Single spin resonance driven by electric modulation of the g-factor anisotropy

Autores
Ferrón, Alejandro; Rodriguez, Santiago Agustín; Gomez, Sergio Santiago; Lado, Jose Luis; Fernandez Rossier, Joaquín
Año de publicación
2019
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
We address the problem of electronic and nuclear spin resonance of an individual atom on a surface driven by a scanning tunneling microscope. Several mechanisms have been proposed so far, some of them based on the modulation of exchange and crystal field associated with a piezoelectric displacement of the adatom driven by the radio frequency (RF) tip electric field. Here we consider another mechanism, where the piezoelectric displacement modulates the g -factor anisotropy, leading both to electronic and nuclear spin flip transitions. We discuss thoroughly the cases of hydrogenated Ti ( S = 1 / 2 ) and Fe ( S = 2 ) on MgO, relevant for recent experiments. We model the system using two approaches. First, an analytical model that includes crystal field, spin orbit coupling, and hyperfine interactions. Second, we carry out density-functional-based calculations. We find that the modulation of the anisotropy of the g tensor due to the piezoelectric displacement of the atom is an additional mechanism for scanning tunneling microscopy (STM)-based single spin resonance that would be effective in S = 1 / 2 adatoms with large spin orbit coupling. In the case of hydrogenated Ti on MgO, we predict a modulation spin resonance frequency driven by the DC electric field of the tip.
Fil: Ferrón, Alejandro. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Nordeste. Instituto de Modelado e Innovación Tecnológica. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas Naturales y Agrimensura. Instituto de Modelado e Innovación Tecnológica; Argentina. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas y Naturales y Agrimensura. Departamento de Física; Argentina
Fil: Rodriguez, Santiago Agustín. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Nordeste. Instituto de Modelado e Innovación Tecnológica. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas Naturales y Agrimensura. Instituto de Modelado e Innovación Tecnológica; Argentina. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas y Naturales y Agrimensura. Departamento de Física; Argentina
Fil: Gomez, Sergio Santiago. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas y Naturales y Agrimensura. Departamento de Física; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Nordeste. Instituto de Modelado e Innovación Tecnológica. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas Naturales y Agrimensura. Instituto de Modelado e Innovación Tecnológica; Argentina
Fil: Lado, Jose Luis. Aalto University; Finlandia
Fil: Fernandez Rossier, Joaquín. International Iberian Nanotechnology Laboratory; Portugal. Universidad de Alicante; España
Materia
STM
SPINTRONIC
G-FACTOR
ESR
ELECTRONIC STRUCTURE
MAGNETIC ANISOTROPY
SPIN-ORBIT COUPLING
MAGNETISM
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/105972
Acceder
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oai_identifier_str oai:ri.conicet.gov.ar:11336/105972
network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Single spin resonance driven by electric modulation of the g-factor anisotropyFerrón, AlejandroRodriguez, Santiago AgustínGomez, Sergio SantiagoLado, Jose LuisFernandez Rossier, JoaquínSTMSPINTRONICG-FACTORESRELECTRONIC STRUCTUREMAGNETIC ANISOTROPYSPIN-ORBIT COUPLINGMAGNETISMhttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1We address the problem of electronic and nuclear spin resonance of an individual atom on a surface driven by a scanning tunneling microscope. Several mechanisms have been proposed so far, some of them based on the modulation of exchange and crystal field associated with a piezoelectric displacement of the adatom driven by the radio frequency (RF) tip electric field. Here we consider another mechanism, where the piezoelectric displacement modulates the g -factor anisotropy, leading both to electronic and nuclear spin flip transitions. We discuss thoroughly the cases of hydrogenated Ti ( S = 1 / 2 ) and Fe ( S = 2 ) on MgO, relevant for recent experiments. We model the system using two approaches. First, an analytical model that includes crystal field, spin orbit coupling, and hyperfine interactions. Second, we carry out density-functional-based calculations. We find that the modulation of the anisotropy of the g tensor due to the piezoelectric displacement of the atom is an additional mechanism for scanning tunneling microscopy (STM)-based single spin resonance that would be effective in S = 1 / 2 adatoms with large spin orbit coupling. In the case of hydrogenated Ti on MgO, we predict a modulation spin resonance frequency driven by the DC electric field of the tip.Fil: Ferrón, Alejandro. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Nordeste. Instituto de Modelado e Innovación Tecnológica. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas Naturales y Agrimensura. Instituto de Modelado e Innovación Tecnológica; Argentina. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas y Naturales y Agrimensura. Departamento de Física; ArgentinaFil: Rodriguez, Santiago Agustín. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Nordeste. Instituto de Modelado e Innovación Tecnológica. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas Naturales y Agrimensura. Instituto de Modelado e Innovación Tecnológica; Argentina. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas y Naturales y Agrimensura. Departamento de Física; ArgentinaFil: Gomez, Sergio Santiago. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas y Naturales y Agrimensura. Departamento de Física; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Nordeste. Instituto de Modelado e Innovación Tecnológica. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas Naturales y Agrimensura. Instituto de Modelado e Innovación Tecnológica; ArgentinaFil: Lado, Jose Luis. Aalto University; FinlandiaFil: Fernandez Rossier, Joaquín. International Iberian Nanotechnology Laboratory; Portugal. Universidad de Alicante; EspañaAmerican Physical Society2019-12info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/105972Ferrón, Alejandro; Rodriguez, Santiago Agustín; Gomez, Sergio Santiago; Lado, Jose Luis; Fernandez Rossier, Joaquín; Single spin resonance driven by electric modulation of the g-factor anisotropy; American Physical Society; Physical Review Research; 1; 3; 12-2019; 1-152643-1564CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://journals.aps.org/prresearch/abstract/10.1103/PhysRevResearch.1.033185info:eu-repo/semantics/altIdentifier/doi/10.1103/PhysRevResearch.1.033185info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-10-22T11:16:54Zoai:ri.conicet.gov.ar:11336/105972instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-10-22 11:16:55.125CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Single spin resonance driven by electric modulation of the g-factor anisotropy
title Single spin resonance driven by electric modulation of the g-factor anisotropy
spellingShingle Single spin resonance driven by electric modulation of the g-factor anisotropy
Ferrón, Alejandro
STM
SPINTRONIC
G-FACTOR
ESR
ELECTRONIC STRUCTURE
MAGNETIC ANISOTROPY
SPIN-ORBIT COUPLING
MAGNETISM
title_short Single spin resonance driven by electric modulation of the g-factor anisotropy
title_full Single spin resonance driven by electric modulation of the g-factor anisotropy
title_fullStr Single spin resonance driven by electric modulation of the g-factor anisotropy
title_full_unstemmed Single spin resonance driven by electric modulation of the g-factor anisotropy
title_sort Single spin resonance driven by electric modulation of the g-factor anisotropy
dc.creator.none.fl_str_mv Ferrón, Alejandro
Rodriguez, Santiago Agustín
Gomez, Sergio Santiago
Lado, Jose Luis
Fernandez Rossier, Joaquín
author Ferrón, Alejandro
author_facet Ferrón, Alejandro
Rodriguez, Santiago Agustín
Gomez, Sergio Santiago
Lado, Jose Luis
Fernandez Rossier, Joaquín
author_role author
author2 Rodriguez, Santiago Agustín
Gomez, Sergio Santiago
Lado, Jose Luis
Fernandez Rossier, Joaquín
author2_role author
author
author
author
dc.subject.none.fl_str_mv STM
SPINTRONIC
G-FACTOR
ESR
ELECTRONIC STRUCTURE
MAGNETIC ANISOTROPY
SPIN-ORBIT COUPLING
MAGNETISM
topic STM
SPINTRONIC
G-FACTOR
ESR
ELECTRONIC STRUCTURE
MAGNETIC ANISOTROPY
SPIN-ORBIT COUPLING
MAGNETISM
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv We address the problem of electronic and nuclear spin resonance of an individual atom on a surface driven by a scanning tunneling microscope. Several mechanisms have been proposed so far, some of them based on the modulation of exchange and crystal field associated with a piezoelectric displacement of the adatom driven by the radio frequency (RF) tip electric field. Here we consider another mechanism, where the piezoelectric displacement modulates the g -factor anisotropy, leading both to electronic and nuclear spin flip transitions. We discuss thoroughly the cases of hydrogenated Ti ( S = 1 / 2 ) and Fe ( S = 2 ) on MgO, relevant for recent experiments. We model the system using two approaches. First, an analytical model that includes crystal field, spin orbit coupling, and hyperfine interactions. Second, we carry out density-functional-based calculations. We find that the modulation of the anisotropy of the g tensor due to the piezoelectric displacement of the atom is an additional mechanism for scanning tunneling microscopy (STM)-based single spin resonance that would be effective in S = 1 / 2 adatoms with large spin orbit coupling. In the case of hydrogenated Ti on MgO, we predict a modulation spin resonance frequency driven by the DC electric field of the tip.
