SBR/BiFeO3 Elastomer Capacitor Films Prepared under Magnetic and Electric Fields Displaying Magnetoelectric Coupling
- Autores
- Saleh Medina, Leila María; Jorge, Guillermo Antonio; Rubi, Diego; D'accorso, Norma Beatriz; Negri, Ricardo Martin
- Año de publicación
- 2015
- Idioma
- inglés
- Tipo de recurso
- artículo
- Estado
- versión publicada
- Descripción
- The dielectric properties of elastomer composites formed by dispersions of bismuth ferrite (BiFeO3) multiferroic filler particles in styrene-butadiene rubber (SBR) were studied. The SBR/BiFeO3 films (10-100 μm) were prepared in the presence of electric (E) or magnetic fields (H), showing remarkable characteristics in comparison with systems obtained in its absence. The dispersed multiferroic fillers form clusters of much smaller size when prepared under E or H. The dielectric constant, ε (measured up to 1 MHz), increases with BiFeO3 concentration until reaching saturation. The rise of ε was obtained at concentrations much lower for samples prepared in the presence of E or H than in its absence. Saturation is assigned to connectivity between filler clusters at the largest concentrations, increasing leakage currents and limiting the dielectric behavior. The whole dependence of ε with BiFeO3 concentration was described using a proposed model. The dc resistivities, ρ, increase with BiFeO3 concentration but remain high (ρ ≈ 10 Gω·cm), allowing using the films as capacitors with filter action between 100 kHz and 7 MHz. The films prepared in the presence of H present strong dependence of the ferroelectric response with magnetic fields applied after preparation; that is, electromagnetic coupling was observed in those samples.
Fil: Saleh Medina, Leila María. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Química, Física de los Materiales, Medioambiente y Energía. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Química, Física de los Materiales, Medioambiente y Energía; Argentina
Fil: Jorge, Guillermo Antonio. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Universidad Nacional de General Sarmiento. Instituto de Ciencias; Argentina
Fil: Rubi, Diego. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Comisión Nacional de Energía Atómica. Centro Atómico Constituyentes; Argentina. Universidad Nacional de San Martín. Escuela de Ciencia y Tecnología; Argentina
Fil: D'accorso, Norma Beatriz. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Centro de Investigaciones en Hidratos de Carbono. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Centro de Investigaciones en Hidratos de Carbono; Argentina
Fil: Negri, Ricardo Martin. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Química, Física de los Materiales, Medioambiente y Energía. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Química, Física de los Materiales, Medioambiente y Energía; Argentina - Materia
-
CAPACITORS
ELECTROMAGNETIC COUPLING
BISMUTH FERRITES
STYRENE BUTADYENE RUBBER - Nivel de accesibilidad
- acceso abierto
- Condiciones de uso
- https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
- Repositorio
- Institución
- Consejo Nacional de Investigaciones Científicas y Técnicas
- OAI Identificador
- oai:ri.conicet.gov.ar:11336/78083
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SBR/BiFeO3 Elastomer Capacitor Films Prepared under Magnetic and Electric Fields Displaying Magnetoelectric CouplingSaleh Medina, Leila MaríaJorge, Guillermo AntonioRubi, DiegoD'accorso, Norma BeatrizNegri, Ricardo MartinCAPACITORSELECTROMAGNETIC COUPLINGBISMUTH FERRITESSTYRENE BUTADYENE RUBBERhttps://purl.org/becyt/ford/1.4https://purl.org/becyt/ford/1The dielectric properties of elastomer composites formed by dispersions of bismuth ferrite (BiFeO3) multiferroic filler particles in styrene-butadiene rubber (SBR) were studied. The SBR/BiFeO3 films (10-100 μm) were prepared in the presence of electric (E) or magnetic fields (H), showing remarkable characteristics in comparison with systems obtained in its absence. The dispersed multiferroic fillers form clusters of much smaller size when prepared under E or H. The dielectric constant, ε (measured up to 1 MHz), increases with BiFeO3 concentration until reaching saturation. The rise of ε was obtained at concentrations much lower for samples prepared in the presence of E or H than in its absence. Saturation is assigned to connectivity between filler clusters at the largest concentrations, increasing leakage currents and limiting the dielectric behavior. The whole dependence of ε with BiFeO3 concentration was described using a proposed model. The dc resistivities, ρ, increase with BiFeO3 concentration but remain high (ρ ≈ 10 Gω·cm), allowing using the films as capacitors with filter action between 100 kHz and 7 MHz. The films prepared in the presence of H present strong dependence of the ferroelectric response with magnetic fields applied after preparation; that is, electromagnetic coupling was observed in those samples.Fil: Saleh Medina, Leila María. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Química, Física de los Materiales, Medioambiente y Energía. