Anomalous continuum scattering and higher-order van Hove singularity in the strongly anisotropic S = 1/2 triangular lattice antiferromagnet
- Autores
- Park, Pyeongjae; Ghioldi, Esteban Agustín; May, Andrew F.; Kolopus, James A.; Podlesnyak, Andrey A.; Calder, Stuart; Paddison, Joseph A. M.; Trumper, Adolfo Emilio; Manuel, Luis Oscar; Batista, Cristian D.; Stone, Matthew B.; Halász, Gábor B.; Christianson, Andrew D.
- Año de publicación
- 2024
- Idioma
- inglés
- Tipo de recurso
- artículo
- Estado
- versión publicada
- Descripción
- The S = 1/2 triangular lattice antiferromagnet (TLAF) is a paradigmatic exampleof frustrated quantum magnetism. An ongoing challenge involves under-standing the influence of exchange anisotropy on the collective behaviorwithin such systems. Using inelastic neutron scattering (INS) and advancedcalculation techniques, we have studied the low and high-temperature spindynamics of Ba2La 2CoTe2O 12 (BLCTO): a Co2+-based Jeff = 1/2 TLAF that exhibits120° order below T_ N = 3.26 K. We determined the spin Hamiltonian by fittingthe energy-resolved paramagnetic excitations measured at T > T_N, revealingexceptionally strong easy-plane XXZ anisotropy. Below T_N , the excitationspectrum exhibits a high energy continuum having a larger spectral weightthan the single-magnon modes, suggesting a scenario characterized by a spi-non confinement length that markedly exceeds the lattice spacing. We con-jecture that this phenomenon arises from the proximity to a quantum meltingpoint, even under strong easy-plane XXZ anisotropy. Finally, we highlightcharacteristic flat features in the excitation spectrum, which are connected tohigher-order van Hove singularities in the magnon dispersion directly inducedby easy-plane XXZ anisotropy. Our results provide a rare experimental insightinto the nature of highly anisotropic S = 1/2 TLAFs between the Heisenberg andXY limits.
Fil: Park, Pyeongjae. Oak Ridge National Laboratory; Estados Unidos
Fil: Ghioldi, Esteban Agustín. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; Argentina. University of Tennessee; Estados Unidos
Fil: May, Andrew F.. Oak Ridge National Laboratory; Estados Unidos
Fil: Kolopus, James A.. Oak Ridge National Laboratory; Estados Unidos
Fil: Podlesnyak, Andrey A.. Oak Ridge National Laboratory; Estados Unidos
Fil: Calder, Stuart. Oak Ridge National Laboratory; Estados Unidos
Fil: Paddison, Joseph A. M.. Oak Ridge National Laboratory; Estados Unidos
Fil: Trumper, Adolfo Emilio. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; Argentina
Fil: Manuel, Luis Oscar. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; Argentina
Fil: Batista, Cristian D.. Oak Ridge National Laboratory; Estados Unidos. University of Tennessee; Estados Unidos
Fil: Stone, Matthew B.. Oak Ridge National Laboratory; Estados Unidos
Fil: Halász, Gábor B.. Oak Ridge National Laboratory; Estados Unidos
Fil: Christianson, Andrew D.. Oak Ridge National Laboratory; Estados Unidos - Materia
-
FRUSTRATION
ANTIFERROMAGNETISM
DYNAMICAL STRUCTURE FACTOR
NEUTRON SCATTERING EXPERIMENT - Nivel de accesibilidad
- acceso abierto
- Condiciones de uso
- https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
- Repositorio
- Institución
- Consejo Nacional de Investigaciones Científicas y Técnicas
- OAI Identificador
- oai:ri.conicet.gov.ar:11336/264170
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Anomalous continuum scattering and higher-order van Hove singularity in the strongly anisotropic S = 1/2 triangular lattice antiferromagnetPark, PyeongjaeGhioldi, Esteban AgustínMay, Andrew F.Kolopus, James A.Podlesnyak, Andrey A.Calder, StuartPaddison, Joseph A. M.Trumper, Adolfo EmilioManuel, Luis OscarBatista, Cristian D.Stone, Matthew B.Halász, Gábor B.Christianson, Andrew D.FRUSTRATIONANTIFERROMAGNETISMDYNAMICAL STRUCTURE FACTORNEUTRON SCATTERING EXPERIMENThttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1The S = 1/2 triangular lattice antiferromagnet (TLAF) is a paradigmatic exampleof frustrated quantum magnetism. An ongoing