Hierarchical nanoparticle ensembles synthesized by liquid phase directed self?assembly

Autores
Fowlkes, J. D.; Roberts, N. A.; Wu, Y.; Diez, Javier Alberto; Gonzalez, Alejandro Guillermo; Hartnett, C.; Mahady, K.; Afkhami, K.; Kondic, L.; Rack, P. D.
Año de publicación
2014
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
A liquid metal filament supported on a dielectric substrate was directed to fragment into an ordered, mesoscale particle ensemble. Imposing an undulated surface perturbation on the filament forced the development of a single unstable mode from the otherwise disperse, multimodal Rayleigh−Plateau instability. The imposed mode paved the way for a hierarchical spatial fragmentation of the filament into particles, previously seen only at much larger scales. Ultimately, nanoparticle radius control is demonstrated using a micrometer scale switch.
Fil: Fowlkes, J. D.. Oak Ridge National Laboratory. Center for Nanophase Materials Sciences; Estados Unidos
Fil: Roberts, N. A.. Utah State University. Mechanical and Aerospace Engineering; Estados Unidos
Fil: Wu, Y.. University of Tennessee. Department of Materials Science and Engineering; Estados Unidos
Fil: Diez, Javier Alberto. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Tandil. Centro de Investigaciones En Física E Ingeniería del Centro de la Provincia de Buenos Aires; Argentina. Universidad Nacional del Centro de la Provincia de Buenos Aires. Facultad de Ciencias Exactas. Instituto de Fisica Arroyo Seco; Argentina
Fil: Gonzalez, Alejandro Guillermo. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Tandil. Centro de Investigaciones En Física E Ingeniería del Centro de la Provincia de Buenos Aires; Argentina. Universidad Nacional del Centro de la Provincia de Buenos Aires. Facultad de Ciencias Exactas. Instituto de Fisica Arroyo Seco; Argentina
Fil: Hartnett, C. . University of Tennessee. Department of Physics and Astronomy; Estados Unidos
Fil: Mahady, K.. New Jersey Institute of Technology. Department of Mathematical Sciences; Estados Unidos
Fil: Afkhami, K.. New Jersey Institute of Technology. Department of Mathematical Sciences; Estados Unidos
Fil: Kondic, L.. New Jersey Institute of Technology. Department of Mathematical Sciences; Estados Unidos
Fil: Rack, P. D.. Oak Ridge National Laboratory. Center for Nanophase Materials Sciences; Estados Unidos. University of Tennessee. Department of Materials Science and Engineering; Estados Unidos
Materia
Nanoparticle
Self-Assembly
Rayleigh-Plateau
Filament Breakup
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/4609
Acceder
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network_name_str CONICET Digital (CONICET)
spelling Hierarchical nanoparticle ensembles synthesized by liquid phase directed self?assemblyFowlkes, J. D.Roberts, N. A.Wu, Y.Diez, Javier AlbertoGonzalez, Alejandro GuillermoHartnett, C. Mahady, K.Afkhami, K.Kondic, L.Rack, P. D.NanoparticleSelf-AssemblyRayleigh-PlateauFilament Breakuphttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1A liquid metal filament supported on a dielectric substrate was directed to fragment into an ordered, mesoscale particle ensemble. Imposing an undulated surface perturbation on the filament forced the development of a single unstable mode from the otherwise disperse, multimodal Rayleigh−Plateau instability. The imposed mode paved the way for a hierarchical spatial fragmentation of the filament into particles, previously seen only at much larger scales. Ultimately, nanoparticle radius control is demonstrated using a micrometer scale switch.Fil: Fowlkes, J. D.. Oak Ridge National Laboratory. Center for Nanophase Materials Sciences; Estados UnidosFil: Roberts, N. A.. Utah State University. Mechanical and Aerospace Engineering; Estados UnidosFil: Wu, Y.. University of Tennessee. Department of Materials Science and Engineering; Estados UnidosFil: Diez, Javier Alberto. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Tandil. Centro de Investigaciones En Física E Ingeniería del Centro de la Provincia de Buenos Aires; Argentina. Universidad Nacional del Centro de la Provincia de Buenos Aires. Facultad de Ciencias Exactas. Instituto de Fisica Arroyo Seco; ArgentinaFil: Gonzalez, Alejandro Guillermo. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Tandil. Centro de Investigaciones En Física E Ingeniería del Centro de la Provincia de Buenos Aires; Argentina. Universidad Nacional del Centro de la Provincia de Buenos Aires. Facultad de Ciencias Exactas. Instituto de Fisica Arroyo Seco; ArgentinaFil: Hartnett, C. . University of Tennessee. Department of Physics and Astronomy; Estados UnidosFil: Mahady, K.. New Jersey Institute of Technology. Department of Mathematical Sciences; Estados UnidosFil: Afkhami, K.. New Jersey Institute of Technology. Department of Mathematical Sciences; Estados UnidosFil: Kondic, L.. New Jersey Institute of Technology. Department of Mathematical Sciences; Estados UnidosFil: Rack, P. D.. Oak Ridge National Laboratory. Center for Nanophase Materials Sciences; Estados Unidos. University of Tennessee. Department of Materials Science and Engineering; Estados UnidosAmerican Chemical Society2014-01info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/4609Fowlkes, J. D.; Roberts, N. A.; Wu, Y.; Diez, Javier Alberto; Gonzalez, Alejandro Guillermo; et al.; Hierarchical nanoparticle ensembles synthesized by liquid phase directed self?assembly; American Chemical Society; Nano Letters; 14; 2; 1-2014; 774-7821530-6984enginfo:eu-repo/semantics/altIdentifier/url/http://pubs.acs.org/doi/abs/10.1021/nl404128dinfo:eu-repo/semantics/altIdentifier/doi/10.1021/nl404128dinfo:eu-repo/semantics/altIdentifier/issn/1530-6984info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-10T13:20:05Zoai:ri.conicet.gov.ar:11336/4609instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-10 13:20:06.089CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Hierarchical nanoparticle ensembles synthesized by liquid phase directed self?assembly
title Hierarchical nanoparticle ensembles synthesized by liquid phase directed self?assembly
spellingShingle Hierarchical nanoparticle ensembles synthesized by liquid phase directed self?assembly
Fowlkes, J. D.
Nanoparticle
Self-Assembly
Rayleigh-Plateau
Filament Breakup
title_short Hierarchical nanoparticle ensembles synthesized by liquid phase directed self?assembly
title_full Hierarchical nanoparticle ensembles synthesized by liquid phase directed self?assembly
title_fullStr Hierarchical nanoparticle ensembles synthesized by liquid phase directed self?assembly
title_full_unstemmed Hierarchical nanoparticle ensembles synthesized by liquid phase directed self?assembly
title_sort Hierarchical nanoparticle ensembles synthesized by liquid phase directed self?assembly
dc.creator.none.fl_str_mv Fowlkes, J. D.
Roberts, N. A.
Wu, Y.
Diez, Javier Alberto
Gonzalez, Alejandro Guillermo
Hartnett, C.
Mahady, K.
Afkhami, K.
Kondic, L.
Rack, P. D.
author Fowlkes, J. D.
author_facet Fowlkes, J. D.
Roberts, N. A.
Wu, Y.
Diez, Javier Alberto
Gonzalez, Alejandro Guillermo
Hartnett, C.
Mahady, K.
Afkhami, K.
Kondic, L.
Rack, P. D.
author_role author
author2 Roberts, N. A.
Wu, Y.
Diez, Javier Alberto
Gonzalez, Alejandro Guillermo
Hartnett, C.
Mahady, K.
Afkhami, K.
Kondic, L.
