Suppression of ferromagnetic order by Ag-doping: A neutron scattering investigation on Ce2(Pd1-xAgx)2In (x = 0.20, 0.50)

Autores
Martinelli, A.; Giovannini, M.; Sereni, Julian Gustavo Renzo; Ritter, C.
Año de publicación
2018
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
The ground state magnetic behaviour of Ce2(Pd0.8Ag0.2)2In and Ce2(Pd0.5Ag0.5)2In, found in the ferromagnetic branch of Ce2Pd2In, has been investigated by neutron powder diffraction at low temperature. Ce2(Pd0.8Ag0.2)2In is characterized by a ferromagnetic structure with the Ce moments aligned along the c-axis and values of 0.96(2) μB. The compound retains the P4/mbm throughout the magnetic transition, although the magnetic ordering is accompanied by a significant decrease of the lattice strain along [0 0 l], suggesting a magnetostructural contribution. The magnetic behaviour of Ce2(Pd0.5Ag0.5)2In is very different; this compound exhibits an extremely reduced magnetic scattering contribution in the diffraction pattern, that can be ascribed to a different kind of ferromagnetic ordering, with extremely reduced magnetic moments (∼0.1 μB) aligned along [0 l 0]. These results point to a competition between different types of magnetic correlations induced by Ag-substitution, giving rise to a magnetically frustrated scenario in Ce2(Pd0.5Ag0.5)2In.
Fil: Martinelli, A.. Consiglio Nazionale delle Ricerche; Italia
Fil: Giovannini, M.. Università degli Studi di Genova; Italia
Fil: Sereni, Julian Gustavo Renzo. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Ritter, C.. Institut Laue Langevin; Francia
Materia
CE COMPOUND
MAGNETIC FRUSTRATION
MAGNETIC STRUCTURE
NEUTRON DIFFRACTION
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/99490
Acceder
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oai_identifier_str oai:ri.conicet.gov.ar:11336/99490
network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Suppression of ferromagnetic order by Ag-doping: A neutron scattering investigation on Ce2(Pd1-xAgx)2In (x = 0.20, 0.50)Martinelli, A.Giovannini, M.Sereni, Julian Gustavo RenzoRitter, C.CE COMPOUNDMAGNETIC FRUSTRATIONMAGNETIC STRUCTURENEUTRON DIFFRACTIONhttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1The ground state magnetic behaviour of Ce2(Pd0.8Ag0.2)2In and Ce2(Pd0.5Ag0.5)2In, found in the ferromagnetic branch of Ce2Pd2In, has been investigated by neutron powder diffraction at low temperature. Ce2(Pd0.8Ag0.2)2In is characterized by a ferromagnetic structure with the Ce moments aligned along the c-axis and values of 0.96(2) μB. The compound retains the P4/mbm throughout the magnetic transition, although the magnetic ordering is accompanied by a significant decrease of the lattice strain along [0 0 l], suggesting a magnetostructural contribution. The magnetic behaviour of Ce2(Pd0.5Ag0.5)2In is very different; this compound exhibits an extremely reduced magnetic scattering contribution in the diffraction pattern, that can be ascribed to a different kind of ferromagnetic ordering, with extremely reduced magnetic moments (∼0.1 μB) aligned along [0 l 0]. These results point to a competition between different types of magnetic correlations induced by Ag-substitution, giving rise to a magnetically frustrated scenario in Ce2(Pd0.5Ag0.5)2In.Fil: Martinelli, A.. Consiglio Nazionale delle Ricerche; ItaliaFil: Giovannini, M.. Università degli Studi di Genova; ItaliaFil: Sereni, Julian Gustavo Renzo. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaFil: Ritter, C.. Institut Laue Langevin; FranciaIOP Publishing2018-06info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/99490Martinelli, A.; Giovannini, M.; Sereni, Julian Gustavo Renzo; Ritter, C.; Suppression of ferromagnetic order by Ag-doping: A neutron scattering investigation on Ce2(Pd1-xAgx)2In (x = 0.20, 0.50); IOP Publishing; Journal of Physics: Condensed Matter; 30; 26; 6-20180953-8984CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/doi/10.1088/1361-648X/aac79binfo:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-03T09:53:30Zoai:ri.conicet.gov.ar:11336/99490instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-03 09:53:30.568CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Suppression of ferromagnetic order by Ag-doping: A neutron scattering investigation on Ce2(Pd1-xAgx)2In (x = 0.20, 0.50)
title Suppression of ferromagnetic order by Ag-doping: A neutron scattering investigation on Ce2(Pd1-xAgx)2In (x = 0.20, 0.50)
spellingShingle Suppression of ferromagnetic order by Ag-doping: A neutron scattering investigation on Ce2(Pd1-xAgx)2In (x = 0.20, 0.50)
Martinelli, A.