challenge involves under-standing the influence of exchange anisotropy on the collective behaviorwithin such systems. Using inelastic neutron scattering (INS) and advancedcalculation techniques, we have studied the low and high-temperature spindynamics of Ba2La 2CoTe2O 12 (BLCTO): a Co2+-based Jeff = 1/2 TLAF that exhibits120° order below T_ N = 3.26 K. We determined the spin Hamiltonian by fittingthe energy-resolved paramagnetic excitations measured at T > T_N, revealingexceptionally strong easy-plane XXZ anisotropy. Below T_N , the excitationspectrum exhibits a high energy continuum having a larger spectral weightthan the single-magnon modes, suggesting a scenario characterized by a spi-non confinement length that markedly exceeds the lattice spacing. We con-jecture that this phenomenon arises from the proximity to a quantum meltingpoint, even under strong easy-plane XXZ anisotropy. Finally, we highlightcharacteristic flat features in the excitation spectrum, which are connected tohigher-order van Hove singularities in the magnon dispersion directly inducedby easy-plane XXZ anisotropy. Our results provide a rare experimental insightinto the nature of highly anisotropic S = 1/2 TLAFs between the Heisenberg andXY limits.Fil: Park, Pyeongjae. Oak Ridge National Laboratory; Estados UnidosFil: Ghioldi, Esteban Agustín. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; Argentina. University of Tennessee; Estados UnidosFil: May, Andrew F.. Oak Ridge National Laboratory; Estados UnidosFil: Kolopus, James A.. Oak Ridge National Laboratory; Estados UnidosFil: Podlesnyak, Andrey A.. Oak Ridge National Laboratory; Estados UnidosFil: Calder, Stuart. Oak Ridge National Laboratory; Estados UnidosFil: Paddison, Joseph A. M.. Oak Ridge National Laboratory; Estados UnidosFil: Trumper, Adolfo Emilio. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Manuel, Luis Oscar. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; ArgentinaFil: Batista, Cristian D.. Oak Ridge National Laboratory; Estados Unidos. University of Tennessee; Estados UnidosFil: Stone, Matthew B.. Oak Ridge National Laboratory; Estados UnidosFil: Halász, Gábor B.. Oak Ridge National Laboratory; Estados UnidosFil: Christianson, Andrew D.. Oak Ridge National Laboratory; Estados UnidosNature Publishing Group2024-08info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/264170Park, Pyeongjae; Ghioldi, Esteban Agustín; May, Andrew F.; Kolopus, James A.; Podlesnyak, Andrey A.; et al.; Anomalous continuum scattering and higher-order van Hove singularity in the strongly anisotropic S = 1/2 triangular lattice antiferromagnet; Nature Publishing Group; Nature Communications; 15; 1; 8-2024; 7264-72642041-1723CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://www.nature.com/articles/s41467-024-51618-winfo:eu-repo/semantics/altIdentifier/doi/10.1038/s41467-024-51618-winfo:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-nd/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T10:45:27Zoai:ri.conicet.gov.ar:11336/264170instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 10:45:27.328CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse |
dc.title.none.fl_str_mv |
Anomalous continuum scattering and higher-order van Hove singularity in the strongly anisotropic S = 1/2 triangular lattice antiferromagnet |
title |
Anomalous continuum scattering and higher-order van Hove singularity in the strongly anisotropic S = 1/2 triangular lattice antiferromagnet |
spellingShingle |
Anomalous continuum scattering and higher-order van Hove singularity in the strongly anisotropic S = 1/2 triangular lattice antiferromagnet Park, Pyeongjae FRUSTRATION ANTIFERROMAGNETISM DYNAMICAL STRUCTURE FACTOR NEUTRON SCATTERING EXPERIMENT |
title_short |
Anomalous continuum scattering and higher-order van Hove singularity in the strongly anisotropic S = 1/2 triangular lattice antiferromagnet |
title_full |
Anomalous continuum scattering and higher-order van Hove singularity in the strongly anisotropic S = 1/2 triangular lattice antiferromagnet |
