Disordered Mott-Hubbard Physics in Nanoparticle Solids: Transitions Driven by Disorder, Interactions, and Their Interplay

Autores
Unruh, Davis; Camjayi, Alberto; Hansen, Chase; Bobadilla, Joel Ivan; Rozenberg, Marcelo J.; Zimanyi, Gergely T.
Año de publicación
2020
Idioma
inglés
Tipo de recurso
artículo
Estado
versión publicada
Descripción
We show that adapting the knowledge developed for the disordered Mott-Hubbard model to Nanoparticle (NP) solids can deliver many very helpful new insights. We developed a ?Hierarchical Nanoparticle Transport Simulator? (HINTS), which builds from localized states to describe the Disorder-localized and Mott-localized phases of NP solids, and the transitions out of these localized phases. We also studied the interplaybetween correlations and disorder in the corresponding multi-orbital Hubbard model at and away from integer filling by Dynamical Mean Field Theory. This DMFT approach is complementary to HINTS, as it builds from the metallic phase of the NP solid. The mobility scenarios produced by the two methods are strikingly similar, and account for the mobilities measured in NP solids. We conclude by constructing the comprehensivephase diagram of PbSe NP solids on the disorder-filling plane.
Fil: Unruh, Davis. University of California; Estados Unidos
Fil: Camjayi, Alberto. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; Argentina
Fil: Hansen, Chase. University of California; Estados Unidos
Fil: Bobadilla, Joel Ivan. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; Argentina
Fil: Rozenberg, Marcelo J.. Université Paris Sud; Francia
Fil: Zimanyi, Gergely T.. University of California; Estados Unidos
Materia
COULOMB BLOCKADE
NANOPARTICLES
HUBBARD
DISORDER
Nivel de accesibilidad
acceso abierto
Condiciones de uso
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
Repositorio
CONICET Digital (CONICET)
Institución
Consejo Nacional de Investigaciones Científicas y Técnicas
OAI Identificador
oai:ri.conicet.gov.ar:11336/145807
Acceder
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spelling Disordered Mott-Hubbard Physics in Nanoparticle Solids: Transitions Driven by Disorder, Interactions, and Their InterplayUnruh, DavisCamjayi, AlbertoHansen, ChaseBobadilla, Joel IvanRozenberg, Marcelo J.Zimanyi, Gergely T.COULOMB BLOCKADENANOPARTICLESHUBBARDDISORDERhttps://purl.org/becyt/ford/1.3https://purl.org/becyt/ford/1We show that adapting the knowledge developed for the disordered Mott-Hubbard model to Nanoparticle (NP) solids can deliver many very helpful new insights. We developed a ?Hierarchical Nanoparticle Transport Simulator? (HINTS), which builds from localized states to describe the Disorder-localized and Mott-localized phases of NP solids, and the transitions out of these localized phases. We also studied the interplaybetween correlations and disorder in the corresponding multi-orbital Hubbard model at and away from integer filling by Dynamical Mean Field Theory. This DMFT approach is complementary to HINTS, as it builds from the metallic phase of the NP solid. The mobility scenarios produced by the two methods are strikingly similar, and account for the mobilities measured in NP solids. We conclude by constructing the comprehensivephase diagram of PbSe NP solids on the disorder-filling plane.Fil: Unruh, Davis. University of California; Estados UnidosFil: Camjayi, Alberto. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; ArgentinaFil: Hansen, Chase. University of California; Estados UnidosFil: Bobadilla, Joel Ivan. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; ArgentinaFil: Rozenberg, Marcelo J.. Université Paris Sud; FranciaFil: Zimanyi, Gergely T.. University of California; Estados UnidosAmerican Chemical Society2020-11info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/145807Unruh, Davis; Camjayi, Alberto; Hansen, Chase; Bobadilla, Joel Ivan; Rozenberg, Marcelo J.; et al.; Disordered Mott-Hubbard Physics in Nanoparticle Solids: Transitions Driven by Disorder, Interactions, and Their Interplay; American Chemical Society; Nano Letters; 11-2020; 1-71530-6984CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/url/https://pubs.acs.org/doi/10.1021/acs.nanolett.0c03141info:eu-repo/semantics/altIdentifier/doi/10.1021/acs.nanolett.0c03141info:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-sa/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-10-15T15:30:23Zoai:ri.conicet.gov.ar:11336/145807instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-10-15 15:30:23.725CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse
dc.title.none.fl_str_mv Disordered Mott-Hubbard Physics in Nanoparticle Solids: Transitions Driven by Disorder, Interactions, and Their Interplay
title Disordered Mott-Hubbard Physics in Nanoparticle Solids: Transitions Driven by Disorder, Interactions, and Their Interplay
spellingShingle Disordered Mott-Hubbard Physics in Nanoparticle Solids: Transitions Driven by Disorder, Interactions, and Their Interplay
Unruh, Davis
COULOMB BLOCKADE
NANOPARTICLES
HUBBARD
DISORDER
title_short Disordered Mott-Hubbard Physics in Nanoparticle Solids: Transitions Driven by Disorder, Interactions, and Their Interplay
title_full Disordered Mott-Hubbard Physics in Nanoparticle Solids: Transitions Driven by Disorder, Interactions, and Their Interplay
title_fullStr Disordered Mott-Hubbard Physics in Nanoparticle Solids: Transitions Driven by Disorder, Interactions, and Their Interplay
title_full_unstemmed Disordered Mott-Hubbard Physics in Nanoparticle Solids: Transitions Driven by Disorder, Interactions, and Their Interplay
title_sort Disordered Mott-Hubbard Physics in Nanoparticle Solids: Transitions Driven by Disorder, Interactions, and Their Interplay
dc.creator.none.fl_str_mv Unruh, Davis
Camjayi, Alberto
Hansen, Chase
Bobadilla, Joel Ivan
Rozenberg, Marcelo J.
