Fast microwave synthesis of Pt-MFI zeolite coatings on silicon micromonoliths: Application to VOC catalytic combustion
- Autores
- Marin, Ingrid; Adrover, María Esperanza; Vega,Didac; Urbiztondo, Miguel; Pina, Maria Pilar; Mallada, Reyes; Santamaría, Jesús
- Año de publicación
- 2012
- Idioma
- inglés
- Tipo de recurso
- artículo
- Estado
- versión publicada
- Descripción
- This paper describes the preparation of a ZSM-5 zeolite layer onto conventional Si wafers and Si micromonoliths, by using microwave-assisted seeded hydrothermal synthesis. A homogeneous ZSM-5 zeolite layer up to 680 nm was obtained over the external surface of a Si micromonolith (surface to volume ratio >300,000 m-1) after only 4 min of hydrothermal synthesis at 453 K. As a proof of concept, the catalytic activity of the prepared ZSM-5 coated micromonoliths, after a conventional Pt ion-exchange process, was demonstrated in the combustion of traces of n-hexane (200 ppmV) in air.
Fil: Marin, Ingrid. Universidad de Zaragoza. Instituto de Nanociencia de Aragón; España
Fil: Adrover, María Esperanza. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Planta Piloto de Ingeniería Química. Universidad Nacional del Sur. Planta Piloto de Ingeniería Química; Argentina
Fil: Vega,Didac. Universidad Politecnica de Catalunya; España
Fil: Urbiztondo, Miguel. Centro Universitario de la Defensa (cud); España
Fil: Pina, Maria Pilar. Universidad de Zaragoza. Instituto de Nanociencia de Aragón; España
Fil: Mallada, Reyes. Universidad de Zaragoza. Instituto de Nanociencia de Aragón; España
Fil: Santamaría, Jesús. Universidad de Zaragoza. Instituto de Nanociencia de Aragón; España - Materia
-
Mfi
Microreactor
Microwave Synthesis
Voc Combustion - Nivel de accesibilidad
- acceso abierto
- Condiciones de uso
- https://creativecommons.org/licenses/by-nc-nd/2.5/ar/
- Repositorio
- Institución
- Consejo Nacional de Investigaciones Científicas y Técnicas
- OAI Identificador
- oai:ri.conicet.gov.ar:11336/53507
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Fast microwave synthesis of Pt-MFI zeolite coatings on silicon micromonoliths: Application to VOC catalytic combustionMarin, IngridAdrover, María EsperanzaVega,DidacUrbiztondo, MiguelPina, Maria PilarMallada, ReyesSantamaría, JesúsMfiMicroreactorMicrowave SynthesisVoc Combustionhttps://purl.org/becyt/ford/2.4https://purl.org/becyt/ford/2This paper describes the preparation of a ZSM-5 zeolite layer onto conventional Si wafers and Si micromonoliths, by using microwave-assisted seeded hydrothermal synthesis. A homogeneous ZSM-5 zeolite layer up to 680 nm was obtained over the external surface of a Si micromonolith (surface to volume ratio >300,000 m-1) after only 4 min of hydrothermal synthesis at 453 K. As a proof of concept, the catalytic activity of the prepared ZSM-5 coated micromonoliths, after a conventional Pt ion-exchange process, was demonstrated in the combustion of traces of n-hexane (200 ppmV) in air.Fil: Marin, Ingrid. Universidad de Zaragoza. Instituto de Nanociencia de Aragón; EspañaFil: Adrover, María Esperanza. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Planta Piloto de Ingeniería Química. Universidad Nacional del Sur. Planta Piloto de Ingeniería Química; ArgentinaFil: Vega,Didac. Universidad Politecnica de Catalunya; EspañaFil: Urbiztondo, Miguel. Centro Universitario de la Defensa (cud); EspañaFil: Pina, Maria Pilar. Universidad de Zaragoza. Instituto de Nanociencia de Aragón; EspañaFil: Mallada, Reyes. Universidad de Zaragoza. Instituto de Nanociencia de Aragón; EspañaFil: Santamaría, Jesús. Universidad de Zaragoza. Instituto de Nanociencia de Aragón; EspañaDe