the many degrees of freedom at play in this material. In this work, acting solely on the magnetic degree of freedom, we reveal an anomalous feature in the electronic transport of V2O3: On cooling, the magnetoresistance changes from positive to negative values well above the MIT temperature, and shows divergent behavior at the transition. The effects are attributed to the magnetic field quenching antiferromagnetic fluctuations above the Néel temperature TN, and preventing long-range antiferromagnetic ordering below TN. In both cases, suppressing the antiferromagnetic ordering prevents the opening of the incipient electronic gap. This interpretation is supported by Hubbard model calculations which fully reproduce the experimental behavior. Our study sheds light on this classic problem providing a clear and physical interpretation of the nature of the metal-insulator transition.
Fil: Trastoy, J.. University of California at San Diego; Estados Unidos
Fil: Camjayi, Alberto. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; Argentina
Fil: Del Valle, J.. University of California at San Diego; Estados Unidos
Fil: Kalcheim, Y.. University of California at San Diego; Estados Unidos
Fil: Crocombette, J. P.. Université Paris-Saclay; Francia
Fil: Gilbert, D.A.. University of Tennessee; Estados Unidos
Fil: Borchers, J.A.. Nist Center For Neutron Research; Estados Unidos
Fil: Villegas, J.E.. Université Paris-Saclay; Francia
Fil: Ravelosona, D.. Center For Nanoscience And Nanotechnology; Francia
Fil: Rozenberg, M.J.. Université Paris-Saclay; Francia
Fil: Schuller, Ivan K.. University of California at San Diego; Estados Unidos
Materia
METAL
INSULATOR
FRUSTRATION
V2O3
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/146094

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spelling Magnetic field frustration of the metal-insulator transition in V2 O3Trastoy, J.Camjayi, AlbertoDel Valle, J.Kalcheim, Y.Crocombette, J. P.Gilbert, D.A.Borchers, J.A.Villegas, J.E.Ravelosona, D.Rozenberg, M.J.Schuller, Ivan K.METALINSULATORFRUSTRATIONV2O3https://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1Despite decades of efforts, the origin of metal-insulator transitions (MITs) in strongly correlated materials remains one of the main long-standing problems in condensed-matter physics. An archetypal example is V2O3, which undergoes simultaneous electronic, structural, and magnetic phase transitions. This remarkable feature highlights the many degrees of freedom at play in this material. In this work, acting solely on the magnetic degree of freedom, we reveal an anomalous feature in the electronic transport of V2O3: On cooling, the magnetoresistance changes from positive to negative values well above the MIT temperature, and shows divergent behavior at the transition. The effects are attributed to the magnetic field quenching antiferromagnetic fluctuations above the Néel temperature TN, and preventing long-range antiferromagnetic ordering below TN. In both cases, suppressing the antiferromagnetic ordering prevents the opening of the incipient electronic gap. This interpretation is supported by Hubbard model calculations which fully reproduce the experimental behavior. Our study sheds light on this classic problem providing a clear and physical interpretation of the nature of the metal-insulator transition.Fil: Trastoy, J.. University of California at San Diego; Estados UnidosFil: Camjayi, Alberto. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; ArgentinaFil: Del Valle, J.. University of California at San Diego; Estados UnidosFil: Kalcheim, Y.. University of California at San Diego; Estados UnidosFil: Crocombette, J. P.. Université Paris-Saclay; FranciaFil: Gilbert, D.A.. University of Tennessee; Estados UnidosFil: Borchers, J.A.. Nist Center For Neutron Research; Estados UnidosFil: Villegas, J.E.. Université Paris-Saclay; FranciaFil: Ravelosona, D.. Center For Nanoscience And Nanotechnology; FranciaFil: Rozenberg, M.J.. Université Paris-Saclay; FranciaFil: Schuller, Ivan K.. University of California at San Diego; Estados UnidosAmerican Physical Society2020-06info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/146094Trastoy, J.; Camjayi, Alberto; Del Valle, J.; Kalcheim, Y.; Crocombette, J. P.; et al.; Magnetic field frustration of the metal-insulator transition in V2 O3; American Physical Society; Physical Review B; 101; 24; 6-2020; 1-62469-9969CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://journals.aps.org/prb/abstract/10.1103/PhysRevB.101.245109info:eu-repo/semantics/altIdentifier/doi/10.1103/PhysRevB.101.245109info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-10-22T11:18:39Zoai:ri.conicet.gov.ar:11336/146094instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-10-22 11:18:39.974CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Magnetic field frustration of the metal-insulator transition in V2 O3
title Magnetic field frustration of the metal-insulator transition in V2 O3
spellingShingle Magnetic field frustration of the metal-insulator transition in V2 O3
Trastoy, J.
METAL
INSULATOR
FRUSTRATION
V2O3
title_short Magnetic field frustration of the metal-insulator transition in V2 O3
title_full Magnetic field frustration of the metal-insulator transition in V2 O3
title_fullStr Magnetic field frustration of the metal-insulator transition in V2 O3
title_full_unstemmed Magnetic field frustration of the metal-insulator transition in V2 O3
title_sort Magnetic field frustration of the metal-insulator transition in V2 O3
dc.creator.none.fl_str_mv Trastoy, J.