Fil: Ferrón, Alejandro. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Nordeste. Instituto de Modelado e Innovación Tecnológica. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas Naturales y Agrimensura. Instituto de Modelado e Innovación Tecnológica; Argentina. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas y Naturales y Agrimensura. Departamento de Física; Argentina
Fil: Rodriguez, Santiago Agustín. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Nordeste. Instituto de Modelado e Innovación Tecnológica. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas Naturales y Agrimensura. Instituto de Modelado e Innovación Tecnológica; Argentina. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas y Naturales y Agrimensura. Departamento de Física; Argentina
Fil: Gomez, Sergio Santiago. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas y Naturales y Agrimensura. Departamento de Física; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Nordeste. Instituto de Modelado e Innovación Tecnológica. Universidad Nacional del Nordeste. Facultad de Ciencias Exactas Naturales y Agrimensura. Instituto de Modelado e Innovación Tecnológica; Argentina
Fil: Lado, Jose Luis. Aalto University; Finlandia
Fil: Fernandez Rossier, Joaquín. International Iberian Nanotechnology Laboratory; Portugal. Universidad de Alicante; España
description We address the problem of electronic and nuclear spin resonance of an individual atom on a surface driven by a scanning tunneling microscope. Several mechanisms have been proposed so far, some of them based on the modulation of exchange and crystal field associated with a piezoelectric displacement of the adatom driven by the radio frequency (RF) tip electric field. Here we consider another mechanism, where the piezoelectric displacement modulates the g -factor anisotropy, leading both to electronic and nuclear spin flip transitions. We discuss thoroughly the cases of hydrogenated Ti ( S = 1 / 2 ) and Fe ( S = 2 ) on MgO, relevant for recent experiments. We model the system using two approaches. First, an analytical model that includes crystal field, spin orbit coupling, and hyperfine interactions. Second, we carry out density-functional-based calculations. We find that the modulation of the anisotropy of the g tensor due to the piezoelectric displacement of the atom is an additional mechanism for scanning tunneling microscopy (STM)-based single spin resonance that would be effective in S = 1 / 2 adatoms with large spin orbit coupling. In the case of hydrogenated Ti on MgO, we predict a modulation spin resonance frequency driven by the DC electric field of the tip.
publishDate 2019
dc.date.none.fl_str_mv 2019-12
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/105972
Ferrón, Alejandro; Rodriguez, Santiago Agustín; Gomez, Sergio Santiago; Lado, Jose Luis; Fernandez Rossier, Joaquín; Single spin resonance driven by electric modulation of the g-factor anisotropy; American Physical Society; Physical Review Research; 1; 3; 12-2019; 1-15
2643-1564
CONICET Digital
CONICET
url http://hdl.handle.net/11336/105972
identifier_str_mv Ferrón, Alejandro; Rodriguez, Santiago Agustín; Gomez, Sergio Santiago; Lado, Jose Luis; Fernandez Rossier, Joaquín; Single spin resonance driven by electric modulation of the g-factor anisotropy; American Physical Society; Physical Review Research; 1; 3; 12-2019; 1-15
2643-1564
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://journals.aps.org/prresearch/abstract/10.1103/PhysRevResearch.1.033185
info:eu-repo/semantics/altIdentifier/doi/10.1103/PhysRevResearch.1.033185
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
application/pdf
dc.publisher.none.fl_str_mv American Physical Society
publisher.none.fl_str_mv American Physical Society
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
_version_ 1846781625322438656
score 12.982451

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