Gruyter2012-04info:eu-repo/semantics/articleinfo:eu-repo/semantics/publishedVersionhttp://purl.org/coar/resource_type/c_6501info:ar-repo/semantics/articuloapplication/pdfapplication/pdfhttp://hdl.handle.net/11336/53507Marin, Ingrid; Adrover, María Esperanza; Vega,Didac; Urbiztondo, Miguel; Pina, Maria Pilar; et al.; Fast microwave synthesis of Pt-MFI zeolite coatings on silicon micromonoliths: Application to VOC catalytic combustion; De Gruyter; Green Processing and Synthesis; 1; 2; 4-2012; 169-1742191-95422191-9550CONICET DigitalCONICETenginfo:eu-repo/semantics/altIdentifier/doi/10.1515/gps-2012-0006info:eu-repo/semantics/altIdentifier/url/https://www.degruyter.com/view/j/gps.2012.1.issue-2/gps-2012-0006/gps-2012-0006.xmlinfo:eu-repo/semantics/openAccesshttps://creativecommons.org/licenses/by-nc-nd/2.5/ar/reponame:CONICET Digital (CONICET)instname:Consejo Nacional de Investigaciones Científicas y Técnicas2025-09-29T10:13:11Zoai:ri.conicet.gov.ar:11336/53507instacron:CONICETInstitucionalhttp://ri.conicet.gov.ar/Organismo científico-tecnológicoNo correspondehttp://ri.conicet.gov.ar/oai/requestdasensio@conicet.gov.ar; lcarlino@conicet.gov.arArgentinaNo correspondeNo correspondeNo correspondeopendoar:34982025-09-29 10:13:11.626CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicasfalse |
dc.title.none.fl_str_mv |
Fast microwave synthesis of Pt-MFI zeolite coatings on silicon micromonoliths: Application to VOC catalytic combustion |
title |
Fast microwave synthesis of Pt-MFI zeolite coatings on silicon micromonoliths: Application to VOC catalytic combustion |
spellingShingle |
Fast microwave synthesis of Pt-MFI zeolite coatings on silicon micromonoliths: Application to VOC catalytic combustion Marin, Ingrid Mfi Microreactor Microwave Synthesis Voc Combustion |
title_short |
Fast microwave synthesis of Pt-MFI zeolite coatings on silicon micromonoliths: Application to VOC catalytic combustion |
title_full |
Fast microwave synthesis of Pt-MFI zeolite coatings on silicon micromonoliths: Application to VOC catalytic combustion |
title_fullStr |
Fast microwave synthesis of Pt-MFI zeolite coatings on silicon micromonoliths: Application to VOC catalytic combustion |
title_full_unstemmed |
Fast microwave synthesis of Pt-MFI zeolite coatings on silicon micromonoliths: Application to VOC catalytic combustion |
title_sort |
Fast microwave synthesis of Pt-MFI zeolite coatings on silicon micromonoliths: Application to VOC catalytic combustion |
dc.creator.none.fl_str_mv |
Marin, Ingrid Adrover, María Esperanza Vega,Didac Urbiztondo, Miguel Pina, Maria Pilar Mallada, Reyes Santamaría, Jesús |
author |
Marin, Ingrid |
author_facet |
Marin, Ingrid Adrover, María Esperanza Vega,Didac Urbiztondo, Miguel Pina, Maria Pilar Mallada, Reyes Santamaría, Jesús |
author_role |
author |
author2 |
Adrover, María Esperanza Vega,Didac Urbiztondo, Miguel Pina, Maria Pilar Mallada, Reyes Santamaría, Jesús |
author2_role |
author author author author author author |
dc.subject.none.fl_str_mv |
Mfi Microreactor Microwave Synthesis Voc Combustion |
topic |
Mfi Microreactor Microwave Synthesis Voc Combustion |
purl_subject.fl_str_mv |
https://purl.org/becyt/ford/2.4 https://purl.org/becyt/ford/2 |
dc.description.none.fl_txt_mv |