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Química, Física de los Materiales, Medioambiente y Energía; ArgentinaFil: Jorge, Guillermo Antonio. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Universidad Nacional de General Sarmiento. Instituto de Ciencias; ArgentinaFil: Rubi, Diego. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Comisión Nacional de Energía Atómica. Centro Atómico Constituyentes; Argentina. Universidad Nacional de San Martín. Escuela de Ciencia y Tecnología; ArgentinaFil: D'accorso, Norma Beatriz. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Centro de Investigaciones en Hidratos de Carbono. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Centro de Investigaciones en Hidratos de Carbono; ArgentinaFil: Negri, Ricardo Martin. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Química, Física de los Materiales, Medioambiente y Energía. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Química, Física de los Materiales, Medioambiente y Energía; ArgentinaAmerican Chemical Society2015-10info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/78083Saleh Medina, Leila María; Jorge, Guillermo Antonio; Rubi, Diego; D'accorso, Norma Beatriz; Negri, Ricardo Martin; SBR/BiFeO3 Elastomer Capacitor Films Prepared under Magnetic and Electric Fields Displaying Magnetoelectric Coupling; American Chemical Society; Journal of Physical Chemistry C; 119; 41; 10-2015; 23319-233281932-7447CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/http://pubs.acs.org/doi/10.1021/acs.jpcc.5b06056info:eu-repo/semantics/altIdentifier/doi/10.1021/acs.jpcc.5b06056info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T09:47:45Zoai:ri.conicet.gov.ar:11336/78083instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 09:47:46.257CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse |
dc.title.none.fl_str_mv |
SBR/BiFeO3 Elastomer Capacitor Films Prepared under Magnetic and Electric Fields Displaying Magnetoelectric Coupling |
title |
SBR/BiFeO3 Elastomer Capacitor Films Prepared under Magnetic and Electric Fields Displaying Magnetoelectric Coupling |
spellingShingle |
SBR/BiFeO3 Elastomer Capacitor Films Prepared under Magnetic and Electric Fields Displaying Magnetoelectric Coupling Saleh Medina, Leila María CAPACITORS ELECTROMAGNETIC COUPLING BISMUTH FERRITES STYRENE BUTADYENE RUBBER |
title_short |
SBR/BiFeO3 Elastomer Capacitor Films Prepared under Magnetic and Electric Fields Displaying Magnetoelectric Coupling |
title_full |
SBR/BiFeO3 Elastomer Capacitor Films Prepared under Magnetic and Electric Fields Displaying Magnetoelectric Coupling |
title_fullStr |
SBR/BiFeO3 Elastomer Capacitor Films Prepared under Magnetic and Electric Fields Displaying Magnetoelectric Coupling |
title_full_unstemmed |
SBR/BiFeO3 Elastomer Capacitor Films Prepared under Magnetic and Electric Fields Displaying Magnetoelectric Coupling |
title_sort |
SBR/BiFeO3 Elastomer Capacitor Films Prepared under Magnetic and Electric Fields Displaying Magnetoelectric Coupling |
dc.creator.none.fl_str_mv |
Saleh Medina, Leila María Jorge, Guillermo Antonio Rubi, Diego D'accorso, Norma Beatriz Negri, Ricardo Martin |
author |
Saleh Medina, Leila María |
author_facet |
Saleh Medina, Leila María Jorge, Guillermo Antonio Rubi, Diego D'accorso, Norma Beatriz Negri, Ricardo Martin |
author_role |
author |
author2 |
Jorge, Guillermo Antonio Rubi, Diego D'accorso, Norma Beatriz Negri, Ricardo Martin |
author2_role |
author author author author |
dc.subject.none.fl_str_mv |
CAPACITORS ELECTROMAGNETIC COUPLING BISMUTH FERRITES STYRENE BUTADYENE RUBBER |
topic |
CAPACITORS ELECTROMAGNETIC COUPLING BISMUTH FERRITES STYRENE BUTADYENE RUBBER |
purl_subject.fl_str_mv |
https://purl.org/becyt/ford/1.4 https://purl.org/becyt/ford/1 |
dc.description.none.fl_txt_mv |
The dielectric properties of elastomer composites formed by dispersions of bismuth ferrite (BiFeO3) multiferroic filler particles in styrene-butadiene rubber (SBR) were studied. The SBR/BiFeO3 films (10-100 μm) were prepared in the presence of electric (E) or magnetic fields (H), showing remarkable characteristics in comparison with systems obtained in its absence. The dispersed multiferroic fillers form clusters of much smaller size when prepared under E or H. The dielectric constant, ε (measured up to 1 MHz), increases with BiFeO3 concentration until reaching saturation. The rise of ε was obtained at concentrations much lower for samples prepared in the presence of E or H than in its absence. Saturation is assigned to connectivity between filler clusters at the largest concentrations, increasing leakage currents and limiting the dielectric behavior. The whole dependence of ε with BiFeO3 concentration was described using a proposed model. The dc resistivities, ρ, increase with BiFeO3 concentration but remain high (ρ ≈ 10 Gω·cm), allowing using the films as capacitors with filter action between 100 kHz and 7 MHz. The films prepared in the presence of H present strong dependence of the ferroelectric response with magnetic fields applied after preparation; that is, electromagnetic coupling was observed in those samples. Fil: Saleh Medina, Leila María. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Química, Física de los Materiales, Medioambiente y Energía. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Química, Física de los Materiales, Medioambiente y Energía; Argentina Fil: Jorge, Guillermo Antonio. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Universidad Nacional de General Sarmiento. Instituto de Ciencias; Argentina Fil: Rubi, Diego. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Comisión Nacional de Energía Atómica. Centro Atómico Constituyentes; Argentina. Universidad Nacional de San Martín. Escuela de Ciencia y Tecnología; Argentina Fil: D'accorso, Norma Beatriz. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Centro de Investigaciones en Hidratos de Carbono. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Centro de Investigaciones en Hidratos de Carbono; Argentina Fil: Negri, Ricardo Martin. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Química, Física de los Materiales, Medioambiente y Energía. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Química, Física de los Materiales, Medioambiente y Energía; Argentina |
description |
The dielectric properties of elastomer composites formed by dispersions of bismuth ferrite (BiFeO3) multiferroic filler particles in styrene-butadiene rubber (SBR) were studied. The SBR/BiFeO3 films (10-100 μm) were prepared in the presence of electric (E) or magnetic fields (H), showing remarkable characteristics in comparison with systems obtained in its absence. The dispersed multiferroic fillers form clusters of much smaller size when prepared under E or H. The dielectric constant, ε (measured up to 1 MHz), increases with BiFeO3 concentration until reaching saturation. The rise of ε was obtained at concentrations much lower for samples prepared in the presence of E or H than in its absence. Saturation is assigned to connectivity between filler clusters at the largest concentrations, increasing leakage currents and limiting the dielectric behavior. The whole dependence of ε with BiFeO3 concentration was described using a proposed model. The dc resistivities, ρ, increase with BiFeO3 concentration but remain high (ρ ≈ 10 Gω·cm), allowing using the films as capacitors with filter action between 100 kHz and 7 MHz. The films prepared in the presence of H present strong dependence of the ferroelectric response with magnetic fields applied after preparation; that is, electromagnetic coupling was observed in those samples. |
publishDate |
2015 |
dc.date.none.fl_str_mv |
2015-10 |
dc.type.none.fl_str_mv |
info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion http://purl.org/coar/resource_type/c_6501 info:ar-repo/semantics/articulo |
format |
article |
status_str |
publishedVersion |
dc.identifier.none.fl_str_mv |
http://hdl.handle.net/11336/78083 Saleh Medina, Leila María; Jorge, Guillermo Antonio; Rubi, Diego; D'accorso, Norma Beatriz; Negri, Ricardo Martin; SBR/BiFeO3 Elastomer Capacitor Films Prepared under Magnetic and Electric Fields Displaying Magnetoelectric Coupling; American Chemical Society; Journal of Physical Chemistry C; 119; 41; 10-2015; 23319-23328 1932-7447 CONICET Digital CONICET |
url |
http://hdl.handle.net/11336/78083 |
identifier_str_mv |
Saleh Medina, Leila María; Jorge, Guillermo Antonio; Rubi, Diego; D'accorso, Norma Beatriz; Negri, Ricardo Martin; SBR/BiFeO3 Elastomer Capacitor Films Prepared under Magnetic and Electric Fields Displaying Magnetoelectric Coupling; American Chemical Society; Journal of Physical Chemistry C; 119; 41; 10-2015; 23319-23328 1932-7447 CONICET Digital CONICET |
dc.language.none.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
info:eu-repo/semantics/altIdentifier/url/http://pubs.acs.org/doi/10.1021/acs.jpcc.5b06056 info:eu-repo/semantics/altIdentifier/doi/10.1021/acs.jpcc.5b06056 |
dc.rights.none.fl_str_mv |
info:eu-repo/semantics/openAccess https://creativecommons.org/licenses/by-nc-sa/2.5/ar/ |
eu_rights_str_mv |
openAccess |
rights_invalid_str_mv |
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/ |
dc.format.none.fl_str_mv |
application/pdf application/pdf application/pdf application/pdf application/pdf application/pdf |
dc.publisher.none.fl_str_mv |
American Chemical Society |
publisher.none.fl_str_mv |
American Chemical Society |
dc.source.none.fl_str_mv |
reponame:CONICET Digital (CONICET) instname:Consejo Nacional de Investigaciones Científicas y Técnicas |
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CONICET Digital (CONICET) |
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CONICET Digital (CONICET) |
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Consejo Nacional de Investigaciones Científicas y Técnicas |
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CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.mail.fl_str_mv |
dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar |
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13.070432 |