title_fullStr |
Anomalous continuum scattering and higher-order van Hove singularity in the strongly anisotropic S = 1/2 triangular lattice antiferromagnet |
title_full_unstemmed |
Anomalous continuum scattering and higher-order van Hove singularity in the strongly anisotropic S = 1/2 triangular lattice antiferromagnet |
title_sort |
Anomalous continuum scattering and higher-order van Hove singularity in the strongly anisotropic S = 1/2 triangular lattice antiferromagnet |
dc.creator.none.fl_str_mv |
Park, Pyeongjae Ghioldi, Esteban Agustín May, Andrew F. Kolopus, James A. Podlesnyak, Andrey A. Calder, Stuart Paddison, Joseph A. M. Trumper, Adolfo Emilio Manuel, Luis Oscar Batista, Cristian D. Stone, Matthew B. Halász, Gábor B. Christianson, Andrew D. |
author |
Park, Pyeongjae |
author_facet |
Park, Pyeongjae Ghioldi, Esteban Agustín May, Andrew F. Kolopus, James A. Podlesnyak, Andrey A. Calder, Stuart Paddison, Joseph A. M. Trumper, Adolfo Emilio Manuel, Luis Oscar Batista, Cristian D. Stone, Matthew B. Halász, Gábor B. Christianson, Andrew D. |
author_role |
author |
author2 |
Ghioldi, Esteban Agustín May, Andrew F. Kolopus, James A. Podlesnyak, Andrey A. Calder, Stuart Paddison, Joseph A. M. Trumper, Adolfo Emilio Manuel, Luis Oscar Batista, Cristian D. Stone, Matthew B. Halász, Gábor B. Christianson, Andrew D. |
author2_role |
author author author author author author author author author author author author |
dc.subject.none.fl_str_mv |
FRUSTRATION ANTIFERROMAGNETISM DYNAMICAL STRUCTURE FACTOR NEUTRON SCATTERING EXPERIMENT |
topic |
FRUSTRATION ANTIFERROMAGNETISM DYNAMICAL STRUCTURE FACTOR NEUTRON SCATTERING EXPERIMENT |
purl_subject.fl_str_mv |
https://purl.org/becyt/ford/1.3 https://purl.org/becyt/ford/1 |
dc.description.none.fl_txt_mv |
The S = 1/2 triangular lattice antiferromagnet (TLAF) is a paradigmatic exampleof frustrated quantum magnetism. An ongoing challenge involves under-standing the influence of exchange anisotropy on the collective behaviorwithin such systems. Using inelastic neutron scattering (INS) and advancedcalculation techniques, we have studied the low and high-temperature spindynamics of Ba2La 2CoTe2O 12 (BLCTO): a Co2+-based Jeff = 1/2 TLAF that exhibits120° order below T_ N = 3.26 K. We determined the spin Hamiltonian by fittingthe energy-resolved paramagnetic excitations measured at T > T_N, revealingexceptionally strong easy-plane XXZ anisotropy. Below T_N , the excitationspectrum exhibits a high energy continuum having a larger spectral weightthan the single-magnon modes, suggesting a scenario characterized by a spi-non confinement length that markedly exceeds the lattice spacing. We con-jecture that this phenomenon arises from the proximity to a quantum meltingpoint, even under strong easy-plane XXZ anisotropy. Finally, we highlightcharacteristic flat features in the excitation spectrum, which are connected tohigher-order van Hove singularities in the magnon dispersion directly inducedby easy-plane XXZ anisotropy. Our results provide a rare experimental insightinto the nature of highly anisotropic S = 1/2 TLAFs between the Heisenberg andXY limits. Fil: Park, Pyeongjae. Oak Ridge National Laboratory; Estados Unidos Fil: Ghioldi, Esteban Agustín. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; Argentina. University of Tennessee; Estados Unidos Fil: May, Andrew F.. Oak Ridge National Laboratory; Estados Unidos Fil: Kolopus, James A.. Oak Ridge National Laboratory; Estados Unidos Fil: Podlesnyak, Andrey A.. Oak Ridge National Laboratory; Estados Unidos Fil: Calder, Stuart. Oak Ridge National Laboratory; Estados Unidos Fil: Paddison, Joseph A. M.. Oak Ridge National Laboratory; Estados Unidos Fil: Trumper, Adolfo Emilio. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; Argentina Fil: Manuel, Luis Oscar. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Rosario. Instituto de Física de Rosario. Universidad Nacional de Rosario. Instituto de Física de Rosario; Argentina Fil: Batista, Cristian D.. Oak Ridge National Laboratory; Estados Unidos. University of Tennessee; Estados Unidos Fil: Stone, Matthew B.. Oak Ridge National Laboratory; Estados Unidos Fil: Halász, Gábor B.. Oak Ridge National Laboratory; Estados Unidos Fil: Christianson, Andrew D.. Oak Ridge National Laboratory; Estados Unidos |
