Experimental analysis of density fingering instability modified by precipitation

Autores
Binda, Leonardo David; El Hasi, Claudio Daniel; Zalts, Anita; D'onofrio, Alejandro Gustavo
Año de publicación
2017
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
We analyze the effect of precipitate formation on the development of density induced hydrodynamic instabilities. In this case the precipitate is BaCO3, obtained by reaction of CO2 with aqueous BaCl2. CO2(g) dissolution increases the local density of the aqueous phase, triggering Rayleigh ?Taylor instabilities and BaCO3 formation. It was observed that at first the precipitate was formed at the finger front. As the particles became bigger, they began to fall down from the front. These particles were used as tracers using PIV technique to visualize the particle streamlines and to obtain the velocity of that movement. This falling produced a downwards flow that might increase the mixing zone. Contrary to expectations, it was observed that finger length decreased, indicating that for the mixing zone development, the consumption of CO2 to form the precipitate is more important than the downwards flow. The mixing zone length was recovered increasing the availability of the reactant (higher CO2 partial pressure), compensating the CO2 used for BaCO3 formation. Mixing zone development rates reached constant values at shorter times when the precipitate is absent than when it is present. An analysis of the non linear regime with and without the precipitate is performed.
Fil: Binda, Leonardo David. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Universidad de Buenos Aires. Facultad de Ingeniería. Departamento de Física. Grupo de Medios Porosos; Argentina. Universidad Nacional de General Sarmiento; Argentina
Fil: El Hasi, Claudio Daniel. Universidad Nacional de General Sarmiento; Argentina
Fil: Zalts, Anita. Universidad Nacional de General Sarmiento; Argentina
Fil: D'onofrio, Alejandro Gustavo. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Universidad de Buenos Aires. Facultad de Ingeniería. Departamento de Física. Grupo de Medios Porosos; Argentina
Materia
Instabilities
Co2
Hele-Shaw
Precipitation
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/40914
Acceder
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oai_identifier_str oai:ri.conicet.gov.ar:11336/40914
network_acronym_str CONICETDig
repository_id_str 3498
network_name_str CONICET Digital (CONICET)
spelling Experimental analysis of density fingering instability modified by precipitationBinda, Leonardo DavidEl Hasi, Claudio DanielZalts, AnitaD'onofrio, Alejandro GustavoInstabilitiesCo2Hele-ShawPrecipitationhttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1We analyze the effect of precipitate formation on the development of density induced hydrodynamic instabilities. In this case the precipitate is BaCO3, obtained by reaction of CO2 with aqueous BaCl2. CO2(g) dissolution increases the local density of the aqueous phase, triggering Rayleigh ?Taylor instabilities and BaCO3 formation. It was observed that at first the precipitate was formed at the finger front. As the particles became bigger, they began to fall down from the front. These particles were used as tracers using PIV technique to visualize the particle streamlines and to obtain the velocity of that movement. This falling produced a downwards flow that might increase the mixing zone. Contrary to expectations, it was observed that finger length decreased, indicating that for the mixing zone development, the consumption of CO2 to form the precipitate is more important than the downwards flow. The mixing zone length was recovered increasing the availability of the reactant (higher CO2 partial pressure), compensating the CO2 used for BaCO3 formation. Mixing zone development rates reached constant values at shorter times when the precipitate is absent than when it is present. An analysis of the non linear regime with and without the precipitate is performed.Fil: Binda, Leonardo David. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Universidad de Buenos Aires. Facultad de Ingeniería. Departamento de Física. Grupo de Medios Porosos; Argentina. Universidad Nacional de General Sarmiento; ArgentinaFil: El Hasi, Claudio Daniel. Universidad Nacional de General Sarmiento; ArgentinaFil: Zalts, Anita. Universidad Nacional de General Sarmiento; ArgentinaFil: D'onofrio, Alejandro Gustavo. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Universidad de Buenos Aires. Facultad de Ingeniería. Departamento de Física. Grupo de Medios Porosos; ArgentinaAmerican Institute of Physics2017-05info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/40914Binda, Leonardo David; El Hasi, Claudio Daniel; Zalts, Anita; D'onofrio, Alejandro Gustavo; Experimental analysis of density fingering instability modified by precipitation; American Institute of Physics; Chaos; 27; 5; 5-2017; 1-71054-1500CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/doi/10.1063/1.4983670info:eu-repo/semantics/altIdentifier/url/https://aip.scitation.org/doi/10.1063/1.4983670info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-03T09:49:14Zoai:ri.conicet.gov.ar:11336/40914instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-03 09:49:14.383CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Experimental analysis of density fingering instability modified by precipitation
title Experimental analysis of density fingering instability modified by precipitation