Camjayi, Alberto
Del Valle, J.
Kalcheim, Y.
Crocombette, J. P.
Gilbert, D.A.
Borchers, J.A.
Villegas, J.E.
Ravelosona, D.
Rozenberg, M.J.
Schuller, Ivan K.
author Trastoy, J.
author_facet Trastoy, J.
Camjayi, Alberto
Del Valle, J.
Kalcheim, Y.
Crocombette, J. P.
Gilbert, D.A.
Borchers, J.A.
Villegas, J.E.
Ravelosona, D.
Rozenberg, M.J.
Schuller, Ivan K.
author_role author
author2 Camjayi, Alberto
Del Valle, J.
Kalcheim, Y.
Crocombette, J. P.
Gilbert, D.A.
Borchers, J.A.
Villegas, J.E.
Ravelosona, D.
Rozenberg, M.J.
Schuller, Ivan K.
author2_role author
author
author
author
author
author
author
author
author
author
dc.subject.none.fl_str_mv METAL
INSULATOR
FRUSTRATION
V2O3
topic METAL
INSULATOR
FRUSTRATION
V2O3
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv Despite decades of efforts, the origin of metal-insulator transitions (MITs) in strongly correlated materials remains one of the main long-standing problems in condensed-matter physics. An archetypal example is V2O3, which undergoes simultaneous electronic, structural, and magnetic phase transitions. This remarkable feature highlights the many degrees of freedom at play in this material. In this work, acting solely on the magnetic degree of freedom, we reveal an anomalous feature in the electronic transport of V2O3: On cooling, the magnetoresistance changes from positive to negative values well above the MIT temperature, and shows divergent behavior at the transition. The effects are attributed to the magnetic field quenching antiferromagnetic fluctuations above the Néel temperature TN, and preventing long-range antiferromagnetic ordering below TN. In both cases, suppressing the antiferromagnetic ordering prevents the opening of the incipient electronic gap. This interpretation is supported by Hubbard model calculations which fully reproduce the experimental behavior. Our study sheds light on this classic problem providing a clear and physical interpretation of the nature of the metal-insulator transition.
Fil: Trastoy, J.. University of California at San Diego; Estados Unidos
Fil: Camjayi, Alberto. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; Argentina
Fil: Del Valle, J.. University of California at San Diego; Estados Unidos
Fil: Kalcheim, Y.. University of California at San Diego; Estados Unidos
Fil: Crocombette, J. P.. Université Paris-Saclay; Francia
Fil: Gilbert, D.A.. University of Tennessee; Estados Unidos
Fil: Borchers, J.A.. Nist Center For Neutron Research; Estados Unidos
Fil: Villegas, J.E.. Université Paris-Saclay; Francia
Fil: Ravelosona, D.. Center For Nanoscience And Nanotechnology; Francia
Fil: Rozenberg, M.J.. Université Paris-Saclay; Francia
Fil: Schuller, Ivan K.. University of California at San Diego; Estados Unidos
description Despite decades of efforts, the origin of metal-insulator transitions (MITs) in strongly correlated materials remains one of the main long-standing problems in condensed-matter physics. An archetypal example is V2O3, which undergoes simultaneous electronic, structural, and magnetic phase transitions. This remarkable feature highlights the many degrees of freedom at play in this material. In this work, acting solely on the magnetic degree of freedom, we reveal an anomalous feature in the electronic transport of V2O3: On cooling, the magnetoresistance changes from positive to negative values well above the MIT temperature, and shows divergent behavior at the transition. The effects are attributed to the magnetic field quenching antiferromagnetic fluctuations above the Néel temperature TN, and preventing long-range antiferromagnetic ordering below TN. In both cases, suppressing the antiferromagnetic ordering prevents the opening of the incipient electronic gap. This interpretation is supported by Hubbard model calculations which fully reproduce the experimental behavior. Our study sheds light on this classic problem providing a clear and physical interpretation of the nature of the metal-insulator transition.
publishDate 2020
dc.date.none.fl_str_mv 2020-06
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/146094
Trastoy, J.; Camjayi, Alberto; Del Valle, J.; Kalcheim, Y.; Crocombette, J. P.; et al.; Magnetic field frustration of the metal-insulator transition in V2 O3; American Physical Society; Physical Review B; 101; 24; 6-2020; 1-6
2469-9969
CONICET Digital
CONICET
url http://hdl.handle.net/11336/146094
identifier_str_mv Trastoy, J.; Camjayi, Alberto; Del Valle, J.; Kalcheim, Y.; Crocombette, J. P.; et al.; Magnetic field frustration of the metal-insulator transition in V2 O3; American Physical Society; Physical Review B; 101; 24; 6-2020; 1-6
2469-9969
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://journals.aps.org/prb/abstract/10.1103/PhysRevB.101.245109
info:eu-repo/semantics/altIdentifier/doi/10.1103/PhysRevB.101.245109
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv American Physical Society
publisher.none.fl_str_mv American Physical Society
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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