Rack, P. D.
author2_role author
author
author
author
author
author
author
author
author
dc.subject.none.fl_str_mv Nanoparticle
Self-Assembly
Rayleigh-Plateau
Filament Breakup
topic Nanoparticle
Self-Assembly
Rayleigh-Plateau
Filament Breakup
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv A liquid metal filament supported on a dielectric substrate was directed to fragment into an ordered, mesoscale particle ensemble. Imposing an undulated surface perturbation on the filament forced the development of a single unstable mode from the otherwise disperse, multimodal Rayleigh−Plateau instability. The imposed mode paved the way for a hierarchical spatial fragmentation of the filament into particles, previously seen only at much larger scales. Ultimately, nanoparticle radius control is demonstrated using a micrometer scale switch.
Fil: Fowlkes, J. D.. Oak Ridge National Laboratory. Center for Nanophase Materials Sciences; Estados Unidos
Fil: Roberts, N. A.. Utah State University. Mechanical and Aerospace Engineering; Estados Unidos
Fil: Wu, Y.. University of Tennessee. Department of Materials Science and Engineering; Estados Unidos
Fil: Diez, Javier Alberto. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Tandil. Centro de Investigaciones En Física E Ingeniería del Centro de la Provincia de Buenos Aires; Argentina. Universidad Nacional del Centro de la Provincia de Buenos Aires. Facultad de Ciencias Exactas. Instituto de Fisica Arroyo Seco; Argentina
Fil: Gonzalez, Alejandro Guillermo. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Tandil. Centro de Investigaciones En Física E Ingeniería del Centro de la Provincia de Buenos Aires; Argentina. Universidad Nacional del Centro de la Provincia de Buenos Aires. Facultad de Ciencias Exactas. Instituto de Fisica Arroyo Seco; Argentina
Fil: Hartnett, C. . University of Tennessee. Department of Physics and Astronomy; Estados Unidos
Fil: Mahady, K.. New Jersey Institute of Technology. Department of Mathematical Sciences; Estados Unidos
Fil: Afkhami, K.. New Jersey Institute of Technology. Department of Mathematical Sciences; Estados Unidos
Fil: Kondic, L.. New Jersey Institute of Technology. Department of Mathematical Sciences; Estados Unidos
Fil: Rack, P. D.. Oak Ridge National Laboratory. Center for Nanophase Materials Sciences; Estados Unidos. University of Tennessee. Department of Materials Science and Engineering; Estados Unidos
description A liquid metal filament supported on a dielectric substrate was directed to fragment into an ordered, mesoscale particle ensemble. Imposing an undulated surface perturbation on the filament forced the development of a single unstable mode from the otherwise disperse, multimodal Rayleigh−Plateau instability. The imposed mode paved the way for a hierarchical spatial fragmentation of the filament into particles, previously seen only at much larger scales. Ultimately, nanoparticle radius control is demonstrated using a micrometer scale switch.
publishDate 2014
dc.date.none.fl_str_mv 2014-01
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/4609
Fowlkes, J. D.; Roberts, N. A.; Wu, Y.; Diez, Javier Alberto; Gonzalez, Alejandro Guillermo; et al.; Hierarchical nanoparticle ensembles synthesized by liquid phase directed self?assembly; American Chemical Society; Nano Letters; 14; 2; 1-2014; 774-782
1530-6984
url http://hdl.handle.net/11336/4609
identifier_str_mv Fowlkes, J. D.; Roberts, N. A.; Wu, Y.; Diez, Javier Alberto; Gonzalez, Alejandro Guillermo; et al.; Hierarchical nanoparticle ensembles synthesized by liquid phase directed self?assembly; American Chemical Society; Nano Letters; 14; 2; 1-2014; 774-782
1530-6984
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/http://pubs.acs.org/doi/abs/10.1021/nl404128d
info:eu-repo/semantics/altIdentifier/doi/10.1021/nl404128d
info:eu-repo/semantics/altIdentifier/issn/1530-6984
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv American Chemical Society
publisher.none.fl_str_mv American Chemical Society
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
_version_ 1842981100902678528
score 12.48226

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