Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope

Autores
Verlhac, Benjamin; Bachellier, N.; Garnier, L.; Ormaza, Maider; Abufager, Paula Natalia; Robles, Robles; Bocquet, Marie Laure; Ternes, Markus; Lorente, Nicolás; Limot, Laurent
Año de publicación
2019
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
Recent advances in scanning probe techniques rely on the chemical functionalization of the probe-tip termination by a single molecule. The success of this approach opens the prospect of introducing spin sensitivity through functionalization by a magnetic molecule. We used a nickelocene-terminated tip (Nc-tip), which offered the possibility of producing spin excitations on the tip apex of a scanning tunneling microscope (STM). When the Nc-tip was 100 picometers away from point contact with a surface-supported object, magnetic effects could be probed through changes in the spin excitation spectrum of nickelocene. We used this detection scheme to simultaneously determine the exchange field and the spin polarization of iron atoms and cobalt films on a copper surface with atomic-scale resolution.
Fil: Verlhac, Benjamin. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia
Fil: Bachellier, N.. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia
Fil: Garnier, L.. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia
Fil: Ormaza, Maider. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia
Fil: Abufager, Paula Natalia. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; Argentina
Fil: Robles, Robles. Consejo Superior de Investigaciones Científicas; España. Universidad del País Vasco; España
Fil: Bocquet, Marie Laure. Ecole Normale Supérieure; Francia
Fil: Ternes, Markus. Helmholtz Gemeinschaft. Forschungszentrum Jülich; Alemania. Aachen University; Alemania
Fil: Lorente, Nicolás. Donostia International Physics Center; España
Fil: Limot, Laurent. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia
Materia
Magnetism
Molecular-tip
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/148780
Acceder
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network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscopeVerlhac, BenjaminBachellier, N.Garnier, L.Ormaza, MaiderAbufager, Paula NataliaRobles, RoblesBocquet, Marie LaureTernes, MarkusLorente, NicolásLimot, LaurentMagnetismMolecular-tiphttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1Recent advances in scanning probe techniques rely on the chemical functionalization of the probe-tip termination by a single molecule. The success of this approach opens the prospect of introducing spin sensitivity through functionalization by a magnetic molecule. We used a nickelocene-terminated tip (Nc-tip), which offered the possibility of producing spin excitations on the tip apex of a scanning tunneling microscope (STM). When the Nc-tip was 100 picometers away from point contact with a surface-supported object, magnetic effects could be probed through changes in the spin excitation spectrum of nickelocene. We used this detection scheme to simultaneously determine the exchange field and the spin polarization of iron atoms and cobalt films on a copper surface with atomic-scale resolution.Fil: Verlhac, Benjamin. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; FranciaFil: Bachellier, N.. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; FranciaFil: Garnier, L.. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; FranciaFil: Ormaza, Maider. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; FranciaFil: Abufager, Paula Natalia. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Robles, Robles. Consejo Superior de Investigaciones Científicas; España. Universidad del País Vasco; EspañaFil: Bocquet, Marie Laure. Ecole Normale Supérieure; FranciaFil: Ternes, Markus. Helmholtz Gemeinschaft. Forschungszentrum Jülich; Alemania. Aachen University; AlemaniaFil: Lorente, Nicolás. Donostia International Physics Center; EspañaFil: Limot, Laurent. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; FranciaAmerican Association for the Advancement of Science2019-11info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/148780Verlhac, Benjamin; Bachellier, N.; Garnier, L.; Ormaza, Maider; Abufager, Paula Natalia; et al.; Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope; American Association for the Advancement of Science; Science; 366; 6465; 11-2019; 623-6270036-8075CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/http://www.sciencemag.org/lookup/doi/10.1126/science.aax8222info:eu-repo/semantics/altIdentifier/doi/10.1126/science.aax8222info:eu-repo/semantics/altIdentifier/url/https://arxiv.org/abs/1901.04862info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-10-22T12:11:42Zoai:ri.conicet.gov.ar:11336/148780instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-10-22 12:11:42.578CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope
title Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope
spellingShingle Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope
Verlhac, Benjamin
Magnetism
Molecular-tip
title_short Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope
title_full Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope
title_fullStr Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope
title_full_unstemmed Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope
title_sort Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope
dc.creator.none.fl_str_mv Verlhac, Benjamin
Bachellier, N.
