Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments

Autores
Brinks, Daan; Hildner, Richard; Stefani, Fernando Daniel; Van Hulst, Niek F.
Año de publicación
2011
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
Diffraction of finite sized laser beams imposes a limit on the control that can be exerted over ultrafast pulses. This limit manifests as spatio-temporal coupling induced in standard implementations of pulse shaping schemes. We demonstrate the influence this has on coherent control experiments that depend on finite excitation, sample, and detection volumes. Based on solutions used in pulse stretching experiments, we introduce a double-pass scheme that reduces the errors produced through spatio-temporal coupling by at least one order of magnitude. Finally, employing single molecules as nanoscale probes, we prove that such a double pass scheme is capable of artifact-free pulse shaping at dimensions two orders of magnitude smaller than the diffraction limit.
Fil: Brinks, Daan. Institut de Ciencies Fotoniques; España
Fil: Hildner, Richard. Institut de Ciencies Fotoniques; España. University of Bayreuth; Alemania
Fil: Stefani, Fernando Daniel. Institut de Ciencies Fotoniques; España. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Parque Centenario. Centro de Investigaciones en Bionanociencias "Elizabeth Jares Erijman"; Argentina
Fil: Van Hulst, Niek F.. Universidad de Barcelona. Institució Catalana de Recerca i Estudis Avançats; España. Institut de Ciencies Fotoniques; España
Materia
ultrafast spectroscopy
pulse shaper
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/68943
Acceder
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oai_identifier_str oai:ri.conicet.gov.ar:11336/68943
network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experimentsBrinks, DaanHildner, RichardStefani, Fernando DanielVan Hulst, Niek F.ultrafast spectroscopypulse shaperhttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1Diffraction of finite sized laser beams imposes a limit on the control that can be exerted over ultrafast pulses. This limit manifests as spatio-temporal coupling induced in standard implementations of pulse shaping schemes. We demonstrate the influence this has on coherent control experiments that depend on finite excitation, sample, and detection volumes. Based on solutions used in pulse stretching experiments, we introduce a double-pass scheme that reduces the errors produced through spatio-temporal coupling by at least one order of magnitude. Finally, employing single molecules as nanoscale probes, we prove that such a double pass scheme is capable of artifact-free pulse shaping at dimensions two orders of magnitude smaller than the diffraction limit.Fil: Brinks, Daan. Institut de Ciencies Fotoniques; EspañaFil: Hildner, Richard. Institut de Ciencies Fotoniques; España. University of Bayreuth; AlemaniaFil: Stefani, Fernando Daniel. Institut de Ciencies Fotoniques; España. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Parque Centenario. Centro de Investigaciones en Bionanociencias "Elizabeth Jares Erijman"; ArgentinaFil: Van Hulst, Niek F.. Universidad de Barcelona. Institució Catalana de Recerca i Estudis Avançats; España. Institut de Ciencies Fotoniques; EspañaOptical Society of America2011-12info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/68943Brinks, Daan; Hildner, Richard; Stefani, Fernando Daniel; Van Hulst, Niek F.; Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments; Optical Society of America; Optics Express; 19; 27; 12-2011; 26486-264991094-4087CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://www.osapublishing.org/oe/abstract.cfm?uri=oe-19-27-26486info:eu-repo/semantics/altIdentifier/doi/10.1364/OE.19.026486info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-17T11:40:17Zoai:ri.conicet.gov.ar:11336/68943instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-17 11:40:17.431CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments
title Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments
spellingShingle Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments
Brinks, Daan
ultrafast spectroscopy
pulse shaper
title_short Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments
title_full Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments
title_fullStr Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments
title_full_unstemmed Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments
title_sort Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments
dc.creator.none.fl_str_mv Brinks, Daan
Hildner, Richard
Stefani, Fernando Daniel
Van Hulst, Niek F.
author Brinks, Daan
author_facet Brinks, Daan
Hildner, Richard
Stefani, Fernando Daniel
Van Hulst, Niek F.
author_role author
author2 Hildner, Richard
Stefani, Fernando Daniel
Van Hulst, Niek F.
author2_role author
author
author
dc.subject.none.fl_str_mv ultrafast spectroscopy
pulse shaper
topic ultrafast spectroscopy
pulse shaper
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv Diffraction of finite sized laser beams imposes a limit on the control that can be exerted over ultrafast pulses. This limit manifests as spatio-temporal coupling induced in standard implementations of pulse shaping schemes. We demonstrate the influence this has on coherent control experiments that depend on finite excitation, sample, and detection volumes. Based on solutions used in pulse stretching experiments, we introduce a double-pass scheme that reduces the errors produced through spatio-temporal coupling by at least one order of magnitude. Finally, employing single molecules as nanoscale probes, we prove that such a double pass scheme is capable of artifact-free pulse shaping at dimensions two orders of magnitude smaller than the diffraction limit.
Fil: Brinks, Daan. Institut de Ciencies Fotoniques; España
Fil: Hildner, Richard. Institut de Ciencies Fotoniques; España. University of Bayreuth; Alemania
Fil: Stefani, Fernando Daniel. Institut de Ciencies Fotoniques; España. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Parque Centenario. Centro de Investigaciones en Bionanociencias "Elizabeth Jares Erijman"; Argentina
Fil: Van Hulst, Niek F.. Universidad de Barcelona. Institució Catalana de Recerca i Estudis Avançats; España. Institut de Ciencies Fotoniques; España
description Diffraction of finite sized laser beams imposes a limit on the control that can be exerted over ultrafast pulses. This limit manifests as spatio-temporal coupling induced in standard implementations of pulse shaping schemes. We demonstrate the influence this has on coherent control experiments that depend on finite excitation, sample, and detection volumes. Based on solutions used in pulse stretching experiments, we introduce a double-pass scheme that reduces the errors produced through spatio-temporal coupling by at least one order of magnitude. Finally, employing single molecules as nanoscale probes, we prove that such a double pass scheme is capable of artifact-free pulse shaping at dimensions two orders of magnitude smaller than the diffraction limit.
publishDate 2011
dc.date.none.fl_str_mv 2011-12
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/68943
Brinks, Daan; Hildner, Richard; Stefani, Fernando Daniel; Van Hulst, Niek F.; Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments; Optical Society of America; Optics Express; 19; 27; 12-2011; 26486-26499
1094-4087
CONICET Digital
CONICET
url http://hdl.handle.net/11336/68943
identifier_str_mv Brinks, Daan; Hildner, Richard; Stefani, Fernando Daniel; Van Hulst, Niek F.; Beating spatio-temporal coupling: Implications for pulse shaping and coherent control experiments; Optical Society of America; Optics Express; 19; 27; 12-2011; 26486-26499
1094-4087
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://www.osapublishing.org/oe/abstract.cfm?uri=oe-19-27-26486
info:eu-repo/semantics/altIdentifier/doi/10.1364/OE.19.026486
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv Optical Society of America
publisher.none.fl_str_mv Optical Society of America
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 13.001348

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