Anisotropy-driven topological quantum phase transition in magnetic impurities

Autores
Blesio, Germán Gabriel; Manuel, Luis Oscar; Aligia, Armando Angel
Año de publicación
2024
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
A few years ago, a topological quantum phase transition (TQPT) has been found in Anderson andKondo 2-channel spin-1 impurity models that include a hard-axis anisotropy term DS2 z with D > 0.The most remarkable manifestation of the TQPT is a jump in the spectral density of localizedelectrons, at the Fermi level, from very high to very low values as D is increased. If the twoconduction channels are equivalent, the transition takes place at the critical anisotropyDc ∼ 2.5 TK, where TK is the Kondo temperature for D = 0. This jump might be important todevelop a molecular transistor. The jump is due to a corresponding one in the Luttinger integral,which has a topological non-trivial value π/2 for D > Dc . Here, we review the main results for thespectral density and highlight the significance of the theory for the interpretation of measurementsconducted on magnetic atoms or molecules on metallic surfaces. In these experiments, where D isheld constant, the energy scale TK is manipulated by some parameters. The resulting variation givesrise to a differential conductance dI/dV, measured by scanning-tunneling spectroscopy, which isconsistent with a TQPT at an intermediate value of TK. For non-equivalent channels and non-zeromagnetic field, the topological phase is lost but still a peculiar behaviour in the spectral density isobtained which agrees with experimental observations. We also show that the theory can beextended to integer spin S > 1 and two-impurity systems. This is also probably true for half-integerspin and non-equivalent channels in some cases.
Fil: Blesio, Germán Gabriel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; Argentina
Fil: Manuel, Luis Oscar. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; Argentina
Fil: Aligia, Armando Angel. Comisión Nacional de Energía Atómica. Gerencia del Área de Energía Nuclear. Instituto Balseiro; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Unidad Ejecutora Instituto de Nanociencia y Nanotecnología. Unidad Ejecutora Instituto de Nanociencia y Nanotecnología - Nodo Bariloche | Comisión Nacional de Energía Atómica. Unidad Ejecutora Instituto de Nanociencia y Nanotecnología. Unidad Ejecutora Instituto de Nanociencia y Nanotecnología - Nodo Bariloche; Argentina
Materia
KONDO EFFECT
TOPOLOGICAL PHASE TRANSITION
MAGNETIC ANISOTROPY
NANOSCOPIC SYSTEMS
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/263274

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network_acronym_str CONICETDig
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network_name_str CONICET Digital (CONICET)
spelling Anisotropy-driven topological quantum phase transition in magnetic impuritiesBlesio, Germán GabrielManuel, Luis OscarAligia, Armando AngelKONDO EFFECTTOPOLOGICAL PHASE TRANSITIONMAGNETIC ANISOTROPYNANOSCOPIC SYSTEMShttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1A few years ago, a topological quantum phase transition (TQPT) has been found in Anderson andKondo 2-channel spin-1 impurity models that include a hard-axis anisotropy term DS2 z with D > 0.The most remarkable manifestation of the TQPT is a jump in the spectral density of localizedelectrons, at the Fermi level, from very high to very low values as D is increased. If the twoconduction channels are equivalent, the transition takes place at the critical anisotropyDc ∼ 2.5 TK, where TK is the Kondo temperature for D = 0. This jump might be important todevelop a molecular transistor. The jump is due to a corresponding one in the Luttinger integral,which has a topological non-trivial value π/2 for D > Dc . Here, we review the main results for thespectral density and highlight the significance of the theory for the interpretation of measurementsconducted on magnetic atoms or molecules on metallic surfaces. In these experiments, where D isheld constant, the energy scale TK is manipulated by some parameters. The resulting variation givesrise to a differential conductance dI/dV, measured by scanning-tunneling spectroscopy, which isconsistent with a TQPT at an intermediate value of TK. For non-equivalent channels and non-zeromagnetic field, the topological phase is lost but still a peculiar behaviour in the spectral density isobtained which agrees with experimental observations. We also show that the theory can beextended to integer spin S > 1 and two-impurity systems. This is also probably true for half-integerspin and non-equivalent channels in some cases.Fil: Blesio, Germán Gabriel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Manuel, Luis Oscar. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Aligia, Armando Angel. Comisión Nacional de Energía Atómica. Gerencia del Área de Energía Nuclear. Instituto Balseiro; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Unidad Ejecutora Instituto de Nanociencia y Nanotecnología. Unidad Ejecutora Instituto de Nanociencia y Nanotecnología - Nodo Bariloche | Comisión Nacional de Energía Atómica. Unidad Ejecutora Instituto de Nanociencia y Nanotecnología. Unidad Ejecutora Instituto de Nanociencia y Nanotecnología - Nodo Bariloche; ArgentinaIOP Publishing2024-12info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/263274Blesio, Germán Gabriel; Manuel, Luis Oscar; Aligia, Armando Angel; Anisotropy-driven topological quantum phase transition in magnetic impurities; IOP Publishing; Materials for Quantum Technology; 4; 4; 12-2024; 1-202633-4356CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://iopscience.iop.org/article/10.1088/2633-4356/ada081info:eu-repo/semantics/altIdentifier/doi/10.1088/2633-4356/ada081info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-10T13:02:38Zoai:ri.conicet.gov.ar:11336/263274instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-10 13:02:39.085CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Anisotropy-driven topological quantum phase transition in magnetic impurities
title Anisotropy-driven topological quantum phase transition in magnetic impurities