Zimanyi, Gergely T.
author Unruh, Davis
author_facet Unruh, Davis
Camjayi, Alberto
Hansen, Chase
Bobadilla, Joel Ivan
Rozenberg, Marcelo J.
Zimanyi, Gergely T.
author_role author
author2 Camjayi, Alberto
Hansen, Chase
Bobadilla, Joel Ivan
Rozenberg, Marcelo J.
Zimanyi, Gergely T.
author2_role author
author
author
author
author
dc.subject.none.fl_str_mv COULOMB BLOCKADE
NANOPARTICLES
HUBBARD
DISORDER
topic COULOMB BLOCKADE
NANOPARTICLES
HUBBARD
DISORDER
purl_subject.fl_str_mv https://purl.org/becyt/ford/1.3
https://purl.org/becyt/ford/1
dc.description.none.fl_txt_mv We show that adapting the knowledge developed for the disordered Mott-Hubbard model to Nanoparticle (NP) solids can deliver many very helpful new insights. We developed a ?Hierarchical Nanoparticle Transport Simulator? (HINTS), which builds from localized states to describe the Disorder-localized and Mott-localized phases of NP solids, and the transitions out of these localized phases. We also studied the interplaybetween correlations and disorder in the corresponding multi-orbital Hubbard model at and away from integer filling by Dynamical Mean Field Theory. This DMFT approach is complementary to HINTS, as it builds from the metallic phase of the NP solid. The mobility scenarios produced by the two methods are strikingly similar, and account for the mobilities measured in NP solids. We conclude by constructing the comprehensivephase diagram of PbSe NP solids on the disorder-filling plane.
Fil: Unruh, Davis. University of California; Estados Unidos
Fil: Camjayi, Alberto. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; Argentina
Fil: Hansen, Chase. University of California; Estados Unidos
Fil: Bobadilla, Joel Ivan. Consejo Nacional de Investigaciones Científicas y Técnicas. Oficina de Coordinación Administrativa Ciudad Universitaria. Instituto de Física de Buenos Aires. Universidad de Buenos Aires. Facultad de Ciencias Exactas y Naturales. Instituto de Física de Buenos Aires; Argentina
Fil: Rozenberg, Marcelo J.. Université Paris Sud; Francia
Fil: Zimanyi, Gergely T.. University of California; Estados Unidos
description We show that adapting the knowledge developed for the disordered Mott-Hubbard model to Nanoparticle (NP) solids can deliver many very helpful new insights. We developed a ?Hierarchical Nanoparticle Transport Simulator? (HINTS), which builds from localized states to describe the Disorder-localized and Mott-localized phases of NP solids, and the transitions out of these localized phases. We also studied the interplaybetween correlations and disorder in the corresponding multi-orbital Hubbard model at and away from integer filling by Dynamical Mean Field Theory. This DMFT approach is complementary to HINTS, as it builds from the metallic phase of the NP solid. The mobility scenarios produced by the two methods are strikingly similar, and account for the mobilities measured in NP solids. We conclude by constructing the comprehensivephase diagram of PbSe NP solids on the disorder-filling plane.
publishDate 2020
dc.date.none.fl_str_mv 2020-11
dc.type.none.fl_str_mv info:eu-repo/semantics/article
info:eu-repo/semantics/publishedVersion
http://purl.org/coar/resource_type/c_6501
info:ar-repo/semantics/articulo
format article
status_str publishedVersion
dc.identifier.none.fl_str_mv http://hdl.handle.net/11336/145807
Unruh, Davis; Camjayi, Alberto; Hansen, Chase; Bobadilla, Joel Ivan; Rozenberg, Marcelo J.; et al.; Disordered Mott-Hubbard Physics in Nanoparticle Solids: Transitions Driven by Disorder, Interactions, and Their Interplay; American Chemical Society; Nano Letters; 11-2020; 1-7
1530-6984
CONICET Digital
CONICET
url http://hdl.handle.net/11336/145807
identifier_str_mv Unruh, Davis; Camjayi, Alberto; Hansen, Chase; Bobadilla, Joel Ivan; Rozenberg, Marcelo J.; et al.; Disordered Mott-Hubbard Physics in Nanoparticle Solids: Transitions Driven by Disorder, Interactions, and Their Interplay; American Chemical Society; Nano Letters; 11-2020; 1-7
1530-6984
CONICET Digital
CONICET
dc.language.none.fl_str_mv eng
language eng
dc.relation.none.fl_str_mv info:eu-repo/semantics/altIdentifier/url/https://pubs.acs.org/doi/10.1021/acs.nanolett.0c03141
info:eu-repo/semantics/altIdentifier/doi/10.1021/acs.nanolett.0c03141
dc.rights.none.fl_str_mv info:eu-repo/semantics/openAccess
https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
eu_rights_str_mv openAccess
rights_invalid_str_mv https://creativecommons.org/licenses/by-nc-sa/2.5/ar/
dc.format.none.fl_str_mv application/pdf
application/pdf
dc.publisher.none.fl_str_mv American Chemical Society
publisher.none.fl_str_mv American Chemical Society
dc.source.none.fl_str_mv reponame:CONICET Digital (CONICET)
instname:Consejo Nacional de Investigaciones Científicas y Técnicas
reponame_str CONICET Digital (CONICET)
collection CONICET Digital (CONICET)
instname_str Consejo Nacional de Investigaciones Científicas y Técnicas
repository.name.fl_str_mv CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas
repository.mail.fl_str_mv dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar
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score 13.22299

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