Searching for suitable catalysts for a passive direct methanol fuel cell cathode
- Autores
- Asteazaran, Mariano; Cespedes, G.; Moreno, Mario Sergio Jesus; Bengió, Silvina; Castro Luna Berenguer, Ana Maria del Carmen
- Año de publicación
- 2015
- Idioma
- inglés
- Tipo de recurso
- artículo
- Estado
- versión publicada
- Descripción
- Trimetallic PtMRu/C cathode catalysts with M = Co or Fe obtained by an impregnation procedure using ethylene glycol and NaBH4 as reducing agent, with suitable activity for the oxygen reduction reaction (ORR) and improved tolerance to methanol, have been physically characterized by HRTEM, EDS and XPS. The examined nanoparticles have a small particle size and are well spread on the carbon support. Pt is mainly found as Pt(0) and Co, Fe and Ru are mostly oxidized. To study their durability and performance for ORR and methanol tolerance over time, the catalysts were subjected to an electrochemical accelerated stress test (AST), consisting in cycling the potential 2000 times. Polarization curves for ORR with and without methanol were recorded. After the AST the trimetallic PtMRu/C catalysts are able to keep their performance for ORR in the presence of methanol.
Fil: Asteazaran, Mariano. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; Argentina
Fil: Cespedes, G.. Universidad Tecnológica Nacional. Facultad Regional La Plata. Centro de Investigación y Desarrollo en Ciencia y Tecnología de Materiales; Argentina
Fil: Moreno, Mario Sergio Jesus. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Bengió, Silvina. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina
Fil: Castro Luna Berenguer, Ana Maria del Carmen. Universidad Tecnológica Nacional. Facultad Regional La Plata. Centro de Investigación y Desarrollo en Ciencia y Tecnología de Materiales; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; Argentina - Materia
-
Methanol Crossover
Methanol Tolerant Catalyst - Nivel de accesibilidad
- acceso abierto
- Condiciones de uso
- https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
- Repositorio
- Institución
- Consejo Nacional de Investigaciones Científicas y Técnicas
- OAI Identificador
- oai:ri.conicet.gov.ar:11336/50157
Ver los metadatos del registro completo
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Searching for suitable catalysts for a passive direct methanol fuel cell cathodeAsteazaran, MarianoCespedes, G.Moreno, Mario Sergio JesusBengió, SilvinaCastro Luna Berenguer, Ana Maria del CarmenMethanol CrossoverMethanol Tolerant Catalysthttps://purl.org/becyt/ford/1.4https://purl.org/becyt/ford/1Trimetallic PtMRu/C cathode catalysts with M = Co or Fe obtained by an impregnation procedure using ethylene glycol and NaBH4 as reducing agent, with suitable activity for the oxygen reduction reaction (ORR) and improved tolerance to methanol, have been physically characterized by HRTEM, EDS and XPS. The examined nanoparticles have a small particle size and are well spread on the carbon support. Pt is mainly found as Pt(0) and Co, Fe and Ru are mostly oxidized. To study their durability and performance for ORR and methanol tolerance over time, the catalysts were subjected to an electrochemical accelerated stress test (AST), consisting in cycling the potential 2000 times. Polarization curves for ORR with and without methanol were recorded. After the AST the trimetallic PtMRu/C catalysts are able to keep their performance for ORR in the presence of methanol.Fil: Asteazaran, Mariano. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; ArgentinaFil: Cespedes, G.. Universidad Tecnológica Nacional. Facultad Regional La Plata. Centro de Investigación y Desarrollo en Ciencia y Tecnología de Materiales; ArgentinaFil: Moreno, Mario Sergio Jesus. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaFil: Bengió, Silvina. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; ArgentinaFil: Castro Luna Berenguer, Ana Maria del Carmen. Universidad Tecnológica Nacional. Facultad Regional La Plata. Centro de Investigación y Desarrollo en Ciencia y Tecnología de Materiales; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; ArgentinaPergamon-Elsevier Science Ltd2015-12info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/50157Asteazaran, Mariano; Cespedes, G.; Moreno, Mario Sergio Jesus; Bengió, Silvina; Castro Luna Berenguer, Ana Maria del Carmen; Searching for suitable catalysts for a passive direct methanol fuel cell cathode; Pergamon-Elsevier Science Ltd; International Journal of Hydrogen Energy; 40; 12-2015; 14632-146390360-3199CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/doi/10.1016/j.ijhydene.2015.05.134info:eu-repo/semantics/altIdentifier/url/https://www.sciencedirect.com/science/article/pii/S0360319915013476info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-nd/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-03T09:48:10Zoai:ri.conicet.gov.ar:11336/50157instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-03 09:48:10.944CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse |
dc.title.none.fl_str_mv |
Searching for suitable catalysts for a passive direct methanol fuel cell cathode |
title |
Searching for suitable catalysts for a passive direct methanol fuel cell cathode |
spellingShingle |
Searching for suitable catalysts for a passive direct methanol fuel cell cathode Asteazaran, Mariano Methanol Crossover Methanol Tolerant Catalyst |
title_short |
Searching for suitable catalysts for a passive direct methanol fuel cell cathode |
title_full |
Searching for suitable catalysts for a passive direct methanol fuel cell cathode |
title_fullStr |
Searching for suitable catalysts for a passive direct methanol fuel cell cathode |
title_full_unstemmed |
Searching for suitable catalysts for a passive direct methanol fuel cell cathode |
title_sort |