CE COMPOUND
MAGNETIC FRUSTRATION
MAGNETIC STRUCTURE
NEUTRON DIFFRACTION
title_short Suppression of ferromagnetic order by Ag-doping: A neutron scattering investigation on Ce2(Pd1-xAgx)2In (x = 0.20, 0.50)
title_full Suppression of ferromagnetic order by Ag-doping: A neutron scattering investigation on Ce2(Pd1-xAgx)2In (x = 0.20, 0.50)
title_fullStr Suppression of ferromagnetic order by Ag-doping: A neutron scattering investigation on Ce2(Pd1-xAgx)2In (x = 0.20, 0.50)
title_full_unstemmed Suppression of ferromagnetic order by Ag-doping: A neutron scattering investigation on Ce2(Pd1-xAgx)2In (x = 0.20, 0.50)
title_sort Suppression of ferromagnetic order by Ag-doping: A neutron scattering investigation on Ce2(Pd1-xAgx)2In (x = 0.20, 0.50)
dc.creator.none.fl_str_mv Martinelli, A.
Giovannini, M.
Sereni, Julian Gustavo Renzo
Ritter, C.
author Martinelli, A.
author_facet Martinelli, A.
Giovannini, M.
Sereni, Julian Gustavo Renzo
Ritter, C.
author_role author
author2 Giovannini, M.
Sereni, Julian Gustavo Renzo
Ritter, C.
author2_role author
author
author
dc.subject.none.fl_str_mv CE COMPOUND
MAGNETIC FRUSTRATION
MAGNETIC STRUCTURE
NEUTRON DIFFRACTION
topic CE COMPOUND
MAGNETIC FRUSTRATION
MAGNETIC STRUCTURE
NEUTRON DIFFRACTION
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv The ground state magnetic behaviour of Ce2(Pd0.8Ag0.2)2In and Ce2(Pd0.5Ag0.5)2In, found in the ferromagnetic branch of Ce2Pd2In, has been investigated by neutron powder diffraction at low temperature. Ce2(Pd0.8Ag0.2)2In is characterized by a ferromagnetic structure with the Ce moments aligned along the c-axis and values of 0.96(2) μB. The compound retains the P4/mbm throughout the magnetic transition, although the magnetic ordering is accompanied by a significant decrease of the lattice strain along [0 0 l], suggesting a magnetostructural contribution. The magnetic behaviour of Ce2(Pd0.5Ag0.5)2In is very different; this compound exhibits an extremely reduced magnetic scattering contribution in the diffraction pattern, that can be ascribed to a different kind of ferromagnetic ordering, with extremely reduced magnetic moments (∼0.1 μB) aligned along [0 l 0]. These results point to a competition between different types of magnetic correlations induced by Ag-substitution, giving rise to a magnetically frustrated scenario in Ce2(Pd0.5Ag0.5)2In.
Fil: Martinelli, A.. Consiglio Nazionale delle Ricerche; Italia
Fil: Giovannini, M.. Università degli Studi di Genova; Italia
Fil: Sereni, Julian Gustavo Renzo. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Ritter, C.. Institut Laue Langevin; Francia
description The ground state magnetic behaviour of Ce2(Pd0.8Ag0.2)2In and Ce2(Pd0.5Ag0.5)2In, found in the ferromagnetic branch of Ce2Pd2In, has been investigated by neutron powder diffraction at low temperature. Ce2(Pd0.8Ag0.2)2In is characterized by a ferromagnetic structure with the Ce moments aligned along the c-axis and values of 0.96(2) μB. The compound retains the P4/mbm throughout the magnetic transition, although the magnetic ordering is accompanied by a significant decrease of the lattice strain along [0 0 l], suggesting a magnetostructural contribution. The magnetic behaviour of Ce2(Pd0.5Ag0.5)2In is very different; this compound exhibits an extremely reduced magnetic scattering contribution in the diffraction pattern, that can be ascribed to a different kind of ferromagnetic ordering, with extremely reduced magnetic moments (∼0.1 μB) aligned along [0 l 0]. These results point to a competition between different types of magnetic correlations induced by Ag-substitution, giving rise to a magnetically frustrated scenario in Ce2(Pd0.5Ag0.5)2In.
publishDate 2018
dc.date.none.fl_str_mv 2018-06
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/99490
Martinelli, A.; Giovannini, M.; Sereni, Julian Gustavo Renzo; Ritter, C.; Suppression of ferromagnetic order by Ag-doping: A neutron scattering investigation on Ce2(Pd1-xAgx)2In (x = 0.20, 0.50); IOP Publishing; Journal of Physics: Condensed Matter; 30; 26; 6-2018
0953-8984
CONICET Digital
CONICET
url http://hdl.handle.net/11336/99490
identifier_str_mv Martinelli, A.; Giovannini, M.; Sereni, Julian Gustavo Renzo; Ritter, C.; Suppression of ferromagnetic order by Ag-doping: A neutron scattering investigation on Ce2(Pd1-xAgx)2In (x = 0.20, 0.50); IOP Publishing; Journal of Physics: Condensed Matter; 30; 26; 6-2018
0953-8984
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/doi/10.1088/1361-648X/aac79b
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv IOP Publishing
publisher.none.fl_str_mv IOP Publishing
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 13.13397

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