Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope
- Autores
- Verlhac, Benjamin; Bachellier, N.; Garnier, L.; Ormaza, Maider; Abufager, Paula Natalia; Robles, Robles; Bocquet, Marie Laure; Ternes, Markus; Lorente, Nicolás; Limot, Laurent
- Año de publicación
- 2019
- Idioma
- inglés
- Tipo de recurso
- artículo
- Estado
- versión publicada
- Descripción
- Recent advances in scanning probe techniques rely on the chemical functionalization of the probe-tip termination by a single molecule. The success of this approach opens the prospect of introducing spin sensitivity through functionalization by a magnetic molecule. We used a nickelocene-terminated tip (Nc-tip), which offered the possibility of producing spin excitations on the tip apex of a scanning tunneling microscope (STM). When the Nc-tip was 100 picometers away from point contact with a surface-supported object, magnetic effects could be probed through changes in the spin excitation spectrum of nickelocene. We used this detection scheme to simultaneously determine the exchange field and the spin polarization of iron atoms and cobalt films on a copper surface with atomic-scale resolution.
Fil: Verlhac, Benjamin. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia
Fil: Bachellier, N.. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia
Fil: Garnier, L.. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia
Fil: Ormaza, Maider. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia
Fil: Abufager, Paula Natalia. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; Argentina
Fil: Robles, Robles. Consejo Superior de Investigaciones Científicas; España. Universidad del País Vasco; España
Fil: Bocquet, Marie Laure. Ecole Normale Supérieure; Francia
Fil: Ternes, Markus. Helmholtz Gemeinschaft. Forschungszentrum Jülich; Alemania. Aachen University; Alemania
Fil: Lorente, Nicolás. Donostia International Physics Center; España
Fil: Limot, Laurent. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia - Materia
-
Magnetism
Molecular-tip - Nivel de accesibilidad
- acceso abierto
- Condiciones de uso
- https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
- Repositorio
- Institución
- Consejo Nacional de Investigaciones Científicas y Técnicas
- OAI Identificador
- oai:ri.conicet.gov.ar:11336/148780
Ver los metadatos del registro completo
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Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscopeVerlhac, BenjaminBachellier, N.Garnier, L.Ormaza, MaiderAbufager, Paula NataliaRobles, RoblesBocquet, Marie LaureTernes, MarkusLorente, NicolásLimot, LaurentMagnetismMolecular-tiphttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1Recent advances in scanning probe techniques rely on the chemical functionalization of the probe-tip termination by a single molecule. The success of this approach opens the prospect of introducing spin sensitivity through functionalization by a magnetic molecule. We used a nickelocene-terminated tip (Nc-tip), which offered the possibility of producing spin excitations on the tip apex of a scanning tunneling microscope (STM). When the Nc-tip was 100 picometers away from point contact with a surface-supported object, magnetic effects could be probed through changes in the spin excitation spectrum of nickelocene. We used this detection scheme to simultaneously determine the exchange field and the spin polarization of iron atoms and cobalt films on a copper surface with atomic-scale resolution.Fil: Verlhac, Benjamin. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; FranciaFil: Bachellier, N.. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; FranciaFil: Garnier, L.. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; FranciaFil: Ormaza, Maider. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; FranciaFil: Abufager, Paula Natalia. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Robles, Robles. Consejo Superior de Investigaciones Científicas; España. Universidad del País Vasco; EspañaFil: Bocquet, Marie Laure. Ecole Normale Supérieure; FranciaFil: Ternes, Markus. Helmholtz Gemeinschaft. Forschungszentrum Jülich; Alemania. Aachen University; AlemaniaFil: Lorente, Nicolás. Donostia International Physics Center; EspañaFil: Limot, Laurent. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; FranciaAmerican Association for the Advancement of Science2019-11info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/148780Verlhac, Benjamin; Bachellier, N.; Garnier, L.; Ormaza, Maider; Abufager, Paula Natalia; et al.; Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope; American Association for the Advancement of Science; Science; 366; 6465; 11-2019; 623-6270036-8075CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/http://www.sciencemag.org/lookup/doi/10.1126/science.aax8222info:eu-repo/semantics/altIdentifier/doi/10.1126/science.aax8222info:eu-repo/semantics/altIdentifier/url/https://arxiv.org/abs/1901.04862info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T10:39:25Zoai:ri.conicet.gov.ar:11336/148780instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 10:39:25.548CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse |
dc.title.none.fl_str_mv |
Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope |
title |
Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope |
spellingShingle |
Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope Verlhac, Benjamin Magnetism Molecular-tip |
title_short |
Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope |
title_full |
Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope |
title_fullStr |
Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope |
title_full_unstemmed |
Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope |
title_sort |
Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope |
dc.creator.none.fl_str_mv |
Verlhac, Benjamin Bachellier, N. Garnier, L. Ormaza, Maider Abufager, Paula Natalia Robles, Robles Bocquet, Marie Laure Ternes, Markus Lorente, Nicolás Limot, Laurent |
author |
Verlhac, Benjamin |
author_facet |
Verlhac, Benjamin Bachellier, N. Garnier, L. Ormaza, Maider Abufager, Paula Natalia Robles, Robles Bocquet, Marie Laure Ternes, Markus Lorente, Nicolás Limot, Laurent |
author_role |
author |
author2 |
Bachellier, N. Garnier, L. Ormaza, Maider Abufager, Paula Natalia Robles, Robles Bocquet, Marie Laure Ternes, Markus Lorente, Nicolás Limot, Laurent |
author2_role |
author author author author author author author author author |
dc.subject.none.fl_str_mv |
Magnetism Molecular-tip |
topic |
Magnetism Molecular-tip |
purl_subject.fl_str_mv |
https://purl.org/becyt/ford/1.3 https://purl.org/becyt/ford/1 |
dc.description.none.fl_txt_mv |
Recent advances in scanning probe techniques rely on the chemical functionalization of the probe-tip termination by a single molecule. The success of this approach opens the prospect of introducing spin sensitivity through functionalization by a magnetic molecule. We used a nickelocene-terminated tip (Nc-tip), which offered the possibility of producing spin excitations on the tip apex of a scanning tunneling microscope (STM). When the Nc-tip was 100 picometers away from point contact with a surface-supported object, magnetic effects could be probed through changes in the spin excitation spectrum of nickelocene. We used this detection scheme to simultaneously determine the exchange field and the spin polarization of iron atoms and cobalt films on a copper surface with atomic-scale resolution. Fil: Verlhac, Benjamin. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia Fil: Bachellier, N.. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia Fil: Garnier, L.. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia Fil: Ormaza, Maider. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia Fil: Abufager, Paula Natalia. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; Argentina Fil: Robles, Robles. Consejo Superior de Investigaciones Científicas; España. Universidad del País Vasco; España Fil: Bocquet, Marie Laure. Ecole Normale Supérieure; Francia Fil: Ternes, Markus. Helmholtz Gemeinschaft. Forschungszentrum Jülich; Alemania. Aachen University; Alemania Fil: Lorente, Nicolás. Donostia International Physics Center; España Fil: Limot, Laurent. Université de Strasbourg; Francia. Institut de physique et de chimie des Matériaux de Strasbourg; Francia. Centre National de la Recherche Scientifique; Francia |
description |
Recent advances in scanning probe techniques rely on the chemical functionalization of the probe-tip termination by a single molecule. The success of this approach opens the prospect of introducing spin sensitivity through functionalization by a magnetic molecule. We used a nickelocene-terminated tip (Nc-tip), which offered the possibility of producing spin excitations on the tip apex of a scanning tunneling microscope (STM). When the Nc-tip was 100 picometers away from point contact with a surface-supported object, magnetic effects could be probed through changes in the spin excitation spectrum of nickelocene. We used this detection scheme to simultaneously determine the exchange field and the spin polarization of iron atoms and cobalt films on a copper surface with atomic-scale resolution. |
publishDate |
2019 |
dc.date.none.fl_str_mv |
2019-11 |
dc.type.none.fl_str_mv |
info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion http://purl.org/coar/resource_type/c_6501 info:ar-repo/semantics/articulo |
format |
article |
status_str |
publishedVersion |
dc.identifier.none.fl_str_mv |
http://hdl.handle.net/11336/148780 Verlhac, Benjamin; Bachellier, N.; Garnier, L.; Ormaza, Maider; Abufager, Paula Natalia; et al.; Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope; American Association for the Advancement of Science; Science; 366; 6465; 11-2019; 623-627 0036-8075 CONICET Digital CONICET |
url |
http://hdl.handle.net/11336/148780 |
identifier_str_mv |
Verlhac, Benjamin; Bachellier, N.; Garnier, L.; Ormaza, Maider; Abufager, Paula Natalia; et al.; Atomic-scale spin sensing with a single molecule at the apex of a scanning tunneling microscope; American Association for the Advancement of Science; Science; 366; 6465; 11-2019; 623-627 0036-8075 CONICET Digital CONICET |
dc.language.none.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
info:eu-repo/semantics/altIdentifier/url/http://www.sciencemag.org/lookup/doi/10.1126/science.aax8222 info:eu-repo/semantics/altIdentifier/doi/10.1126/science.aax8222 info:eu-repo/semantics/altIdentifier/url/https://arxiv.org/abs/1901.04862 |
dc.rights.none.fl_str_mv |
info:eu-repo/semantics/openAccess https://creativecommons.org/licenses/by-nc-sa/2.5/ar/ |
eu_rights_str_mv |
openAccess |
rights_invalid_str_mv |
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/ |
dc.format.none.fl_str_mv |
application/pdf application/pdf application/pdf |
dc.publisher.none.fl_str_mv |
American Association for the Advancement of Science |
publisher.none.fl_str_mv |
American Association for the Advancement of Science |
dc.source.none.fl_str_mv |
reponame:CONICET Digital (CONICET) instname:Consejo Nacional de Investigaciones Científicas y Técnicas |
reponame_str |
CONICET Digital (CONICET) |
collection |
CONICET Digital (CONICET) |
instname_str |
Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.name.fl_str_mv |
CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.mail.fl_str_mv |
dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar |
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1844614419203489792 |
score |
13.070432 |