Searching for suitable catalysts for a passive direct methanol fuel cell cathode |
dc.creator.none.fl_str_mv |
Asteazaran, Mariano Cespedes, G. Moreno, Mario Sergio Jesus Bengió, Silvina Castro Luna Berenguer, Ana Maria del Carmen |
author |
Asteazaran, Mariano |
author_facet |
Asteazaran, Mariano Cespedes, G. Moreno, Mario Sergio Jesus Bengió, Silvina Castro Luna Berenguer, Ana Maria del Carmen |
author_role |
author |
author2 |
Cespedes, G. Moreno, Mario Sergio Jesus Bengió, Silvina Castro Luna Berenguer, Ana Maria del Carmen |
author2_role |
author author author author |
dc.subject.none.fl_str_mv |
Methanol Crossover Methanol Tolerant Catalyst |
topic |
Methanol Crossover Methanol Tolerant Catalyst |
purl_subject.fl_str_mv |
https://purl.org/becyt/ford/1.4 https://purl.org/becyt/ford/1 |
dc.description.none.fl_txt_mv |
Trimetallic PtMRu/C cathode catalysts with M = Co or Fe obtained by an impregnation procedure using ethylene glycol and NaBH4 as reducing agent, with suitable activity for the oxygen reduction reaction (ORR) and improved tolerance to methanol, have been physically characterized by HRTEM, EDS and XPS. The examined nanoparticles have a small particle size and are well spread on the carbon support. Pt is mainly found as Pt(0) and Co, Fe and Ru are mostly oxidized. To study their durability and performance for ORR and methanol tolerance over time, the catalysts were subjected to an electrochemical accelerated stress test (AST), consisting in cycling the potential 2000 times. Polarization curves for ORR with and without methanol were recorded. After the AST the trimetallic PtMRu/C catalysts are able to keep their performance for ORR in the presence of methanol. Fil: Asteazaran, Mariano. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; Argentina Fil: Cespedes, G.. Universidad Tecnológica Nacional. Facultad Regional La Plata. Centro de Investigación y Desarrollo en Ciencia y Tecnología de Materiales; Argentina Fil: Moreno, Mario Sergio Jesus. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina Fil: Bengió, Silvina. Comisión Nacional de Energía Atómica. Centro Atómico Bariloche; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina Fil: Castro Luna Berenguer, Ana Maria del Carmen. Universidad Tecnológica Nacional. Facultad Regional La Plata. Centro de Investigación y Desarrollo en Ciencia y Tecnología de Materiales; Argentina. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - La Plata. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas. Universidad Nacional de La Plata. Facultad de Ciencias Exactas. Instituto de Investigaciones Fisicoquímicas Teóricas y Aplicadas; Argentina |
description |
Trimetallic PtMRu/C cathode catalysts with M = Co or Fe obtained by an impregnation procedure using ethylene glycol and NaBH4 as reducing agent, with suitable activity for the oxygen reduction reaction (ORR) and improved tolerance to methanol, have been physically characterized by HRTEM, EDS and XPS. The examined nanoparticles have a small particle size and are well spread on the carbon support. Pt is mainly found as Pt(0) and Co, Fe and Ru are mostly oxidized. To study their durability and performance for ORR and methanol tolerance over time, the catalysts were subjected to an electrochemical accelerated stress test (AST), consisting in cycling the potential 2000 times. Polarization curves for ORR with and without methanol were recorded. After the AST the trimetallic PtMRu/C catalysts are able to keep their performance for ORR in the presence of methanol. |
publishDate |
2015 |
dc.date.none.fl_str_mv |
2015-12 |
dc.type.none.fl_str_mv |
info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion http://purl.org/coar/resource_type/c_6501 info:ar-repo/semantics/articulo |
format |
article |
status_str |
publishedVersion |
dc.identifier.none.fl_str_mv |
http://hdl.handle.net/11336/50157 Asteazaran, Mariano; Cespedes, G.; Moreno, Mario Sergio Jesus; Bengió, Silvina; Castro Luna Berenguer, Ana Maria del Carmen; Searching for suitable catalysts for a passive direct methanol fuel cell cathode; Pergamon-Elsevier Science Ltd; International Journal of Hydrogen Energy; 40; 12-2015; 14632-14639 0360-3199 CONICET Digital CONICET |
url |
http://hdl.handle.net/11336/50157 |
identifier_str_mv |
Asteazaran, Mariano; Cespedes, G.; Moreno, Mario Sergio Jesus; Bengió, Silvina; Castro Luna Berenguer, Ana Maria del Carmen; Searching for suitable catalysts for a passive direct methanol fuel cell cathode; Pergamon-Elsevier Science Ltd; International Journal of Hydrogen Energy; 40; 12-2015; 14632-14639 0360-3199 CONICET Digital CONICET |
dc.language.none.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
info:eu-repo/semantics/altIdentifier/doi/10.1016/j.ijhydene.2015.05.134 info:eu-repo/semantics/altIdentifier/url/https://www.sciencedirect.com/science/article/pii/S0360319915013476 |
dc.rights.none.fl_str_mv |
info:eu-repo/semantics/openAccess https://creativecommons.org/licenses/by-nc-nd/2.5/ar/ |
eu_rights_str_mv |
openAccess |
rights_invalid_str_mv |
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/ |
dc.format.none.fl_str_mv |
application/pdf application/pdf application/pdf |
dc.publisher.none.fl_str_mv |
Pergamon-Elsevier Science Ltd |
publisher.none.fl_str_mv |
Pergamon-Elsevier Science Ltd |
dc.source.none.fl_str_mv |
reponame:CONICET Digital (CONICET) instname:Consejo Nacional de Investigaciones Científicas y Técnicas |
reponame_str |
CONICET Digital (CONICET) |
collection |
CONICET Digital (CONICET) |
instname_str |
Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.name.fl_str_mv |
CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.mail.fl_str_mv |
dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar |
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1842268908128567296 |
score |
13.13397 |