spellingShingle Experimental analysis of density fingering instability modified by precipitation
Binda, Leonardo David
Instabilities
Co2
Hele-Shaw
Precipitation
title_short Experimental analysis of density fingering instability modified by precipitation
title_full Experimental analysis of density fingering instability modified by precipitation
title_fullStr Experimental analysis of density fingering instability modified by precipitation
title_full_unstemmed Experimental analysis of density fingering instability modified by precipitation
title_sort Experimental analysis of density fingering instability modified by precipitation
dc.creator.none.fl_str_mv Binda, Leonardo David
El Hasi, Claudio Daniel
Zalts, Anita
D'onofrio, Alejandro Gustavo
author Binda, Leonardo David
author_facet Binda, Leonardo David
El Hasi, Claudio Daniel
Zalts, Anita
D'onofrio, Alejandro Gustavo
author_role author
author2 El Hasi, Claudio Daniel
Zalts, Anita
D'onofrio, Alejandro Gustavo
author2_role author
author
author
dc.subject.none.fl_str_mv Instabilities
Co2
Hele-Shaw
Precipitation
topic Instabilities
Co2
Hele-Shaw
Precipitation
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv We analyze the effect of precipitate formation on the development of density induced hydrodynamic instabilities. In this case the precipitate is BaCO3, obtained by reaction of CO2 with aqueous BaCl2. CO2(g) dissolution increases the local density of the aqueous phase, triggering Rayleigh ?Taylor instabilities and BaCO3 formation. It was observed that at first the precipitate was formed at the finger front. As the particles became bigger, they began to fall down from the front. These particles were used as tracers using PIV technique to visualize the particle streamlines and to obtain the velocity of that movement. This falling produced a downwards flow that might increase the mixing zone. Contrary to expectations, it was observed that finger length decreased, indicating that for the mixing zone development, the consumption of CO2 to form the precipitate is more important than the downwards flow. The mixing zone length was recovered increasing the availability of the reactant (higher CO2 partial pressure), compensating the CO2 used for BaCO3 formation. Mixing zone development rates reached constant values at shorter times when the precipitate is absent than when it is present. An analysis of the non linear regime with and without the precipitate is performed.
Fil: Binda, Leonardo David. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Universidad de Buenos Aires. Facultad de Ingeniería. Departamento de Física. Grupo de Medios Porosos; Argentina. Universidad Nacional de General Sarmiento; Argentina
Fil: El Hasi, Claudio Daniel. Universidad Nacional de General Sarmiento; Argentina
Fil: Zalts, Anita. Universidad Nacional de General Sarmiento; Argentina
Fil: D'onofrio, Alejandro Gustavo. Consejo Nacional de Investigaciones Científicas y Técnicas; Argentina. Universidad de Buenos Aires. Facultad de Ingeniería. Departamento de Física. Grupo de Medios Porosos; Argentina
description We analyze the effect of precipitate formation on the development of density induced hydrodynamic instabilities. In this case the precipitate is BaCO3, obtained by reaction of CO2 with aqueous BaCl2. CO2(g) dissolution increases the local density of the aqueous phase, triggering Rayleigh ?Taylor instabilities and BaCO3 formation. It was observed that at first the precipitate was formed at the finger front. As the particles became bigger, they began to fall down from the front. These particles were used as tracers using PIV technique to visualize the particle streamlines and to obtain the velocity of that movement. This falling produced a downwards flow that might increase the mixing zone. Contrary to expectations, it was observed that finger length decreased, indicating that for the mixing zone development, the consumption of CO2 to form the precipitate is more important than the downwards flow. The mixing zone length was recovered increasing the availability of the reactant (higher CO2 partial pressure), compensating the CO2 used for BaCO3 formation. Mixing zone development rates reached constant values at shorter times when the precipitate is absent than when it is present. An analysis of the non linear regime with and without the precipitate is performed.
publishDate 2017
dc.date.none.fl_str_mv 2017-05
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/40914
Binda, Leonardo David; El Hasi, Claudio Daniel; Zalts, Anita; D'onofrio, Alejandro Gustavo; Experimental analysis of density fingering instability modified by precipitation; American Institute of Physics; Chaos; 27; 5; 5-2017; 1-7
1054-1500
CONICET Digital
CONICET
url http://hdl.handle.net/11336/40914
identifier_str_mv Binda, Leonardo David; El Hasi, Claudio Daniel; Zalts, Anita; D'onofrio, Alejandro Gustavo; Experimental analysis of density fingering instability modified by precipitation; American Institute of Physics; Chaos; 27; 5; 5-2017; 1-7
1054-1500
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/doi/10.1063/1.4983670
info:eu-repo/semantics/altIdentifier/url/https://aip.scitation.org/doi/10.1063/1.4983670
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
application/pdf
dc.publisher.none.fl_str_mv American Institute of Physics
publisher.none.fl_str_mv American Institute of Physics
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 13.13397

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