This paper describes the preparation of a ZSM-5 zeolite layer onto conventional Si wafers and Si micromonoliths, by using microwave-assisted seeded hydrothermal synthesis. A homogeneous ZSM-5 zeolite layer up to 680 nm was obtained over the external surface of a Si micromonolith (surface to volume ratio >300,000 m-1) after only 4 min of hydrothermal synthesis at 453 K. As a proof of concept, the catalytic activity of the prepared ZSM-5 coated micromonoliths, after a conventional Pt ion-exchange process, was demonstrated in the combustion of traces of n-hexane (200 ppmV) in air. Fil: Marin, Ingrid. Universidad de Zaragoza. Instituto de Nanociencia de Aragón; España Fil: Adrover, María Esperanza. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Bahía Blanca. Planta Piloto de Ingeniería Química. Universidad Nacional del Sur. Planta Piloto de Ingeniería Química; Argentina Fil: Vega,Didac. Universidad Politecnica de Catalunya; España Fil: Urbiztondo, Miguel. Centro Universitario de la Defensa (cud); España Fil: Pina, Maria Pilar. Universidad de Zaragoza. Instituto de Nanociencia de Aragón; España Fil: Mallada, Reyes. Universidad de Zaragoza. Instituto de Nanociencia de Aragón; España Fil: Santamaría, Jesús. Universidad de Zaragoza. Instituto de Nanociencia de Aragón; España |
description |
This paper describes the preparation of a ZSM-5 zeolite layer onto conventional Si wafers and Si micromonoliths, by using microwave-assisted seeded hydrothermal synthesis. A homogeneous ZSM-5 zeolite layer up to 680 nm was obtained over the external surface of a Si micromonolith (surface to volume ratio >300,000 m-1) after only 4 min of hydrothermal synthesis at 453 K. As a proof of concept, the catalytic activity of the prepared ZSM-5 coated micromonoliths, after a conventional Pt ion-exchange process, was demonstrated in the combustion of traces of n-hexane (200 ppmV) in air. |
publishDate |
2012 |
dc.date.none.fl_str_mv |
2012-04 |
dc.type.none.fl_str_mv |
info:eu-repo/semantics/article info:eu-repo/semantics/publishedVersion http://purl.org/coar/resource_type/c_6501 info:ar-repo/semantics/articulo |
format |
article |
status_str |
publishedVersion |
dc.identifier.none.fl_str_mv |
http://hdl.handle.net/11336/53507 Marin, Ingrid; Adrover, María Esperanza; Vega,Didac; Urbiztondo, Miguel; Pina, Maria Pilar; et al.; Fast microwave synthesis of Pt-MFI zeolite coatings on silicon micromonoliths: Application to VOC catalytic combustion; De Gruyter; Green Processing and Synthesis; 1; 2; 4-2012; 169-174 2191-9542 2191-9550 CONICET Digital CONICET |
url |
http://hdl.handle.net/11336/53507 |
identifier_str_mv |
Marin, Ingrid; Adrover, María Esperanza; Vega,Didac; Urbiztondo, Miguel; Pina, Maria Pilar; et al.; Fast microwave synthesis of Pt-MFI zeolite coatings on silicon micromonoliths: Application to VOC catalytic combustion; De Gruyter; Green Processing and Synthesis; 1; 2; 4-2012; 169-174 2191-9542 2191-9550 CONICET Digital CONICET |
dc.language.none.fl_str_mv |
eng |
language |
eng |
dc.relation.none.fl_str_mv |
info:eu-repo/semantics/altIdentifier/doi/10.1515/gps-2012-0006 info:eu-repo/semantics/altIdentifier/url/https://www.degruyter.com/view/j/gps.2012.1.issue-2/gps-2012-0006/gps-2012-0006.xml |
dc.rights.none.fl_str_mv |
info:eu-repo/semantics/openAccess https://creativecommons.org/licenses/by-nc-nd/2.5/ar/ |
eu_rights_str_mv |
openAccess |
rights_invalid_str_mv |
https://creativecommons.org/licenses/by-nc-nd/2.5/ar/ |
dc.format.none.fl_str_mv |
application/pdf application/pdf |
dc.publisher.none.fl_str_mv |
De Gruyter |
publisher.none.fl_str_mv |
De Gruyter |
dc.source.none.fl_str_mv |
reponame:CONICET Digital (CONICET) instname:Consejo Nacional de Investigaciones Científicas y Técnicas |
reponame_str |
CONICET Digital (CONICET) |
collection |
CONICET Digital (CONICET) |
instname_str |
Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.name.fl_str_mv |
CONICET Digital (CONICET) - Consejo Nacional de Investigaciones Científicas y Técnicas |
repository.mail.fl_str_mv |
dasensio@conicet.gov.ar; lcarlino@conicet.gov.ar |
_version_ |
1844614046384390144 |
score |
13.070432 |