description |
The S = 1/2 triangular lattice antiferromagnet (TLAF) is a paradigmatic exampleof frustrated quantum magnetism. An ongoing challenge involves under-standing the influence of exchange anisotropy on the collective behaviorwithin such systems. Using inelastic neutron scattering (INS) and advancedcalculation techniques, we have studied the low and high-temperature spindynamics of Ba2La 2CoTe2O 12 (BLCTO): a Co2+-based Jeff = 1/2 TLAF that exhibits120° order below T_ N = 3.26 K. We determined the spin Hamiltonian by fittingthe energy-resolved paramagnetic excitations measured at T > T_N, revealingexceptionally strong easy-plane XXZ anisotropy. Below T_N , the excitationspectrum exhibits a high energy continuum having a larger spectral weightthan the single-magnon modes, suggesting a scenario characterized by a spi-non confinement length that markedly exceeds the lattice spacing. We con-jecture that this phenomenon arises from the proximity to a quantum meltingpoint, even under strong easy-plane XXZ anisotropy. Finally, we highlightcharacteristic flat features in the excitation spectrum, which are connected tohigher-order van Hove singularities in the magnon dispersion directly inducedby easy-plane XXZ anisotropy. Our results provide a rare experimental insightinto the nature of highly anisotropic S = 1/2 TLAFs between the Heisenberg andXY limits. |
publishDate |
2024 |
dc.date.none.fl_str_mv |
2024-08 |
dc.type.none.fl_str_mv |
info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion http://purl.org/coar/resource_type/c_6501 info:ar-repo/semantics/articulo |
format |
article |
status_str |
publishedVersion |
dc.identifier.none.fl_str_mv |
http://hdl.handle.net/11336/264170 Park, Pyeongjae; Ghioldi, Esteban Agustín; May, Andrew F.; Kolopus, James A.; Podlesnyak, Andrey A.; et al.; Anomalous continuum scattering and higher-order van Hove singularity in the strongly anisotropic S = 1/2 triangular lattice antiferromagnet; Nature Publishing Group; Nature Communications; 15; 1; 8-2024; 7264-7264 2041-1723 CONICET Digital CONICET |
url |
http://hdl.handle.net/11336/264170 |
identifier_str_mv |
Park, Pyeongjae; Ghioldi, Esteban Agustín; May, Andrew F.; Kolopus, James A.; Podlesnyak, Andrey A.; et al.; Anomalous continuum scattering and higher-order van Hove singularity in the strongly anisotropic S = 1/2 triangular lattice antiferromagnet; Nature Publishing Group; Nature Communications; 15; 1; 8-2024; 7264-7264 2041-1723 CONICET Digital CONICET |
dc.language.none.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
info:eu-repo/semantics/altIdentifier/url/https://www.nature.com/articles/s41467-024-51618-w info:eu-repo/semantics/altIdentifier/doi/10.1038/s41467-024-51618-w |
dc.rights.none.fl_str_mv |
info:eu-repo/semantics/openAccess https://creativecommons.org/licenses/by-nc-nd/2.5/ar/ |
eu_rights_str_mv |
openAccess |
rights_invalid_str_mv |
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/ |
dc.format.none.fl_str_mv |
application/pdf application/pdf application/pdf application/pdf application/pdf |
dc.publisher.none.fl_str_mv |
Nature Publishing Group |
publisher.none.fl_str_mv |
Nature Publishing Group |
dc.source.none.fl_str_mv |
reponame:CONICET Digital (CONICET) instname:Consejo Nacional de Investigaciones Científicas y Técnicas |
reponame_str |
CONICET Digital (CONICET) |
collection |
CONICET Digital (CONICET) |
instname_str |
Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.name.fl_str_mv |
CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.mail.fl_str_mv |
dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar |
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1844614494272094208 |
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13.070432 |