spellingShingle Anisotropy-driven topological quantum phase transition in magnetic impurities
Blesio, Germán Gabriel
KONDO EFFECT
TOPOLOGICAL PHASE TRANSITION
MAGNETIC ANISOTROPY
NANOSCOPIC SYSTEMS
title_short Anisotropy-driven topological quantum phase transition in magnetic impurities
title_full Anisotropy-driven topological quantum phase transition in magnetic impurities
title_fullStr Anisotropy-driven topological quantum phase transition in magnetic impurities
title_full_unstemmed Anisotropy-driven topological quantum phase transition in magnetic impurities
title_sort Anisotropy-driven topological quantum phase transition in magnetic impurities
dc.creator.none.fl_str_mv Blesio, Germán Gabriel
Manuel, Luis Oscar
Aligia, Armando Angel
author Blesio, Germán Gabriel
author_facet Blesio, Germán Gabriel
Manuel, Luis Oscar
Aligia, Armando Angel
author_role author
author2 Manuel, Luis Oscar
Aligia, Armando Angel
author2_role author
author
dc.subject.none.fl_str_mv KONDO EFFECT
TOPOLOGICAL PHASE TRANSITION
MAGNETIC ANISOTROPY
NANOSCOPIC SYSTEMS
topic KONDO EFFECT
TOPOLOGICAL PHASE TRANSITION
MAGNETIC ANISOTROPY
NANOSCOPIC SYSTEMS
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv A few years ago, a topological quantum phase transition (TQPT) has been found in Anderson andKondo 2-channel spin-1 impurity models that include a hard-axis anisotropy term DS2 z with D > 0.The most remarkable manifestation of the TQPT is a jump in the spectral density of localizedelectrons, at the Fermi level, from very high to very low values as D is increased. If the twoconduction channels are equivalent, the transition takes place at the critical anisotropyDc ∼ 2.5 TK, where TK is the Kondo temperature for D = 0. This jump might be important todevelop a molecular transistor. The jump is due to a corresponding one in the Luttinger integral,which has a topological non-trivial value π/2 for D > Dc . Here, we review the main results for thespectral density and highlight the significance of the theory for the interpretation of measurementsconducted on magnetic atoms or molecules on metallic surfaces. In these experiments, where D isheld constant, the energy scale TK is manipulated by some parameters. The resulting variation givesrise to a differential conductance dI/dV, measured by scanning-tunneling spectroscopy, which isconsistent with a TQPT at an intermediate value of TK. For non-equivalent channels and non-zeromagnetic field, the topological phase is lost but still a peculiar behaviour in the spectral density isobtained which agrees with experimental observations. We also show that the theory can beextended to integer spin S > 1 and two-impurity systems. This is also probably true for half-integerspin and non-equivalent channels in some cases.
Fil: Blesio, Germán Gabriel. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; Argentina
Fil: Manuel, Luis Oscar. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; Argentina
Fil: Aligia, Armando Angel. Comisión Nacional de Energía Atómica. Gerencia del Área de Energía Nuclear. Instituto Balseiro; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Unidad Ejecutora Instituto de Nanociencia y Nanotecnología. Unidad Ejecutora Instituto de Nanociencia y Nanotecnología - Nodo Bariloche | Comisión Nacional de Energía Atómica. Unidad Ejecutora Instituto de Nanociencia y Nanotecnología. Unidad Ejecutora Instituto de Nanociencia y Nanotecnología - Nodo Bariloche; Argentina
description A few years ago, a topological quantum phase transition (TQPT) has been found in Anderson andKondo 2-channel spin-1 impurity models that include a hard-axis anisotropy term DS2 z with D > 0.The most remarkable manifestation of the TQPT is a jump in the spectral density of localizedelectrons, at the Fermi level, from very high to very low values as D is increased. If the twoconduction channels are equivalent, the transition takes place at the critical anisotropyDc ∼ 2.5 TK, where TK is the Kondo temperature for D = 0. This jump might be important todevelop a molecular transistor. The jump is due to a corresponding one in the Luttinger integral,which has a topological non-trivial value π/2 for D > Dc . Here, we review the main results for thespectral density and highlight the significance of the theory for the interpretation of measurementsconducted on magnetic atoms or molecules on metallic surfaces. In these experiments, where D isheld constant, the energy scale TK is manipulated by some parameters. The resulting variation givesrise to a differential conductance dI/dV, measured by scanning-tunneling spectroscopy, which isconsistent with a TQPT at an intermediate value of TK. For non-equivalent channels and non-zeromagnetic field, the topological phase is lost but still a peculiar behaviour in the spectral density isobtained which agrees with experimental observations. We also show that the theory can beextended to integer spin S > 1 and two-impurity systems. This is also probably true for half-integerspin and non-equivalent channels in some cases.
publishDate 2024
dc.date.none.fl_str_mv 2024-12
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/263274
Blesio, Germán Gabriel; Manuel, Luis Oscar; Aligia, Armando Angel; Anisotropy-driven topological quantum phase transition in magnetic impurities; IOP Publishing; Materials for Quantum Technology; 4; 4; 12-2024; 1-20
2633-4356
CONICET Digital
CONICET
url http://hdl.handle.net/11336/263274
identifier_str_mv Blesio, Germán Gabriel; Manuel, Luis Oscar; Aligia, Armando Angel; Anisotropy-driven topological quantum phase transition in magnetic impurities; IOP Publishing; Materials for Quantum Technology; 4; 4; 12-2024; 1-20
2633-4356
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://iopscience.iop.org/article/10.1088/2633-4356/ada081
info:eu-repo/semantics/altIdentifier/doi/10.1088/2633-4356/ada081
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
application/pdf
dc.publisher.none.fl_str_mv IOP Publishing
publisher.none.fl_str_mv IOP Publishing
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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