Garnier, L.
Ormaza, Maider
Abufager, Paula Natalia
Robles, Robles
Bocquet, Marie Laure
Ternes, Markus
Lorente, Nicolás
Limot, Laurent
author Verlhac, Benjamin
author_facet Verlhac, Benjamin
Bachellier, N.
Garnier, L.
Ormaza, Maider
Abufager, Paula Natalia
Robles, Robles
Bocquet, Marie Laure
Ternes, Markus
Lorente, Nicolás
Limot, Laurent
author_role author
author2 Bachellier, N.
Garnier, L.
Ormaza, Maider
Abufager, Paula Natalia
Robles, Robles
Bocquet, Marie Laure
Ternes, Markus
Lorente, Nicolás
Limot, Laurent
author2_role author
author
author
author
author
author
author
author
author
dc.subject.none.fl_str_mv Magnetism
Molecular-tip
topic Magnetism
Molecular-tip
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv Recent advances in scanning probe techniques rely on the chemical functionalization of the probe-tip termination by a single molecule. The success of this approach opens the prospect of introducing spin sensitivity through functionalization by a magnetic molecule. We used a nickelocene-terminated tip (Nc-tip), which offered the possibility of producing spin excitations on the tip apex of a scanning tunneling microscope (STM). When the Nc-tip was 100 picometers away from point contact with a surface-supported object, magnetic effects could be probed through changes in the spin excitation spectrum of nickelocene. We used this detection scheme to simultaneously determine the exchange field and the spin polarization of iron atoms and cobalt films on a copper surface with atomic-scale resolution.
Fil: Verlhac, Benjamin. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia
Fil: Bachellier, N.. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia
Fil: Garnier, L.. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia
Fil: Ormaza, Maider. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia
Fil: Abufager, Paula Natalia. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; Argentina
Fil: Robles, Robles. Consejo Superior de Investigaciones Científicas; España. Universidad del País Vasco; España
Fil: Bocquet, Marie Laure. Ecole Normale Supérieure; Francia
Fil: Ternes, Markus. Helmholtz Gemeinschaft. Forschungszentrum Jülich; Alemania. Aachen University; Alemania
Fil: Lorente, Nicolás. Donostia International Physics Center; España
Fil: Limot, Laurent. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia
description Recent advances in scanning probe techniques rely on the chemical functionalization of the probe-tip termination by a single molecule. The success of this approach opens the prospect of introducing spin sensitivity through functionalization by a magnetic molecule. We used a nickelocene-terminated tip (Nc-tip), which offered the possibility of producing spin excitations on the tip apex of a scanning tunneling microscope (STM). When the Nc-tip was 100 picometers away from point contact with a surface-supported object, magnetic effects could be probed through changes in the spin excitation spectrum of nickelocene. We used this detection scheme to simultaneously determine the exchange field and the spin polarization of iron atoms and cobalt films on a copper surface with atomic-scale resolution.
publishDate 2019
dc.date.none.fl_str_mv 2019-11
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/148780
Verlhac, Benjamin; Bachellier, N.; Garnier, L.; Ormaza, Maider; Abufager, Paula Natalia; et al.; Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope; American Association for the Advancement of Science; Science; 366; 6465; 11-2019; 623-627
0036-8075
CONICET Digital
CONICET
url http://hdl.handle.net/11336/148780
identifier_str_mv Verlhac, Benjamin; Bachellier, N.; Garnier, L.; Ormaza, Maider; Abufager, Paula Natalia; et al.; Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope; American Association for the Advancement of Science; Science; 366; 6465; 11-2019; 623-627
0036-8075
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/http://www.sciencemag.org/lookup/doi/10.1126/science.aax8222
info:eu-repo/semantics/altIdentifier/doi/10.1126/science.aax8222
info:eu-repo/semantics/altIdentifier/url/https://arxiv.org/abs/1901.04862
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
application/pdf
dc.publisher.none.fl_str_mv American Association for the Advancement of Science
publisher.none.fl_str_mv American Association for the Advancement of Science
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
_version_ 1846782510053195776
score 12.982451

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